SearcharxivSearch

arXiv subjects

Michael M. Fogler

Publications and source records attributed to Michael M. Fogler.

At least 19 recordsLinked to original sources

Excitonic pattern formation from a wrinkling instability in a van der Waals heterostructure

We studied photoluminescence of spatially indirect excitons (IXs) in a MoSe$_2$/WSe$_2$ van der Waals heterostructure. We observed a quasi-periodic triangular pattern of IXs with a characteristic spatial wavelength $\sim{}2.6\,μ\mathrm{m}$. Our theoretical analysis using a Föppl-von Kármán theory finds an elastic instability that produces triangular patterns with micrometer-scale wavelengths. This mechanism is consistent with the wavelength, symmetry, excitation power dependence, and temperature dependence of the observed IX pattern.

cond-mat.mes-hall

Quantum Light Nano-Imaging

Entanglement and quantum correlations are central to the physics of quantum materials, yet they have remained notoriously difficult to access experimentally. Accessing these phenomena in solids requires quantum optical probes that operate at the native length and time scales of material excitations, below the diffraction limit of light. Developing the requisite tools has previously been infeasible due to the weak intensities of state-of-the-art quantum light sources and the inefficiency of light coupling in near-field light-matter interactions. In this work, we address these challenges and report the development of a quantum light scattering-type scanning near-field optical microscope (q-SNOM) that enables quantum-optical studies of solid-state systems with nanoscale spatial resolution. As a first demonstration, we visualize the self-interference of single hybrid light-matter polaritons in the prototypical van der Waals semiconductor MoS2. We also introduce a polaritonic time-of-flight metrology that exploits the temporal correlations among entangled photons to observe the quasiparticle propagation dynamics at femtosecond time scales. This work establishes a new experimental paradigm for exploring quantum effects in materials at the nanoscale.

cond-mat.mes-hall

Plasmon dynamics in graphene

Plasmon are collective oscillations of mobile electrons with dynamics controlled by their charge stiffness("Drude weight"). Using terahertz spacetime metrology, we probe Plasmon dynamics of mono- and bi-layer graphene. In both systems, the experimentally measured Drude weight systematically exceeds the prediction based on non-interacting electronic system. The relative enhancement increases as the carrier density decreases. We attribute the observed deviation to the interplay of interactions and wave function structure of the Dirac fermions in multi-layer graphene. Our results establish that pseudospin structure of the single-particle electronic wave function can directly influence collective excitations, with implications that extend beyond graphene to a broad class of quantum materials.

cond-mat.mes-hall

Twisted bilayer graphene as a terahertz plasmonic crystal

We study surface plasmons in minimally-twisted gapped bilayer graphene that contains a triangular network of partial dislocations (or AB-BA domain walls) hosting topologically protected one-dimensional electronic states. We show that this system behaves as a plasmonic crystal and we calculate its band structure by solving classical equations of motion for charge dynamics on the network links with impedance boundary conditions at the network nodes. The plasmon dispersion exhibits several notable features such as multiple gapless branches, flat bands, and dissipationless modes at high-symmetry points. We compare our network-based formalism with the conventional random phase approximation and discuss when each approach is valid. Calculations of plasmon waves launched by local scatterers are presented to simulate terahertz nano-imaging experiments.

cond-mat.mes-hall

Application of deep neural networks for computing the renormalization group flow of the two-dimensional phi^4 field theory

We introduce RGFlow, a deep neural network-based real-space renormalization group (RG) framework tailored for continuum scalar field theories. Leveraging generative capabilities of flow-based neural networks, RGFlow autonomously learns real-space RG transformations from data without prior knowledge of the underlying model. In contrast to conventional approaches, RGFlow is bijective (information-preserving) and is optimized based on the principle of minimal mutual information. We demonstrate the method on two examples. The first one is a one-dimensional Gaussian model, where RGFlow is shown to learn the classical decimation rule. The second is the two-dimensional phi^4 theory, where the network successfully identifies a Wilson-Fisher-like critical point and provides an estimate of the correlation-length critical exponent.

cond-mat.dis-nn

Imaging the diffusive-to-ballistic crossover of magnetotransport in graphene

Scanning tunneling potentiometry (STP) is used to probe the local, current-induced electrochemical potential of carriers in graphene near circular electrostatic barriers in an out-of-plane magnetic field ranging from 0 to 1.4 T. These measurements provide nanometer-resolved information about the local motion of carriers, revealing significant changes in carrier dynamics with increasing field strength. At low magnetic fields the electrochemical potential displays a spiral-like pattern, while at high fields it exhibits distinct changes at particular radii. We show that the observed behavior indicates a transition from diffusive to ballistic transport. Additionally, the sharp changes in the measured potential profile at high fields result from the `spirograph' motion of carriers, which creates a local enhancement of the Hall field one cyclotron diameter away from the semiclassical turning point near the electrostatic barrier.

cond-mat.mes-hall

Electronic interactions in Dirac fluids visualized by nano-terahertz spacetime interference of electron-photon quasiparticles

Ultraclean graphene at charge neutrality hosts a quantum critical Dirac fluid of interacting electrons and holes. Interactions profoundly affect the charge dynamics of graphene, which is encoded in the properties of its electron-photon collective modes: surface plasmon polaritons (SPPs). Here we show that polaritonic interference patterns are particularly well suited to unveil the interactions in Dirac fluids by tracking polaritonic interference in time at temporal scales commensurate with the electronic scattering. Spacetime SPP interference patterns recorded in tera-hertz (THz) frequency range provided unobstructed readouts of the group velocity and lifetime of polariton that can be directly mapped onto the electronic spectral weight and the relaxation rate. Our data uncovered prominent departures of the electron dynamics from the predictions of the conventional Fermi-liquid theory. The deviations are particularly strong when the densities of electrons and holes are approximately equal. The proposed spacetime imaging methodology can be broadly applied to probe the electrodynamics of quantum materials.

cond-mat.str-el

Nano-Imaging of Landau-Phonon Polaritons in Dirac Heterostructures

Polaritons are light-matter quasiparticles that govern the optical response of quantum materials and enable their nanophotonic applications. We have studied a new type of polaritons arising in magnetized graphene encapsulated in hexagonal boron nitride (hBN). These polaritons stem from hybridization of Dirac magnetoexciton modes of graphene with waveguide phonon modes of hBN crystals. We refer to these quasiparticles as the Landau-phonon polaritons (LPPs). Using infrared magneto nanoscopy, we imaged LPPs and controlled their real-space propagation by varying the magnetic field. These LLPs have large in-plane momenta and are not bound by the conventional optical selection rules, granting us access to the "forbidden" inter-Landau level transitions (ILTs). We observed avoided crossings in the LPP dispersion - a hallmark of the strong coupling regime - occurring when the magnetoexciton and hBN phonon frequencies matched. Our LPP-based nanoscopy also enabled us to resolve two fundamental many-body effects: the graphene Fermi velocity renormalization and ILT-dependent magnetoexciton binding energies. These results indicate that magnetic-field-tuned Dirac heterostructures are promising platforms for precise nanoscale control and sensing of light-matter interaction.

physics.optics

Feshbach resonance of heavy exciton-polaritons

We study interactions between polaritons formed by hybridization of excitons in a two-dimensional (2D) semiconductor with surface optical phonons or plasmons. These quasiparticles have a high effective mass and can bind into bipolaritons near a Feshbach-like scattering resonance. We analyze the phase diagram of a many-body condensate of heavy polaritons and bipolaritons and calculate their absorption and luminescence spectra, which can be measured experimentally.

cond-mat.mes-hall

Can A Neural Network Hear the Shape of A Drum?

We have developed a deep neural network that reconstructs the shape of a polygonal domain given the first hundred of its Laplacian eigenvalues. Having an encoder-decoder structure, the network maps input spectra to a latent space and then predicts the discretized image of the domain on a square grid. We tested this network on randomly generated pentagons. The prediction accuracy is high and the predictions obey the Laplacian scaling rule. The network recovers the continuous rotational degree of freedom beyond the symmetry of the grid. The variation of the latent variables under the scaling transformation shows they are strongly correlated with Weyl' s parameters (area, perimeter, and a certain function of the angles) of the test polygons.

cs.SD

Machine Learning for Optical Scanning Probe Nanoscopy

The ability to perform nanometer-scale optical imaging and spectroscopy is key to deciphering the low-energy effects in quantum materials, as well as vibrational fingerprints in planetary and extraterrestrial particles, catalytic substances, and aqueous biological samples. The scattering-type scanning near-field optical microscopy (s-SNOM) technique has recently spread to many research fields and enabled notable discoveries. In this brief perspective, we show that the s-SNOM, together with scanning probe research in general, can benefit in many ways from artificial intelligence (AI) and machine learning (ML) algorithms. We show that, with the help of AI- and ML-enhanced data acquisition and analysis, scanning probe optical nanoscopy is poised to become more efficient, accurate, and intelligent.

physics.optics

Deep-Learning-Aided Extraction of Optical Constants in Scanning Near-Field Optical Microscopy

Scanning near-field optical microscopy is one of the most effective techniques for spectroscopy of nanoscale systems. However, inferring optical constants from the measured near-field signal can be challenging because of a complicated and highly nonlinear interaction between the scanned probe and the sample. Conventional fitting methods applied to this problem often suffer from the lack of convergence or require human intervention. Here we develop an alternative approach where the optical parameter extraction is automated by a deep learning network. Compared to its traditional counterparts, our method demonstrates superior accuracy, stability against noise, and computational speed when applied to simulated near-field spectra.

physics.optics

Hyperbolic enhancement of photocurrent patterns in minimally twisted bilayer graphene

Quasi-periodic moiré patterns and their effect on electronic properties of twisted bilayer graphene (TBG) have been intensely studied. At small twist angle $θ$, due to atomic reconstruction, the moiré superlattice morphs into a network of narrow domain walls separating micron-scale AB and BA stacking regions. We use scanning probe photocurrent imaging to resolve nanoscale variations of the Seebeck coefficient occurring at these domain walls. The observed features become enhanced in a range of mid-infrared frequencies where the hexagonal boron nitride (hBN), which we use as a TBG substrate, is optically hyperbolic. Our results illustrate new capabilities of nano-photocurrent technique for probing nanoscale electronic inhomogeneities in two-dimensional materials.

cond-mat.mes-hall

Graphene/$α$-RuCl$_3$: An Emergent 2D Plasmonic Interface

Work function-mediated charge transfer in graphene/$α$-RuCl$_3$ heterostructures has been proposed as a strategy for generating highly-doped 2D interfaces. In this geometry, graphene should become sufficiently doped to host surface and edge plasmon-polaritons (SPPs and EPPs, respectively). Characterization of the SPP and EPP behavior as a function of frequency and temperature can be used to simultaneously probe the magnitude of interlayer charge transfer while extracting the optical response of the interfacial doped $α$-RuCl$_3$. We accomplish this using scanning near-field optical microscopy (SNOM) in conjunction with first-principles DFT calculations. This reveals massive interlayer charge transfer (2.7 $\times$ 10$^{13}$ cm$^{-2}$) and enhanced optical conductivity in $α$-RuCl$_3$ as a result of significant electron doping. Our results provide a general strategy for generating highly-doped plasmonic interfaces in the 2D limit in a scanning probe-accessible geometry without need of an electrostatic gate.

cond-mat.mtrl-sci

Nano-photocurrent mapping of local electronic structure in twisted bilayer graphene

We report a combined nano-photocurrent and infrared nanoscopy study of twisted bilayer graphene (TBG) enabling access to the local electronic phenomena at length scales as short as 20 nm. We show that the photocurrent changes sign at carrier densities tracking the local superlattice density of states of TBG. We use this property to identify domains of varying local twist angle by local photo-thermoelectric effect. Consistent with the photocurrent study, infrared nano-imaging experiments reveal optical conductivity features dominated by twist-angle dependent interband transitions. Our results provide a fast and robust method for mapping the electronic structure of TBG and suggest that similar methods can be broadly applied to probe electronic inhomogeneities of moiré superlattices in other van der Waals heterostructures.

cond-mat.mes-hall

Photo-enhanced metastable c-axis electrodynamics in stripe ordered cuprate La$_{1.885}$Ba$_{0.115}$CuO$_{4}$

Quantum materials are amenable to non-equilibrium manipulation with light, enabling modification and control of macroscopic properties. Light-based augmentation of superconductivity is particularly intriguing. Copper-oxide superconductors exhibit complex interplay between spin order, charge order and superconductivity, offering the prospect of enhanced coherence by altering the balance between competing orders. We utilize terahertz time domain spectroscopy to monitor the c-axis Josephson Plasma Resonance (JPR) in La$_{2-x}$Ba$_{x}$CuO$_{4}$ (x = 0.115) as a direct probe of superconductivity dynamics following excitation with near infrared pulses. Starting from the superconducting state, c-axis polarized excitation with a fluence of 100 $μ$J/cm2 results in an increase of the far-infrared spectral weight by more than an order of magnitude as evidenced by a blueshift of the JPR, interpreted as resulting from non-thermal collapse of the charge order. The photo-induced signal persists well beyond our measurement window of 300 ps and exhibits signatures of spatial inhomogeneity. The electrodynamic response of this new metastable state is consistent with enhanced superconducting fluctuations. Our results reveal that La$_{2-x}$Ba$_{x}$CuO$_{4}$ is highly sensitive to non-equilibrium excitation over a wide fluence range, providing an unambiguous example of photo-induced modification of order-parameter competition.

cond-mat.supr-con

Theory of plasmon reflection by a 1D junction

We present a comprehensive study of the reflection of normally incident plasmon waves from a low-conductivity 1D junction in a 2D conductive sheet. Rigorous analytical results are derived in the limits of wide and narrow junctions. Two types of phenomena determine the reflectance, the cavity resonances within the junction and the capacitive coupling between the leads. The resonances give rise to alternating strong and weak reflection but are vulnerable to plasmonic damping. The capacitive coupling, which is immune to damping, induces a near perfect plasmon reflection in junctions narrower than $1/10$ of the plasmon wavelength. Our results are important for infrared 2D plasmonic circuits utilizing slot antennas, split gates or nanowire gates. They are also relevant for the implementation of nanoscale terahertz detectors, where optimal light absorption coincides with the maximal junction reflectance.

cond-mat.mes-hall

Nanoscale mapping and spectroscopy of non-radiative hyperbolic modes in hexagonal boron nitride nanostructures

The inherent crystal anisotropy of hexagonal boron nitride (hBN) sustains naturally hyperbolic phonon polaritons, i.e. polaritons that can propagate with very large wavevectors within the material volume, thereby enabling optical confinement to exceedingly small dimensions. Indeed, previous research has shown that nanometer-scale truncated nanocone hBN cavities, with deep subwavelength dimensions, support three-dimensionally confined optical modes in the mid-infrared. Due to optical selection rules, only a few of many such modes predicted theoretically have been observed experimentally via far-field reflection and scattering-type scanning near-field optical microscopy. The Photothermal induced resonance (PTIR) technique probes optical and vibrational resonances overcoming weak far-field emission by leveraging an atomic force microscope (AFM) probe to transduce local sample expansion due to light absorption. Here we show that PTIR enables the direct observation of previously unobserved, dark hyperbolic modes of hBN nanostructures. Leveraging these optical modes could yield a new degree of control over the electromagnetic near-field concentration, polarization and angular momentum in nanophotonic applications.

cond-mat.mes-hall