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Mayia A. Vranas

Publications and source records attributed to Mayia A. Vranas.

2 recordsLinked to original sources

Anisotropic Kitaev Spin Glass in Li$_{2}$Ru$_{x}$Ir$_{1-x}$O$_{3}$

Kitaev iridates have emerged as an important class of spin-orbit-entangled quantum materials in which bond-directional exchange interactions generate strong magnetic frustration and unconventional correlated states. Rather than realizing simple ordered magnets, members of the alpha,beta,gamma-Li2IrO3 family exhibit fragile and highly anisotropic magnetic behavior, including incommensurate counter-rotating order, strong field sensitivity, and pressure-driven electronic reconstruction. These phenomena place the iridates in close proximity to the Kitaev quantum spin liquid (QSL) regime, while simultaneously revealing the importance of competing interactions, lattice distortions, and spin-orbit-assisted hopping processes beyond the ideal Kitaev limit. Understanding how chemical substitution perturbs these competing interactions provides a route toward probing the underlying frustrated magnetic state. Here, we study single crystals of beta-Li2RuxIr1-xO3 with dilute Ru substitution, x<~10%. Through a combination of magnetometry, resonant elastic X-ray scattering, ac-heat capacity, and muon spin relaxation/rotation, we show that weak magnetic disorder continuously suppresses the incommensurate antiferromagnetic ground state without stabilizing an alternative long-range ordered phase. Instead, the system evolves into a bulk static spin glass characterized by slow relaxation, aging behavior, and frozen local magnetic fields. Despite the loss of long-range magnetic order, the glassy state retains substantial directional anisotropy without significant distortion to the honeycomb lattice, suggesting that disorder freezes spins within a still-active bond-directional exchange environment. In this picture, dilute Ru substitution provides a controlled pathway into an anisotropic Kitaev spin glass regime that preserves essential fingerprints of the underlying Kitaev exchange network.

cond-mat.str-el↗

Low-Temperature Suppression of Intertwined Orders in La$_{1/3}$Sr$_{2/3}$FeO$_{3}$ Thin Films

The strong coupling between spin, charge, and lattice degrees of freedom in perovskite oxides leads to an array of exotic phenomena, giving these materials rich phase diagrams that can include coupled orders. This is exemplified by the A-site doped ferrite La$_{1/3}$Sr$_{2/3}$FeO$_{3}$ (LSFO), which exhibits a coupled paramagnetic-antiferromagnetic and charge ordering phase transition at $\sim$190 K that has been well studied in thin films, bulk, and polycrystalline samples. However, the low temperature behavior of LSFO thin films below $\sim$100 K has not been thoroughly explored. This work uses several X-ray scattering and spectroscopy techniques to directly probe LSFO's magnetic and charge order down to low temperature. Using resonant X-ray scattering, we observe a complete suppression of LSFO's known antiferromagnetic and charge order below $\sim$25 K. Further spectroscopy and coherent scattering measurements provide insight into LSFO's electronic structure and domain dynamics in this new low temperature phase, and we propose possible explanations for the observed order suppression based on reduced dimensionality of domains in our thin films. Our findings provide insight into the effects of competing interactions in strongly correlated materials, particularly those with coupled orders.

cond-mat.str-el↗