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Matthias Eschrig

Publications and source records attributed to Matthias Eschrig.

At least 19 recordsLinked to original sources

Anomalous Superfluid Response in Altermagnetic Superconductors

We report on the emergence of the anomalous (paramagnetic) superfluid response in altermagnetic superconductors at arbitrary impurity concentrations. Due to anisotropic gapless superconductivity, altermagnetic superconductors with an out-of-plane Zeeman field display an anisotropic paramagnetic Meissner effect. The effect is strongest for parallel altermagnetic and Zeeman exchange field vectors and in the clean sample. The presence of nonmagnetic impurities leads to isotropisation and, consequently, weakens the effect; however, the paramagnetic response sustains intermediate amounts of impurities in the system. As demonstrated in recent experiments, microwave superfluid stiffness measurements can serve as a sensitive probe of gapless superconductivity.

cond-mat.supr-con

Free Energy of Non-uniform Disordered Superconductors

We extend the Luttinger-Ward free energy functional to disordered superconductors and superfluids with arbitrary scattering mechanisms, including both impurity disorder and the presence of interfaces. The disorder is taken into account within the self-consistent $t$-matrix approximation, thus allowing for arbitrary impurity scattering strengths. It is shown that both the interface and the impurity scattering self-energy appear in the functional only implicitly, through self-consistently determined fermionic propagators. The free energy functional is formulated in terms of a generalized integral in the complex energy plane, which encompasses formulations both in terms of retarded/advanced propagators and in terms of Matsubara Green's functions by appropriately choosing the integration path. It can be applied, e.g., to spatially non-uniform and hybrid systems, triplet and other unconventional condensates, and strongly-correlated Fermi liquids. A particularly useful formulation in terms of the quasiclassical propagators is applied to unconventional non-uniform singlet and triplet superconductors and superfluids in an external Zeeman magnetic field.

cond-mat.supr-con

Spin-polarized supercurrents and Josephson diode effect in altermagnets

We present a systematic theoretical study of the Josephson effect in junctions consisting of a d-wave altermagnet (AM) placed between two BCS superconductors (SC). In general, the SC/AM interfaces are spin-active and modeled by spin-dependent $\delta$ potentials, allowing for an arbitrary direction of the local exchange field vector. The model is formulated within the fully quantum (Gor'kov) and quasiclassical (Eilenberger) Green's function technique, applied to two distinct cases of (i) a weakly spin-polarized AM (exchange field much smaller compared to the Fermi energy) and (ii) a strongly spin-polarized AM (exchange field comparable to the Fermi energy). We apply our model to the SC/AM/SC geometry, accounting for the Josephson current-phase relation (CPR). In the weakly spin-polarized regime, the CPR displays the normal Josephson effect. Irrespective of the orientation of the altermagnet, the junction undergoes the $0-\pi$ transition. Depending on the orientation, the system displays the features similar to those of a ferromagnetic or an antiferromagnetic junction. To investigate the spin-polarized currents and nonreciprocal transport as the central results of the present work, we put the main focus on the strongly spin-polarized regime. Within this regime, we distinguish two cases. A coplanar exchange field profile across the junctions displays the normal Josephson effect; however, with a pure and stable long-range second harmonic in the CPR. In contrast, a noncoplanar exchange field profile gives rise to the so-called quantum geometric phases across the junction, leading to the absence of the phase-inversion center in the Josephson CPR. As a result, a Josephson diode effect emerges with a significant charge diode efficiency larger than 30% and a perfect spin diode efficiency of 100%.

cond-mat.supr-con

Light-driven octupolar inverse Faraday effect and multipolar order in Mott insulators

Hidden multipolar orders in spin-orbit-coupled Mott insulators provide a promising setting for correlated quantum matter, yet their control and detection remain major challenges. Here, we demonstrate that circularly polarized light enables both in $4d^2/5d^2$ systems with edge-sharing octahedra. Using a Floquet Schrieffer-Wolff expansion of a driven Hubbard-Kanamori model, we derive a low-energy multipolar Hamiltonian with two qualitatively new light-driven terms. One is an effective static field that couples linearly to the magnetic octupole, realizing an octupolar inverse Faraday effect. The other is a bond-dependent anisotropic exchange interaction absent in equilibrium. These two couplings are the key result of this work: the first provides a direct optical handle on hidden octupolar order, while the second reorganizes the multipolar exchange landscape and opens an enlarged Kitaev-like multipolar liquid regime. Their interplay produces a nonequilibrium multipolar phase space inaccessible in equilibrium, enabling optical tuning among antiferro-octupolar, ferro-octupolar, partially polarized ferro-quadrupolar, Ising octupolar, and multipolar liquid phases. We further show that the induced multipolar order couples to the lattice, generating reversible trigonal and tetragonal distortions that provide structural fingerprints in pump-probe experiments. Our work establishes a general mechanism for the optical generation, control, and detection of hidden multipolar quantum states.

cond-mat.str-el

Necessary conditions for spin-resolved Josephson diode effect across strongly spin-polarized magnetic materials

We present a set of necessary conditions for the appearance of charge and spin Josephson diode effects across strongly spin-polarized inhomogeneous magnetic materials (FM) placed between two spin-singlet superconductors. Noncoplanarity of the FM's spin texture gives rise to quantum geometric phases, $\Delta\varphi'$, that enter the Josephson current-phase relation (CPR) similarly to the superconducting phase difference, resulting in charge and spin Josephson diode effects. Our study shows that such effects appear if the CPR possesses no phase-inversion center, achieved under the following conditions. First, noncoplanarity of the spin texture is necessary to break the spatial inversion symmetry. Second, both spin bands have to contribute to the transport, i.e., the effect is absent in half-metallic junctions. Third, different band-specific densities of states are required, and this condition is ensured by the strong spin polarization of the FM. Finally, higher harmonics in the CPR are necessary, i.e., the effect is absent in the tunneling limit. However, even in this case, the CPR must not have a phase-inversion center, which is ensured by the restriction of the quantum geometric phase to values $\Delta\varphi'\neq k\pi/2, k\in\mathbb{Z}$. We formulate a minimal phenomenological model that incorporates all these points, qualitatively illustrating our theory.

cond-mat.supr-con

Purely even harmonic Josephson current due to crossed pair transmission across strongly spin-polarized materials

We revisit the problem of the second harmonic generation in the current-phase relation across ferromagnetic bilayers placed between BCS superconductors. In particular, we consider a strongly spin-polarized metallic ferromagnet coupled to two superconducting leads via thin spin-active (left) and non-spin-active (right) insulating layers. The system is examined in the framework of the quasiclassical Green$^\prime$s function formalism, both in the ballistic (Eilenberger) and the diffusive (Usadel) limit. Strong spin polarization allows for neglecting short-range mixed-spin correlations, and the Josephson supercurrent across the ferromagnet is fully mediated by long-range equal-spin triplet correlations. Using a diagrammatic technique for ballistic propagators introduced in Refs. [1-3], we describe the relevant Andreev processes responsible for the effective conversion of two spin-singlet Cooper pairs in the superconductor into two $\uparrow\uparrow$ and $\downarrow\downarrow$ pairs in the ferromagnet. Contrary to the naive picture of direct conversion, we show that the lowest order process involves four Cooper pairs in the superconductor, among which three are incoming, and one is outgoing, giving rise to net charge transport of 4e across the non-spin-active interface. The self-consistent numerical treatment of the diffusive junction, typically more relevant in experiments, confirms this picture quantitatively.

cond-mat.supr-con

Spin-resolved Josephson diode effect through strongly spin-polarized conical magnets

We present a theoretical study of the spin-resolved Josephson diode effect in junctions comprising strongly spin-polarized conical magnets (FM) coupled to singlet superconductors (SC). The system is treated by making use of the Gor$^\prime$kov and quasiclassical Green$^\prime$s function methods. Modeling the SC/FM interfaces as spin-dependent $\delta$-potentials, we apply our model to an SC/FM/SC junction and account for the Josephson current-phase relation (CPR). The nontrivial coupling between the spin bands in the conical magnet gives rise to a strong Josephson diode effect with an efficiency greater than 40%. The effect essentially depends on the quantum spin-geometric phase that enters the Josephson CPR in a very similar manner to the superconducting phase difference. The former is generated non-locally by the intrinsically noncoplanar spin arrangement of the conical magnet, which breaks the time-reversal and inversion symmetries. Strong spin polarization and a helical pitch of the conical magnet comparable to the superconducting coherence length are essential for the effect. We perform a harmonic analysis of the Josephson CPR and interpret the effect in terms of coherent transfer of multiple equal-spin triplet Cooper pairs across the conical magnet.

cond-mat.supr-con

Theory of quantum-geometric charge and spin Josephson diode effects in strongly spin-polarized hybrid structures with noncoplanar spin textures

We present a systematic study of the spin-resolved Josephson diode effect (JDE) in strongly spin-polarized ferromagnets (sFM) coupled to singlet superconductors (SC) via ferromagnetic insulating interfaces (FI). All metallic parts are described in the framework of the quasiclassical Usadel Green's function theory applicable to diffusive systems. The interfaces are characterized by an S-matrix obtained for a model potential with exchange vectors pointing in an arbitrary direction with respect to the magnetization in the sFM. Our theory predicts a large charge Josephson diode effect with an efficiency exceeding $33\%$ and a perfect spin diode effect with $100\%$ efficiency. To achieve these the following conditions are necessary: (i) a noncoplanar profile of the three magnetization vectors in the system and (ii) different densities of states of spin-$\uparrow$ and spin-$\downarrow$ bands in the sFM achieved by a strong spin polarization. The former gives rise to the quantum-geometric phase, $\Delta\varphi$, that enters the theory in a very similar manner as the superconducting phase difference across the junction, $\Delta\chi$. We perform a harmonic analysis of the Josephson current in both variables and find symmetries between Fourier coefficients allowing an interpretation in terms of transfer processes of multiple equal-spin Cooper pairs across the two ferromagnetic spin bands. We point out the importance of crossed pair transmission processes. Finally, we study a spin-switching effect of an equal-spin supercurrent by reversing the magnetic flux in a SQUID device incorporating the mentioned junction and propose a way for measuring it.

cond-mat.supr-con

Quantum-geometric spin and charge Josephson diode effects

We present a general mechanism for large charge and spin Josephson diode effects in strongly spin-polarized superconductor-ferromagnet hybrid structures with a noncoplanar spin texture, formulated in terms of quantum-geometric phases. We present necessary conditions for this effect to occur, and show numerical results for disordered materials, relevant for applications. We calculate Josephson diode efficiencies for both charge- and spin-diodes and show that a spin-diode efficiency of 100% can be reached. Finally, we present a SQUID device that can switch between nearly pure spin-up and spin-down equal-spin supercurrents across the ferromagnet by reversing the flux. These findings establish functionalities that are absent for coplanar spin textures.

cond-mat.supr-con

Chiral Current Inversion Induced by Flat-Band Andreev Bound States

We study the spontaneous chiral surface current circulating in a three-dimensional disk of a chiral superconductor (SC) utilizing the quasiclassical Eilenberger theory. We obtain spatial profiles of the chiral current for both a ($d_{zx} + i d_{yz}$)-wave and a ($p_{x} + i p_{y}$)-wave SCs (where the top and bottom surfaces of the disk are perpendicular to the $z$-axis). Whereas the chiral current for a ($p_{x} + i p_{y}$)-wave SC does not depend on $z$, a reversal of the chiral current takes place at the top and bottom surfaces in the case of a ($d_{zx} + i d_{yz}$)-wave SC. In this latter case, flat-band Andreev bound states appear at the top and bottom surfaces in addition to the chiral surface states at the lateral surface. The chiral current reversal is explained in terms of hybridization between the two types of Andreev bound states. As a result, the magnetic field around the disk differs drastically between the two cases.

cond-mat.supr-con

Controlling spin pumping into superconducting Nb by proximity-induced spin-triplet Cooper pairs

Proximity-induced long-range spin-triplet supercurrents, important for the field of superconducting spintronics, are generated in superconducting/ferromagnetic heterostructures when interfacial magnetic inhomogeneities responsible for spin mixing and spin flip scattering are present. The multilayer stack Nb/Cr/Fe/Cr/Nb has been shown to support such exotic currents when fabricated into Josephson junction devices. However, creating pure spin currents controllably in superconductors outside of the Josephson junction architecture is a bottleneck to progress. Recently, ferromagnetic resonance was proposed as a possible direction, the signature of pure supercurrent creation being an enhancement of the Gilbert damping below the superconducting critical temperature, but the necessary conditions are still poorly established. Consistent with theoretical prediction, we demonstrate conclusively that pumping pure spin currents into a superconductor is only possible when conditions supporting proximity-induced spin-triplet effects are satisfied. Our study is an important step forward for superconducting pure spin current creation and manipulation, considerably advancing the field of superconducting spintronics.

cond-mat.supr-con

FeSe and the missing electron pocket problem

The nature and origin of electronic nematicity remains a significant challenge in our understanding of the iron-based superconductors. This is particularly evident in the iron chalcogenide, FeSe, where it is currently unclear how the experimentally determined Fermi surface near the M point evolves from having two electron pockets in the tetragonal state to exhibiting just a single electron pocket in the nematic state. This has posed a major theoretical challenge, which has become known as the missing electron pocket problem of FeSe, and is of central importance if we wish to uncover the secrets behind nematicity and superconductivity in the wider iron-based superconductors. Here, we review the recent experimental work uncovering this nematic Fermi surface of FeSe from both ARPES and STM measurements, as well as current theoretical attempts to explain this missing electron pocket of FeSe, with a particular focus on the emerging importance of incorporating the $d_{xy}$ orbital into theoretical descriptions of the nematic state. Furthermore, we will discuss the consequence this missing electron pocket has on the theoretical understanding of superconductivity in this system and present several remaining open questions and avenues for future research.

cond-mat.supr-con

Non-local $d_{xy}$ nematicity and the missing electron pocket in FeSe

The origin of spontaneous electronic nematic ordering provides important information for understanding iron-based superconductors. Here, we analyze a scenario where the $d_{xy}$ orbital strongly contributes to nematic ordering in FeSe. We show that the addition of $d_{xy}$ nematicity to a pure $d_{xz}/d_{yz}$ order provides a natural explanation for the unusual Fermi surface and correctly reproduces the strongly anisotropic momentum dependence of the superconducting gap. We predict a Lifshitz transition of an electron pocket mediated by temperature and sulphur doping, whose signatures we discuss by analysing available experimental data. We present the variation of momentum dependence of the superconducting gap upon suppression of nematicity. Our quantitatively accurate model yields the transition from tetragonal to nematic FeSe and the FeSe$_{1-x}$S$_{x}$ series, and puts strong constraints on possible nematic mechanisms.

cond-mat.supr-con

Anomalous inverse proximity effect in unconventional-superconductor junctions

We investigate the effects of Andreev bound states due to the unconventional pairing on the inverse proximity effect of ferromagnet/superconductor junctions. Utilizing quasiclassical Eilenberger theory, we obtain the magnetization penetrating into the superconductor. We show that in a wide parameter range the direction of the induced magnetization is determined by two factors: whether Andreev bound states are present at the junction interface and the sign of the spin-mixing angle. In particular, when Andreev bound states appear at the interface, the direction of the induced magnetization is opposite to that without Andreev bound states. We also clarify the conditions under which the inverted induced magnetization appears. Applying this novel effect helps distinguishing the pairing symmetry of a superconductor.

cond-mat.supr-con

The inverse proximity effect in strong ferromagnet-superconductor structures

The magnetization in a superconductor induced due to the inverse proximity effect is investigated in hybrid bilayers containing a superconductor and a ferromagnetic insulator or a strongly spin-polarized ferromagnetic metal. The study is performed within a quasiclassical Green function framework, wherein Usadel equations are solved with boundary conditions appropriate for strongly spin-polarized ferromagnetic materials. A comparison with recent experimental data is presented. The singlet to triplet conversion of the superconducting correlations as a result of the proximity effect with a ferromagnet is studied.

cond-mat.supr-con

$k_z$ selective scattering within Quasiparticle Interference measurements of FeSe

Quasiparticle interference (QPI) provides a wealth of information relating to the electronic structure of a material. However, it is often assumed that this information is constrained to two-dimensional electronic states. Here, we show that this is not necessarily the case. For FeSe, a system dominated by surface defects, we show that it is actually all electronic states with negligible group velocity in the $z$ axis that are contained within the experimental data. By using a three-dimensional tight binding model of FeSe, fit to photoemission measurements, we directly reproduce the experimental QPI scattering dispersion, within a T-matrix formalism, by including both $k_z = 0$ and $k_z = π$ electronic states. This result unifies both tunnelling and photoemission based experiments on FeSe and highlights the importance of $k_z$ within surface sensitive measurements of QPI.

cond-mat.supr-con

Magnetic Skyrmion Lattice by Fourier Transform Method

We demonstrate a fast numerical method of theoretical studies of skyrmion lattice or spiral order in magnetic materials with Dzyaloshinsky-Moriya interaction. The method is based on the Fourier expansion of the magnetization combined with a minimization of the free energy functional of the magnetic material in Fourier space, yielding the optimal configuration of the system for any given set of parameters. We employ a Lagrange multiplier technique in order to satisfy micromagnetic constraints. We apply this method to a system that exhibits, depending on the parameter choice, ferromagnetic, skyrmion lattice, or spiral (helical) order. Known critical fields corresponding to the helical-skyrmion as well as the skyrmion-ferromagnet phase transitions are reproduced with high precision. Using this numerical method we predict new types of excited (metastable) states of the skyrmion lattice, which may be stabilized by coupling the skyrmion lattice with a superconducting vortex lattice. The method can be readily adapted to other micromagnetic systems.

cond-mat.str-el

Effect of Meissner screening and trapped magnetic flux on magnetization dynamics in thick Nb/Ni80Fe20/Nb trilayers

We investigate the influence of Meissner screening and trapped magnetic flux on magnetization dynamics for a Ni80Fe20 film sandwiched between two thick Nb layers (100 nm) using broadband (5-20 GHz) ferromagnetic resonance (FMR) spectroscopy. Below the superconducting transition Tc of Nb, significant zero-frequency line broadening (5-6 mT) and DC resonance field shift (50 mT) to a low field are both observed if the Nb thickness is comparable to the London penetration depth of Nb films (>= 100 nm). We attribute the observed peculiar behaviors to the increased incoherent precession near the Ni80Fe20/Nb interface and the effectively focused magnetic flux in the middle Ni80Fe20 caused by strong Meissner screening and (defect-)trapped flux of the thick adjacent Nb layers. This explanation is supported by static magnetic properties of the samples and comparison with FMR data on thick Nb/Ni80Fe20 bilayers. Great care should therefore be taken in the analysis of FMR response in ferromagnetic Josephson structures with thick superconductors, a fundamental property for high-frequency device applications of spin-polarized supercurrents.

cond-mat.mes-hall