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Matthias Schröter

Publications and source records attributed to Matthias Schröter.

At least 37 records · Page 2Linked to original sources

A cohesive granular material with tunable elasticity

By mixing glass beads with a curable polymer we create a well-defined cohesive granular medium, held together by solidified, and hence elastic, capillary bridges. This material has a geometry similar to a wet packing of beads, but with an additional control over the elasticity of the bonds holding the particles together. We show that its mechanical response can be varied over several orders of magnitude by adjusting the size and stiffness of the bridges, and the size of the particles. We also investigate its mechanism of failure under unconfined uniaxial compression in combination with in situ x-ray microtomography. We show that a broad linear-elastic regime ends at a limiting strain of about 8%, whatever the stiffness of the agglomerate, which corresponds to the beginning of shear failure. The possibility to finely tune the stiffness, size and shape of this simple material makes it an ideal model system for investigations on, for example, fracturing of porous rocks, seismology, or root growth in cohesive porous media.

cond-mat.soft↗

High refractive index immersion liquid for super-resolution 3D imaging using sapphire-based aNAIL optics

Optically-transparent immersion liquids with refractive index (n ~ 1.77) to match sapphire-based aplanatic numerical aperture increasing lens (aNAIL) are necessary for achieving deep 3D imaging with high spatial resolution. We report that antimony tribromide (SbBr$_{3}$) salt dissolved in liquid diiodomethane (CH$_{2}$I$_{2}$) provides a new high refractive index immersion liquid for optics applications. The refractive index is tunable from n = 1.74 (pure) to n = 1.873 (saturated), by adjusting either salt concentration or temperature; this allows it to match (or even exceed) the refractive index of sapphire. Importantly, the solution gives excellent light transmittance in the ultraviolet to near-infrared range, an improvement over commercially-available immersion liquids. This refractive index matched immersion liquid formulation has enabled us to develop a sapphire-based aNAIL objective that has both high numerical aperture (NA = 1.17) and long working distance (WD = 12 mm). This opens up new possibilities for deep 3D imaging with high spatial resolution.

physics.optics↗

The mechanism of long-term coarsening of granular mixtures in rotating drums

Three fundamental segregation and pattern formation processes are known in granular mixtures in a rotating cylindrical drum: radial segregation, axial banding, and coarsening of the band pattern. While the mechanism for the first effect is well understood and for the second effect, several models have been proposed, the long-term coarsening mechanism remained unexplained so far. We demonstrate that the unidirectional flow between the bands in an axially segregated pattern is driven by small differences in size of the small beads at the band edges. Due to a process of microsegregation inside each band of small particles, which was so far unrecognized, this difference in diameter will be effective in all experiments with polydisperse beads. In consequence the stability of individual bands can be easily controlled by minor alterations of their composition. Our results make evident that a new mechanism as the driving force behind the axial particle flow has to be sought. We suggest possible hypotheses for such a mechanism.

cond-mat.soft↗

Non-universal Voronoi cell shapes in amorphous ellipsoid packings

In particulate systems with short-range interactions, such as granular matter or simple fluids, local structure plays a pivotal role in determining the macroscopic physical properties. Here, we analyse local structure metrics derived from the Voronoi diagram of configurations of oblate ellipsoids, for various aspect ratios $α$ and global volume fractions $ϕ_g$. We focus on jammed static configurations of frictional ellipsoids, obtained by tomographic imaging and by discrete element method simulations. In particular, we consider the local packing fraction $ϕ_l$, defined as the particle's volume divided by its Voronoi cell volume. We find that the probability $P(ϕ_l)$ for a Voronoi cell to have a given local packing fraction shows the same scaling behaviour as function of $ϕ_g$ as observed for random sphere packs. Surprisingly, this scaling behaviour is further found to be independent of the particle aspect ratio. By contrast, the typical Voronoi cell shape, quantified by the Minkowski tensor anisotropy index $β=β_0^{2,0}$, points towards a significant difference between random packings of spheres and those of oblate ellipsoids. While the average cell shape $β$ of all cells with a given value of $ϕ_l$ is very similar in dense and loose jammed sphere packings, the structure of dense and loose ellipsoid packings differs substantially such that this does not hold true. This non-universality has implications for our understanding of jamming of aspherical particles.

cond-mat.soft↗

Local origin of global contact numbers in frictional ellipsoid packings

In particulate soft matter systems the average number of contacts $Z$ of a particle is an important predictor of the mechanical properties of the system. Using X-ray tomography, we analyze packings of frictional, oblate ellipsoids of various aspect ratios $α$, prepared at different global volume fractions $ϕ_g$. We find that $Z$ is a monotonously increasing function of $ϕ_g$ for all $α$. We demonstrate that this functional dependence can be explained by a local analysis where each particle is described by its local volume fraction $ϕ_l$ computed from a Voronoi tessellation. $Z$ can be expressed as an integral over all values of $ϕ_l$: $Z(ϕ_g, α, X) = \int Z_l (ϕ_l, α, X) \; P(ϕ_l | ϕ_g) \; dϕ_l$. The local contact number function $ Z_l (ϕ_l, α, X)$ describes the relevant physics in term of locally defined variables only, including possible higher order terms $X$. The conditional probability $P(ϕ_l | ϕ_g)$ to find a specific value of $ϕ_l$ given a global packing fraction $ϕ_g$ is found to be independent of $α$ and $X$. Our results demonstrate that for frictional particles a local approach is not only a theoretical requirement but also feasible.

cond-mat.soft↗

Wetting heterogeneity in mixed-wet porous media controls flow dissipation

Pressure controlled displacement of an oil/water interface is studied in dense packings of functionalized glass beads with well-defined spatial wettability correlations. An enhanced dissipation is observed if the typical extension $ξ$ of the same-type wetting domains is smaller than the average bead diameter $d$. Three dimensional imaging using X-ray microtomography shows that the frequency $n(s)$ of residual droplet volumes $s$ for different $ξ$ collapse onto the same curve. This indicates that the additional dissipation for small $ξ$ is due to contact line pinning rather than an increase of capillary break-up/coalescence events.

physics.flu-dyn↗

Measuring the configurational temperature of a binary disc packing

Jammed packings of granular materials differ from systems normally described by statistical mechanics in that they are athermal. In recent years a statistical mechanics of static granular media has emerged where the thermodynamic temperature is replaced by a configurational temperature X which describes how the number of mechanically stable configurations depends on the volume. Four different methods have been suggested to measure X. Three of them are computed from properties of the Voronoi volume distribution, the fourth takes into account the contact number and the global volume fraction. This paper answers two questions using experimental binary disc packings: First we test if the four methods to measure compactivity provide identical results when applied to the same dataset. We find that only two of the methods agree quantitatively. Secondly, we test if X is indeed an intensive variable; this becomes true only for samples larger than roughly 200 particles. This result is shown to be due to recently found correlations between the particle volumes [Zhao et al., Europhys. Lett., 2012, 97, 34004].

cond-mat.soft↗

Granular transport in a horizontally vibrated sawtooth channel

We present a new mode of transport of spherical particles in a horizontally vibrated channel with sawtooth shaped side walls. The underlying driving mechanism is based on an interplay of directional energy injection transformed by the sidewall collisions and density dependent interparticle collisions. Experiments and matching numerics show that the average particle velocity reaches a maximum at 60% of the maximal filling density. Introducing a spatial phase shift between the channel boundaries increases the transport velocity by an order of magnitude.

cond-mat.stat-mech↗

Jammed frictional tetrahedra are hyperstatic

We prepare packings of frictional tetrahedra with volume fractions ϕ ranging from 0.469 to 0.622 using three different experimental protocols under isobaric conditions. Analysis via X-ray micro-tomography reveals that the contact number Z grows with ϕ, but does depend on the preparation protocol. While there exist four different types of contacts in tetrahedra packings, our analysis shows that the edge-to-face contacts contribute about 50% of the total increase in Z. The number of constraints per particle C increases also with ϕ and even the loosest packings are strongly hyperstatic i.e. mechanically over-determined with C approximately twice the degrees of freedom each particle possesses.

cond-mat.soft↗

Performance of Polarization-based Stereoscopy Screens

The screen is a key part of stereoscopic display systems using polarization to separate the different channels for each eye. The system crosstalk, characterizing the imperfection of the screen in terms of preserving the polarization of the incoming signal, and the scattering rate, characterizing the ability of the screen to deliver the incoming light to the viewers, determine the image quality of the system. Both values will depend on the viewing angle. In this work we measure the performance of three silver screens and three rear-projection screens. Additionally, we measure the surface texture of the screens using white-light interferometry. While part of our optical results can be explained by the surface roughness, more work is needed to understand the optical properties of the screens from a microscopic model.

physics.optics↗

Granular segregation in dense systems: the role of statistical mechanics and entropy

Granular segregation is ubiquitous in industrial, geological or daily-life context, but there is still no unifying theoretical approach. In this review, we examine two examples of granular segregation -- shallow rapid flows and rotating drums -- which suggest that the dynamics of systems at intermediate and high density might be amenable to a statistical mechanics approach.

cond-mat.soft↗

Correlation between Voronoi volumes in disc packings

We measure the two-point correlation of free Voronoi volumes in binary disc packings, where the packing fraction $ϕ_{\rm avg}$ ranges from 0.8175 to 0.8380. We observe short-ranged correlations over the whole range of $ϕ_{\rm avg}$ and anti-correlations for $ϕ_{\rm avg}>0.8277$. The spatial extent of the anti-correlation increases with $ϕ_{\rm avg}$ while the position of the maximum of the anti-correlation and the extent of the positive correlation shrink with $ϕ_{\rm avg}$. We conjecture that the onset of anti-correlation corresponds to dilatancy onset in this system.

cond-mat.stat-mech↗

Tailoring the frictional properties of granular media

A method of modifying the roughness of soda-lime glass spheres is presented, with the purpose of tuning inter-particle friction. The effect of chemical etching on the surface topography and the bulk frictional properties of grains is systematically investigated. The surface roughness of the grains is measured using white light interferometry and characterised by the lateral and vertical roughness length scales. The underwater angle of repose is measured to characterise the bulk frictional behaviour. We observe that the co-efficient of friction depends on the vertical roughness length scale. We also demonstrate a bulk surface roughness measurement using a carbonated soft drink.

cond-mat.stat-mech↗

Sound speed in water-saturated glass beads as a function of frequency and porosity

Sound propagation in water-saturated granular sediments is known to depend on the sediment porosity, but few data in the literature address both the frequency and porosity dependency. To begin to address this deficiency, a fluidized bed technique was used to control the porosity of an artificial sediment composed of glass spheres of 265 μm diameter. Time-of-flight measurements and the Fourier phase technique were utilized to determine the sound speed for frequencies from 300 to 800 kHz and porosities from 0.37 to 0.43. A Biot-based model qualitatively describes the porosity dependence.

cond-mat.soft↗

Shearing of frictional sphere packings

We measure shear response in packings of glass beads by pulling a thin, rough, metal plate vertically through a bed of volume fraction phi, which is set, before the plate is pulled, in the range 0.575 to 0.628. The yield stress is velocity independent over 4 decades and increases exponentially with phi, with a transition at phi approximately 0.595. An analysis of the measured force fluctuations indicates that the shear modulus is significantly smaller than the bulk modulus.

cond-mat.soft↗

Onset of mechanical stability in random packings of frictional spheres

Using sedimentation to obtain precisely controlled packings of noncohesive spheres, we find that the volume fraction $ϕ_{\rm RLP}$ of the loosest mechanically stable packing is in an operational sense well defined by a limit process. This random loose packing volume fraction decreases with decreasing pressure $p$ and increasing interparticle friction coefficient $μ$. Using X-ray tomography to correct for a container boundary effect that depends on particle size, we find for rough particles in the limit $p \to 0$ a new lower bound, $ϕ_{\rm RLP} = 0.550 \pm 0.001$.

cond-mat.soft↗

Influence of friction on granular segregation

Vertical shaking of a mixture of small and large beads can lead to segregation where the large beads either accumulate at the top of the sample, the so called Brazil Nut effect (BNE), or at the bottom, the Reverse Brazil Nut effect (RBNE). Here we demonstrate experimentally a sharp transition from the RBNE to the BNE when the particle coefficient of friction increases due to aging of the particles. This result can be explained by the two competing mechanisms of buoyancy and sidewall-driven convection, where the latter is assumed to grow in strength with increasing friction.

cond-mat.dis-nn↗

Geometry-induced asymmetric diffusion

Past work has shown that ions can pass through a membrane more readily in one direction than the other. We demonstrate here in a model and an experiment that for a mixture of small and large particles such asymmetric diffusion can arise solely from an asymmetry in the geometry of the pores of the membrane. Our deterministic simulation considers a two-dimensional gas of elastic disks of two sizes diffusing through a membrane, and our laboratory experiment examines the diffusion of glass beads of two sizes through a metal membrane. In both experiment and simulation, the membrane is permeable only to the smaller particles, and the asymmetric pores lead to an asymmetry in the diffusion rates of these particles. The presence of even a small percentage of large particles can clog a membrane, preventing passage of the small particles in one direction while permitting free flow of the small particles in the other direction. The purely geometric kinetic constraints may play a role in common biological contexts such as membrane ion channels.

cond-mat.soft↗