arXiv subjects

Michael Weinert

Publications and source records attributed to Michael Weinert.

At least 19 recordsLinked to original sources

arXiv2026

Precision masses of neutron-rich platinum and gold nuclei reveal enhanced $N=126$ shell strength below doubly-magic $^{208}$Pb

The heaviest stable nuclei in the universe owe their existence to quantum shell structure, the grouping of protons and neutrons into discrete energy levels separated by gaps. The largest known neutron shell gap in stable nuclei, at $N=126$, stabilizes doubly-magic $^{208}$Pb and is responsible for the characteristic abundance peak of heavy elements near gold and platinum produced by the rapid neutron-capture process (r-process). Whether this shell gap persists as protons are removed from lead is a question central to both nuclear structure and the modeling of heavy-element synthesis, yet it has remained unanswered due to the extraordinary difficulty of producing the relevant neutron-rich nuclei. Direct experimental knowledge in this region was essentially absent. Here we report the first precision mass measurements of $^{203,204}$Pt and $^{204,205,206}$Au, performed at GSI using a novel combination of Schottky and isochronous mass spectrometry in a heavy-ion storage ring. The $N=126$ isotones $^{204}$Pt and $^{205}$Au are more strongly bound than the extrapolated trend of the previously known mass surface by 403 and 464~keV, respectively, revealing an unexpectedly enhanced $N=126$ shell strength below doubly-magic $^{208}$Pb. Furthermore, the proton-neutron interaction strength exhibits a hitherto unobserved bifurcation at $N=126$ as protons are removed from $^{208}$Pb. Our results redefine the nuclear mass surface in the neutron-rich heavy-element region and provide direct experimental benchmarks for theoretical models whose extrapolations toward more exotic nuclei are essential for r-process nucleosynthesis calculations.

nucl-ex↗

arXiv2025

Origin of sublattice particle-hole asymmetry in monolayer FeSe superconductors

In iron-based superconductors, the two Fe atoms in the unit cell are typically related by crystal symmetries; therefore, we expect no intra-unit cell variations in the superconducting gap. However, recent experiments have challenged this expectation, reporting intra-unit cell variations in the gap with an unusual particle-hole asymmetry. Here, we examine the origin of this asymmetry between the two Fe sublattices in monolayer FeSe grown on SrTiO$_3$. We reveal that, in addition to the substrate-induced broken inversion symmetry, substrate nematic symmetry breaking is key to observing this asymmetry. We further identify two possible mechanisms through which this can occur. The first is through an odd-parity gap function that coexists with an extended $s$-wave function. The second is via a nodeless $d$-wave gap function that develops in the presence of a symmetry-breaking substrate. We argue that the latter mechanism is more physical. To test our theory, we performed scanning tunneling spectroscopy measurements across the nematic domain walls, which exhibit a clear enhancement of the asymmetry between the two Fe sublattices. In addition, we reveal that the observed sublattice particle-hole asymmetry is associated with odd-frequency pairing correlations, providing an experimental realization of this unusual pairing correlation.

cond-mat.supr-con↗

arXiv2025

Symmetry-required Orbital Selectivity in Monolayer FeSe

Orbital-selective correlations have been observed to play an important role in Fe-based superconductors. Here, in contrast to previous site-local Mott transition-based origins, we present a band-theory-based mechanism for orbital-selective physics in monolayer FeSe, for which only electron pockets appear. Underlying our mechanism is the observation in density functional theory (DFT) calculations that around the M point in the Brillouin zone, antiferromagnetic fluctuations are strongly coupled to electrons in $x^2-y^2$ orbitals but weakly coupled to those in $\{xz,yz\}$ orbitals. Symmetry-arguments reveal that this orbital selective coupling originates from the different intertwined orbital and Fe-site sublattice Bloch wavefunctions for these two sets of orbitals at the M point, specifically, the $x^2-y^2$ orbitals can be Fe-site localized. The strong coupling of electrons in $x^2-y^2$ orbitals to the magnetic fluctuations enables orbital-selective electronic renormalizations that can account for important features of our angle-resolved photoemission spectroscopy (ARPES) measurements. Our symmetry-required mechanism for orbital selective physics can be generalized to a range of crystal space groups with four-fold and six-fold screw axes.

cond-mat.str-el↗

arXiv2025

Rigid muffin-tin approximation in plane-wave codes for fast modeling of phonon-mediated superconductors

We present a pseudopotential-based plane-wave implementation of the rigid muffin-tin approximation (RMTA), offering a computationally efficient alternative to its traditional use in all-electron codes. This approach enables the evaluation of angular-momentum-resolved electron-phonon matrix elements and McMillan-Hopfield parameters of not only elemental transition metals but also their compounds. The results are benchmarked against full-potential linearized augmented plane wave calculations, showing excellent agreement. We further outline a practical route to extract atom- and symmetry-type-resolved electron-phonon coupling constants. By enabling the use of RMTA descriptors within high-throughput workflows, this framework significantly lowers the computational cost of screening candidate superconductors, providing a valuable tool for materials discovery.

cond-mat.supr-con↗

arXiv2025

Correlation Enhanced Electron-Phonon Coupling in FeSe/SrTiO$_3$ at a Magic Angle

While a predictive theory for unconventional superconductivity in Fe-based superconductors remains elusive, an extensively debated aspect is the interaction between phonons and strongly correlated electrons, and its potential role in the pairing mechanism. Here, through the combination of first principles dynamical mean field theory calculations and epitaxial growth of the single-layer FeX (X=Se, S, Te) on SrTiO$_3$ (STO)(001) substrate, which facilitates the controlled distortion of the FeX$_4$ tetrahedron, we demonstrate an unique superconducting dome where the superconducting gap peaks at a `magic' angle of the FeX$_4$ tetrahedron and the electron-phonon coupling (EPC) for the A$_{1g}$ mode is maximized for the FeSe film. Our findings uncover a significant role of electronic correlations in strengthening Cooper pairing in unconventional superconductors by enhancing EPC.

cond-mat.str-el↗

arXiv2025

Light-driven lattice metastability for enhanced superconductivity in FeSe/SrTiO3

Driven quantum materials with on demand properties controlled by external stimuli are critical for emergent quantum technology. In optically tunable superconducting heterostructures, the lattice responses at the buried interface may hold the key to the light susceptibility but is very challenging to detect. In this work, a nondestructive synchrotron-based X-ray scattering phase-retrieval technique is implemented in monolayer-FeSe/SrTiO3 heterostructures to capture the three-dimensional interfacial atomic displacements in-situ as the interface superconductivity is actively manipulated by light. It is found that the interlayer sliding between FeSe and SrTiO3 can drastically alter how the lattice responds to the light. In domains with selected stacking configurations, the interface transforms the very weak photoexcitation in SrTiO3 into significant Fe-atom displacements in FeSe and generate metastable interfacial structures that can lead to a persistent superconductivity enhancement. These findings demonstrate an effective strategy for achieving greatly amplified light-lattice coupling for efficient quantum phase manipulations at designed interfaces.

cond-mat.mtrl-sci↗

arXiv2025

Anisotropic response of defect bound states to magnetic field in epitaxial FeSn films

Crystal defects, whether intrinsic or engineered, drive many fundamental phenomena and novel functionalities of quantum materials. Here, we report symmetry-breaking phenomena induced by Sn-vacancy defects on the surface of epitaxial Kagome antiferromagnet FeSn films using low-temperature scanning tunneling microscopy and spectroscopy. Near the Sn-vacancy defects, anisotropic quasiparticle interference patterns are observed in the differential conductance dI/dV maps, indicating two-fold electronic states that break the 6-fold rotational symmetry of the Kagome layer. Furthermore, the Sn-vacancy defects induce bound states that exhibit anomalous Zeeman shifts under an out-of-plane magnetic field, where their energy shifts linearly towards higher energy independent of the direction of the magnetic field. Under an in-plane magnetic field, the shift of the bound state energy also shows a two-fold oscillating behavior as a function of the azimuth angle. These findings demonstrate defect-enabled new functionalities in Kagome antiferromagnets for potential applications in nanoscale spintronic devices.

cond-mat.mtrl-sci↗

arXiv2025

Unraveling Enhanced Superconductivity in Single-layer FeSe through Substrate Surface Terminations

Single-layer FeSe films grown on (001) SrTiO3 substrates have shown a significant increase in superconducting transition temperature compared to bulk FeSe. Several mechanisms have been proposed to explain such enhancement, including electron doping, interfacial electron-phonon coupling, and strong electron correlations. To pinpoint the primary driver, we grew FeSe films on SrTiO3 substrates with coexisting TiO2 and SrO surface terminations. Scanning tunneling spectroscopy revealed a larger superconducting gap of 17 meV for FeSe on TiO2 compared to 11 meV on SrO. Tunneling spectroscopy also showed a larger work function on SrO, leading to reduced charge transfer, as confirmed by angle-resolved photoemission spectroscopy. Scanning transmission electron microscopy revealed distinctive interfacial atomic-scale structures, with the Se-Fe-Se tetrahedral angle changing from 109.9{\deg} on SrO to 105.1{\deg} on TiO2. Compared to dynamical mean field theory calculations, these results suggest optimal electron correlations in FeSe/TiO2 for enhancing high-temperature superconductivity.

cond-mat.supr-con↗

arXiv2025

Odd-parity Magnetism Driven by Antiferromagnetic Exchange

Realizing odd-parity, time-reversal-preserving, non-relativistic spin splitting is a central goal for spintronics applications. We propose a group-theory-based microscopic framework to induce odd-parity spin splitting from coplanar antiferromagnetic (AFM) states without spin-orbit coupling (SOC). We develop phenomenological models for 421 conventional period-doubling AFM systems in non-symmorphic space groups and construct minimal microscopic models for 119 of these. We find that these AFM states can attain three possible competing ground states. These ground states all break symmetries in addition to those broken by the usual AFM order. Specifically, they give rise to either odd-parity spin-splitting, nematic order, or scalar odd-parity order related to multiferroicity. Our microscopic theories reveal that the odd-parity spin-splitting energy scale is generically large and further reveal that the scalar odd-parity order gives a non-zero Berry curvature dipole without SOC. We identify 67 materials in the Magndata database for which our theory applies. We provide DFT calculations on FeSe that reveal an $h$-wave spin splitting consistent with our symmetry arguments and apply our microscopic model to determine the non-relativistic Edelstein response for CeNiAsO.

cond-mat.str-el↗

arXiv2024

Large critical fields in superconducting Ti$_{4}$Ir$_2$O from spin-orbit coupling

The recently synthesized $\eta$-carbide-type superconductors exhibit large critical fields. A notable example is Ti$_4$Ir$_2$O, for which the upper critical field strongly violates the Pauli paramagnetic limit, behavior that is unusual for cubic materials that preserve inversion symmetry. Here, by combining density functional theory (DFT) and analytic modeling, we provide an explanation for this enhanced Pauli limiting field. We show that the nonsymmorphic Fd$\overline{3}$m symmetry implies that the electronic states near the X points exhibit strong spin-orbit coupling (SOC), which leads to a vanishing effective $g$-factor and enables the enhanced Pauli limiting field. Furthermore, our DFT results reveal a Van Hove singularity (VHS) peak near the X points, accounting for $\sim$65\% of the total density of states (DOS), occurring near the chemical potential. We propose that the strong SOC and enhanced DOS in the vicinity of the X points provide the origin of the observed enhanced critical field. This leads to a prediction that the magnetic field will lead to a strongly momentum-dependent gap suppression. The gap due to electronic states away from (near to) the X points will be rapidly (slowly) suppressed by fields.

cond-mat.supr-con↗

arXiv2024

GEO600 beam splitter thermal compensation system: new design and commissioning

Gravitational waves have revolutionised the field of astronomy by providing scientists with a new way to observe the universe and gain a better understanding of exotic objects like black holes. Several large-scale laser interferometric gravitational wave detectors (GWDs) have been constructed worldwide, with a focus on achieving the best sensitivity possible. However, in order for a detector to operate at its intended sensitivity, its optics must be free from imperfections such as thermal lensing effects. In the GEO\,600 gravitational wave detector, the beam splitter (BS) experiences a significant thermal lensing effect due to the high power build-up in the Power Recycling Cavity (PRC) combined with a very small beam waist. This causes the fundamental mode to be converted into higher order modes (HOMs), subsequently impacting the detector's performance. To address this issue, the GEO\,600 detector is equipped with a thermal compensation system (TCS) applied to the BS. This involves projecting a spatially tunable heating pattern through an optical system onto the beam splitter. The main objective of the TCS is to counteract the thermal lens at the BS and restore the detector to its ideal operating condition. This paper presents the new beam splitter TCS in GEO\,600, its commissioning, and its effect on strain sensitivity. It also outlines the planned upgrade to further enhance the performance of the TCS.

astro-ph.IM↗

arXiv2023

Tuning quantum paramagnetism and d-wave superconductivity in single-layer iron chalcogenides by chemical pressure

By substituting S into single-layer FeSe/SrTiO3, chemical pressure is applied to tune its paramagnetic state that is modeled as an incoherent superposition of spin-spiral states. The resulting electronic bands resemble an ordered checkerboard antiferromagnetic structure, consistent with angle-resolved photoemission spectroscopy measurements. Scanning tunneling spectroscopy reveals a gap evolving from U-shaped for FeSe to V-shaped for FeS with decreasing size, attributed to a d-wave superconducting state for which nodes emerge once the gap size is smaller than the effective spin-orbit coupling.

cond-mat.supr-con↗

arXiv2023

Spin-orbit enabled unconventional Stoner magnetism

The Stoner instability remains a cornerstone for understanding metallic ferromagnets. This instability captures the interplay of Coulomb repulsion, Pauli exclusion, and two-fold fermionic spin degeneracy. In materials with spin-orbit coupling, this fermionic spin is generalized to a two-fold degenerate pseudospin which is typically believed to have symmetry properties as spin. Here we identify a distinct symmetry of this pseudospin that forbids it to couple to a Zeeman field. This `spinless' property is required to exist in five non-symmorphic space groups and has non-trivial implications for superconductivity and magnetism. With Coulomb repulsion, Fermi surfaces composed primarily of this spinless pseudospin feature give rise to Stoner instabilities into magnetic states that are qualitatively different than ferromagnets. These spinless-pseudospin ferromagnets break time-reversal symmetry, have a vanishing magnetization, are non-collinear, and exhibit altermagnetic-like energy band spin-splittings. In superconductors, for all pairing symmetries and field orientations, this spinless pseudospin extinguishes paramagnetic limiting. We discuss applications to superconducting UCoGe and magnetic NiS$_{2-x}$Se$_x$.

cond-mat.str-el↗

arXiv2023

Characterization and evasion of backscattered light in the squeezed-light enhanced gravitational wave interferometer GEO 600

Squeezed light is injected into the dark port of gravitational wave interferometers, in order to reduce the quantum noise. A fraction of the interferometer output light can reach the OPO due to sub-optimal isolation of the squeezing injection path. This backscattered light interacts with squeezed light generation process, introducing additional measurement noise. We present a theoretical description of the noise coupling mechanism. We propose a control scheme to achieve a de-amplification of the backscattered light inside the OPO with a consequent reduction of the noise caused by it. The scheme was implemented at the GEO 600 detector and has proven to be crucial in maintaining a good level of quantum noise reduction of the interferometer for high parametric gain of the OPO. In particular, the mitigation of the backscattered light noise helped in reaching 6dB of quantum noise reduction [Phys. Rev. Lett. 126, 041102 (2021)]. The impact of backscattered-light-induced noise on the squeezing performance is phenomenologically equivalent to increased phase noise of the squeezing angle control. The results discussed in this paper provide a way for a more accurate estimation of the residual phase noise of the squeezed light field.

physics.optics↗

arXiv2023

First demonstration of neural sensing and control in a kilometer-scale gravitational wave observatory

Suspended optics in gravitational wave (GW) observatories are susceptible to alignment perturbations, particularly slow drifts over time, due to variations in temperature and seismic levels. Such misalignments affect the coupling of the incident laser beam into the optical cavities, degrade both circulating power and optomechanical photon squeezing and thus decrease the astrophysical sensitivity to merging binaries. Traditional alignment techniques involve differential wavefront sensing using multiple quadrant photodiodes but are often restricted in bandwidth and are limited by the sensing noise. We present the first-ever successful implementation of neural network-based sensing and control at a gravitational wave observatory and demonstrate low-frequency control of the signal recycling mirror at the GEO 600 detector. Alignment information for three critical optics is simultaneously extracted from the interferometric dark port camera images via a CNN-LSTM network architecture and is then used for MIMO control using soft actor-critic-based deep reinforcement learning. Overall sensitivity improvement achieved using our scheme demonstrates deep learning's capabilities as a viable tool for real-time sensing and control for current and next-generation GW interferometers.

physics.ins-det↗

arXiv2023

Giant periodic pseudo-magnetic fields in strained kagome magnet FeSn epitaxial films on SrTiO$_3$(111) substrate

Quantum materials, particularly Dirac materials with linearly dispersing bands, can be effectively tuned by strain-induced lattice distortions leading to a pseudo-magnetic field that strongly modulates their electronic properties. Here, we grow kagome magnet FeSn films, consisting of alternatingly stacked Sn$_2$ honeycomb (stanene) and Fe$_3$Sn kagome layers, on SrTiO$_3$(111) substrates by molecular beam epitaxy. Using scanning tunneling microscopy/spectroscopy, we show that the Sn honeycomb layer can be periodically deformed by epitaxial strain for film thickness below 10 nm, resulting in differential conductance peaks consistent with Landau levels generated by a pseudo-magnetic field greater than 1000 T. Our findings demonstrate the feasibility of strain engineering the electronic properties of topological magnets at the nanoscale.

cond-mat.mtrl-sci↗

arXiv2023

Resonant Ultrasound Spectroscopy for Irregularly-Shaped Samples and its Application to Uranium Ditelluride

Resonant ultrasound spectroscopy (RUS) is a powerful technique for measuring the full elastic tensor of a given material in a single experiment. Previously, this technique was limited to regularly-shaped samples such as rectangular parallelepipeds, spheres, and cylinders. We demonstrate a new method for determining the elastic moduli of irregularly-shaped samples, extending the applicability of RUS to a much larger set of materials. We apply this new approach to the recently-discovered unconventional superconductor UTe$_2$ and provide its elastic tensor at both 300 and 4 kelvin.

cond-mat.str-el↗

arXiv2023

Superconductivity of anomalous pseudospin

Spin-orbit coupling driven by broken inversion symmetry ($I$) is known to lead to unusual magnetic response of superconductors, including extremely large critical fields for spin-singlet superconductors. This unusual response is also known to appear in materials that have $I$, provided there is local $I$-breaking: fermions participating in superconductivity reside on crystal sites that lack $I$. Here we show that this unusual response exists even when the crystal sites preserve $I$. Indeed, we argue that the symmetry of Kramers degenerate fermionic pseudospin is more relevant than the local crystal site symmetry. We examine and classify non-symmorphic materials with momentum space spin-textures that exhibit an anomalous pseudospin with different symmetry properties than usual spin-1/2. We find that this anomalous pseudospin does not depend on the existence of local $I$ breaking crystal sites and it optimizes the unusual magnetic response traditionally associated with locally noncentrosymmetric superconductors, dramatically extending the range of relevant materials. We further show this anomalous pseudospin leads to fully gapped `nodal' superconductors and provides additional insight into the breakdown of Blount's theorem for pseudospin triplet superconductors. We apply our results to UPt$_3$, BiS$_2$-based superconductors, Fe-based superconductors, and paramagnetic UCoGe.

cond-mat.supr-con↗