arXiv subjects

Maurice S. Skolnick

Publications and source records attributed to Maurice S. Skolnick.

At least 19 recordsLinked to original sources

arXiv2026

All-optical nonlinear phase modulation in open semiconductor microcavities

We report a significant advancement in ultra low power light-by-light phase modulation using open semiconductor microcavities in the strong light-matter coupling regime. We achieve cross-phase modulation of up to 247$\pm$17 mrad per particle between laser beams attenuated to single-photon average intensities. This breakthrough extends the potential for quantum information processing and nonlinear quantum optics in strongly coupled light-matter systems, setting a new benchmark in the field without relying on atom-like emitters. Our findings suggest promising new avenues for scalable quantum optical technologies.

physics.optics↗

arXiv2026

Observation of Electrically Tunable Chirality Inversion in a Slow-Light Waveguide

We identify chiral inversion points in slow-light, glide-plane-symmetric, photonic-crystal waveguides, defined as fixed locations where the local optical chirality changes sign over a narrow wavelength range. We experimentally access this behaviour using a waveguide-embedded InAs/InGaAs quantum dot. The slow-light spectral region is determined from time-integrated and time-resolved photoluminescence, and the dot exciton is electrically tuned across the slow-light bandwidth via the quantum-confined Stark effect. As the emission wavelength is swept through the slow-light region, the directional emission contrast shows a strong wavelength dependence and a sign reversal, consistent with the identified chiral inversion point. Numerical simulations attribute the switching primarily to the pronounced spectral variation of the local optical chirality for emitters displaced from the waveguide center. These results demonstrate on-demand electrical switching of chiral light-matter coupling in nanophotonic waveguides and enable tunable chiral interfaces for integrated quantum photonic devices.

physics.optics↗

arXiv2025

Flat-band compactons in a two-dimensional driven-dissipative Lieb lattice

We experimentally study the effect of inter-particle interactions on the flat-band states of a two-dimensional Lieb lattice with drive and dissipation. Exploiting the giant nonlinear interactions of exciton polaritons we observe compactly localised solitons (compactons) embedded within the continuum of propagating state bands -- a form of nonlinear bound state in the continuum (BIC). The driven-dissipative nature of the system leads to a sudden self-localisation into the compacton state above a threshold power. The experimental results agree well with numerical simulations. These results have implications for the physics of interacting quantum particles in flat-band systems and for generation of quantum-correlated light and spatially multiplexed coherent information transport.

cond-mat.other↗

arXiv2025

Electro-mechanically tunable, waveguide-coupled photonic-crystal cavities with embedded quantum dots

On-chip micro-cavities with embedded quantum emitters provide an excellent platform for high-performance quantum technologies. A major difficulty for such devices is overcoming the detrimental effects of fluctuations in the device dimensions caused by the limitations of the fabrication processes. We present a fully tunable system based on a 1D photonic-crystal cavity with an embedded quantum dot, which enables tuning of both the quantum dot emission energy and the cavity mode wavelength. A micro-electromechanical cantilever is used to tune the cavity mode wavelength via index modulation and the quantum-confined Stark effect is used to tune the quantum dot emission energy, mitigating the effect of fabrication imperfections. To demonstrate the operation of the device, a maximum, voltage-controllable cavity tuning range of $Δλ= 1.8$ nm is observed. This signal is measured at the end of a bus waveguide which side-couples to the cavity, enabling the coupling of multiple cavities to a common waveguide, a key requirement for scale-up in these systems. Additionally, a quantum dot is tuned into resonance with the cavity mode, exhibiting an enhanced emission rate with a resolution limited Purcell factor of $F_P = 3.5$.

physics.optics↗

arXiv2025

Waveguide Excitation and Spin Pumping of Chirally Coupled Quantum Dots

We report on an integrated semiconductor chip where a single quantum dot (QD) is excited in-plane via a photonic-crystal waveguide through its nearest p-shell optical transition. The chirality of the waveguide mode is exploited to achieve both directional absorption and directional emission, resulting in a substantial enhancement in directional contrast, as measured for the Zeeman components of the waveguide-coupled QD. This remote excitation scheme enables high directionality (greater than or equal to 0.95) across approximately 56% of the waveguide area, with significant overlap with the Purcell-enhanced region, where the electric field intensity profile is near its peak. In contrast, local excitation methods using an out-of-plane excitation beam focused directly over the area of the QD achieve only approximately 25% overlap. This enhancement increases the likelihood of locating Purcell-enhanced QDs in regions that support high directionality, enabling the experimental demonstration of a six-fold enhancement in the decay rate of a QD with greater than 90% directionality. The remote p-shell excitation protocol establishes a new benchmark for waveguide quantum optics in terms of the combination of Purcell enhancement and high directionality, thereby paving the way for on-chip excitation of spin-based solid-state quantum technologies in regimes of high beta-factor.

cond-mat.mes-hall↗

arXiv2025

Purcell-Enhanced, Directional Light-Matter Interaction in a Waveguide-Coupled Nanocavity

We demonstrate electrically tunable, spin-dependent, directional coupling of single photons by embedding quantum dots (QDs) in a waveguide-coupled nanocavity. The directional behavior arises from direction-dependent interference between two cavity modes when coupled to the device waveguides. The small mode volume cavity enables simultaneous Purcell enhancement (${10.8\pm0.7}$) and peak directional contrast (${88\pm1\%}$), exceeding current state-of-the-art waveguide-only systems. We also present a scattering matrix model for the transmission through this structure, alongside a quantum trajectory-based model for predicting the system's directionality, which we use to explain the observed asymmetry in directional contrast seen in QD devices. Furthermore, the nanocavity enables wide-range electrical tuning of the emitter's directional contrast. We present results showing precise tuning of a QD emission line from a directional contrast of ${2\%}$ to ${96\%}$. In combination, these characteristics make this cavity-waveguide approach promising for use as a building block in directional nanophotonic circuits.

physics.optics↗

arXiv2024

Optical Spin Initialisation and Readout with a Cavity-Coupled Quantum Dot in an In-Plane Magnetic Field

The spin of a charged semiconductor quantum dot (QD) coupled to an optical cavity is a promising candidate for high fidelity spin-photon interfaces; the cavity selectively modifies the decay rates of optical transitions such that spin initialisation, manipulation, and readout are all possible in a single magnetic field geometry. By performing cavity QED calculations, we show that a cavity with a single, linearly-polarised mode can simultaneously support both high-fidelity optical spin initialisation and readout in a single, in-plane (Voigt geometry) magnetic field. Furthermore, we demonstrate that single mode cavities always outperform bi-modal cavities in experimentally favourable driving regimes. Our analysis, when combined with established methods of control in a Voigt geometry field, provides optimal parameter regimes for high-fidelity initialisation and readout, and coherent control in both cavity configurations, providing insights for the design and development of QD spin-photon interfaces as the basis of quantum network nodes and for the generation of photonic graph states.

quant-ph↗

arXiv2024

Realization of Z$_2$ topological photonic insulators made from multilayer transition metal dichalcogenides

Monolayers of semiconducting transition metal dichalcogenides (TMDs) have long attracted interest for their intriguing optical and electronic properties. Recently TMDs in their quasi-bulk form have started to show considerable promise for nanophotonics thanks to their high refractive indices, large optical anisotropy, wide transparency windows reaching to the visible, and robust room temperature excitons promising for nonlinear optics. Adherence of TMD layers to any substrate via van der Waals forces is a further key enabler for nanofabrication of sophisticated photonic structures requiring heterointegration. Here, we capitalize on these attractive properties and realize topological spin-Hall photonic lattices made of arrays of triangular nanoholes in 50 to 100 nm thick WS$_2$ flakes exfoliated on SiO$_2$/Si substrates. High quality structures are achieved taking advantage of anisotropic dry etching dictated by the crystal axes of WS$_2$. Reflectance measurements at room temperature show a photonic gap opening in the near-infrared in trivial and topological phases. Unidirectional propagation along the domain interface is demonstrated in real space via circularly polarized laser excitation in samples with both zigzag and armchair domain boundaries. Finite-difference time-domain simulations are used to interpret optical spectroscopy results. Our work opens the way for future sophisticated nanophotonic devices based on the layered (van der Waals) materials platform.

physics.optics↗

arXiv2024

Electrostatic control of nonlinear photonic-crystal polaritons in a monolayer semiconductor

Integration of 2D semiconductors with photonic crystal slabs provides an attractive approach to achieve strong light--matter coupling and exciton-polariton formation in a planar chip-compatible geometry. However, for the development of practical devices, it is crucial that the polariton excitations in the structure are easily tunable and exhibit strong nonlinear response. Here we study neutral and charged exciton-polaritons in an electrostatically gated planar photonic crystal slab with an embedded monolayer semiconductor MoSe$_2$ and experimentally demonstrate strong polariton nonlinearity, which can be tuned via gate voltage. We find that modulation of dielectric environment within the photonic crystal results in the formation of two distinct resonances with significantly different nonlinear response, which enables optical switching with ultrashort laser pulses. Our results open new avenues towards development of active polaritonic devices in a compact chip-compatible implementation.

cond-mat.mes-hall↗

arXiv2023

Purcell-Enhanced Single Photons at Telecom Wavelengths from a Quantum Dot in a Photonic Crystal Cavity

Quantum dots are promising candidates for telecom single photon sources due to their tunable emission across the different low-loss telecommunications bands, making them compatible with existing fiber networks. Their suitability for integration into photonic structures allows for enhanced brightness through the Purcell effect, supporting efficient quantum communication technologies. Our work focuses on InAs/InP QDs created via droplet epitaxy MOVPE to operate within the telecoms C-band. We observe a short radiative lifetime of 340 ps, arising from a Purcell factor of 5, owing to interaction of the QD within a low-mode-volume photonic crystal cavity. Through in-situ control of the sample temperature, we show both temperature tuning of the QD's emission wavelength and a preserved single photon emission purity at temperatures up to 25K. These findings suggest the viability of QD-based, cryogen-free, C-band single photon sources, supporting applicability in quantum communication technologies.

quant-ph↗

arXiv2023

Probing and control of guided exciton-polaritons in a 2D semiconductor-integrated slab waveguide

Guided 2D exciton-polaritons, resulting from the strong coupling of excitons in semiconductors with non-radiating waveguide modes, provide an attractive approach towards developing novel on-chip optical devices. These quasiparticles are characterized by long propagation distances and efficient nonlinear interaction but cannot be directly accessed from the free space. Here we demonstrate a powerful approach for probing and manipulating guided polaritons in a Ta2O5 slab integrated with a WS2 monolayer using evanescent coupling through a high-index solid immersion lens. Tuning the nanoscale lens-sample gap allows for extracting all the intrinsic parameters of the system. We also demonstrate the transition from weak to strong coupling accompanied by the onset of the motional narrowing effect: with the increase of exciton-photon coupling strength, the inhomogeneous contribution to polariton linewidth, inherited from the exciton resonance, becomes fully lifted. Our results enable the development of integrated optics employing room-temperature exciton-polaritons in 2D semiconductor-based structures.

physics.optics↗

arXiv2023

Observation of Zitterbewegung in photonic microcavities

We present and experimentally study the effects of the photonic spin-orbit coupling on real space propagetion of polariton wavepackets in planar semiconductor microcavities and polaritonic analogs of graphene. In particular, we demonstrate the appearance of an analog Zitterbewegung effect, a term which translates as 'trembling motion' in english, which was originally proposed for relativistic Dirac electrons and consists of the oscillations of the center of mass of a wavepacket in the direction perpendicular to its propagation. For a planar microcavity we observe regular Zitterbewegung oscillations whose amplitude and period depend on the wavevector of the polaritons. We then extend these results to a honeycomb lattice of coupled microcavity resonators. Compared to the planar cavity such lattices are inherently more tuneable and versatile, allowing simulation of the Hamilitonians of a wide range of important physical systems. We observe an oscillation pattern related to the presence of the spin-split Dirac cones in the dispersion. In both cases the experimentally observed oscillations are in good agreement with theoretical modelling and independently measured bandstructure parameters, providing strong evidence for the observation of Zitterbewegung.

physics.optics↗

arXiv2022

Polariton lasing in AlGaN microring with GaN/AlGaN quantum wells

Microcavity polaritons are strongly interacting hybrid light-matter quasiparticles, which are promising for the development of novel light sources and active photonic devices. Here, we report polariton lasing in the UV spectral range in microring resonators based on GaN/AlGaN slab waveguides, with experiments carried out from 4 K up to room temperature. Stimulated polariton relaxation into multiple ring resonator modes is observed, which exhibit threshold-like dependence of the emission intensity with pulse energy. The strong exciton-photon coupling regime is confirmed by the significant reduction of the free spectral range with energy and the blueshift of the exciton-like modes with increasing pulse energy. Importantly, the exciton emission shows no broadening with power, further confirming that lasing is observed at electron-hole densities well below the Mott transition. Overall, our work paves the way towards development of novel UV devices based on the high-speed slab waveguide polariton geometry operating up to room temperature with potential to be integrated into complex photonic circuits.

physics.optics↗

arXiv2022

Observation of large spontaneous emission rate enhancement of quantum dots in a broken-symmetry slow-light waveguide

Quantum states of light and matter can be manipulated on the nanoscale to provide a technological resource for aiding the implementation of scalable photonic quantum technologies [1-3]. Experimental progress relies on the quality and efficiency of the coupling between photons and internal states of quantum emitters [4-6]. Here we demonstrate a nanophotonic waveguide platform with embedded quantum dots (QDs) that enables both Purcell-enhanced emission and strong chiral coupling. The design uses slow-light effects in a glide-plane photonic crystal waveguide with QD tuning to match the emission frequency to the slow-light region. Simulations were used to map the chirality and Purcell enhancement depending on the position of a dipole emitter relative to the air holes. The highest Purcell factors and chirality occur in separate regions, but there is still a significant area where high values of both can be obtained. Based on this, we first demonstrate a record large radiative decay rate of 17 ns^-1 (60 ps lifetime) corresponding to a 20 fold Purcell enhancement. This was achieved by electric-field tuning of the QD to the slow-light region and quasi-resonant phonon-sideband excitation. We then demonstrate a 5 fold Purcell enhancement for a dot with high degree of chiral coupling to waveguide modes, substantially surpassing all previous measurements. Together these demonstrate the excellent prospects for using QDs in scalable implementations of on-chip spin-photonics relying on chiral quantum optics.

physics.optics↗

arXiv2021

Few-photon all-optical phase rotation in a quantum-well micropillar cavity

Photonic platforms are an excellent setting for quantum technologies because weak photon-environment coupling ensures long coherence times. The second key ingredient for quantum photonics is interactions between photons, which can be provided by optical nonlinearities in the form of cross-phase-modulation (XPM). This approach underpins many proposed applications in quantum optics and information processing, but achieving its potential requires strong single-photon-level nonlinear phase shifts and also scalable nonlinear elements. In this work we show that the required nonlinearity can be provided by exciton-polaritons in micropillars with embedded quantum wells. These combine the strong interactions of excitons with the scalability of micrometer-sized emitters. We observe XPM up to $3 \pm 1$ mrad per particle using laser beams attenuated to below single photon average intensity. With our work serving as a first stepping stone, we lay down a route for quantum information processing in polaritonic lattices.

physics.optics↗

arXiv2021

Ultrafast-nonlinear ultraviolet pulse modulation in an AlInGaN polariton waveguide operating up to room temperature

Ultrafast nonlinear photonics enables a host of applications in advanced on-chip spectroscopy and information processing. These rely on a strong intensity dependent (nonlinear) refractive index capable of modulating optical pulses on sub-picosecond timescales and on length scales suitable for integrated photonics. Currently there is no platform that can provide this for the UV spectral range where broadband spectra generated by nonlinear modulation can pave the way to new on-chip ultrafast (bio-) chemical spectroscopy devices. We demonstrate the giant nonlinearity of UV hybrid light-matter states (exciton-polaritons) up to room temperature in an AlInGaN waveguide. We experimentally measure ultrafast nonlinear spectral broadening of UV pulses in a compact 100 $μ$m long device and deduce a nonlinearity 1000 times that in common UV nonlinear materials and comparable to non-UV polariton devices. Our demonstration promises to underpin a new generation of integrated UV nonlinear light sources for advanced spectroscopy and measurement.

physics.optics↗

arXiv2020

Chiral topological photonics with an embedded quantum emitter

Topological photonic interfaces support topologically non-trivial optical modes with helical character. When combined with an embedded quantum emitter that has a circularly polarised transition dipole moment, a chiral quantum optical interface is formed due to spin-momentum locking. Here, we experimentally realise such an interface by integrating semiconductor quantum dots into a valley-Hall topological photonic crystal waveguide. We harness the robust waveguide transport to create a ring resonator which supports helical modes. Chiral coupling of quantum dot transitions, with directional contrast as high as $75\%$, is demonstrated. The interface also supports a topologically trivial mode, comparison with which allows us to clearly demonstrate the protection afforded by topology to the non-trivial mode.

physics.optics↗

arXiv2020

Photon Statistics of Filtered Resonance Fluorescence

Spectral filtering of resonance fluorescence is widely employed to improve single photon purity and indistinguishability by removing unwanted backgrounds. For filter bandwidths approaching the emitter linewidth, complex behaviour is predicted due to preferential transmission of components with differing photon statistics. We probe this regime using a Purcell-enhanced quantum dot in both weak and strong excitation limits, finding excellent agreement with an extended sensor theory model. By changing only the filter width, the photon statistics can be transformed between antibunched, bunched, or Poissonian. Our results verify that strong antibunching and a sub-natural linewidth cannot simultaneously be observed, providing new insight into the nature of coherent scattering.

quant-ph↗