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Maxim V. Gorkunov

Publications and source records attributed to Maxim V. Gorkunov.

17 recordsLinked to original sources

Plasmonic Fourier Surfaces Revisited: Relating Bandgaps with Bound States in the Continuum

Periodically corrugated metal interfaces supporting surface plasmon polaritons (SPPs) belong to the earliest nanoplasmonic platforms. Even simplest reliefs described by a few harmonics - plasmonic Fourier surfaces - display markedly different far-field signatures depending on the corrugation depth and symmetry: shallow reliefs exhibit a plasmonic bandgap (PBG) between two hybridized SPP standing waves, while deeper reliefs support asymmetry-induced single sharp resonances, termed over the last decade as quasi-bound states in the continuum (qBICs). Although these spectral features have long been observed experimentally and treated empirically, the underlying eigenmode evolution connecting the shallow and deep corrugation regimes has remained largely unexplored. Here we revisit this long-standing problem by analyzing it in terms of modern eigenstate formalism. Starting from the Rayleigh hypothesis, we develop a concise first-principle analytical description that explicitly captures how one eigenmode transforms from a dark bound state into an observable qBIC, while the other turns from bright into an overcoupled, unobservable state - thus unifying the SPP manifestations featuring PBG and qBIC within the same eigenmode framework. Finally, we demonstrate the practical relevance of the theory by showing how precise eigenstate engineering can enhance the SPP refractive index sensitivity.

physics.optics↗

Rewritable Chirality of Metasurfaces with Permittivity-Asymmetric Flatband Quasi-Bound States in the Continuum

Flatband eigenstates are widely applied to enhance angle-robust light-matter interactions in metaphotonics. However, controlling the polarization of flatbands remains challenging, as it is usually fixed once the metasurface is fabricated, with no options of post-fabrication modification. Here, we present a rewritable permittivity-asymmetric quasi-bound state in the continuum (ε-qBIC) metasurface platform, where selective polymethyl methacrylate (PMMA) coating of a silicon double-nanorod unit cell establishes a circularly polarized flatband state. By varying the PMMA thickness, the polarization of this state can be further controlled in the range from the right-circular to linear and to left-elliptical. The flatbands maintain stable resonance positions and robust far-field polarizations for the incidence angles up to 10 degrees. Importantly, the PMMA layer can be removed, recoated, and re-patterned on the same nanostructure, providing a pathway to rewrite the optical response. Building on this capability, we experimentally demonstrate the chirality encoding by spatially selective PMMA coating. The results establish a practical strategy for realizing high quality factor flatband metasurfaces with rewritable chirality, thus opening opportunities for applications in chiral encoding and chiroptical photonic devices in general.

physics.optics↗

Topological Control of Polaritonic Flatbands in Anisotropic van der Waals Metasurfaces

Anisotropic van der Waals (vdW) materials exhibit direction-dependent optical and electronic properties, making them valuable for tailoring directional light-matter interactions. Rhenium disulfide (ReS$_2$) stands out for its strong in-plane anisotropy and its thickness-independent direct-bandgap excitons, which can hybridize with light to form exciton-polaritons. In parallel, metasurfaces, engineered arrays of nanoscale subwavelength resonators, can support ultra-sharp photonic modes in the form of quasi-bound states in the continuum (qBICs). Topological transformations of photonic modes can give rise to flatbands, i.e., dispersionless states with quenched kinetic energy and vanishing group velocity. Intrinsic material anisotropy offers an unexplored route to robust far-field flatband formation and control. Here, we demonstrate how structuring an intrinsically anisotropic excitonic material into a resonant metasurface fundamentally transforms its photonic topological features and light-matter coupling behavior, allowing us to drive and topologically control extended far-field flatband formation. To this end, we fabricate C$_4$-symmetric metasurfaces directly from bulk ReS$_2$. The intrinsic anisotropy lifts the initial double degeneracy of the qBIC mode and yields two distinctly polarized resonances. It also reshapes the topological landscape: the integer topological charge of the qBIC mode splits into momentum-separated half-integer singularities, thereby flattening the far-field photonic dispersion. The resulting topologically-controlled photonic flatbands are then tuned in resonance with the linearly polarized excitonic transitions of ReS$_2$, resulting in two distinct, directionally hybridized exciton-polariton flatband regimes. These findings establish anisotropic vdW metasurfaces as a new platform for topologically engineered flatbands and flatband-driven light-matter coupling.

physics.optics↗

Observation of Janus Chirality for Coherent Thermal Emission from Metasurfaces

Metasurfaces emerged as a powerful tool for controlling thermal radiation, yet achieving coherent emission with opposite circular handednesses remains a highly challenging problem. Here, we demonstrate experimentally the Janus chiral thermal emission from metasurfaces with opposite circular handednesses on either side of a single device. We employ anisotropic metasurfaces supporting high-Q resonances with photonic flatbands enabling near-unity circular dichroism through in-plane symmetry control. Our experiments confirm the Janus coherent emission, and they are validated by the results of the coupled-mode theory. The flatband resonant metasurfaces enabling a control of chiral thermal emission provide an efficient platform for spin-controlled light-matter interaction.

physics.optics↗

Nonlinear chiral light generation from resonant metasurfaces

Chiral nonlinear response has been explored for decades due to its extreme sensitivity to molecular and structural dissymmetry. Conventional approaches often require bulky systems and produce only static nonlinear chirality. Here, we report on a generic mechanism for the generation and control of nonlinear chiral light in resonant optical systems. We reveal that nonlinear resonant generation of circularly polarized light from achiral dielectric metasurfaces is extremely sensitive to the polarization state of the fundamental wave, and a resonant metasurface can produce light with arbitrary degree of nonlinear chirality (DNC). Experimentally, we demonstrate that the chirality of nonlinear radiation from one metasurface can be continuously tuned from DNC = -0.86 to DNC = 0.94 by simply varying the polarization angle of the incident wave. By further exploiting the instantaneous polarization state, nonlinear chirality has been switched in a delay time step of 3.2 fs, which is orders of magnitude more sensitive than the current state-of-the-art polarization modulation. These results promise to enrich our understanding of nonlinear processes in chiral structures and their manipulation with resonant photonic structures.

physics.optics↗

Chiral Nonlinear Polaritonics with van der Waals Metasurfaces

In the strong-coupling regime, the interaction between light and matter reaches a hybridization state where the photonic and material components are inseparably linked. Using tailored states of light to break symmetries in such systems can facilitate the development of novel non-equilibrium quantum materials. Chiral optical cavities offer a promising approach for this, enabling either temporal or spatial symmetry-breaking, both of which are unachievable with conventional mirror cavities. For spatial symmetry-breaking, a cavity must discriminate the handedness of circularly polarized light, a functionality uniquely provided by chiral metamaterials. Here, we propose and demonstrate experimentally a chiral transition metal dichalcogenide (TMDC) metasurface with broken out-of-plane symmetry, allowing for the selective formation of self-hybridized exciton-polaritons with specific handedness. Our metasurface maintains maximal chirality for oblique incidence up to 20°, significantly outperforming all previously known designs, thereby transforming the angle of incidence from a constraint into a new degree of freedom for sub-nanometer-precise tuning of the cavity's resonant wavelength. Moreover, we study the chiral strong-coupling regime in nonlinear experiments and reveal the polariton-driven nature of chiral third-harmonic generation. Our results demonstrate a clear pathway towards van der Waals (vdW) metasurfaces as a novel and potent platform for chiral polaritonics with implications in a wide range of photonics research, such as non-reciprocal photonic devices and valleytronics.

physics.optics↗

Substrate-induced maximum optical chirality of planar dielectric structures

Resonant dielectric planar structures can interact selectively with light of particular helicity thus providing an attractive platform for chiral flat optics. The absence of mirror-symmetry planes defines geometric chirality, and it remains the main condition for achieving strong circular dichroism. For planar optical structures such as photonic-crystal membranes and metasurfaces, breaking of out-of-plane mirror symmetry is especially challenging, as it requires to fabricate meta-atoms with a tilt, variable height, or vertically shifted positions. Although transparent substrates formally break out-of-plane mirror symmetries, their optical effect is typically subtle being rarely considered for enhancing optical chirality. Here we reveal that low-refractive-index substrates can induce up to maximum optical chirality in otherwise achiral metastructures so that the transparency to waves of one helicity is combined with resonant blocking of waves of the opposite helicity. This effect originates from engineering twisted photonic eigenstates of different parities. Our perturbation analysis developed in terms of the resonant-state expansion reveals how the eigenstate coupling induced by a substrate gives rise to a pair of chiral resonances of opposite handedness. Our general theory is confirmed by the specific examples of light transmission in the normal and oblique directions by a rotation-symmetric photonic-crystal membrane placed on different transparent substrates.

physics.optics↗

Chiral electroluminescence from thin-film perovskite metacavities

Chiral light sources realized in ultracompact device platforms are highly desirable for various applications. Among active media employed for thin-film emission devices, lead-halide perovskites have been extensively studied for photoluminescence due to their exceptional properties. However, up to date, there have been no demonstrations of chiral electroluminescence with a substantial degree of circular polarization (DCP), being critical for the development of practical devices. Here, we propose a new concept of chiral light sources based on a thin-film perovskite metacavity and experimentally demonstrate chiral electroluminescence with DCP approaching 0.38. We design a metacavity created by a metal and a dielectric metasurface supporting photonic eigenstates with close-to-maximum chiral response. Chiral cavity modes facilitate asymmetric electroluminescence of pairs of left and right circularly polarized waves propagating in the opposite oblique directions. The proposed ultracompact light sources are especially advantageous for many applications requiring chiral light beams of both helicities.

physics.optics↗

Towards chiral polaritons

Coupling between light and material excitations underlies a wide range of optical phenomena. Polaritons are eigenstates of a coupled system with hybridized wave function. Owing to their hybrid composition, polaritons exhibit at the same time properties typical for photonic and electronic excitations, thus offering new ways for controlling electronic transport and even chemical kinetics. While most theoretical and experimental efforts have been focused on polaritons with electric-dipole coupling between light and matter, in chiral quantum emitters, electronic transitions are characterized by simultaneously nonzero electric and magnetic dipole moments. Geometrical chirality affects the optical properties of materials in a profound way and enables phenomena that underlie our ability to discriminate enantiomers of chiral molecules. Thus, it is natural to wonder what kinds of novel effects chirality may enable in the realm of strong light-matter coupling. Right now, this field located at the intersection of nanophotonics, quantum optics, and chemistry is in its infancy. In this Perspective, we offer our view towards chiral polaritons. We review basic physical concepts underlying chirality of matter and electromagnetic field, discuss the main theoretical and experimental challenges that need to be solved, and consider novel effects that could be enabled by strong coupling between chiral light and matter.

physics.optics↗

Unlocking the out-of-plane dimension for photonic bound states in the continuum to achieve maximum optical chirality

The realization of lossless metasurfaces with true chirality crucially requires the fabrication of three-dimensional structures, constraining their feasibility for experiments and hampering practical implementations. Even though the three-dimensional assembly of metallic nanostructures has been demonstrated previously, the resulting plasmonic resonances suffer from high intrinsic and radiative losses. The concept of photonic bound states in the continuum (BICs) is instrumental for tailoring radiative losses in diverse geometries, especially when implemented using lossless dielectrics, but applications have so far been limited to planar and intrinsically achiral structures. Here, we introduce a novel nanofabrication approach to unlock the height of generally flat all-dielectric metasurfaces as an accessible parameter for efficient resonance and functionality control. In particular, we realize out-of-plane symmetry breaking in quasi-BIC metasurfaces and leverage this design degree of freedom to demonstrate, for the first time, an optical all-dielectric quasi-BIC metasurface with maximum intrinsic chirality that responds selectively to light of a particular circular polarization depending on the structural handedness. Our experimental results not only open a new paradigm for all-dielectric BICs and chiral nanophotonics but also promise advances in the realization of efficient generation of optical angular momentum, holographic metasurfaces, and parity-time symmetry-broken optical systems.

physics.optics↗

Single-handedness chiral optical cavities

Geometrical chirality is a universal property encountered on very different length scales ranging from geometrical shapes of living organisms to protein and DNA molecules. Interaction of chiral matter with chiral light - that is, electromagnetic field possessing a certain handedness - underlies our ability to discriminate enantiomers of chiral molecules. In this context, it is often desired to have an optical cavity that efficiently couples to only a specific (right or left) molecular enantiomer, and does not couple to the opposite one. Here, we demonstrate a single-handedness chiral optical cavity supporting only an eigenmode of a given handedness and lacking modes having the opposite one. Resonant excitation of the cavity with light of appropriate handedness enables formation of a helical standing wave with a uniform chirality density, while the light of opposite handedness does not cause any resonant effects. Furthermore, only chiral emitters of the matching handedness efficiently interact with such a chiral eigenmode, enabling the handedness-selective strength of light-matter coupling. The proposed system expands the set of tools available for investigations of chiral matter and opens the door to studies of chiral electromagnetic vacuum.

physics.optics↗

Metasurfaces with maximum chirality empowered by bound states in the continuum

We demonstrate that rotationally symmetric chiral metasurfaces can support arbitrarily sharp resonances with the maximum optical chirality determined by precise shaping of bound states in the continuum (BICs). Being uncoupled from one circular polarisation of light and resonantly coupled to its counterpart, a metasurface hosting the chiral BIC resonance exhibits a narrow peak in the circular dichroism spectrum. We propose a realization of such chiral BIC metasurfaces based on pairs of dielectric bars and validate the concept of maximum chirality by numerical simulations

physics.optics↗

Corrugated silicon metasurface optimized within the Rayleigh hypothesis for anomalous refraction at large angles

We optimize optical performance of metasurfaces based on periodically corrugated silicon layers by adjusting the Fourier coefficients of their surface profile. For smooth corrugations, we demonstrate an excellent quantitative accuracy of semi-analytical approach based on the Rayleigh hypothesis. We employ the approach to design metasurfaces with anomalous refraction due to dominant first order diffraction. Unlike conventional Huygens' dielectric metasurfaces, corrugated silicon layers are capable of efficient anomalous refraction in grazing directions: we obtain corrugation shapes allowing to deflect 70-80% of the energy of normally incident green light into the range of 68°-85° of angles with respect to the normal.

physics.optics↗

Enhanced sensing of molecular optical activity with plasmonic nanohole arrays

Prospects of using metal hole arrays for the enhanced optical detection of molecular chirality in nanosize volumes are investigated. Light transmission through the holes filled with an optically active material is modeled and the activity enhancement by more than an order of magnitude is demonstrated. The spatial resolution of the chirality detection is shown to be of a few tens of nanometers. From comparing the effect in arrays of cylindrical holes and holes of complex chiral shape, it is concluded that the detection sensitivity is determined by the plasmonic near field enhancement. The intrinsic chirality of the arrays due to their shape appears to be less important.

physics.optics↗

Suppressed absolute negative conductance and generation of high-frequency radiation in semiconductor superlattices

We show that space-charge instabilities (electric field domains) in semiconductor superlattices are the attribute of absolute negative conductance induced by small constant and large alternating electric fields. We propose the efficient method for suppression of this destructive phenomenon in order to obtain a generation at microwave and THz frequencies in devices operating at room temperature. We theoretically proved that an unbiased superlattice with a moderate doping subjected to a microwave pump field provides a strong gain at third, fifth, seventh, etc. harmonics of the pump frequency in the conditions of suppressed domains.

cond-mat.mes-hall↗

Enhanced parametric processes in binary metamaterials

We suggest double-resonant (binary) metamaterials composed of two types of magnetic resonant elements, and demonstrate that in the nonlinear regime such metamaterials provide unique possibilities for phase-matched parametric interaction and enhanced second-harmonic generation.

physics.optics↗

Generation of high-frequency radiation in semiconductor superlattices with suppressed space-charge instabilities

We theoretically investigated the scheme allowing to avoid destructive space-charge instabilities and to obtain a strong gain at microwave and THz frequencies in semiconductor superlattice devices. Superlattice is subjected to a microwave field and a generation is achieved at some odd harmonics of the pump frequency. Gain arises because of parametric amplification seeded by harmonic generation. Negative differential conductance (NDC) is not a necessary condition for the generation. For the mode of operation with NDC, a limited space-charge accumulation does not sufficiently reduce the gain.

cond-mat.mes-hall↗