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Michael Förster

Publications and source records attributed to Michael Förster.

5 recordsLinked to original sources

Non-adiabatic ponderomotive effects in photoemission from nanotips in intense mid-infrared laser fields

Transient near-fields around metallic nanotips drive many applications, including the generation of ultrafast electron pulses and their use in electron microscopy. We have investigated the electron emission from a gold nanotip driven by mid-infrared few-cycle laser pulses. We identify a low-energy peak in the kinetic energy spectrum and study its shift to higher energies with increasing laser intensities from $1.7$ to $3.7\cdot10^{11} \mathrm{W}/\mathrm{cm}^2$. The experimental observation of the upshift of the low-energy peak is compared to a simple model and numerical simulations, which show that the decay of the near-field on a nanometer scale results in non-adiabatic transfer of the ponderomotive potential to the kinetic energy of emitted electrons and in turn to a shift of the peak. We derive an analytic expression for the non-adiabatic ponderomotive shift, which, after the previously found quenching of the quiver motion, completes the understanding of the role of inhomogeneous fields in strong-field photoemission from nanostructures.

physics.optics↗

High Visibility in Two-Color Above-Threshold Photoemission from Tungsten Nanotips in a Coherent Control Scheme

In this article we present coherent control of above-threshold photoemission from a tungsten nanotip achieving nearly perfect modulation. Depending on the pulse delay between fundamental (1560 nm) and second harmonic (780 nm) pulses of a femtosecond fiber laser at the nanotip, electron emission is significantly enhanced or depressed during temporal overlap. Electron emission is studied as a function of pulse delay, optical near-field intensities, DC bias field, and final photoelectron energy. Under optimized conditions modulation amplitudes of the electron emission of 97.5% are achieved. Experimental observations are discussed in the framework of quantum- pathway interference supported by local density of states (LDOS) simulations.

physics.optics↗

Two-color coherent control of femtosecond above-threshold photoemission from a tungsten nanotip

We demonstrate coherent control of multiphoton and above-threshold photoemission from a single solid-state nanoemitter driven by a fundamental and a weak second harmonic laser pulse. Depending on the relative phase of the two pulses, electron emission is modulated with a contrast of the oscillating current signal of up to 94%. Electron spectra reveal that all observed photon orders are affected simultaneously and similarly. We confirm that photoemission takes place within 10 fs. Accompanying simulations indicate that the current modulation with its large contrast results from two interfering quantum pathways leading to electron emission.

physics.optics↗

Probing of optical near-fields by electron rescattering on the 1 nm scale

We present a new method of measuring optical near-fields within ~1 nm of a metal surface, based on rescattering of photoemitted electrons. With this method, we precisely measure the field enhancement factor for tungsten and gold nanotips as a function of tip radius. The agreement with Maxwell simulations is very good. Further simulations yield a field enhancement map for all materials, which shows that optical near-fields at nanotips are governed by a geometric effect under most conditions, while plasmon resonances play only a minor role. Last, we consider the implications of our results on quantum mechanical effects near the surface of nanostructures and discuss features of quantum plasmonics.

physics.optics↗

A tip-based source of femtosecond electron pulses at 30keV

We present a nano-scale photoelectron source, optimized towards ultrashort pulse durations and well-suited for time-resolved diffraction experiments. A tungsten tip, mounted in a suppressor-extractor electrode configuration, allows the generation of 30 keV electron pulses with an estimated pulse duration of 37 fs at the gun exit. We infer the pulse duration from particle tracking simulations, which are in excellent agreement with experimental measurements of the electron-optical properties of the source. We furthermore demonstrate femtosecond laser-triggered operation. Besides the short electron pulse duration, a tip-based source is expected to feature a large transverse coherence as well as a nanometric emittance.

physics.acc-ph↗