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Mauro Sbragaglia

Publications and source records attributed to Mauro Sbragaglia.

At least 55 records · Page 3Linked to original sources

Convective heat transfer of a model emulsion at the droplet scale

We numerically study the Rayleigh-Bénard (RB) convection in two-dimensional model emulsions confined between two parallel walls at fixed temperatures. The systems under study are heterogeneous, with finite-size droplets dispersed in a continuous phase. The droplet concentration is chosen to explore the convective heat transfer of both Newtonian (low droplet concentration) and non-Newtonian (high droplet concentration) emulsions, the latter exhibiting shear-thinning rheology, with a noticeable increase of viscosity at low shear rates. It is well known that the transition to convection of a homogeneous Newtonian system is accompanied by the onset of steady flow and time-independent heat flux; in marked contrast, the heterogeneity of emulsions brings in an additional and previously unexplored phenomenology. As a matter of fact, when the droplet concentration increases, we observe that the heat transfer process is mediated by a non-steady flow, with neat heat-flux fluctuations, obeying a non-Gaussian statistics. The observed findings are ascribed to the emergence of space correlations among distant droplets, which we highlight via direct measurements of the droplets displacement and the characterisation of the associated correlation functions.

physics.flu-dyn↗

Rayleigh-Bénard convection of a model emulsion: anomalous heat-flux fluctuations and finite-size droplets effects

We present mesoscale numerical simulations of Rayleigh-Bénard (RB) convection in a two-dimensional model emulsion. The systems under study are constituted of finite-size droplets, whose concentration Phi_0 is systematically varied from small (Newtonian emulsions) to large values (non-Newtonian emulsions). We focus on the characterisation of the heat transfer properties close to the transition from conductive to convective states, where it is known that a homogeneous Newtonian system exhibits a steady flow and a time-independent heat flux. In marked contrast, emulsions exhibit a non-steady dynamics with fluctuations in the heat flux. In this paper, we aim at the characterisation of such non-steady dynamics via detailed studies on the time-averaged heat flux and its fluctuations. To understand the time-averaged heat flux, we propose a side-by-side comparison between the emulsion system and a single-phase (SP) system, whose viscosity is constructed from the shear rheology of the emulsion. We show that such local closure works well only when a suitable degree of coarse-graining (at the droplet scale) is introduced in the local viscosity. To delve deeper into the fluctuations in the heat flux, we propose a side-by-side comparison between a Newtonian emulsion and a non-Newtonian emulsion, at fixed time-averaged heat flux. This comparison elucidates that finite-size droplets and the non-Newtonian rheology cooperate to trigger enhanced heat-flux fluctuations at the droplet scales. These enhanced fluctuations are rooted in the emergence of space correlations among distant droplets, which we highlight via direct measurements of the droplets displacement and the characterisation of the associated correlation function. The observed findings offer insights on heat transfer properties for confined systems possessing finite-size constituents.

physics.flu-dyn↗

Lattice Boltzmann simulations on the tumbling to tank-treading transition: effects of membrane viscosity

The tumbling to tank-treading (TB-TT) transition for red blood cells (RBCs) has been widely investigated, with a main focus on the effects of the viscosity ratio $λ$ (i.e., the ratio between the viscosities of the fluids inside and outside the membrane) and the shear rate $\dotγ$ applied to the RBC. However, the membrane viscosity $μ_m$ plays a major role in a realistic description of RBC's dynamics, and only a few works have systematically focused on its effects on the TB-TT transition. In this work, we provide a parametric investigation on the effect of membrane viscosity $μ_m$ on the TB-TT transition, for a single RBC. It is found that, at fixed viscosity ratios $λ$, larger values of $μ_m$ lead to an increased range of values of capillary number at which the TB-TT transition occurs. We systematically quantify such an increase by means of mesoscale numerical simulations based on the lattice Boltzmann models.

cond-mat.soft↗

Lattice Boltzmann simulations of droplet breakup in confined and time-dependent flows

We study droplet dynamics and breakup in generic time-dependent flows via a multicomponent Lattice Boltzmann algorithm, with emphasis on flow start up conditions. We first study droplet breakup in a confined oscillatory shear flow via two different protocols. In one set up, we start from an initially spherical droplet and turn on the flow abruptly ("shock method"); in the other protocol, we start from an initially spherical droplet as well, but we progressively increase the amplitude of the flow, by allowing the droplet to relax to the steady state for each increase in amplitude, before increasing the flow amplitude again ("relaxation method"). The two protocols are shown to produce substantially different breakup scenarios. The mismatch between these two protocols is also studied for variations in the flow topology, the degree of confinement and the inertia of the fluid. All results point to the fact that under extreme conditions of confinement the relaxation protocols can drive the droplets into metastable states, which break only for very intense flow amplitudes, but their stability is prone to external perturbations, such as an oscillatory driving force.

physics.flu-dyn↗

Unified theoretical and experimental view on transient shear banding

Dense emulsions, colloidal gels, microgels, and foams all display a solid-like behavior at rest characterized by a yield stress, above which the material flows like a liquid. Such a fluidization transition often consists of long-lasting transient flows that involve shear-banded velocity profiles. The characteristic time for full fluidization, $τ_\text{f}$, has been reported to decay as a power-law of the shear rate $\dot γ$ and of the shear stress $σ$ with respective exponents $α$ and $β$. Strikingly, the ratio of these exponents was empirically observed to coincide with the exponent of the Herschel-Bulkley law that describes the steady-state flow behavior of these complex fluids. Here we introduce a continuum model, based on the minimization of a "free energy", that captures quantitatively all the salient features associated with such \textit{transient} shear-banding. More generally, our results provide a unified theoretical framework for describing the yielding transition and the steady-state flow properties of yield stress fluids.

cond-mat.soft↗

Hydrodynamic behavior of the Pseudo-Potential lattice Boltzmann method for interfacial flows

The lattice Boltzmann method (LBM) is routinely employed in the simulation of complex multiphase flows comprising bulk phases separated by non-ideal interfaces. LBM is intrinsically mesoscale with an hydro-dynamic equivalence popularly set by the Chapman-Enskog analysis, requiring that fields slowly vary in space and time. The latter assumptions become questionable close to interfaces, where the method is also known to be affected by spurious non hydrodynamical contributions. This calls for quantitative hydrodynamical checks. In this paper we analyze the hydrodynamic behaviour of LBM pseudo-potential models for the problem of break-up of a liquid ligament triggered by the Plateau-Rayleigh instability. Simulations are performed at fixed interface thickness, while increasing the ligament radius, i.e. in the "sharp interface" limit. Influence of different LBM collision operators is also assessed. We find that different distributions of spurious currents along the interface may change the outcome of the pseudo-potential model simulations quite sensibly, which suggests that a proper fine-tuning of pseudo-potential models in time-dependent problems is needed before the utilization in concrete applications. Taken all together, we argue that the results of the proposed study provide a valuable insight for engineering pseudo-potential model applications involving the hydrodynamics of liquid jets.

physics.comp-ph↗

Ligament break-up simulation through pseudo-potential Lattice Boltzmann Method

The Plateau-Rayleigh instability causes the fragmentation of a liquid ligament into smaller droplets. In this study a numerical study of this phenomenon based on a single relaxation time (SRT) pseudo-potential lattice Boltzmann method (LBM) is proposed. If systematically analysed, this test case allows to design appropriate parameters sets to deal with engineering applications involving the hydrodynamics of a jet. Grid convergence simulations are performed in the limit where the interface thickness is asymptotically smaller than the characteristic size of the ligament. These simulations show a neat asymptotic behaviour, possibly related to the convergence of LBM diffuse-interface physics to sharp interface hydrodynamics.

physics.comp-ph↗

Avalanche statistics during coarsening dynamics

We study the coarsening dynamics of a two dimensional system via lattice Boltzmann numerical simulations. The system under consideration is a biphasic system consisting of domains of a dispersed phase closely packed together in a continuous phase and separated by thin interfaces. Such system is elastic and typically out of equilibrium. The equilibrium state is attained via the coarsening dynamics, wherein the dispersed phase slowly diffuses through the interfaces, causing domains to change in size and eventually rearrange abruptly. The effect of rearrangements is propagated throughout the system via the intrinsic elastic interactions and may cause rearrangements elsewhere, resulting in intermittent bursts of activity and avalanche behaviour. Here we aim at quantitatively characterizing the corresponding avalanche statistics (i.e. size, duration, inter-avalanche time). Despite the coarsening dynamics is triggered by an internal driving mechanism, we find quantitative indications that such avalanche statistics displays scaling-laws very similar to those observed in the response of disordered materials to external loads.

cond-mat.soft↗

A numerical tool for the study of the hydrodynamic recovery of the Lattice Boltzmann Method

We investigate the hydrodynamic recovery of Lattice Boltzmann Method (LBM) by analyzing exact balance relations for energy and enstrophy derived from averaging the equations of motion on sub-volumes of different sizes. In the context of 2D isotropic homogeneous turbulence, we first validate this approach on decaying turbulence by comparing the hydrodynamic recovery of an ensemble of LBM simulations against the one of an ensemble of Pseudo-Spectral (PS) simulations. We then conduct a benchmark of LBM simulations of forced turbulence with increasing Reynolds number by varying the input relaxation times of LBM. This approach can be extended to the study of implicit subgrid-scale (SGS) models, thus offering a promising route to quantify the implicit SGS models implied by existing stabilization techniques within the LBM framework.

physics.comp-ph↗

Effects of thermal fluctuations in the fragmentation of a nano-ligament

We study the effects of thermally induced capillary waves in the fragmentation of a liquid ligament into multiple nano-droplets. Our numerical implementation is based on a fluctuating lattice Boltzmann (LB) model for non-ideal multicomponent fluids, including non-equilibrium stochastic fluxes mimicking the effects of molecular forces at the nanoscales. We quantitatively analyze the statistical distribution of the break-up times and the droplet volumes after the fragmentation process, at changing the two relevant length scales of the problem, i.e., the thermal length-scale and the ligament size. The robustness of the observed findings is also corroborated by quantitative comparisons with the predictions of sharp interface hydrodynamics. Beyond the practical importance of our findings for nanofluidic engineering devices, our study also explores a novel application of LB in the realm of nanofluidic phenomena.

physics.flu-dyn↗

Lattice Boltzmann Simulations of Non-Equilibrium Fluctuations in a Non-Ideal Binary Mixture

In the recent years the lattice Boltzmann (LB) methodology has been fruitfully extended to include the effects of thermal fluctuations. So far, all studied cases pertain equilibrium fluctuations, i.e. fluctuations with respect to an equilibrium background state. In this paper we take a step further and present results of fluctuating LB simulations of a binary mixture confined between two parallel walls in presence of a constant concentration gradient in the wall-to-wall direction. This is a paradigmatic set-up for the study of non-equilibrium (NE) fluctuations, i.e. fluctuations with respect to a non- equilibrium state. We analyze the dependence of the structure factors for the hydrodynamical fields on the wave vector $\boldsymbol{q}$ in both the directions parallel and perpendicular to the walls, as well as the finite-size effects induced by confinement, highlighting the long-range ($\sim |\boldsymbol{q}|^{-4}$) nature of correlations in the NE framework. Results quantitatively agree with the predictions of fluctuating hydrodynamics. Moreover, in presence of a non-ideal (NI) equation of state of the mixture, we also observe that the (spatially homogeneous) average pressure changes, due to a genuinely new contribution triggered by the long-range nature of NE fluctuations. These NE pressure effects are studied at changing the system size and the concentration gradient. Taken all together, we argue that these findings are instrumental to boost the applicability of the fluctuating LB methodology in the framework of NE fluctuations, possibly in conjunction with experiments.

physics.comp-ph↗

Metastability at the Yield-Stress Transition in Soft Glasses

We study the solid-to-liquid transition in a two-dimensional fully periodic soft-glassy model with an imposed spatially heterogeneous stress. The model we consider consists of droplets of a dispersed phase jammed together in a continuous phase. When the peak value of the stress gets close to the yield stress of the material, we find that the whole system intermittently tunnels to a metastable "fluidized" state, which relaxes back to a metastable "solid" state by means of an elastic-wave dissipation. This macroscopic scenario is studied through the microscopic displacement field of the droplets, whose time statistics displays a remarkable bimodality. Metastability is rooted in the existence, in a given stress range, of two distinct stable rheological branches as well as long-range correlations (e.g., large dynamic heterogeneity) developed in the system. Finally, we show that a similar behavior holds for a pressure-driven flow, thus suggesting possible experimental tests.

cond-mat.soft↗

Droplet breakup driven by shear thinning solutions in a microfluidic T-Junction

Droplet-based microfluidics turned out to be an efficient and adjustable platform for digital analysis, encapsulation of cells, drug formulation, and polymerase chain reaction. Typically, for most biomedical applications, the handling of complex, non-Newtonian fluids is involved, e.g. synovial and salivary fluids, collagen, and gel scaffolds. In this study we investigate the problem of droplet formation occurring in a microfluidic T-shaped junction, when the continuous phase is made of shear thinning liquids. At first, we review in detail the breakup process providing extensive, side-by-side comparisons between Newtonian and non-Newtonian liquids over unexplored ranges of flow conditions and viscous responses. The non-Newtonian liquid carrying the droplets is made of Xanthan solutions, a stiff rod-like polysaccharide displaying a marked shear thinning rheology. By defining an effective Capillary number, a simple yet effective methodology is used to account for the shear-dependent viscous response occurring at the breakup. The droplet size can be predicted over a wide range of flow conditions simply by knowing the rheology of the bulk continuous phase. Experimental results are complemented with numerical simulations of purely shear thinning fluids using Lattice Boltzmann models. The good agreement between the experimental and numerical data confirm the validity of the proposed rescaling with the effective Capillary number.

cond-mat.soft↗

A one dimensional modal approach for flows controlled by contact line motion

The hydrodynamics of a liquid-vapour interface in contact with an heterogeneous surface is largely impacted by the presence of defects at the smaller scales. Such defects introduce morphological disturbances on the contact line and ultimately determine the force exerted on the wedge of liquid in contact with the surface. From the mathematical point of view, defects introduce perturbation modes, whose space-time evolution is governed by the interfacial hydrodynamic equations of the contact line. In this paper we derive the response function of the contact line to such generic perturbations. The contact line response may be used to design simplified 1+1 dimensional models accounting for the complexity of interfacial flows coupled to nanoscale defects, yet offering a more tractable mathematical framework to include thermal fluctuations and explore thermally activated contact line motion through a disordered energy landscape.

physics.flu-dyn↗

Stretching of viscoelastic drops by steady sliding

The sliding of non-Newtonian drops down planar surfaces results in a complex, entangled balance between interfacial forces and non linear viscous dissipation, which has been scarcely inspected. In particular, a detailed understanding of the role played by the polymer flexibility and the resulting elasticity of the polymer solution is still lacking. To this aim, we have considered polyacrylamide (PAA) solutions of different molecular weights, suspended either in water or glycerol/water mixtures. In contrast to drops with stiff polymers, drops with flexible polymers exhibit a remarkable elongation in steady sliding. This difference is most likely attributed to different viscous bending as a consequence of different shear thinning. Moreover, an "optimal elasticity" of the polymer seems to be required for this drop elongation to be visible. We have complemented experimental results with numerical simulations of a viscoelastic FENE-P drop. This has been a decisive step to unravel how a change of the elastic parameters (e.g. polymer relaxation time, maximum extensibility) affects the dimensionless sliding velocity.

cond-mat.soft↗

Deformation and break-up of viscoelastic droplets Using Lattice Boltzmann Models

We investigate the break-up of Newtonian/viscoelastic droplets in a viscoelastic/Newtonian matrix under the hydrodynamic conditions of a confined shear flow. Our numerical approach is based on a combination of Lattice-Boltzmann models (LBM) and Finite Difference (FD) schemes. LBM are used to model two immiscible fluids with variable viscosity ratio (i.e. the ratio of the droplet to matrix viscosity); FD schemes are used to model viscoelasticity, and the kinetics of the polymers is introduced using constitutive equations for viscoelastic fluids with finitely extensible non-linear elastic dumbbells with Peterlin's closure (FENE-P). We study both strongly and weakly confined cases to highlight the role of matrix and droplet viscoelasticity in changing the droplet dynamics after the startup of a shear flow. Simulations provide easy access to quantities such as droplet deformation and orientation and will be used to quantitatively predict the critical Capillary number at which the droplet breaks, the latter being strongly correlated to the formation of multiple neckings at break-up. This study complements our previous investigation on the role of droplet viscoelasticity (A. Gupta \& M. Sbragaglia, {\it Phys. Rev. E} {\bf 90}, 023305 (2014)), and is here further extended to the case of matrix viscoelasticity.

cond-mat.soft↗

A Lattice Boltzmann study of the effects of viscoelasticity on droplet formation in microfluidic cross-junctions

Based on mesoscale lattice Boltzmann (LB) numerical simulations, we investigate the effects of viscoelasticity on the break-up of liquid threads in microfluidic cross-junctions, where droplets are formed by focusing a liquid thread of a dispersed (d) phase into another co-flowing continuous (c) immiscible phase. Working at small Capillary numbers, we investigate the effects of non-Newtonian phases in the transition from droplet formation at the cross-junction (DCJ) to droplet formation downstream of the cross-junction (DC) (Liu $\&$ Zhang, ${\it Phys. ~Fluids.}$ ${\bf 23}$, 082101 (2011)). We will analyze cases with ${\it Droplet ~Viscoelasticity}$ (DV), where viscoelastic properties are confined in the dispersed phase, as well as cases with ${\it Matrix ~Viscoelasticity}$ (MV), where viscoelastic properties are confined in the continuous phase. Moderate flow-rate ratios $Q \approx {\cal O}(1)$ of the two phases are considered in the present study. Overall, we find that the effects are more pronounced in the case with MV, where viscoelasticity is found to influence the break-up point of the threads, which moves closer to the cross-junction and stabilizes. This is attributed to an increase of the polymer feedback stress forming in the corner flows, where the side channels of the device meet the main channel. Quantitative predictions on the break-up point of the threads are provided as a function of the Deborah number, i.e. the dimensionless number measuring the importance of viscoelasticity with respect to Capillary forces.

physics.flu-dyn↗

Effects of viscoelasticity on droplet dynamics and break-up in microfluidic T-Junctions: a lattice Boltzmann study

The effects of viscoelasticity on the dynamics and break-up of fluid threads in microfluidic T-junctions are investigated using numerical simulations of dilute polymer solutions at changing the Capillary number ($\mbox {Ca}$), i.e. at changing the balance between the viscous forces and the surface tension at the interface, up to $\mbox{Ca} \approx 3 \times 10^{-2}$. A Navier-Stokes (NS) description of the solvent based on the lattice Boltzmann models (LBM) is here coupled to constitutive equations for finite extensible non-linear elastic dumbbells with the closure proposed by Peterlin (FENE-P model). We present the results of three-dimensional simulations in a range of $\mbox{Ca}$ which is broad enough to characterize all the three characteristic mechanisms of breakup in the confined T-junction, i.e. ${\it squeezing}$, ${\it dripping}$ and ${\it jetting}$ regimes. The various model parameters of the FENE-P constitutive equations, including the polymer relaxation time $τ_P$ and the finite extensibility parameter $L^2$, are changed to provide quantitative details on how the dynamics and break-up properties are affected by viscoelasticity. We will analyze cases with ${\it Droplet ~Viscoelasticity}$ (DV), where viscoelastic properties are confined in the dispersed (d) phase, as well as cases with ${\it Matrix ~Viscoelasticity}$ (MV), where viscoelastic properties are confined in the continuous (c) phase. Moderate flow-rate ratios $Q \approx {\cal O}(1)$ of the two phases are considered in the present study. Overall, we find that the effects are more pronounced in the case with MV, as the flow driving the break-up process upstream of the emerging thread can be sensibly perturbed by the polymer stresses.

physics.flu-dyn↗