arXiv subjects

Matthias C. Velsink

Publications and source records attributed to Matthias C. Velsink.

4 recordsLinked to original sources

arXiv2025

Improving signal-to-noise ratios in pump-probe spectroscopy on light-sensitive samples by adapting pulse repetition rates

Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction, resulting in dynamics that can be detected using a time-delayed probe pulse. In addition to the desired dynamics, the initial interaction may also lead to unwanted effects that may result in irreversible changes and even damage. Therefore, the achievable signal strength is often limited by the pumping conditions that a sample can sustain. Here we investigate the optimization of ultrafast photoacoustics in various solid thin films. We perform systematic experiments aimed at maximizing the achievable signal-to-noise (SNR) ratio in a given measurement time while limiting sample damage. By varying pump and probe pulse energies, average pump fluence, and repetition rate, we identify different paths towards optimal SNR depending on material properties. Our results provide a strategy for the design of pump-probe experiments, to optimize achievable SNR for samples in which different damage mechanisms may dominate.

physics.optics↗

arXiv2021

Comparison of round- and square-core fibers for sensing, imaging and spectroscopy

Multimode fibers (MMFs) show great promise as miniature probes for sensing, imaging and spectroscopy applications. Different parameters of the fibers, such as numerical aperture, refractive index profile and length, have been already optimized for better performance. Here we investigate the role of the core shape, in particular for wavefront shaping applications where a focus is formed at the output of the MMF. We demonstrate that in contrast to a conventional round-core MMF, a square-core design doesn't suffer from focus aberrations. Moreover, we find that how the interference pattern behind a square-core fiber decorrelates with the input frequency is largely independent of the input light coupling. Finally, we demonstrate that a square core shape provides an on-average uniform distribution of the output intensity, free from the input-output correlations seen in round fibers, showing great promise for imaging and spectroscopy applications.

physics.optics↗

arXiv2020

Spatiotemporal focusing through a multimode fiber via time-domain wavefront shaping

We shape fs optical pulses and deliver them in a single spatial mode to the input of a multimode fiber. The pulse is shaped in time such that at the output of the multimode fiber an ultrashort pulse appears at a predefined focus. Our result shows how to raster scan an ultrashort pulse at the output of a stiff piece of square-core step-index multimode fiber and in this way the potential for making a nonlinear fluorescent image of the scene behind the fiber, while the connection to the multimode fiber can be established via a thin and flexible single-mode fiber. The experimental results match our numerical simulation well.

physics.optics↗

arXiv2019

Uniform line fillings

Deterministic fabrication of random metamaterials requires filling of a space with randomly oriented and randomly positioned chords with an on-average homogenous density and orientation, which is a nontrivial task. We describe a method to generate fillings with such chords, lines that run from edge to edge of the space, in any dimension. We prove that the method leads to random but on-average homogeneous and rotationally invariant fillings of circles, balls and arbitrary-dimensional hyperballs from which other shapes such as rectangles and cuboids can be cut. We briefly sketch the historic context of Bertrand's paradox and Jaynes' solution by the principle of maximum ignorance. We analyse the statistical properties of the produced fillings, mapping out the density profile and the line-length distribution and comparing them to analytic expressions. We study the characteristic dimensions of the space in between the chords by determining the largest enclosed circles and balls in this pore space, finding a lognormal distribution of the pore sizes. We apply the algorithm to the direct-laser-writing fabrication design of optical multiple-scattering samples as three-dimensional cubes of random but homogeneously positioned and oriented chords.

cond-mat.soft↗