arXiv subjects

Michael A. Famiano

Publications and source records attributed to Michael A. Famiano.

18 recordsLinked to original sources

arXiv2025

Single-Crystal NMR for 17O in Alanine Enantiomers

Single-crystal solid-state nuclear magnetic resonance (ssNMR) spectroscopy, which enables detailed analysis of the electronic structures of crystalline molecules, offers a unique opportunity to investigate molecular chirality -- an essential feature with broad implications for understanding the origin and function of life. In this study, we employ single-crystal ssNMR spectroscopy, in combination with X-ray diffraction and density functional theory (DFT) calculations, to examine the electronic structure of 17O nuclei in crystalline forms of alanine enantiomers. Eight magnetically nonequivalent 17O resonances within the unit cell were observed and successfully assigned, and their corresponding NMR tensor parameters were determined. The experimental findings were compared with previous NMR studies as well as with DFT calculations performed in this work. The DFT results not only supported the assignment of crystallographically distinct 17O sites but also revealed previously unobserved antisymmetric components of the chemical shift tensors. This study presents the first comprehensive characterization of 17O NMR tensors in alanine enantiomers and underscores the power of integrating single-crystal ssNMR with X-ray diffraction and DFT calculations to advance our understanding of molecular chirality in amino acids.

physics.chem-ph↗

arXiv2024

New Experimentally Observable Gamma-ray Emissions from 241Am Nuclear Decay

With the high resolution of microcalorimeter detectors, previously unresolvable gamma-ray lines are now clearly resolvable. A careful measurement of Am-241 decay with a large array of gamma-ray microcalorimeters has revealed never before seen or predicted gamma lines at 207.72 +/- 0.02 keV and 208.21 +/- 0.01 keV. These results were made possible by new microwave-multiplexing readout to increase the array size and improved analysis algorithms to eliminate spectral artifacts. We suggest nuclear levels from which these gamma-rays might originate and calculate branching ratios for these transitions from measurements of both mixed Pu-Am standards and a pure Am-241 source. These results have implications for nuclear material safeguards and accounting, particularly for microcalorimeter gamma spectrometers, which are now being adopted in nuclear safeguards analytical laboratories.

nucl-ex↗

arXiv2021

Relativistic Coulomb Screening in Pulsational Pair Instability Supernovae

Context. Pulsational pair-instabilitye supernovae (PPISNe) and pair instability supernovae (PISNe) are the result of a thermonuclear runaway in the presence of a background electron-positron pair plasma. As such, their evolution and resultant black hole (BH) masses could possibly be affected by screening corrections due to the electron pair plasma. Aims. Sensitivity of PISNe and PPISNe to relativistic weak screening has been explored. Methods. In this paper a weak screening model that includes effects from relativistic pair production has been developed and applied at temperatures approaching and exceeding the thresh old for pair production. This screening model replaces "classical" screening commonly used in astrophysics. Modifications to the weak screening electron Debye length are incorporated in a computationally tractable analytic form with. Results. In PPISNe the BH masses were found to increase somewhat at high temperatures, though this increase is small. The BH collapse is also found to occur at earlier times, and the pulsational morphology also changes. In addition to the resultant BH mass, the sensitivity to the screening model of the pulsational period, the pulse structure, the PPISN-to-PISN transition, and the shift in the BH mass gap has been analyzed. The dependence of the composition of the ejected mass was also examined.

astro-ph.SR↗

arXiv2021

Chiral Selection, Isotopic Abundance Shifts, and Autocatalysis of Meteoritic Amino Acids

The discovery of amino acids in meteorites has presented two clues to the origin of their processing subsequent to their formation: a slight preference for left-handedness in some of them, and isotopic anomalies in some of their constituent atoms. In this article we present theoretical results from the Supernova Neutrino Amino Acid Processing (SNAAP) model, which uses electron anti-neutrinos and the magnetic fields from source objects such as supernovae or colliding neutron stars to selectively destroy one amino acid chirality and to create isotopic abundance shifts. For plausible magnetic fields and electron anti-neutrino fluxes, non-zero, positive enantiomeric excesses, $ee$s, defined to be the relative left/right asymmetry in an amino acid population, are reviewed for two amino acids, and conditions are suggested that would produce $ee>0$ for all of the $α$-amino acids. The relatively high energy anti-neutrinos that produce the $ee$s would inevitably also produce isotopic anomalies. A nuclear reaction network was developed to describe the reactions resulting from them and the nuclides in the meteorites. At similar anti-neutrino fluxes, assumed recombination of the detritus from the anti-neutrino interactions is shown to produce appreciable isotopic anomalies in qualitative agreement with those observed for D/$^1$H and $^{15}$N/$^{14}$N. The isotopic anomalies for $^{13}$C/$^{12}$C are predicted to be small, as are also observed. Autocatalysis may be necessary for any model to produce the largest $ee$s observed in meteorites. This allows the constraints of the original SNAAP model to be relaxed, increasing the probability of meteoroid survival in sites where amino acid processing is possible. These results have obvious implications for the origin of life on Earth.

astro-ph.EP↗

arXiv2021

Enhancement of Lithium in Red Clump Stars by the Additional Energy Loss Induced by New Physics

Since 7Li is easily destroyed in low temperatures, the surface lithium abundance decreases as stars evolve. This is supported by the lithium depletion observed in the atmosphere of most red giants. However, recent studies show that almost all of red clump stars have high lithium abundances A(Li)>-0.9, which are not predicted by the standard theory of the low-mass stellar evolution. In order to reconcile the discrepancy between the observations and the model, we consider additional energy loss channels which may come from physics beyond the Standard Model. A(Li) slightly increases near the tip of the red giant branch even in the standard model with thermohaline mixing because of the 7Be production by the Cameron-Fowler mechanism, but the resultant 7Li abundance is much lower than the observed values. We find that the production of 7Be becomes more active if there are additional energy loss channels, because themohaline mixing becomes more efficient and a heavier helium core is formed.

astro-ph.SR↗

arXiv2021

Contribution of collapsars, supernovae, and neutron star mergers to the evolution of r-process elements in the Galaxy

We study the evolution of rapid neutron-capture process (r-process) isotopes in the Galaxy. We analyze relative contributions from core collapse supernovae (CCSNe), neutron star mergers (NSMs) and collapsars under a range of astrophysical conditions and nuclear input data. Although the r-process in each of these sites can lead to similar (or differing) isotopic abundances, our simulations reveal that the early contribution of r-process material to the Galaxy was dominated by CCSNe and collapsar r-process nucleosynthesis, while the NSM contribution is unavoidably delayed even under the assumption of the shortest possible minimum merger time.

astro-ph.GA↗

arXiv2020

Screening Effects on Electron Capture Rates and Type Ia Supernova Nucleosynthesis

Type Ia supernovae (SNe Ia) are believed to be a thermonuclear explosion of a white dwarf, but the mass of their progenitors is still an open problem. In near-Chandrasekhar-mass (near-M_Ch) models of SNe Ia, the central density reaches >10^9 g cm^{-3}. The electron chemical potential becomes higher than the Q-values of electron capture (EC) transitions between fp-shell nuclei, so a portion of the available electrons is captured by iron group elements and thus neutron-rich isotopes are formed. Since EC reaction rates are sensitive to the density, the degree of neutronization is a key to distinguish near- and sub-M_Ch models. In order to compare observations and theoretical models, an accurate treatment of EC reactions is necessary. In previous theoretical works, however, effects of electron screening on ECs are ignored. Screening lowers EC rates and thus leads to a higher electron fraction. We implement electron screening on ECs to calculate explosive SN Ia nucleosynthesis in a near-M_Ch single degenerate model. It is found that some of neutron-rich nuclear abundances, namely those of 46,48Ca, 50Ti, 54Cr, 58Fe, 64Ni and 67,70Zn, decrease when screening effects on ECs are considered. Of these, 50Ti, 54Cr and 58Fe are particularly interesting because a significant portion of the solar abundance of these nuclei is presumed to originate from SNe Ia. We conclude that implementing the screening effect on ECs in modern SN Ia models is desirable to precisely calculate abundances of neutron-rich nuclides.

astro-ph.HE↗

arXiv2020

Elimination of the Blue Loops in the Evolution of Intermediate-mass Stars by the Neutrino Magnetic Moment and Large Extra Dimensions

For searching beyond Standard Model physics, stars are laboratories which complement terrestrial experiments. Massless neutrinos in the Standard Model of particle physics cannot have a magnetic moment, but massive neutrinos have a finite magnetic moment in the minimal extension of the Standard Model. Large extra dimensions are a possible solution of the hierarchy problem. Both of these provide additional energy loss channels in stellar interiors via the electromagnetic interaction and radiation into extra dimensions, respectively, and thus affect stellar evolution. We perform simulations of stellar evolution with such additional energy losses and find that they eliminate the blue loops in the evolution of intermediate-mass stars. The existence of Cepheid stars can be used to constrain the neutrino magnetic moment and large extra dimensions. In order for Cepheids to exist, the neutrino magnetic moment should be smaller than the range ~2x10^{-10} to 4x10^{-11}mu_B, where mu_B is the Bohr magneton, and the fundamental scale in the (4+2)-spacetime should be larger than ~2 to 5 TeV, depending on the rate of the ^{12}C(alpha, gamma)^{16}O reaction. The fundamental scale also has strong dependence on the metallicity. This value of the magnetic moment is in the range explored in the reactor experiments, but higher than the limit inferred from globular clusters. Similarly the fundamental scale value we constrain corresponds to a size of the compactified dimensions comparable to those explored in the torsion balance experiments, but is smaller than the limits inferred from collider experiments and low-mass stars.

astro-ph.SR↗

arXiv2020

Explaining the Variations in Isotopic Ratios in Meteoritic Amino Acids

Measurements of the isotopic abundances in meteoritic amino acids have found enhancements of $^2$H/H, $^{15}$N/$^{14}$N, and $^{13}$C/$^{12}$C in the amino acids in the meteorites studied. We show that they are consistent with the processing of the constituents of the meteorites by electron anti-neutrinos that would be expected from a core-collapse supernova or neutron-star merger. Using theoretical electron anti-neutrino cross sections we are able to predict these isotopic ratio variations depending on the time-integrated anti-neutrino flux at the site where the amino acids were processed.

astro-ph.EP↗

arXiv2020

Screening corrections to Electron Capture Rates and resulting constraints on Primordial Magnetic Fields

We explore screening effects arising from a relativistic magnetized plasma with applications to Big Bang nucleosynthesis (BBN). %Specifically, due to their small magnetic moments, energies of electrons and positrons can be easily quantized via Landau quantization. The screening potential which depends on the thermodynamics of charged particles in the plasma is altered by the magnetic field. We focus on the impact of screening on the electron capture interaction. Taking into account the correction in BBN arising from a homogeneous primordial magnetic field (PMF), we constrain the epoch at which the PMF was generated and its strength during BBN. Considering such screening corrections to the electron capture rates and using up-to-date observations of primordial elemental abundances, we also discuss the possibility of solving the problem of under-estimation of the deuterium abundance. We find for certain values of the PMF strength predicted D and $^4$He abundances are both consistent with the observational constraints.

astro-ph.CO↗

arXiv2019

Nuclear Mass Measurements With Radioactive Ion Beams

Nuclear masses are the most fundamental of all nuclear properties, yet they can provide a wealth of knowledge, including information on astrophysical sites, constraints on existing theory, and fundamental symmetries. In nearly all applications, it is necessary to measure nuclear masses with very high precision. As mass measurements push to more short-lived and more massive nuclei, the practical constraints on mass measurement techniques become more exacting. Various techniques used to measure nuclear masses, including their advantages and disadvantages are described. Descriptions of some of the world facilities at which the nuclear mass measurements are performed are given, and brief summaries of planned facilities are presented. Future directions are mentioned, and conclusions are presented which provide a possible outlook and emphasis on upcoming plans for nuclear mass measurements at existing facilities, those under construction, and those being planned.

nucl-ex↗

arXiv2018

Impacts of the New Carbon Fusion Cross Sections on Type Ia Supernovae

Type Ia supernovae (SNe Ia) are thought to be thermonuclear explosion of white dwarfs (WDs). Their progenitors are not well understood. One popular scenario is the double-degenerate (DD) scenario, which attributes SNe Ia to WD-WD binary mergers. The fates of the WD mergers depend on the rate of $^{12}$C+$^{12}$C reaction. Recently, the $^{12}$C+$^{12}$C cross sections have been measured and the analysis of the data using the Trojan Horse Method suggested that the astrophysical reaction rate is larger than conventional rates at astrophysical temperatures due to possible resonances. The resonance contribution results in a decrease of the carbon burning ignition temperature. Therefore accretion induced collapse occurs more easily and increases the birthrate of Galactic neutron stars with the contribution of the DD scenario to the SNe Ia rate becoming even smaller.

astro-ph.HE↗

arXiv2018

Nucleosynthesis Constraints on the Explosion Mechanism for Type Ia Supernovae

Observations of type Ia supernovae include information about the characteristic nucleosynthesis associated with these thermonuclear explosions. We consider observational constraints from iron-group elemental and isotopic ratios, to compare with various models obtained with the most-realistic recent treatment of electron captures. The nucleosynthesis is sensitive to the highest white-dwarf central densities. Hence, nucleosynthesis yields can distinguish high-density Chandrasekhar-mass models from lower-density burning models such as white-dwarf mergers. We discuss new results of post-processing nucleosynthesis for two spherical models (deflagration and/or delayed detonation models) based upon new electron capture rates. We also consider cylindrical and 3D explosion models (including deflagration, delayed-detonation, or a violent merger model). Although there are uncertainties in the observational constraints, we identify some trends in observations and the models. We make a new comparison of the models with elemental and isotopic ratios from five observed supernovae and three supernova remnants. We find that the models and data tend to fall into two groups. In one group low-density cores such as in a 3D merger model are slightly more consistent with the nucleosynthesis data, while the other group is slightly better identified with higher-density cores such as in single-degenerate 1D-3D deflagration models. Hence, we postulate that both types of environments appear to contribute nearly equally to observed SNIa. We also note that observational constraints on the yields of $^{54}$Cr and $^{54}$Fe, if available, might be used as a means to clarify the degree of geometrical symmetry of SNIa explosions.

astro-ph.HE↗

arXiv2018

First Calorimetric Measurement of Electron Capture in ${}^{193}$Pt with a Transition Edge Sensor

The neutrino mass can be extracted from a high statistics, high resolution calorimetric spectrum of electron capture in ${}^{163}$Ho. In order to better understand the shape of the calorimetric electron capture spectrum, a second isotope was measured with a close to ideal absorber-source configuration. ${}^{193}$Pt was created by irradiating a ${}^{192}$Pt-enriched platinum foil in a nuclear reactor. This Pt-in-Pt absorber was designed to have a nearly ideal absorber-source configuration. The measured ${}^{193}$Pt calorimetric electron-capture spectrum provides an independent check on the corresponding theoretical calculations, which have thus far been compared only for ${}^{163}$Ho. The first experimental and theoretically-calculated spectra from this ${}^{193}$Pt-in-Pt absorber are presented and overlaid for preliminary comparison of theory with experiment.

physics.atom-ph↗

arXiv2018

Sites That Can Produce Left-Handed Amino Acids in the Supernova Neutrino Amino Acid Processing Model

The Supernova Neutrino Amino Acid Processing model, which uses electron anti-neutrinos and the magnetic field from a source object such as a supernova to selectively destroy one amino acid chirality, is studied for possible sites that would produce meteoroids having partially left-handed amino acids. Several sites appear to provide the requisite magnetic field intensities and electron anti-neutrino fluxes. These results have obvious implications for the origin of life on Earth.

physics.bio-ph↗

arXiv2016

Impact of New Gamow-Teller Strengths on Explosive Type Ia Supernova Nucleosynthesis

Recent experimental results have confirmed a possible reduction in the GT$_+$ strengths of pf-shell nuclei. These proton-rich nuclei are of relevance in the deflagration and explosive burning phases of Type Ia supernovae. While prior GT strengths result in nucleosynthesis predictions with a lower-than-expected electron fraction, a reduction in the GT$_+$ strength can result in an slightly increased electron fraction compared to previous shell model predictions, though the enhancement is not as large as previous enhancements in going from rates computed by Fuller, Fowler, and Newman based on an independent particle model. A shell model parametrization has been developed which more closely matches experimental GT strengths. The resultant electron-capture rates are used in nucleosynthesis calculations for carbon deflagration and explosion phases of Type Ia supernovae, and the final mass fractions are compared to those obtained using more commonly-used rates.

astro-ph.HE↗

arXiv2016

Low-lying Resonances and Relativistic Screening in Big Bang Nucleosynthesis

We explore effects of the screening due to the relativistic electron-positron plasma and presence of resonances in the secondary reactions leading to A=7 nuclei during the Big Bang Nucleosynthesis. In particular, we investigate and examine possible low-lying resonances in the $^7$Be($^3$He, $γ$)$^{10}$C reaction and examine the resultant destruction of $^7$Be for various resonance locations and strengths. While a resonance in the $^{10}$C compound nucleus is thought to have negligible effects we explore the possibility of an enhancement from plasma screening that may adjust the final $^7$Be abundance. We find the effects of relativistic screening and possible low-lying resonances to be relatively small in the standard Early Universe models.

astro-ph.CO↗

arXiv2010

Identification of 45 New Neutron-Rich Isotopes Produced by In-Flight Fission of a 238U Beam at 345 MeV/nucleon

A search for new isotopes using in-flight fission of a 345 MeV/nucleon 238U beam has been carried out at the RI Beam Factory at the RIKEN Nishina Center. Fission fragments were analyzed and identified by using the superconducting in-flight separator BigRIPS. We observed 45 new neutron-rich isotopes: 71Mn, 73,74Fe, 76Co, 79Ni, 81,82Cu, 84,85Zn, 87Ga, 90Ge, 95Se, 98Br, 101Kr, 103Rb, 106,107Sr, 108,109Y, 111,112Zr, 114,115Nb, 115,116,117Mo, 119,120Tc, 121,122,123,124Ru, 123,124,125,126Rh, 127,128Pd, 133Cd, 138Sn, 140Sb, 143Te, 145I, 148Xe, and 152Ba.

nucl-ex↗