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Menglan Liu

Publications and source records attributed to Menglan Liu.

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Precision masses of neutron-rich platinum and gold nuclei reveal enhanced $N=126$ shell strength below doubly-magic $^{208}$Pb

The heaviest stable nuclei in the universe owe their existence to quantum shell structure, the grouping of protons and neutrons into discrete energy levels separated by gaps. The largest known neutron shell gap in stable nuclei, at $N=126$, stabilizes doubly-magic $^{208}$Pb and is responsible for the characteristic abundance peak of heavy elements near gold and platinum produced by the rapid neutron-capture process (r-process). Whether this shell gap persists as protons are removed from lead is a question central to both nuclear structure and the modeling of heavy-element synthesis, yet it has remained unanswered due to the extraordinary difficulty of producing the relevant neutron-rich nuclei. Direct experimental knowledge in this region was essentially absent. Here we report the first precision mass measurements of $^{203,204}$Pt and $^{204,205,206}$Au, performed at GSI using a novel combination of Schottky and isochronous mass spectrometry in a heavy-ion storage ring. The $N=126$ isotones $^{204}$Pt and $^{205}$Au are more strongly bound than the extrapolated trend of the previously known mass surface by 403 and 464~keV, respectively, revealing an unexpectedly enhanced $N=126$ shell strength below doubly-magic $^{208}$Pb. Furthermore, the proton-neutron interaction strength exhibits a hitherto unobserved bifurcation at $N=126$ as protons are removed from $^{208}$Pb. Our results redefine the nuclear mass surface in the neutron-rich heavy-element region and provide direct experimental benchmarks for theoretical models whose extrapolations toward more exotic nuclei are essential for r-process nucleosynthesis calculations.

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Level structure of light neutron-rich La isotopes beyond the N=82 shell closure

The high spin excited states of Lanthanum isotopes $^{140-143}$La, above the $N=82$ closed shell, have been populated in fission reactions. The prompt $\gamma$-ray transitions were measured using two complementary methods; a) in coincidence with the isotopically identified fragments produced in the fission of the $^{238}$U+$^{9}$Be system using the VAMOS++ and the AGATA spectrometers and b) high statistics three-fold $\gamma-\gamma-\gamma$ and four-fold $\gamma-\gamma-\gamma-\gamma$ coincidence data from the spontaneous fission of $^{252}$Cf using the Gammasphere. This work reports the first identification of a pair of parity doublet structures in $^{143}$La and the new high spin level structure in $^{140-142}$La from prompt $\gamma$-ray spectroscopy. The level structures are interpreted in terms of the systematics of neighbouring odd-$Z$ nuclei above $Z=50$ shell closure and large-scale shell model calculations. The present results indicate the presence of stable octupole deformation, in $^{143}$La. The excitation energy pattern and their comparison with neighbouring isotones, moving away from the N=82 closed shell, point towards a transition from single particle structures to an alternating parity rotational band structure in the La isotopic chain.

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Recent progress in configuration-interaction shell model

Since Mayer and Jensen employed the single-particle shell model to interpret the magic numbers, various microscopic nuclear models have been developed to study the nuclear force and structure. The confguration-interaction shell model (CISM), performed in truncated model space with the inclusion of the residual interaction, is one widely-used nuclear structure model. In the last decade, CISM has progressed in investigating the cross-shell excitation in exotic light nuclei, the similarity and diference in mirror nuclei, and the isomerism and seniority conservation in medium and heavy nuclei. Additionally, researchers have attempted to construct effective Hamiltonians for nuclei near 132Sn and 208Pb through a unifed way in the CISM framework. In parallel, related models, including the nucleon-pair approximation (NPA) approach, the Monte Carlo shell model (MCSM), the projected shell model (PSM), the Gamow shell model (GSM), etc., have also been extensively developed and validated in the last decade. This paper reviews the recent progress in CISM and some related models.

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Systematic shell-model study on spectroscopic properties in the south region of $^{208}$Pb

We aim to study the properties of nuclei in the south region of $^{208}$Pb systematically, including the binding and excitation energies and electromagnetic properties, in order to predict unknown properties of these nuclei, such as isomerism, utilizing a theoretical model which describes the experimentally known properties precisely. We also address whether the $N=126$ shell closure is robust or not when the proton number decreases from $^{208}$Pb. We performed large-scale shell-model calculations with a new Hamiltonian suggested in the present work. The model space is taken as the five proton orbits within $50<Z\leqslant82$ and the thirteen neutron orbits within $82<N\leqslant184$. And one-particle one-hole excitation is allowed across the $N=126$ gap. The Hamiltonian is constructed by combining the existing Hamiltonians, KHHE (with adjustment of its proton-proton part) and KHPE, and the monopole based universal interaction. The shell-model results well reproduce the experimentally observed binding energies and spectroscopic properties, such as isomerism, core excitation, and electromagnetic properties. Some possible isomeric states in neutron-rich Pb, Tl, and Hg isotopes are predicted with transition energies and half-lives. We also examine the effective charges and the quenching of the $g$ factors suitable for this region by systematic comparisons between observed and calculated electromagnetic properties. A new Hamiltonian is constructed for nuclei in the south region of $^{208}$Pb, mainly including Pb, Tl, Hg, Au, Pt, Ir, Os, Re, and W isotopes around $N=126$, and provides them reasonable descriptions on nuclear properties including binding energies, excitation energies and electromagnetic properties through comprehensive and systematic studies.

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