arXiv subjects
Publications and source records attributed to Michael Köhl.
In this chapter we review the progress in experiments with hybrid systems of trapped ions and ultracold neutral atoms. We give a theoretical overview over the atom-ion interactions in the cold regime and give a summary of the most important experimental results. We conclude with an overview of remaining open challenges and possible applications in hybrid quantum systems of ions and neutral atoms.
We derive analytical expressions for the frequency and damping of the lowest collective modes of a two-dimensional Fermi gas using kinetic theory. For strong coupling, we furthermore show that pairing correlations overcompensate the effects of Pauli blocking on the collision rate for a large range of temperatures, resulting in a rate which is larger than that of a classical gas. Our results agree well with experimental data, and they recover the observed cross-over from collisionless to hydrodynamic behaviour with increasing coupling for the quadruple mode. Finally, we show that a trap anisotropy within the experimental bounds results in a damping of the breathing mode which is comparable to what is observed, even for a scale invariant system.
Harnessing spins as carriers for information has emerged as an elegant extension to the transport of electrical charges. The coherence of such spin transport in spintronic circuits is determined by the lifetime of spin excitations and by spin diffusion. Fermionic quantum gases are a unique system to study the fundamentals of spin transport from first principles since interactions can be precisely tailored and the dynamics is on time scales which are directly observable. In particular at unitarity, spin transport is dictated by diffusion and is expected to reach a universal, quantum-limited diffusivity on the order of hbar/m. Here, we study the non-equilibrium dynamics of a two-dimensional Fermi gas following a quench into a metastable, transversely polarized spin state. Using the spin-echo technique, we measure the yet lowest transverse spin diffusion constant of 0.25(3) hbar/m. For weak interactions, we observe a coherent collective transverse spin-wave mode that exhibits mode softening when approaching the hydrodynamic regime.
We present the realization of a combined trapped-ion and optical cavity system, in which a single Yb^+ ion is confined by a micron-scale ion trap inside a 230 mum-long optical fiber cavity. We characterize the spatial ion-cavity coupling and measure the ion-cavity coupling strength using a cavity-stimulated Lambda-transition. Owing to the small mode volume of the fiber resonator, the coherent coupling strength between the ion and a single photon exceeds the natural decay rate of the dipole moment. This system can be integrated into ion-photon quantum networks and is a step towards cavity quantum-electrodynamics (cavity-QED) based quantum information processing with trapped ions.
The control of chemical reactions is a recurring theme in physics and chemistry. Traditionally, chemical reactions have been investigated by tuning thermodynamic parameters, such as temperature or pressure. More recently, physical methods such as laser or magnetic field control have emerged to provide completely new experimental possibilities, in particular in the realm of cold collisions. The control of reaction pathways is also a critical component to implement molecular quantum information processing. For these undertakings, single particles provide a clean and well-controlled experimental system. Here, we report on the experimental tuning of the exchange reaction rates of a single trapped ion with ultracold neutral atoms by exerting control over both their quantum states. We observe the influence of the hyperfine interaction on chemical reaction rates and branching ratios, and monitor the kinematics of the reaction products. These investigations advance chemistry with single trapped particles towards achieving quantum-limited control of chemical reactions and indicate limits for buffer gas cooling of single ion clocks.
The line shape of radio frequency spectra of tightly bound Feshbach molecules in strong transverse confinement can be described by a simple analytic formula that includes final state interactions. By direct comparison to experimental data, we clarify the role of effective range corrections to two-body bound-state energies in lower dimensions.
The dynamics of a single impurity in an environment is a fundamental problem in many-body physics. In the solid state, a well-known case is an impurity coupled to a bosonic bath, for example lattice vibrations. Here the impurity together with its accompanying lattice distortion form a new entity, a polaron. This quasiparticle plays an important role in the spectral function of high-Tc superconductors as well as in colossal-magnetoresistance in manganites. For impurities in a fermionic bath, the attention so far has been mostly on heavy or immobile impurities which exhibit Anderson's orthogonality catastrophe and the Kondo effect. Only recently, mobile impurities have moved into the focus of research and they have been found to form new quasiparticles, so called Fermi polarons. The Fermi polaron problem constitutes the extreme, but conceptually simple, limit of two important quantum many-body problems: the BEC-BCS crossover with spin-imbalance for attractive interactions and Stoner's itinerant ferromagnetism for repulsive interactions. It has been proposed that this and other yet elusive exotic quantum phases might become realizable in Fermi gases confined to two dimensions. Their stability and observability is intimately related to the theoretically debated properties of the Fermi polaron in two dimensional Fermi gas. Here we create and investigate these Fermi polarons and measure their spectral function using momentum-resolved photoemission spectroscopy. For attractive interactions we find evidence for the disputed pairing transition between polarons and tightly bound dimers, which provides insight into the elementary pairing mechanism of imbalanced, strongly-coupled two-dimensional Fermi gases. Additionally, for repulsive interactions we study novel quasiparticles, repulsive polarons, whose lifetime determine the possibility of stabilizing repulsively interacting Fermi systems.
We investigate the collective excitations of a harmonically trapped two-dimensional Fermi gas from the collisionless (zero sound) to the hydrodynamic (first sound) regime. The breathing mode, which is sensitive to the equation of state, is observed at a frequency two times the dipole mode frequency for a large range of interaction strengths and temperatures, and the amplitude of the breathing mode is undamped. This provides evidence for a dynamical SO(2,1) scaling symmetry of the two-dimensional Fermi gas. Moreover, we investigate the quadrupole mode to measure the shear viscosity of the two-dimensional gas and study its temperature dependence.
We perform laser spectroscopy of Yb+ ions on the 4f14 6s 2S_{1/2} - 4f13 5d 6s 3D[3/2]_{1/2} transition at 297 nm. The frequency measurements for 170Yb+, 172Yb+, 174Yb+, and 176Yb+ reveal the specific mass shift as well as the field shifts. In addition, we demonstrate laser cooling of Yb+ ions using this transition and show that light at 297 nm can be used as the second step in the photoionization of neutral Yb atoms.
Pairing of fermions is ubiquitous in nature and it is responsible for a large variety of fascinating phenomena like superconductivity, superfluidity of $^3$He, the anomalous rotation of neutron stars, and the BEC-BCS crossover in strongly interacting Fermi gases. When confined to two dimensions, interacting many-body systems bear even more subtle effects, many of which lack understanding at a fundamental level. Most striking is the, yet unexplained, effect of high-temperature superconductivity in cuprates, which is intimately related to the two-dimensional geometry of the crystal structure. In particular, the questions how many-body pairing is established at high temperature and whether it precedes superconductivity are crucial to be answered. Here, we report on the observation of pairing in a harmonically trapped two-dimensional atomic Fermi gas in the regime of strong coupling. We perform momentum-resolved photoemission spectroscopy, analogous to ARPES in the solid state, to measure the spectral function of the gas and we detect a many-body pairing gap above the superfluid transition temperature. Our observations mark a significant step in the emulation of layered two-dimensional strongly correlated superconductors using ultracold atomic gases.
The immersion of a single ion confined by a radiofrequency trap in an ultracold atomic gas extends the concept of buffer gas cooling to a new temperature regime. The steady state energy distribution of the ion is determined by its kinetics in the radiofrequency field rather than the temperature of the buffer gas. Moreover, the finite size of the ultracold gas facilitates the observation of back-action of the ion onto the buffer gas. We numerically investigate the system's properties depending on atom-ion mass ratio, trap geometry, differential cross-section, and non-uniform neutral atom density distribution. Experimental results are well reproduced by our model considering only elastic collisions. We identify excess micromotion to set the typical scale for the ion energy statistics and explore the applicability of the mobility collision cross-section to the ultracold regime.
We have investigated $4s\;^2S_{1/2} \rightarrow 5p\;^2P_{1/2}$ transition ($D_1$ line) of the potassium isotopes $^{39}$K, $^{40}$K, and $^{41}$K using Doppler-free laser saturation spectroscopy. Our measurements reveal the hyperfine splitting of the $5p\;^2P_{1/2}$ state of $^{40}$K and we have determined the specific mass shift and the nuclear field shift constants for the blue $D_1$ line.
We realize and study a strongly interacting two-component atomic Fermi gas confined to two dimensions in an optical lattice. Using radio-frequency spectroscopy we measure the interaction energy of the strongly interacting gas. We observe the confinement-induced Feshbach resonance and find the existence of confinement-induced molecules in very good agreement with theoretical predictions.
In recent years, ultracold atoms have emerged as an exceptionally controllable experimental system to investigate fundamental physics, ranging from quantum information science to simulations of condensed matter models. Here we go one step further and explore how cold atoms can be combined with other quantum systems to create new quantum hybrids with tailored properties. Coupling atomic quantum many-body states to an independently controllable single-particle gives access to a wealth of novel physics and to completely new detection and manipulation techniques. We report on recent experiments in which we have for the first time deterministically placed a single ion into an atomic Bose Einstein condensate. A trapped ion, which currently constitutes the most pristine single particle quantum system, can be observed and manipulated at the single particle level. In this single-particle/many-body composite quantum system we show sympathetic cooling of the ion and observe chemical reactions of single particles in situ.
Improved control of the motional and internal quantum states of ultracold neutral atoms and ions has opened intriguing possibilities for quantum simulation and quantum computation. Many-body effects have been explored with hundreds of thousands of quantum-degenerate neutral atoms and coherent light-matter interfaces have been built. Systems of single or a few trapped ions have been used to demonstrate universal quantum computing algorithms and to detect variations of fundamental constants in precision atomic clocks. Until now, atomic quantum gases and single trapped ions have been treated separately in experiments. Here we investigate whether they can be advantageously combined into one hybrid system, by exploring the immersion of a single trapped ion into a Bose-Einstein condensate of neutral atoms. We demonstrate independent control over the two components within the hybrid system, study the fundamental interaction processes and observe sympathetic cooling of the single ion by the condensate. Our experiment calls for further research into the possibility of using this technique for the continuous cooling of quantum computers. We also anticipate that it will lead to explorations of entanglement in hybrid quantum systems and to fundamental studies of the decoherence of a single, locally controlled impurity particle coupled to a quantum environment.
We study cold heteronuclear atom ion collisions by immersing a trapped single ion into an ultracold atomic cloud. Using ultracold atoms as reaction targets, our measurement is sensitive to elastic collisions with extremely small energy transfer. The observed energy-dependent elastic atom-ion scattering rate deviates significantly from the prediction of Langevin but is in full agreement with the quantum mechanical cross section. Additionally, we characterize inelastic collisions leading to chemical reactions at the single particle level and measure the energy-dependent reaction rate constants. The reaction products are identified by in-trap mass spectrometry, revealing the branching ratio between radiative and non-radiative charge exchange processes.
We investigate the propagation of spin impurity atoms through a strongly interacting one-dimensional Bose gas. The initially well localized impurities are accelerated by a constant force, very much analogous to electrons subject to a bias voltage, and propagate as a one-dimensional impurity spin wave packet. We follow the motion of the impurities in situ and characterize the interaction induced dynamics. We observe a very complex non-equilibrium dynamics, including the emergence of large density fluctuations in the remaining Bose gas, and multiple scattering events leading to dissipation of the impurity's motion.
We propose an experimental procedure to cool fermionic atoms loaded into an optical lattice. The central idea is to spatially divide the system into entropy-rich and -poor regions by shaping the confining potential profile. Atoms in regions of high entropy per particle are subsequently isolated from the system. We discuss how to experimentally carry out this proposal, and perform a quantitative study of its efficiency. We find that the entropy per particle, $s$, can typically be reduced by a factor of 10 such that entropies lower than $s/k_B \sim 0.2$ can be reached. Cooling into highly sought-after quantum phases (such as an antiferromagnet) can thus be achieved. We show that this procedure is robust against variations of the experimental conditions.