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Michael Vogl

Publications and source records attributed to Michael Vogl.

36 records · Page 2Linked to original sources

Light driven magnetic transitions in transition metal dichalcogenide heterobilayers

Motivated by the recent excitement around the physics of twisted transition metal dichalcogenide (TMD) multilayer systems, we study strongly correlated phases of TMD heterobilayers under the influence of light. We consider both waveguide light and circularly polarized light. The former allows for longitudinally polarized light, which in the high frequency limit can be used to selectively modify interlayer hoppings in a tight-binding model. We argue based on quasi-degenerate perturbation theory that changes to the interlayer hoppings can be captured as a modulation to the strength of the moiré potential in a continuum model. As a consequence, waveguide light can be used to drive transitions between a myriad of different magnetic phases, including a transition from a $120^\circ$ Neel phase to a stripe ordered magnetic phase, or from a spin density wave phase to a paramagnetic phase, among others. When the system is subjected to circularly polarized light we find that the effective mass of the active TMD layer is modified by an applied electromagnetic field. By simultaneously applying waveguide light and circularly polarized light to a system, one has a high level of control in moving through the phase diagram in-situ. Lastly, we comment on the experimental feasibility of Floquet state preparation and argue that it is within reach of available techniques when the system is coupled to a judiciously chosen bath.

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Deep learning of deformation-dependent conductance in thin films: nanobubbles in graphene

Motivated by the ever-improving performance of deep learning techniques, we design a mixed input convolutional neural network approach to predict transport properties in deformed nanoscale materials using a height map of deformations (from scanning probe information) as input. We employ our approach to study electrical transport in a graphene nanoribbon deformed by a number of randomly positioned nano-bubbles. Our network is able to make conductance predictions valid to an average error of 4.3\%. We demonstrate that such low average errors are achieved by including additional inputs like energy in a highly redundant fashion, which allows predictions that are 30-40\% more accurate than conventional architectures. We demonstrate that the same method can learn to predict the valley-resolved conductance, with success specifically in identifying the energy at which inter-valley scattering becomes prominent. We demonstrate the robustness of the approach by testing the pre-trained network on samples with deformations differing in number and shape from the training data. We employ a graph theoretical analysis of the structure and outputs of the network and conclude that a tight-binding Hamiltonian is effectively encoded in the first layer of the network. We confirm our graph theoretical analysis numerically for different hopping processes in a trained network and find the result to be accurate within an error of 1\%. Our approach contributes a new theoretical understanding and a refined methodology to the application of deep learning for the determination transport properties based on real-space disorder information.

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Fidelity of the Kitaev honeycomb model under a quench

Motivated by rapid developments in the field of quantum computing and the increasingly diverse nature of qubits, we theoretically study the influence that quenched outside disturbances have in an intermediately long time limit. We consider localized imperfections, uniform fields, noise, and couplings to an environment which we study in a unified framework using a prototypical but idealized interacting quantum device - the Kitaev honeycomb model. Our study focuses on the quantum state robustness in response to an outside magnetic field, a magnetic bath, magnetic noise, magnetic impurities, and a noisy impurity. As indicators for quantum robustness, we use the Uhlmann fidelty of the ground state and excited spinon states after a quench. We find that the time dependence of the fidelity often depends crucially on whether the system is gapped. We find that in the gapped case the fidelity decays to a constant value under noiseless quenches, while in a gapless system it exhibits algebraic decay. In all other situations studied, such as coupling to a bath and noisy quenches, both gapped and gapless systems exhibit a universal form for the long-time fidelity, $Ce^{-αt}t^{-β}$, where the values of $C$, $α$, and $β$ depend on physical parameters such as system size, disturbance strength, etc. Therefore, our work provides estimates for the intermediate-long time stability of a quantum device and it suggests under what conditions there appear the hallmarks of an orthogonality catastrophe in the time-dependence of the fidelity. Our work provides engineering guidelines for quantum devices in quench design and system size.

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Tunneling phase diagrams in anisotropic Multi-Weyl semimetals

Motivated by the exciting prediction of Multi-Weyl topological semimetals that are stabilized by point group symmetries [Phys. Rev. Lett. 108 (2012) 266802], we study tunneling phenomena for a class of anisotropic Multi-Weyl semimetals. We find that a distant detector for different ranges of an anisotropy parameter $λ$ and incident angle $θ$ will measure a different number of propagating transmitted modes. We present these findings in terms of phase diagrams that is valid for an incoming wave with fixed wavenumber $k$--energy is not fixed. To gain a deeper understanding of this phenomenon we then focus on the simplest case of an anisotropic quadratic Weyl-semimetal and analyze tunneling coefficients analytically and numerically to confirm the observations from the phase diagram. Our results show non-analytical behavior, which is the hallmark of a phase transition. This serves as a motivation to make a formal analogy with phase transitions that are known from statistical mechanics. Specifically, we argue that the long distance limit in our tunneling problem takes the place of the thermodynamic limit in statistical mechanics. More precisely, find a direct formal connection to the recently developed formalism for dynamical phase transitions [Reports on Progress in Physics 81 (5) (2018) 054001]. We propose that this analogy to phase transitions can help classify transport properties in exotic semimetals.

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Chiral limits and effect of light on the Hofstadter butterfly in twisted bilayer graphene

We study the magnetic field induced Hofstadter butterfly in twisted bilayer graphene (TBG) in various kinds of situations. First, we study the equilibrium case and identify the interlayer hopping processes that are most crucial for the appearance of a Hofstadter butterfly. Surprisingly, the hopping processes that are important for the appearance of the Hofstadter butterfly can be categorized as AA stacking type - that is interlayer hoppings between equivalent sublattices. This is in contrast to AB/BA-type hoppings that are important for the appearance of flat bands in magic angle TBG and were discussed in [Phys. Rev. Lett. 122, 106405 (2019)]. We also find that if AB-type interlayer-hopping processes are turned off the resulting model is chiral but differs from the model discussed in \cite{Tarnopolsky}. Therefore, TBG has two separate chiral limits - one of them is important to understand the formation of flat bands and the other for the Hofstadter butterfly. Taking this as motivation we discuss how the role of AA-type hoppings in combination with lattice relaxation effects can make individual Landau levels slightly harder to resolve in an experimental setting than one would expect from a non-relaxed lattice setting. Finally, we consider the impact of different forms of light on the fractal structure of the butterfly. Particularly, we study the impact of circularly polarized light and longitudinal light originating from a waveguide. As the system is exposed to circularly polarized light we find butterflies with increasingly pronounced asymmetry with respect to energy $E=0$. This is due to the introduction of a gap term that breaks the chiral symmetries for both of the two chiral limits mentioned above. Lastly, we study the effect of longitudinal light that can be produced at the exit of a waveguide, in a slightly simplified model. Here, we find ...

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Direct driving of electronic and phononic degrees of freedom in a honeycomb bilayer with infrared light

We study theoretically AB-stacked honeycomb bilayers driven by light in resonance with an infrared phonon within a tight-binding description. We characterize the phonon properties of honeycomb bilayers with group theory and construct an electronic time-dependent tight-binding model for the system following photo-excitation in resonance with an infrared phonon. We adopt an "atomically adiabatic" approximation, introduced by Mohantya and Heller PNAS 116, 18316 (2019) to describe classically vibrating nuclei, but obtain the Floquet quasienergy spectrum associated with the time-dependent model exactly. We introduce a general scheme to disentangle the complex low-frequency Floquet spectrum to elucidate the relevant Floquet bands. As a prototypical example, we consider bilayer graphene. We find that light in the low-frequency regime can induce a bandgap in the quasienergy spectrum in the vicinity of the K points even if it is linearly polarized, in contrast with the expectations within the Born-Oppenheimer approximation and the high-frequency regime. Finally, we analyze the diabaticity of the driven electron and driven phonon processes and found contrasting effects on the autocorrelation functions at the same driving frequency: driven phonons preserve the character of the initial state while driven electrons exhibit strong deviations within a few drive cycles. The procedure outlined here can be applied to other materials to describe the combined effects of low-frequency light on phonons and electrons.

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Floquet engineering and non-equilibrium topological maps in twisted trilayer graphene

Motivated by the recent experimental realization of twisted trilayer graphene and the observed superconductivity that is associated with its flat bands at specific angles, we study trilayer graphene under the influence of different forms of light in the non-interacting limit. Specifically, we study four different types of stacking configurations with a single twisted layer. In all four cases, we study the impact of circularly polarized light and longitudinal light coming from a waveguide. We derive effective time-independent Floquet Hamiltonians and review light-induced changes to the band structure. For circularly polarized light, we find band flattening effects as well as band gap openings. We emphasize that there is a rich band topology, which we summarize in Chern number maps that are different for all four studied lattice configurations. The case of a so-called ABC stacking with top layer twist is especially rich and shows a different phase diagram depending on the handedness of the circularly polarized light. Consequently, we propose an experiment where this difference in typologies could be captured via optical conductivity measurements. In contrast for the case of longitudinal light that is coming from a waveguide, we find that the band structure is very closely related to the equilibrium one but the magic angles can be tuned in-situ by varying the intensity of the incident beam of light.

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Fractional Spin fluctuations and quantum liquid signature in Gd2ZnIrO6

Hitherto, the discrete identification of quantum spin liquid phase, holy grail of condensed matter physics, remains a challenging task experimentally. However, the precursor of quantum spin liquid state may reflect in the spin dynamics even in the paramagnetic phase over a wide temperature range as conjectured theoretically. Here we report comprehensive inelastic light (Raman) scattering measurements on the Ir based double perovskite, Gd2ZnIrO6, as a function of different incident photon energies and polarization in a broad temperature range. Our results evidenced the spin fractionalization within the paramagnetic phase reflected in the emergence of a polarization independent quasi-elastic peak at low energies with lowering temperature. Also, the fluctuating scattering amplitude measured via dynamic Raman susceptibility increases with lowering temperature and decreases mildly upon entering into long-range magnetic ordering phase, below 23 K, suggesting the magnetic origin of these fluctuations. This anomalous scattering response is thus indicative of fluctuating fractional spin evincing the quantum spin liquid phase in a three-dimensional double perovskite system.

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Tunneling in an anisotropic cubic Dirac semi-metal

Motivated by a recent first principles prediction of an anisotropic cubic Dirac semi-metal in a real material Tl(TeMo)$_3$, we study the behavior of electrons tunneling through a potential barrier in such systems. To clearly investigate effects from different contributions to the Hamiltonian we study the model in various limits. First, in the limit of a very thin material where the linearly dispersive $z$-direction is frozen out at zero momentum and the dispersion in the $x$-$y$ plane is rotationally symmetric. In this limit we find a Klein tunneling reminiscent of what is observed in single layer graphene and linearly dispersive Dirac semi-metals. Second, an increase in thickness of the material leads to the possibility of a non-zero momentum eigenvalue $k_z$ that acts as an effective mass term in the Hamiltonian. We find that these lead to a suppression of Klein tunneling. Third, the inclusion of an anisotropy parameter $λ\neq 1$ leads to a breaking of rotational invariance. Furthermore, we observed that for different values of incident angle $θ$ and anisotropy parameter $λ$ the Hamiltonian supports different numbers of modes propagating to infinity. We display this effect in form of a diagram that is similar to a phase diagram of a distant detector. Fourth, we consider coexistence of both anisotropy and non-zero $k_z$ but do not find any effect that is unique to the interplay between non-zero momentum $k_z$ and anisotropy parameter $λ$. Last, we studied the case of a barrier that was placed in the linearly dispersive direction and found Klein tunneling $T-1\propto θ^6+\mathcal{O}(θ^8)$ that is enhanced when compared to the Klein tunneling in linear Dirac semi-metals or graphene where $T-1\propto θ^2+\mathcal{O}(θ^4)$.

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Low-frequency and Moiré Floquet engineering: a review

We review recent work on low-frequency Floquet engineering and its application to quantum materials driven by light, emphasizing van der Waals systems hosting Moiré superlattices. These non-equilibrium systems combine the twist-angle sensitivity of the band structures with the flexibility of light drives. The frequency, amplitude, and polarization of light can be easily tuned in experimental setups, leading to platforms with on-demand properties. First, we review recent theoretical developments to derive effective Floquet Hamiltonians in different frequency regimes. We apply some of these theories to study twisted graphene and twisted transition metal dichalcogenide systems irradiated by light in free space and inside a waveguide. We study the changes induced in the quasienergies and steady-states, which can lead to topological transitions. Next, we consider van der Waals magnetic materials driven by low-frequency light pulses in resonance with the phonons. We discuss the phonon dynamics induced by the light and resulting magnetic transitions from a Floquet perspective. We finish by outlining new directions for Moiré-Floquet engineering in the low-frequency regime and their relevance for technological applications.

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Floquet-engineering topological transitions in a twisted transition metal dichalcogenide homobilayer

Motivated by the recent experimental realization of twisted transition metal dichalcogenide bilayers, we study a simplified model driven by different forms of monochromatic light. As a concrete and representative example we use parameters that correspond to a twisted MoTe$_2$ homobilayer. First, we consider irradiation with circularly polarized light in free space and demonstrate that the corresponding Floquet Hamiltonian takes the same form as the static Hamiltonian, only with a constant overall shift in quasi-energy. This is in stark contrast to twisted bilayer graphene, where new terms are typically generated under an analagous drive. Longitudinal light, on the other hand, which can be generated from the transverse magnetic mode in a waveguide, has a much more dramatic effect--it renormalizes the tunneling strength between the layers, which effectively permits the tuning of the twist angle {\em in-situ}. We find that, by varying the frequency and amplitude of the drive, one can induce a topological transition that cannot be obtained with the traditional form of the Floquet drive in free space. Furthermore, we find that strong drives can have a profound effect on the layer pseudospin texture of the twisted system, which coincides with multiple simultaneous band gap closings in the infinite-frequency limit. Surprisingly, these bandgap closings are not associated with topological transitions. For high but finite drive frequencies near $0.7$eV, the infinite-frequency band crossings become band gap minima of the order of $10^{-6}$ eV or smaller.

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Exact resummation of the Holstein-Primakoff expansion and differential equation approach to operator square-roots

Operator square-roots are ubiquitous in theoretical physics. They appear, for example, in the Holstein-Primakoff representation of spin operators and in the Klein-Gordon equation. Often the use of a perturbative expansion is the only recourse when dealing with them. In this work we show that under certain conditions differential equations can be derived which can be used to find perturbatively inaccessible approximations to operator square-roots. Specifically, for the number operator $\hat n=\hat a^†a$ we show that the square-root $\sqrt{\hat n}$ near $\hat n=0$ can be approximated by a polynomial in $\hat n$. This result is unexpected because a Taylor expansion fails. A polynomial expression in $\hat n$ is possible because $\hat n$ is an operator, and its constituents $a$ and $a^†$ have a non-trivial commutator $[a,a^†]=1$ and do not behave as scalars. We apply our approach to the zero mass Klein-Gordon Hamiltonian in a constant magnetic field, and as a main application, the Holstein-Primakoff representation of spin operators, where we are able to find new expressions that are polynomial in bosonic operators. We prove that these new expressions exactly reproduce spin operators. Our expressions are manifestly Hermitian, which offer an advantage over other methods, such as the Dyson-Maleev representation.

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Floquet engineering of twisted double bilayer graphene

Motivated by the recent experimental realization of twisted double bilayer graphene (TDBG) samples we study, both analytically and numerically, the effects of circularly polarized light propagating in free space and confined into a waveguide on the band structure and topological properties of these systems. These two complementary Floquet protocols allow us to selectively tune different parameters of the system by varying the intensity and the frequency of the light. For the drive protocol in free space, in the high-frequency regime, we find that in TDBG with AB/BA stacking, we can selectively close the zone-center quasienergy gaps around one valley while increasing the gaps near the opposite valley by tuning the parameters of the drive. In TDBG with AB/AB stacking, a similar effect can be obtained upon the application of a perpendicular static electric field. Furthermore, we study the topological properties of the driven system in different settings, provide accurate effective Floquet Hamiltonians, and show that relatively strong drives can generate flat bands. On the other hand, longitudinal light confined into a waveguide couples to the components of the interlayer hopping that are perpendicular to the TDBG sheet, allowing for selective engineering of the bandwidth of Floquet zone center quasienergy bands without breaking the symmetries of the static system.

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Effective Floquet Hamiltonians for periodically-driven twisted bilayer graphene

We derive effective Floquet Hamiltonians for twisted bilayer graphene driven by circularly polarized light in two different regimes beyond the weak-drive, high frequency regime. First, we consider a driving protocol relevant for experiments with frequencies smaller than the bandwidth and weak amplitudes and derive an effective Hamiltonian, which through a symmetry analysis, provides analytical insight into the rich effects of the drive. We find that circularly polarized light at low frequencies can selectively decrease the strength of AA-type interlayer hopping while leaving the AB-type unaffected. Then, we consider the intermediate frequency, and intermediate-strength drive regime. We provide a compact and accurate effective Hamiltonian which we compare with the Van Vleck expansion and demonstrate that it provides a significantly improved representation of the exact quasienergies. Finally, we discuss the effect of the drive on the symmetries, Fermi velocity and the gap of the Floquet flat bands.

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Floquet engineering of interlayer couplings: Tuning the magic angle of twisted bilayer graphene at the exit of a waveguide

We introduce a new approach that allows one complete control over the modulation of the effective twist angle change in few-layer van der Waals heterostructures by irradiating them with longitudinal waves of light at the end of a waveguide. As a specific application, we consider twisted bilayer graphene and show that one can tune the magic angles to be either larger or smaller, allowing in-situ experimental control of the phase diagram of this and other related materials. A waveguide allows one to circumvent the free-space constraints on the absence of longitudinal electric field components of light. We propose to place twisted bilayer graphene at a specific location at the exit of a waveguide, such that it is subjected to purely longitudinal components of a transverse magnetic modes (TM) wave.

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Effective Floquet Hamiltonian in the low-frequency regime

We develop a theory to derive effective Floquet Hamiltonians in the weak drive and low-frequency regime. We construct the theory in analogy with band theory for electrons in a spatially-periodic and weak potential, such as occurs in some crystalline materials. As a prototypical example, we apply this theory to graphene driven by circularly polarized light of low intensity. We find an analytic expression for the effective Floquet Hamiltonian in the low-frequency regime which accurately predicts the quasienergy spectrum and the Floquet states. Furthermore, we identify self-consistency as the crucial feature effective Hamiltonians in this regime need to satisfy to achieve a high accuracy. The method is useful in providing a realistic description of off-resonant drives for multi-band solid state systems where light-induced topological band structure changes are sought.

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Analogue of Hamilton-Jacobi theory for the time-evolution operator

In this paper we develop an analogue of Hamilton-Jacobi theory for the time-evolution operator of a quantum many-particle system. The theory offers a useful approach to develop approximations to the time-evolution operator, and also provides a unified framework and starting point for many well-known approximations to the time-evolution operator. In the important special case of periodically driven systems at stroboscopic times, we find relatively simple equations for the coupling constants of the Floquet Hamiltonian, where a straightforward truncation of the couplings leads to a powerful class of approximations. Using our theory, we construct a flow chart that illustrates the connection between various common approximations, which also highlights some missing connections and associated approximation schemes. These missing connections turn out to imply an analytically accessible approximation that is the "inverse" of a rotating frame approximation and thus has a range of validity complementary to it. We numerically test the various methods on the one-dimensional Ising model to confirm the ranges of validity that one would expect from the approximations used. The theory provides a map of the relations between the growing number of approximations for the time-evolution operator. We describe these relations in a table showing the limitations and advantages of many common approximations, as well as the new approximations introduced in this paper.

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A flow equation approach to periodically driven quantum systems

We present a theoretical method to generate a highly accurate {\em time-independent} Hamiltonian governing the finite-time behavior of a time-periodic system. The method exploits infinitesimal unitary transformation steps, from which renormalization group-like flow equations are derived to produce the effective Hamiltonian. Our tractable method has a range of validity reaching into frequency regimes that are usually inaccessible via high frequency $ω$ expansions in the parameter $h/ω$, where $h$ is the upper limit for the strength of local interactions. We demonstrate our approach on both interacting and non-interacting many-body Hamiltonians where it offers an improvement over the more well-known Magnus expansion and other high frequency expansions. For the interacting models, we compare our approximate results to those found via exact diagonalization. While the approximation generally performs better globally than other high frequency approximations, the improvement is especially pronounced in the regime of lower frequencies and strong external driving. This regime is of special interest because of its proximity to the resonant regime where the effect of a periodic drive is the most dramatic. Our results open a new route towards identifying novel non-equilibrium regimes and behaviors in driven quantum many-particle systems.

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