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Maxim R. Shcherbakov

Publications and source records attributed to Maxim R. Shcherbakov.

17 recordsLinked to original sources
arXiv2026

Multifunctional Barophotonic Control of Resonators and Metasurfaces

Actively tunable nanophotonic platforms that control light-matter interactions enable reconfigurable optical systems and programmable photonic integrated circuits. Hydrostatic pressure provides a noninvasive and material-agnostic mechanism for modulating the refractive index and resonance conditions without introducing free carriers or structural damage. Here, we demonstrate multiple pressure-dependent functionalities in silicon nitride nanostructures, including resonance tuning, refractive index modulation, and polarization state conversion. Applying a pressure of up to 5 GPa, we observe a Fabry-P\'erot resonance shift of up to 30 nm and a relative refractive index decrease of up to 4%. Based on the results, we design and examine, to the best of our knowledge, the first extreme-pressure-tunable, polarization-converting metasurface, which tunes the ellipticity and orientation angle of the output light. These findings establish pressure-controllable silicon nitride as a viable platform for reconfigurable photonics and extreme-environment nanophotonic systems, including deep-ocean exploration, planetary interiors, and space applications.

physics.optics↗
arXiv2026

Second-Harmonic Generation at a Fourth-Order Exceptional Point Degeneracy

An anomalous flat-band dispersion provided by a degenerate band edge (DBE) of longitudinal optical modes in a double-grating waveguide is used to enhance second-harmonic generation (SHG). The DBE is a fourth-order exceptional point degeneracy (EPD) in a lossless and gainless waveguide, characterized by the coalescence of four eigenmodes that establish a frozen mode in a cavity. At a DBE resonance, the cavity quality factor scales $Q\propto N^5$, where $N$ is the number of unit cells of the grating waveguide. In our numerical experiments, we observe the peak intensity of the fundamental field in the edge-excited cavity scaling as $I_1\propto N^{3.6}$. This leads to a highly efficient SHG process that is radiated vertically from the cavity (i.e., normal to the grating) without requiring collinear phase matching, with a conversion efficiency scaling as $\eta\propto N^{8.27}$. These results establish DBE-based waveguides as promising platforms for miniaturized efficient nonlinear photonic devices.

physics.optics↗
arXiv2025

Highly Tunable Phonon Polaritons via Metal Intercalation

Phonon polaritons in van der Waals crystals offer mid-infrared light confinement deep below the diffraction limit, making them promising for nanophotonics applications. However, the practical use of phonon polaritons remains limited, in part due to the lack of precise control over the phonon polariton dispersion, as crystal lattice vibrations are often inert to external stimuli. Here, we address this challenge by zerovalent metal intercalation of $\alpha$-MoO$_3$. Photo-induced force microscopy shows that introducing tin into the van der Waals gap modulates the phonon polariton dispersion by up to $38.5\pm0.5\%$, which is the highest amount of tunability among non-mechanical modulation approaches, to the best of our knowledge. Intercalation with various metal species preserves the phonon polariton lifetimes, while modulating the dielectric permittivity in agreement with the density functional theory and analytical calculations. Our results establish metal intercalation as a practical route to reconfigurable mid-infrared nanophotonics.

cond-mat.mtrl-sci↗
arXiv2024

Site-Controlled Purcell-Induced Bright Single Photon Emitters in Hexagonal Boron Nitride

Single photon emitters (SPEs) hosted in hexagonal boron nitride (hBN) are essential elementary building blocks for enabling future on-chip quantum photonic technologies that operate at room temperature. However, fundamental challenges, such as managing non-radiative decay, competing incoherent processes, as well as engineering difficulties in achieving deterministic placement and scaling of the emitters, limit their full potential. In this work, we experimentally demonstrate large-area arrays of plasmonic nanoresonators for Purcell-induced site-controlled SPEs by engineering emitter-cavity coupling and enhancing radiative emission at room temperature. The plasmonic nanoresonator architecture consists of gold-coated silicon pillars capped with an alumina spacer layer, enabling a 10-fold local field enhancement in the emission band of native hBN defects. Confocal photoluminescence and second-order autocorrelation measurements show bright SPEs with sub-30 meV bandwidth and a saturated emission rate of more than 3.8 million counts per second. We measure a Purcell factor of 4.9, enabling average SPE lifetimes of 480 ps, a five-fold reduction as compared to emission from gold-free devices, along with an overall SPE yield of 21%. Density functional theory calculations further reveal the beneficial role of an alumina spacer between defected hBN and gold, as an insulating layer can mitigate the electronic broadening of emission from defects proximal to gold. Our results offer arrays of bright, heterogeneously integrated quantum light sources, paving the way for robust and scalable quantum information systems.

physics.optics↗
arXiv2024

Arbitrary control over multimode wave propagation for machine learning

Controlled multimode wave propagation can enable more space-efficient photonic processors than architectures based on discrete components connected by single-mode waveguides. Instead of defining discrete elements, one can sculpt the continuous substrate of a photonic processor to perform computations through multimode interference in two dimensions. Here we designed and demonstrated a device with a refractive index that can be rapidly reprogrammed across space, allowing arbitrary control of wave propagation. The device, a two-dimensional programmable waveguide, uses parallel electro-optic modulation of the refractive index of a slab waveguide with about $10^4$ programmable spatial degrees of freedom. We implemented neural network inference on benchmark tasks with up to $49$-dimensional vectors in a single pass, without digital pre-processing or post-processing. Theoretical and numerical analyses further indicated that two-dimensional programmable waveguides may offer not only a constant-factor reduction in device area but also a scaling benefit, with the area required growing as $N^{1.5}$ rather than $N^2$.

physics.optics↗
arXiv2023

Vacancy-Engineered Phonon Polaritons in a van der Waals Crystal

Phonon-polaritons (PhPs) in low-symmetry van der Waals materials confine mid-infrared electromagnetic radiation well below the diffraction limit for nanoscale optics, sensing, and energy control. However, controlling the PhP dispersion at the nanoscale through intrinsic material properties$-$without external fields, lithography, or intercalants$-$remains elusive. Here, we demonstrate vacancy-engineered tuning of PhPs in $\alpha$-phase molybdenum trioxide ($\alpha$-MoO$_3$) via oxygen vacancy formation and lattice strain. Near-field nanoimaging of PhPs in processed $\alpha$-MoO$_3$ reveals an average polariton wavevector modulation of $\Delta k/k \approx 0.13 $ within the lower Restrahlen band. Stoichiometric analysis, density functional theory, and finite-difference time-domain simulations show agreement with the experimental results and suggest an induced vacancy concentration of $1\% - 2\%$ along with $(1.2\pm 0.2)\%$ compressive strain, resulting in a non-volatile dielectric permittivity modulation of up to $\Delta \varepsilon / \varepsilon \approx 0.15$. Despite these lattice modifications, the lifetimes of thermomechanically tuned PhPs remain high at $1.2 \pm 0.31$ ps. These results establish thermomechanical vacancy engineering as a general strategy to reprogram polaritonic response in vdW crystals, offering a new degree of freedom for embedded, non-volatile nanophotonics.

physics.optics↗
arXiv2023

Giant Thermomechanical Bandgap Engineering in Quasi-two-dimensional Tellurium

Mechanical straining-induced bandgap modulation in two-dimensional (2D) materials has been confined to volatile and narrow modulation due to substrate slippage and poor strain transfer. We report the thermomechanical modulation of the inherent bandgap in quasi-2D tellurium nanoflakes (TeNFs) via non-volatile strain induction during hot-press synthesis. We leveraged the coefficient of thermal expansion (CTE) mismatch between TeNFs and growth substrates by maintaining a high-pressure enforced non-slip condition during thermal relaxation (623 to 300K) to achieve the optimal biaxial compressive strain of -4.6 percent in TeNFs/sapphire. This resulted in an enormous bandgap modulation of 2.3 eV, at a rate of up to ~600 meV/%, which is two-fold larger than reported modulation rate. Strained TeNFs display robust band-to-band radiative excitonic blue photoemission with an intrinsic quantum efficiency (IQE) of c.a. 79.9%, making it promising for energy efficient blue LEDs and nanolasers. Computational studies reveal that biaxial compressive strain inhibits exciton-exciton annihilation by evading van-Hove singularities, hence promoting radiative-recombination. Bandgap modulation by such nonvolatile straining is scalable to other 2D semiconductors for on-demand nano(opto)-electronics.

physics.optics↗
arXiv2021

Electrically actuated varifocal lens based on liquid-crystal-embedded dielectric metasurfaces

Compact varifocal lenses are essential to various imaging and vision technologies. However, existing varifocal elements typically rely on mechanically-actuated systems with limited tuning speeds and scalability. Here, an ultrathin electrically controlled varifocal lens based on a liquid crystal (LC) encapsulated semiconductor metasurface is demonstrated. Enabled by the field-dependent LC anisotropy, applying a voltage bias across the LC cell modifies the local phase response of the silicon meta-atoms, in turn modifying the focal length of the metalens. In a numerical implementation, a voltage-actuated metalens with continuous zoom and up to 20% total focal shift is demonstrated. The concept of LC-based metalens is experimentally verified through the design and fabrication of a bifocal metalens that facilitates high-contrast switching between two discrete focal lengths upon application of a 3.2 V$_{\rm pp}$ voltage bias. Owing to their ultrathin thickness and adaptable design, LC-driven semiconductor metasurfaces open new opportunities for compact varifocal lensing in a diversity of modern imaging applications.

physics.optics↗
arXiv2021

Third-harmonic light polarization control in magnetically-resonant silicon metasurfaces

Nonlinear metasurfaces have become prominent tools for controlling and engineering light at the nanoscale. Usually, the polarization of the total generated third harmonic is studied. However, diffraction orders may present different polarizations. Here, we design an high quality factor silicon metasurface for third harmonic generation and perform back focal plane imaging of the diffraction orders, which present a rich variety of polarization states. Our results demonstrate the possibility of tailoring the polarization of the generated nonlinear diffraction orders paving the way to a higher degree of wavefront control.

physics.optics↗
arXiv2020

Externally driven nonlinear time-variant metasurfaces

Resonant photonic nanostructures exhibiting enhanced nonlinear responses and efficient frequency conversion are an emergent platform in nonlinear optics. High-index semiconductor metasurfaces with rapidly tuned high-Q resonances enable a novel class of time-variant metasurfaces, which expands the toolbox of color management at the nanoscale. Here, we report on the dynamic control of the nonlinear optical response in time-variant semiconductor metasurfaces supporting high-quality factor resonances in the near-infrared spectral range. Pump-probe measurements of germanium metasurfaces at negative pump-probe time delays reveals frequency conversion in the fundamental beam and a blue-shift of 10~nm (3.05$ω$) and 40% broadening in the third harmonic signal due to the photoinduced time-variant refractive index. A time-dependent coupled-mode theory, in excellent agreement with the experimental data, validated the time-variant nature of the system. Our findings expand the scope of time-variant metasurfaces and may serve as base for the next generation of nanoscale pulse shapers, optical switches and light sources.

physics.optics↗
arXiv2020

Generation of even and odd high harmonics in resonant metasurfaces using single and multiple ultra-intense laser pulses

High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in nanostructures is an attractive route to overcoming the well-known limitations of gases and bulk solids. We demonstrate a nanoscale platform for highly efficient HHG driven by strong mid-infrared laser pulses: an ultra-thin resonant gallium phosphide (GaP) metasurface. The wide bandgap and the lack of inversion symmetry of the GaP crystal enable the generation of even and odd harmonics covering a wide range of photon energies between 1.3 and 3 eV with minimal reabsorption. The resonantly enhanced conversion efficiency facilitates single-shot measurements that avoid material damage and pave the way to controllable transition between perturbative and non-perturbative regimes of light-matter interactions at the nanoscale.

physics.optics↗
arXiv2019

Overcoming the efficiency-bandwidth tradeoff for optical harmonics generation using nonlinear time-variant resonators

Highly resonant photonic structures, such as cavities and metasurfaces, can dramatically enhance the efficiency of nonlinear processes by utilizing strong optical field enhancement at the resonance. The latter, however, comes at the expense of the bandwidth. Here, we overcome such tradeoff by utilizing time-varying resonant structures. Using harmonics generation as an example, we show that the amplitude and phase format of the excitation, as well as the time evolution of the resonator, can be optimized to yield the strongest nonlinear response. We find the conditions for an efficient synthesis of electromagnetic signals that surpass the cavity bandwidth, and discuss a potential experimental realization of this concept.

physics.optics↗
arXiv2019

Nonlinear manifestations of photon acceleration in time-dependent metasurfaces: tunable broadband harmonics generation

Time-dependent nonlinear media, such as rapidly generated plasmas produced via laser ionization of gases, can increase the energy of individual laser photons and generate tunable high-order harmonic pulses. This phenomenon, known as photon acceleration, has traditionally required extreme-intensity laser pulses and macroscopic propagation lengths. Here, we report on a novel nonlinear material$-$an ultrathin semiconductor metasurface$-$that exhibits efficient photon acceleration at low intensities. We observe a signature nonlinear manifestation of photon acceleration: third-harmonic generation of near-infrared photons with tunable frequencies reaching up to $\approx3.1ω$. A simple time-dependent coupled-mode theory, found to be in good agreement with experimental results, is utilized to predict a new path towards nonlinear radiation sources that combine resonant upconversion with broadband operation.

physics.optics↗
arXiv2018

Perfect Diffraction with Bianisotropic Metagratings

One highly desirable function of a diffraction grating is its ability to deflect incident light into a specific diffraction order with near-perfect efficiency. While such asymmetry can be achieved in a variety of ways, e.g., by using a sawtooth (blazed) geometry, a recently emerged approach is to use a planar metagrating comprised of designer multi-resonant periodic units (metamolecules). Here we demonstrate that a bianisotropic unit cell supporting four resonances interfering in the far field can be used as a building block for achieving the prefect deflection. A coupled mode analysis shows that these modes provide a small number of orthogonal electromagnetic radiation patterns that are needed to suppress transmission/reflection into all but one diffraction order. Bianisotropy caused by a mirror symmetry breaking enables a normally incident wave to excite, through near-field couplings, two otherwise "dark" resonant modes. We design and experimentally realize bianisotropic metamolecules which are sub-wavelength in all three dimensions, and whose optical properties are desensitized to fabrication imperfections by their geometric simplicity. We show that optical beams tightly focused onto the metagratings with just a few unit cells can also be asymmetrically deflected with high efficiency, paving the way for compact broadband optical devices.

physics.optics↗
arXiv2018

Optical coupling between resonant dielectric nanoparticles and dielectric waveguides probed by third harmonic generation microscopy

Localized electromagnetic modes and negligible Ohmic losses dictate the growing interest in subwavelength all-dielectric nanoparticles. Although an exhaustive volume of study dealt with interaction of all-dielectric nanostructures with free-space electromagnetic fields, their performance as integrated photonics elements remains untackled. We present an experimental study of optical coupling between a resonant subwavelength silicon nanodisk and a non-resonant silicon waveguide, as probed by third harmonic generation microscopy. By placing the nanodisks at different distances from the waveguide, we observe third harmonic intensity modulation by a factor of up to 4.5. This modulation is assigned to changes in the local field enhancement within the nanodisks caused by their coupling to the waveguides and subsequent modulation of their magnetic-type resonances. Interestingly, although the waveguide presents an additional loss channel for the nanodisk, we observe an increase in the local field strength within the nanodisk, as verified by rigorous full-wave simulations. This work makes a step toward integration of all-dielectric nanoparticles on photonic chips.

physics.optics↗
arXiv2014

Plasmon ruler with gold nanorod dimers: utilizing the second-order resonance

The idea of utilizing the second-order plasmon resonance of the gold nanorod π-dimers for plasmon rulers is introduced. We report on a qualitatively different dependence of the plasmon resonance shift on the interparticle distance for the first- and second-order longitudinal modes, extending the working range of plasmon rulers up to the distance values of 400 nm.

physics.optics↗