arXiv subjects

Michael Potthoff

Publications and source records attributed to Michael Potthoff.

At least 19 recordsLinked to original sources

arXiv2026

Topology and Quantum-Spin-Classical-Spin Crossover of the Gapped Kondo Effect

The gapped Kondo effect describes the screening of an $S=\frac12$ impurity spin locally coupled via an antiferromagnetic exchange interaction to a conduction-electron system exhibiting a finite hard gap. Using a combination of a Lanczos transformation and a self-consistent configuration-interaction scheme, we numerically investigate the local phase diagram. Furthermore, we show that the different phases can be characterized by several topological invariants: the conventional momentum-space Chern number of the underlying two-dimensional host system, corresponding to a Chern insulator; the B-space Chern number, defined by coupling the impurity spin to a fictitious local magnetic field $\boldsymbol B$, in the limit $B \to 0$; and the S-space Chern number, defined for a classical impurity spin, i.e., a vector of fixed length. The classical-spin limit is obtained for $B \to \infty$. By varying the field strength, we can therefore continuously interpolate between quantum-impurity-spin and classical-impurity-spin Hamiltonians and investigate whether the corresponding phase diagrams are likewise continuously connected. The gapped underscreened Kondo effect is studied for an impurity spin $S>\frac12$ as well as in the classical-spin limit approached via $B \to \infty$ or $S \to \infty$. Different variants of scattering theory are employed to interpret the resulting phases. Finally, the gapped two-channel overscreened Kondo effect, realized by coupling a quantum impurity spin equally to the local electron spins of both orbitals within a unit cell, is shown to be characterized by spontaneous particle-hole symmetry breaking. This leads to a highly nontrivial quantum-classical phase diagram.

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arXiv2026

Disorder-Induced Topological Phases in a Two-Dimensional Chern Insulator with Strong Magnetic Disorder

Strong directional disorder in local magnetic moments coupled to a Chern insulator gives rise to topological phases that cannot be continuously connected to the clean limit and are therefore genuinely disorder-driven. We demonstrate this in a spinful Qi-Wu-Zhang model of a two-dimensional Chern insulator coupled to disordered classical spins of unit length. The topological phase diagram is computed numerically using two complementary approaches: twisted boundary conditions and the topological Hamiltonian technique. Our results show that strong disorder can act as a fundamental topological mechanism rather than merely a perturbation. For strong exchange coupling, tuning the mass parameter reveals a transition between phases with different Chern numbers $C$. Remarkably, this transition is driven by zeros, rather than poles, of the disorder-averaged Green's function crossing the chemical potential, and has no analogue in any clean system. We further identify a strong-coupling phase with $C = 0$ that is nonetheless topologically nontrivial, characterized by a distinct Chern number $C^{(\mathrm{S})} \neq 0$ over the manifold of classical spin configurations. This phase is also disorder-driven, as $C^{(\mathrm{S})} = 0$ in the clean limit.

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arXiv2025

Exchangeless braiding of Majorana zero modes in weakly coupled Kitaev chains

Exchangeless braiding of Majorana modes is studied in minimal networks of weakly hybridized Kitaev chains of finite length using a rigorous many-body framework. In particular, for two coupled chains it is shown that exchangeless braiding is achieved by $2\pi$ rotations of the phase $\phi$ of the superconducting order parameter of one of the chains. This braiding protocol is verified by the numerical calculation of the non-Abelian Wilczek-Zee phase of the low-energy many-body subspaces ${\cal H}_{0}(\phi)$ based on the Bertsch-Robledo ground-state overlap formula. In the parameter space spanned by the total chain length, the strength of the weak hybridization connecting the chains, and the on-site potential, we identify two regions with different braiding outcomes, i.e., a projective $\sigma_{x}$-gate and a projective $\sigma_{z}$-gate phase. The transition between these phases is a continuous crossover, the location of which is reliably given by a simple four-Majorana mode model. This demonstrates the resilience of the anyonic properties of the Majorana modes against finite-size effects and weak links between Kitaev chains.

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arXiv2024

Microscopic theory of spin friction and dissipative spin dynamics

The real-time dynamics of local magnetic moments exchange coupled to a metallic system of conduction electrons is subject to dissipative friction even in the absence of spin-orbit coupling. Phenomenologically, this is usually described by a local Gilbert damping constant. Here, we use both linear response theory and adiabatic response theory to derive the spin friction microscopically for a generic single-band tight-binding model of the electronic structure. The resulting Gilbert damping is time-dependent and nonlocal. For a one-dimensional model, we compare the emergent relaxation dynamics as obtained from LRT and ART against each other and against the full solution of the microscopic equations of motion and demonstrate the importance of nonlocality, while the time dependence turns out to be irrelevant. In two dimensions and for a few magnetic moments in different geometries, it is found that the inclusion of nonlocal Gilbert damping can counterintuitively lead to longer relaxation times. Besides the distance dependence, the directional dependence of the nonlocal Gilbert damping turns out as very important. Our results are based on an expression relating the nonlocal Gilbert damping to the nonlocal tight-binding density of states close to the Fermi energy. This is exact in case of noninteracting electrons. Effects due to electronic correlations are studied within the random-phase approximation. For the Hubbard model at half filling and with increasing interaction strength, we find a strong enhancement of the nonlocality of spin friction.

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arXiv2024

Kondo Screening and Indirect Magnetic Exchange through a Conventional Superconductor Studied by the Density-Matrix Renormalization Group

The competition between the Kondo screening and indirect magnetic exchange in systems with two magnetic impurities coupled to a conventional s-wave superconductor gives rise to a nontrivial ground-state phase diagram. Here, we utilize the density-matrix renormalization group (DMRG) method and exploit the non-abelian spin-SU(2) symmetry to study the phase diagram for two quantum-spin-$\frac12$ impurities locally exchange coupled to large one-dimensional chains. The nonlocal inter-impurity exchange is treated as an emergent Ruderman-Kittel-Kasuya-Yosida (RKKY) coupling. We find qualitatively different phase diagrams for impurity spins coupled to sites with odd or even distances $d$ on the chain and a partial-Kondo-screened spin-doublet phase that extends over the whole range of local exchange couplings $J$ in the limit of weak superconducting pairing strength $\Delta$. Our numerical studies are complemented by exact diagonalization of small (quantum-box) systems and by perturbative-in-$J$ computations of the $d$ and $\Delta$ dependent RKKY interaction. It is thereby demonstrated that the specific system geometry is essential for our understanding of magnetic impurity interactions in superconducting hosts, and thus for insights into the control of quantum-state properties in nanoparticle systems and topological superconductivity.

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arXiv2024

Prerelaxation in quantum, classical, and quantum-classical two-impurity models

We numerically study the relaxation dynamics of impurity-host systems, focusing on the presence of long-lived metastable states in the non-equilibrium dynamics after an initial excitation of the impurities. In generic systems, an excited impurity coupled to a large bath at zero temperature is expected to relax and approach its ground state over time. However, certain exceptional cases exhibit metastability, where the system remains in an excited state on timescales largely exceeding the typical relaxation time. We study this phenomenon for three prototypical impurity models: a tight-binding quantum model of independent spinless fermions on a lattice with two stub impurities, a classical-spin Heisenberg model with two weakly coupled classical impurity spins, and a tight-binding quantum model of independent electrons with two classical impurity spins. Through numerical integration of the fundamental equations of motion, we find that all three models exhibit similar qualitative behavior: complete relaxation for nearest-neighbor impurities and incomplete or strongly delayed relaxation for next-nearest-neighbor impurities. The underlying mechanisms leading to this behavior differ between models and include impurity-induced bound states, emergent approximately conserved local observables, and exact cancellation of local and nonlocal dissipation effects.

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arXiv2023

Bound states and local topological phase diagram of classical impurity spins coupled to a Chern insulator

The existence of bound states induced by local impurities coupled to an insulating host depends decisively on the global topological properties of the host's electronic structure. In this context, we consider magnetic impurities modelled as classical unit-length spins that are exchange-coupled to the spinful Haldane model on the honeycomb lattice. We investigate the spectral flow of bound states with the coupling strength $J$ in both the topologically trivial and Chern-insulating phases. In addition to conventional $k$-space topology, an additional, spatially local topological feature is available, based on the space of impurity-spin configurations forming, in case of $R$ impurities, an $R$-fold direct product of two-dimensional spheres. Global $k$-space and local $S$-space topology are represented by different topological invariants, the first ($k$-space) Chern number and the $R$-th ($S$-space) spin-Chern number. We demonstrate that there is a local $S$-space topological transition as a function of $J$ associated with a change in the spin Chern number and work out the implications of this for the $J$-dependent local electronic structure close to the impurities and, in particular, for in-gap bound states. The critical exchange couplings' dependence on the parameters of the Haldane model, and thus on the $k$-space topological state, is obtained numerically to construct local topological phase diagrams for systems with $R=1$ and $R=2$ impurity spins.

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arXiv2023

Geometrical torque on magnetic moments coupled to a correlated antiferromagnet

The geometrical spin torque mediates an indirect interaction of magnetic moments, which are weakly exchange coupled to a system of itinerant electrons. It originates from a finite spin-Berry curvature and leads to a non-Hamiltonian magnetic-moment dynamics. We demonstrate that there is an unprecedentedly strong geometrical spin torque in case of an electron system, where correlations cause antiferromagnetic long-range order. The key observation is that the anomalous torque is strongly boosted by low-energy magnon modes emerging in the two-electron spin-excitation spectrum due to spontaneous breaking of SU(2) spin-rotation symmetry. As long as single-electron excitations are gapped out, the effect is largely universal, i.e., essentially independent of the details of the electronic structure, but decisively dependent on the lattice dimension and spatial and spin anisotropies. Analogous to the reasoning that leads to the Mermin-Wagner theorem, there is a lower critical dimension at and below which the spin-Berry curvature diverges.

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arXiv2022

Spin Berry curvature of the Haldane model

The feedback of the geometrical Berry phase, accumulated in an electron system, on the slow dynamics of classical degrees of freedom is governed by the Berry curvature. Here, we study local magnetic moments, modelled as classical spins, which are locally exchange coupled to the (spinful) Haldane model for a Chern insulator. In the emergent equations of motion for the slow classical-spin dynamics there is a an additional anomalous geometrical spin torque, which originates from the corresponding spin-Berry curvature. Due to the explicitly broken time-reversal symmetry, this is nonzero but usually small in a condensed-matter system. We develop the general theory and compute the spin-Berry curvature, mainly in the limit of weak exchange coupling, in various parameter regimes of the Haldane model, particularly close to a topological phase transition and for spins coupled to sites at the zigzag edge of the model in a ribbon geometry. The spatial structure of the spin-Berry curvature tensor, its symmetry properties, the distance dependence of its nonlocal elements and further properties are discussed in detail. For the case of two classical spins, the effect of the geometrical spin torque leads to an anomalous non-Hamiltonian spin dynamics. It is demonstrated that the magnitude of the spin-Berry curvature is decisively controlled by the size of the insulating gap, the system size and the strength of local exchange coupling.

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arXiv2022

Emergent Non-Abelian Gauge Theory in Coupled Spin-Electron Dynamics

A clear separation of the time scales governing the dynamics of "slow" and "fast" degrees of freedom often serves as a prerequisite for the emergence of an independent low-energy theory. Here, we consider (slow) classical spins exchange coupled to a tight-binding system of (fast) conduction electrons. The effective equations of motion are derived under the constraint that the quantum state of the electron system at any instant of time $t$ lies in the $n$-dimensional low-energy subspace for the corresponding spin configuration at $t$. The effective low-energy theory unfolds itself straightforwardly and takes the form of a non-abelian gauge theory with the gauge freedom given by the arbitrariness of the basis spanning the instantaneous low-energy sector. The holonomic constraint generates a gauge covariant spin-Berry curvature tensor in the equations of motion for the classical spins. In the non-abelian theory for $n>1$, opposed to the $n=1$ adiabatic spin dynamics theory, the spin-Berry curvature is generically nonzero, even for time-reversal symmetric systems. Its expectation value with the representation of the electron state is gauge invariant and gives rise to an additional {\em geometrical} spin torque. Besides anomalous precession, the $n\ge 2$ theory also captures the spin nutational motion, which is usually considered as a retardation effect. This is demonstrated by proof-of-principle numerical calculations for a minimal model with a single classical spin. Already for $n=2$ and in parameter regimes where the $n=1$ adiabatic theory breaks down, we find good agreement with results obtained from the full (unconstrained) theory.

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arXiv2021

Controlling the real-time dynamics of a spin coupled to the helical edge states of the Kane-Mele model

The time-dependent state of a classical spin locally exchange coupled to an edge site of a Kane-Mele model in the topologically non-trivial phase is studied numerically by solving the full set of coupled microscopic equations of motion for the spin and the electron system. Dynamics in the long-time limit is accessible thanks to dissipative boundary conditions, applied to all but the zigzag edge of interest. We study means to control the state of the spin via transport of a spin-polarization cloud through the helical edge states. The cloud is formed at a distant edge site using a local magnetic field to inject an electron spin density and released by suddenly switching off the injection field. This basic process, consisting of spin injection, propagation of the spin-polarization cloud, and scattering of the cloud from the classical spin, can be used to steer the spin state in a controlled way. We find that the effect of a single basic process can be reverted to a high degree with a subsequent process. Furthermore, we show that by concatenating several basic injection-propagation-scattering processes, the spin state can be switched completely and that a full reversal can be achieved.

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arXiv2020

Long-time relaxation dynamics of a spin coupled to a Chern insulator

The relaxation of a classical spin, exchange coupled to the local magnetic moment at an edge site of the one-dimensional spinful Su-Schrieffer-Heeger model is studied numerically by solving the full set of equations of motion. A Lindblad coupling of a few sites at the opposite edge to an absorbing bath ensures that convergence with respect to the system size is achieved with only a moderate number of core sites. This allows us to numerically exactly study the long-time limit and to determine the parameter regimes where spin relaxation takes place. Corresponding dynamical phase diagrams for the topologically trivial and the nontrivial cases are constructed. The dynamical phase boundaries, the role of the topological edge state and its internal Zeeman splitting for the spin-relaxation process, as well as incomplete spin relaxation on long time scales can be explained within the framework of a renormalized linear-response approach when explicitly taking retardation effects and nonequilibrium spin-exchange processes into account.

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arXiv2020

Interacting Chern Insulator in Infinite Spatial Dimensions

We study a generic model of a Chern insulator supplemented by a Hubbard interaction in arbitrary even dimension $D$ and demonstrate that the model remains well-defined and nontrivial in the $D \to \infty$ limit. Dynamical mean-field theory is applicable and predicts a phase diagram with a continuum of topologically different phases separating a correlated Mott insulator from the trivial band insulator. We discuss various features, such as the elusive distinction between insulating and semi-metal states, which are unconventional already in the non-interacting case. Topological phases are characterized by a non-quantized Chern density replacing the Chern number as $D\to \infty$.

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arXiv2020

Non-Hamiltonian dynamics of indirectly coupled classical impurity spins

We discuss the emergence of an effective low-energy theory for the real-time dynamics of two classical impurity spins within the framework of a prototypical and purely classical model of indirect magnetic exchange: Two classical impurity spins are embedded in a host system which consists of a finite number of classical spins localized on the sites of a lattice and interacting via a nearest-neighbor Heisenberg exchange. An effective low-energy theory for the slow impurity-spin dynamics is derived for the regime, where the local exchange coupling between impurity and host spins is weak. To this end we apply the recently developed adiabatic spin dynamics (ASD) theory. Besides the Hamiltonian-like classical spin torques, the ASD additionally accounts for a novel topological spin torque that originates as a holonomy effect in the close-to-adiabatic-dynamics regime. It is shown that the effective low-energy precession dynamics cannot be derived from an effective Hamilton function and is characterized by a non-vanishing precession frequency even if the initial state deviates only slightly from a ground state. The effective theory is compared to the fully numerical solution of the equations of motion for the whole system of impurity and host spins to identify the parameter regime where the adiabatic effective theory applies. Effective theories beyond the adiabatic approximation must necessarily include dynamic host degrees of freedom and go beyond the idea of a simple indirect magnetic exchange. We discuss an example of a generalized constrained spin dynamics which does improve the description but also fails for certain geometrical setups.

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arXiv2020

Accessing long timescales in the relaxation dynamics of spins coupled to a conduction-electron system using absorbing boundary conditions

The relaxation time of a classical spin interacting with a large conduction-electron system is computed for a weak magnetic field, which initially drives the spin out of equilibrium. We trace the spin and the conduction-electron dynamics on a time scale, which exceeds the characteristic electronic scale that is set by the inverse nearest-neighbor hopping by more than five orders of magnitude. This is achieved with a novel construction of absorbing boundary conditions, which employs a generalized Lindblad master-equation approach to couple the edge sites of the conduction-electron tight-binding model to an external bath. The failure of the standard Lindblad approach to absorbing boundaries is traced back to artificial excitations initially generated due to the coupling to the bath. This can be cured by introducing Lindblad parameter matrices and by fixing those matrices to perfectly suppress initial-state artifacts as well as reflections of physical excitations propagating to the system boundaries. Numerical results are presented and discussed for generic one-dimensional models of the electronic structure.

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arXiv2020

Topological spin torque emerging in classical-spin systems with different time scales

In classical spin systems with two largely different inherent time scales, the configuration of the fast spins almost instantaneously follows the slow-spin dynamics. We develop the emergent effective theory for the slow-spin degrees of freedom and demonstrate that this generally includes a topological spin torque. This torque gives rise to anomalous real-time dynamics. It derives from the holonomic constraints defining the fast-spin configuration space and is given in terms of a topological charge density which becomes a quantized homotopy invariant when integrated.

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arXiv2019

Magnetic Doublon Bound States in the Kondo Lattice Model

We present a novel pairing mechanism for electrons, mediated by magnons. These paired bound states are termed ``magnetic doublons''. Applying numerically exact techniques (full diagonalization and the density-matrix renormalization group, DMRG) to the Kondo lattice model at strong exchange coupling $J$ for different fillings and magnetic configurations, we demonstrate that magnetic doublon excitations exist as composite objects with very weak dispersion. They are highly stable, support a novel ``inverse'' colossal magnetoresistance and potentially other effects.

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arXiv2019

Pump-probe Auger-electron spectroscopy of Mott insulators

In high-resolution core-valence-valence (CVV) Auger electron spectroscopy from the surface of a solid at thermal equilibrium, the main correlation satellite, visible in the case of strong valence-electron correlations, corresponds to a bound state of the two holes in the final state of the CVV Auger process. We discuss the physical significance of this satellite in nonequilibrium pump-probe Auger spectroscopy by numerical analysis of a single-band Hubbard-type model system including core states and a continuum of high-energy scattering states. It turns out that the spectrum of the photo-doped system, due to the increased double occupancy, shares features with the equilibrium spectrum at higher fillings. The pumping of doublons can be watched when working with overlapping pulses at short $\Delta t$. For larger pump-probe delays $\Delta t$ and on the typical femtosecond time scale for electronic relaxation processes, spectra are hardly $\Delta t$-dependent, reflecting the high stability of bound two-hole states for strong Hubbard-$U$. We argue that taking into account the spatial expansion of single-particle orbitals when these are doubly occupied, as described by the dynamical Hubbard model, produces an oscillation of the barycenter of the satellite as a function of $\Delta t$. Pump-probe Auger-electron spectroscopy is thus highly sensitive to dynamical screening of the Coulomb interaction.

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