arXiv subjects

Michael J. Newburger

Publications and source records attributed to Michael J. Newburger.

3 recordsLinked to original sources

arXiv2026

Lanthanide Ion Electronic Structure Controls Magnetic Excitations in Topological Quantum Ferrimagnets $LnMn_{6}Sn_{6}$ (Ln = Tb, Dy, Ho)

The $LnMn_{6}Sn_{6}$ family of topological magnets is a promising platform for next-generation spintronic and magnonic technologies. However, the influence of the lanthanide ion ($Ln^{3+}$) on the excited-state spin dynamics, or magnons, remains a critical knowledge gap. Here, we present the first comparative study of the magnetic dynamics in $LnMn_{6}Sn_{6}$ materials (Ln = Tb, Dy, Ho) using Brillouin light scattering. Our findings reveal a direct correlation between the lanthanide ion's intrinsic properties and the magnon behavior. We demonstrate that the magnon frequency in the absence of an applied magnetic field is primarily dictated by the strength of the lanthanide exchange coupling, as modeled by its relationship with the de Gennes factor. The response of the magnon to an applied field is influenced by material's gyromagnetic ratio and the overall anisotropy of the material, which are dictated by total angular momentum and the anisotropy of the lanthanide sublattice, respectively. These results establish that simple lanthanide substitution provides a powerful and predictable method for tuning magnon properties, enabling the rational design of materials for advanced technological applications.

cond-mat.mtrl-sci↗

arXiv2026

Raman and Terahertz Spectroscopy of Low-Frequency Chiral Phonons in Amino Acids

Chiral phonons are mirror-symmetric vibrations that correspond to twisting and rotational motions of atoms. In chiral biomolecules, they correspond to low-energy terahertz (THz)-range vibrations of the molecular segments involving dozens of atoms whose energies are sensitive to the chirality of the molecules and local atomic geometries. Here we present spectral signatures of chiral phonons in circularly polarized low-frequency Raman and Raman optical activity (ROA) spectra from crystals of several amino acids in different enantiomeric forms. Along with complementary THz circular dichroism (TCD) measurements, our ROA data reveal two sets of bisignate peaks in valine, alanine, tyrosine and proline between 1 and 4.5 THz that are more intense than the ROA peaks in the fingerprint region. Density functional theory (DFT) calculations on L-alanine attribute these modes to twisting and shearing molecular motions. The strong agreement between the ROA and TCD data demonstrates the power of these complementary vibrational spectroscopy techniques to identify chiral phonons in biomolecules, and offers new insights into their vibrational properties and interactions with circularly polarized light.

cond-mat.mtrl-sci↗

arXiv2023

Magnon Diffusion Length and Longitudinal Spin Seebeck Effect in Vanadium Tetracyanoethylene (V[TCNE]$_x$, $x \sim 2$)

Spintronic, spin caloritronic, and magnonic phenomena arise from complex interactions between charge, spin, and structural degrees of freedom that are challenging to model and even more difficult to predict. This situation is compounded by the relative scarcity of magnetically-ordered materials with relevant functionality, leaving the field strongly constrained to work with a handful of well-studied systems that do not encompass the full phase space of phenomenology predicted by fundamental theory. Here we present an important advance in this coupled theory-experiment challenge, wherein we extend existing theories of the spin Seebeck effect (SSE) to explicitly include the temperature-dependence of magnon non-conserving processes. This expanded theory quantitatively describes the low-temperature behavior of SSE signals previously measured in the mainstay material yttrium iron garnet (YIG) and predicts a new regime for magnonic and spintronic materials that have low saturation magnetization, $M_S$, and ultra-low damping. Finally, we validate this prediction by directly observing the spin Seebeck resistance (SSR) in the molecule-based ferrimagnetic semiconductor vanadium tetracyanoethylene (V[TCNE]$_x$, $x \sim 2$). These results validate the expanded theory, yielding SSR signals comparable in magnitude to YIG and extracted magnon diffusion length ($λ_m>1$ $μ$ m) and magnon lifetime for V[TCNE]$_x$ ($τ_{th}\approx 1-10$ $μ$ s) exceeding YIG ($τ_{th}\sim 10$ ns). Surprisingly, these properties persist to room temperature despite relatively low spin wave stiffness (exchange). This identification of a new regime for highly efficient SSE-active materials opens the door to a new class of magnetic materials for spintronic and magnonic applications.

cond-mat.mtrl-sci↗