arXiv subjects

Meifang Zhu

Publications and source records attributed to Meifang Zhu.

5 recordsLinked to original sources

arXiv2026

Tunable Flat Bands and magnetism in Triangulene-based Superatomic Graphene

Superatomic graphene platforms host a rich portfolio of flat-band-driven exotic quantum properties, yet their experimental realization remains challenging. Here, we report the bottom-up on-surface synthesis of superatomic graphene using phosphorus-doped triangulene as building blocks. Scanning tunneling microscopy and spectroscopy measurements resolve the well-defined honeycomb lattice of as-fabricated superatomic graphene and demonstrate the characteristic Dirac band and flat band electronic structures. Density functional theory calculations reveal that the flat bands originate from the in-plane p$_x,_y$-like frontier orbitals of the phosphorus-doped triangulene units, leading to intrinsic half-metallic behavior. Furthermore, oxygen functionalization of the molecular precursor enables deterministic modulation of the electronic structure and magnetic ordering. This work establishes a general platform for designing correlated quantum materials with tunable flat band properties.

cond-mat.mtrl-sci↗

arXiv2024

Half-Metallicity in Triangulene-based Superatomic Graphene

The discovery of two-dimensional (2D) magnets has opened up new possibilities for miniaturizing spintronic devices to the monolayer limit. 2D half-metals, capable of conducting fully spin-polarized currents when spin-orbit coupling is minimal, provide a key advantage in improving device performance. Extensive theoretical research has been carried out to discover 2D half-metals, yet their realization remains elusive. Here we report the bottom-up synthesis of superatomic graphene and the demonstration of its half-metallic properties. The produced graphene half-metal is fabricated through an on-surface synthetic approach with phosphorus-doped triangulene as its building block. Scanning tunneling microscopy measurements reveal its metallic band structures and identify its ferromagnetism through magnon excitation under varying magnetic fields. Density functional theory simulations accurately capture its half-metallic characteristics, uncovering the origin of spin-polarized bands from the p$_x,_y$-like orbital of superatomic graphene. Our work demonstrates intrinsic 2D carbon magnetism, paving the way for harnessing its advantages in spintronics.

cond-mat.mes-hall↗

arXiv2024

Shear-enhanced Liquid Crystal Spinning of Conjugated Polymer Fibers

Conjugated polymer fibers can be used to manufacture various soft fibrous optoelectronic devices, significantly advancing wearable devices and smart textiles. Recently, conjugated polymer-based fibrous electronic devices have been widely used in energy conversion, electrochemical sensing, and human-machine interaction. However, the insufficient mechanical properties of conjugated polymer fibers, the difficulty in solution processing semiconductors with rigid main chains, and the challenges in large-scale continuous production have limited their further development in the wearable field. We regulated the pi - pi stacking interactions in conjugated polymer molecules below their critical liquid crystal concentration by applying fluid shear stress. We implemented secondary orientation, leading to the continuous fabrication of anisotropic semiconductor fibers. This strategy enables conjugated polymers with rigid backbones to synergistically enhance the mechanical and semiconductor properties of fibers through liquid crystal spinning. Furthermore, conjugated polymer fibers, exhibiting excellent electrochemical performance and high mechanical strength (600 MPa) that essentially meet the requirements for industrialized preparation, maintain stability under extreme temperatures, radiation, and chemical reagents. Lastly, we have demonstrated logic circuits using semiconductor fiber organic electrochemical transistors, showcasing its application potential in the field of wearable fabric-style logic processing. These findings confirm the importance of the liquid crystalline state and solution control in optimizing the performance of conjugated polymer fibers, thus paving the way for developing a new generation of soft fiber semiconductor devices.

cond-mat.soft↗

arXiv2023

Enhanced Effective Aperture Distribution Function for Characterizing Large-Scale Antenna Arrays

Accurate characterization of large-scale antenna arrays is growing in importance and complexity for the fifth-generation (5G) and beyond systems, as they feature more antenna elements and require increased overall performance. The full 3D patterns of all antenna elements in the array need to be characterized because they are in general different due to construction inaccuracy, coupling, antenna array's asymmetry, etc. The effective aperture distribution function (EADF) can provide an analytic description of an antenna array based on a full-sphere measurement of the array in an anechoic chamber. However, as the array aperture increases, denser spatial samples are needed for EADF due to large distance offsets of array elements from the reference point in the anechoic chamber, leading to a prohibitive measurement time and increased complexity of EADF. In this paper, we present the EADF applied to large-scale arrays and highlight issues caused by the large array aperture. To overcome the issues, an enhanced EADF is proposed with a low complexity that is intrinsically determined by the characteristic of each array element rather than the array aperture. The enhanced EADF is validated using experimental measurements conducted at 27-30 GHz frequency band with a relatively large planar array.

eess.SP↗

arXiv2021

Beamspace Multidimensional ESPRIT Approaches for Simultaneous Localization and Communications

Modern wireless communication systems operating at high carrier frequencies are characterized by a high dimensionality of the underlying parameter space (including channel gains, angles, delays, and possibly Doppler shifts). Estimating these parameters is valuable for communication purposes, but also for localization and sensing, making channel estimation a critical component in any joint communication and localization or sensing application. The high dimensionality make it difficult to use search-based methods such as maximum likelihood. Search-free methods such as ESPRIT provide an attractive alternative, but require a complex decomposition step in both the tensor and matrix version of ESPRIT. To mitigate this, we propose, develop, and analyze a reduced complexity beamspace ESPRIT method. Complexity is reduced both by beampace processing as well as low-complex implementation of the singular value decomposition. A novel perturbation analysis provides important insights for both channel estimation and localization performance. The proposed method is compared to the tensor ESPRIT method, in terms of channel estimation, communication, localization, and sensing performance, further validating the perturbation analysis.

eess.SP↗