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Michal Urbánek

Publications and source records attributed to Michal Urbánek.

At least 19 recordsLinked to original sources

Ultrafast formation of a large dynamic magnetic soliton

Nonlinear magnetization dynamics offers a rich variety of phenomena ranging from bistability to chaos. Here, we report the ultrafast formation of a dynamic magnetic soliton in thin ferrimagnetic garnet films with perpendicular magnetic anisotropy, driven by the microwave magnetic field of a microstrip antenna. Using time-resolved Brillouin light scattering microscopy and scanning transmission X-ray microscopy, we directly track the build-up of the large-angle precession state. The observed soliton is distinct from other nonlinear magnetic excitations in two key aspects: (i) it forms inside the linear spin-wave frequency band, and (ii) it is exceptionally large, reaching tens of microns beyond the antenna. We explain the soliton formation by the self-limiting mechanism upon a positive nonlinear frequency shift and the spatial extent of the near-field of the antenna. At large distances from the drive, the soliton collapses and emits short-wavelength spin waves via almost instantaneous spatial wavenumber conversion. Time-resolved measurements further reveal a small finite delay during soliton formation, while coherent long-range oscillations appear essentially simultaneously over distances up to 40 micrometers. These results establish microwave-driven solitons as a robust nonlinear phenomenon in thin-film garnets and suggest opportunities for fast, nonlocal manipulation of magnetic states and for applications in novel computational schemes.

cond-mat.mes-hall↗

Sculpting Spin-Wave Landscapes via Curvature of 2D Magnonic Crystals

Engineering the dispersion relation is one of the key ingredients enabling the application of spin waves in computational elements. One way to engineer the spin-wave band structure is to create an artificial magnonic crystal, which can be used to design specific band gaps or dispersion branches. However, creating a two-dimensional magnonic crystal usually requires removing material, which dramatically decreases the decay lengths of spin waves. Here, we present a method to manipulate the demagnetizing field landscape by utilizing large-area curvilinear nanotemplates consisting of three-dimensional nanopyramids arranged in a square lattice with a period of 400 nm. In a 50-nm-thick Permalloy film grown on these curvilinear templates, we experimentally observe a complete in-plane band gap together with flat-band modes that exhibit strong real-space localization of the spin waves in the pyramid valleys. Micro-focused Brillouin light scattering measurements corroborate the numerically predicted dispersion and reveal the possibility of opening and closing this gap by varying the external magnetic field. Our results establish three-dimensional-templated continuous films as a versatile platform for two-dimensional signal processing and magnonic computing elements.

cond-mat.mes-hall↗

Laterally Differentiated Polymorphs: a route to multifunctional nanostructures

Multifunctional materials can exhibit emergent behavior from the coupling of two or more different properties. For example, coupling between magnetic and ferroelectric order enables electrical control of the magnetic state, enabling for example magnetoelectric memory or logic devices that combine the nonvolatility of magnetic order with the energy efficiency of voltage control. Magnetic iron garnets have outstanding magnonic and magnetooptical properties making them valuable in a range of technologies, but they have not been successfully incorporated into thin film two-phase magnetoelectric nanocomposites. Taking advantage of heterogeneously patterned substrates, this work demonstrates the engineering of garnet-perovskite composites in which both phases are polymorphs with the same composition but dramatically different structures and properties. Applying an electric field to the perovskite phase modulates the magnon dispersion and magnetooptical response of the garnet, opening a path to voltage-controlled garnet devices.

cond-mat.mtrl-sci↗

Precise control of crystallography and magnetism in focused-ion-beam transformed iron-nickel thin films

Focused ion beam irradiation of metastable Fe$_{78}$Ni$_{22}$ thin films grown on Cu(100) substrates results in the localized transformation of the originally paramagnetic, face-centered-cubic continuous film into ferromagnetic patterns with body-centered-cubic structure. The direction of the magnetic easy axis can be controlled by the focused ion beam scanning strategy, resulting in eight differently oriented crystallographic domains with different magnetic properties. We study the local crystallographic orientations of the transformed areas by electron backscatter diffraction and correlate these results with local magnetometry measurements. The observed magnetic anisotropy can be explained as a result of residual lattice strain after the fcc$\to$bcc transformation. These results extend the understanding of this material system and its transformation and allow for the patterning of high-quality magnetic nanostructures with precisely controlled magnetization landscapes.

cond-mat.mtrl-sci↗

Polarization-resolved measurement of forward volume spin waves by micro-focused Brillouin light scattering

We show how the micro-focused BLS signal of forward volume spin waves is formed and why it remains observable despite symmetry-based "suppression" expectations. A reciprocity-theorem based model with vectorial diffraction-limited focusing identifies the nonnegligible longitudinal focal-field component as the key element responsible for BLS sensitivity in the forward volume geometry. We further demonstrate that full polarization analysis, implemented through polarizer-analyzer maps of coherently excited spin waves, provides information beyond the conventional crossed polarizer-analyzer readout. In a BiYIG thin film, the measured maps exhibit Stokes/anti-Stokes polarization asymmetries and nontrivial patterns that stem from quadratic magneto-optical coupling terms. Fitting the data with a model including Voigt and Cotton-Mouton contributions yields an effective Cotton-Mouton constant and shows that the quadratic response is comparable to the linear Voigt contribution.

cond-mat.mes-hall↗

Nanoscale spin-wave frequency-selective limiter for 5G technology

Power limiters are essential devices in modern radio frequency (RF) communications systems to protect highly sensitive input channels from large incoming signals. Nowadays-used semiconductor limiters suffer from high electronic noise and switching delays when approaching the GHz range, which is crucial for the modern generation of 5G communication technologies aiming to operate at the EU 5G high band (24.25-27.5 GHz). The proposed solution is to use ferrite-based Frequency Selective Limiters (FSLs), which maintain their efficiency at high GHz frequencies, although they have only been studied at the macroscale so far. In this study, we demonstrate a proof of concept of nanoscale FSLs. The devices are based on spin-wave transmission affected by four-magnon scattering phenomena in a 97-nm-thin Yttrium Iron Garnet (YIG) film. Spin waves were excited and detected using coplanar waveguide (CPW) transducers of the smallest feature size of 250 nm. The FSLs are tested in the frequency range up to 25 GHz, and the key parameters are extracted (power threshold, power limiting level, insertion losses, bandwidth) for different spin-wave modes and transducer lengths. An analytical theory has been formulated to describe the fundamental physical processes, and a numerical model has been developed to quantitatively describe the insertion losses and power characteristics of the FSLs. Additionally, the perspective of the spin-wave devices is discussed, including the possibility of simultaneously integrating three devices into one: a frequency-selective limiter, an RF filter, and a delay line, allowing for more efficient use of space and energy.

cond-mat.other↗

SpinWaveToolkit: Python package for (semi-)analytical calculations in the field of spin-wave physics

We present an open-source Python package, SpinWaveToolkit (SWT), for (semi-)analytical modeling of spin-wave dynamics in thin ferromagnetic films and exchange-coupled magnetic bilayers. SWT combines analytical models based on the Kalinikos-Slavin theory with a semi-analytical dynamic-matrix approach, enabling the calculation of dispersion relations, group velocities, decay lengths, mode profiles, and static equilibrium magnetization states. In addition, SWT implements a quantitative model of micro-focused Brillouin light scattering (BLS) that incorporates vectorial optical focusing, spin-wave Bloch functions, magneto-optical coupling, and Green-function propagation to simulate experimentally measured BLS spectra. The package is validated against finite-element dynamic-matrix simulations performed with TetraX for Damon-Eshbach, backward-volume, forward-volume, and oblique-field geometries, showing excellent agreement while reducing computation times by nearly two orders of magnitude in comparison to the numerical simulations. Thanks to the easiness of the use and fast calculation times, SWT can be used not only for exploratory mapping of the parameter space, but also for the fitting of the measured dispersion relations and related parameters. Thus, it provides a versatile and efficient framework for experiment design, interpretation, and parameter optimization for magnonics research.

cond-mat.mes-hall↗

Ultrafast propagation of magnon-polaritons

The manipulation of magnetization lies at the heart of spintronic and magnonic technologies, with the ultimate performance of such systems limited by the velocity at which magnetic excitations can propagate. Here, we demonstrate ultrafast propagation of magnon-polaritons-hybrid quasiparticles arising from the coupling between spin waves and electromagnetic fields in thin pure, bismuth-, and gallium substituted yttrium iron garnet (YIG, Bi:YIG and Ga:YIG) films. Using time- and phase-resolved Brillouin light scattering microscopy and time-resolved scanning transmission microscopy, we show that magnon-polaritons can propagate faster than 100 km/s, nearly three orders of magnitude more than conventional spin waves, and can be observed at distances exceeding 40 micrometers in 20 nm thick films. Analytical modeling based on retarded Maxwell equations and Polder tensor formalism confirms the hybridized nature of the excitations and captures the nontrivial dispersion and attenuation profiles. Notably, the magnon-polaritons maintain high initial magnetization amplitudes and long decay lengths, enabling ultrafast manipulation of the magnetization far away from the excitation source. We show, that they can move domain walls or stabilize nonlinear magnetization processes. The unprecedentedly high propagation velocities make magnon-polaritons promising candidates for high-speed information transfer in future spin-based computing architectures, potentially overcoming long-standing group delay bottlenecks in magnonic logic circuits.

physics.app-ph↗

YSGAG: The Ideal Substrate for YIG in Quantum Magnonics

Quantum magnonics leverages the quantum properties of magnons to advance nanoscale quantum information technologies. Ferrimagnetic yttrium iron garnet (YIG), known for exceptionally long magnon lifetimes, is a cornerstone material typically grown as thin films on gadolinium gallium garnet (GGG) for lattice matching. However, paramagnetic GGG introduces detrimental damping at low temperatures due to substrate magnetization, undermining quantum applications. Here, we study magnetic damping in a 150$\,$nm-thick YIG film on a yttrium scandium gallium aluminum garnet (YSGAG) substrate, a newly developed diamagnetic alternative to GGG. Using ferromagnetic resonance spectroscopy down to 30$\,$mK, we compare YIG/YSGAG with a conventional YIG/GGG reference system. We demonstrate that the YIG/YSGAG system maintains low damping from 300$\,$K to 30$\,$mK, with $α= 4.29\times10^{-5}$ at room temperature, comparable to the best YIG/GGG films and bulk YIG, with no low-temperature upturn. The diamagnetic substrate eliminates the dissipation mechanisms that dominate on magnetized GGG, preserving low magnetic damping across the full temperature range. Consequently, YSGAG serves as an ideal substrate for YIG films in quantum magnonics and is paving the way for the development of spin-wave-based quantum technologies.

cond-mat.mes-hall↗

Exchange spin-wave propagation in Ga:YIG nanowaveguides

Spin-wave-based computing has emerged as a promising approach to overcome the fundamental limitations of CMOS technologies. However, the increasing demand for device miniaturization down to a 100 nm scale presents significant challenges for long-distance spin-wave transport. Gallium-substituted yttrium iron garnet (Ga:YIG) offers a potential solution to these challenges due to its unique magnetic properties. The reduced saturation magnetization in Ga:YIG enables efficient excitation of exchange-dominated spin waves, which exhibit enhanced transport characteristics compared to dipolar-dominated modes in conventional materials. Here, we present the first comprehensive study combining experimental, analytical, and numerical investigations of spin-wave propagation in Ga:YIG waveguides down to 145 nm width and 73 nm thickness. Using micro-focused Brillouin light scattering spectroscopy, TetraX simulations, and analytical dispersion calculations, we demonstrate that Ga:YIG waveguides support spin waves with significantly higher group velocities up to 600 m/s. This value remains constant for structures with different widths, leading to longer spin-wave propagation lengths in nanowaveguides compared to non-substituted YIG. These results reveal that gallium substitution provides access to faster and longer-lived spin waves, opening new possibilities for implementing this material in nanoscale magnonic devices.

cond-mat.other↗

Modeling of the micro-focused Brillouin light scattering spectra

Although micro-focused Brillouin light scattering (BLS) has been used for more than twenty years, it lacks a complete theoretical description. This complicates the analysis of experimental data and significantly limits the information that can be obtained. To fill this knowledge gap, we have developed a semi-analytical model based on the mesoscopic continuous medium approach. The model consists of the following steps: calculation of the incident electric field and the dynamic susceptibility, calculation of the induced polarisation, and calculation of the emitted electric field and its propagation towards the detector. We demonstrate the model on the examples of the measurements of thermal and coherently excited spin waves. However, the used approach is general and can describe any micro-focused Brillouin light scattering experiment. The model can also bring new analytical approaches to mechanobiology experiments or to characterization of acoustic wave based devices.

cond-mat.mes-hall↗

Mie-enhanced micro-focused Brillouin light scattering with wavevector resolution

Magnons, the quanta of spin waves, are magnetic excitations of matter spanning through the entire crystal's Brillouin zone and covering a wide range of frequencies ranging from sub-gigahertz to hundreds of terahertz. Magnons play a crucial role in many condensed matter phenomena, such as the reduction of saturation magnetization with increasing temperature or Bose-Einstein condensation. However, current experimental techniques cannot resolve magnons with wavevectors between 30 and 300$\,$rad$\,μ$m$^{-1}$. In this letter, we address this gap by tailoring the light in Brillouin light scattering process with dielectric periodic nanoresonators and thus gaining access to the previously unmeasurable spin waves with full wavevector resolution using table-top optical setup. Filling this gap can stimulate further experimental investigations of the fundamental phenomena associated with magnons but also stimulate the application of magnonics in computational and microwave devices. In addition, the same methodology can be applied to other excitations of matter, such as phonons, opening up new possibilities in e.g. mechanobiological studies.

cond-mat.mes-hall↗

Elimination of substrate-induced FMR linewidth broadening in the epitaxial system YIG-GGG by microstructuring

Modern quantum technologies and hybrid quantum systems offer the opportunity to utilize magnons on the level of single excitations. Long lifetimes, low decoherence rates, and a strong coupling rate to other subsystems propose the ferrimagnet yttrium iron garnet (YIG), grown on a gadolinium gallium garnet (GGG) substrate, as a suitable platform to host magnonic quantum states. However, the magnetic damping at cryogenic temperatures significantly increases due to the paramagnetic character and the highly inhomogeneous stray field of GGG, as recent experiments and simulations pointed out. Here, we report on temperature dependent ferromagnetic resonance (FMR) spectroscopy studies in YIG-GGG thin-films with different sample geometries. We experimentally demonstrate how to eliminate the asymmetric stray field-induced linewidth broadening via microstructuring of the YIG film. Additionally, our experiments reveal evidence of a non-Gilbert like behavior of the linewidth at cryogenic temperatures, independent of the inhomogeneous GGG stray field.

cond-mat.mes-hall↗

YIG/CoFeB bilayer magnonic diode

We demonstrate a magnonic diode based on a bilayer structure of Yttrium Iron Garnet (YIG) and Cobalt Iron Boron (CoFeB). The bilayer exhibits pronounced non-reciprocal spin-wave propagation, enabled by dipolar coupling and the magnetic properties of the two layers. The YIG layer provides low damping and efficient spin-wave propagation, while the CoFeB layer introduces strong magnetic anisotropy, critical for achieving diode functionality. Experimental results, supported by numerical simulations, show unidirectional propagation of Magnetostatic Surface Spin Waves (MSSW), significantly suppressing backscattered waves. This behavior was confirmed through wavevector-resolved and micro-focused Brillouin Light Scattering measurements and is supported by numerical simulations. The proposed YIG/SiO$_2$/CoFeB bilayer magnonic diode demonstrates the feasibility of leveraging non-reciprocal spin-wave dynamics for functional magnonic devices, paving the way for energy-efficient, wave-based signal processing technologies.

physics.app-ph↗

Damping Enhancement in YIG at Millikelvin Temperatures due to GGG Substrate

Quantum magnonics aims to exploit the quantum mechanical properties of magnons for nanoscale quantum information technologies. Ferrimagnetic yttrium iron garnet (YIG), which offers the longest magnon lifetimes, is a key material typically grown on gadolinium gallium garnet (GGG) substrates for structural compatibility. However, the increased magnetic damping in YIG/GGG systems below 50$\,$K poses a challenge for quantum applications. Here, we study the damping in a 97$\,$nm-thick YIG film on a 500$\,μ$m-thick GGG substrate at temperatures down to 30$\,$mK using ferromagnetic resonance (FMR) spectroscopy. We show that the dominant physical mechanism for the observed tenfold increase in FMR linewidth at millikelvin temperatures is the non-uniform bias magnetic field generated by the partially magnetized paramagnetic GGG substrate. Numerical simulations and analytical theory show that the GGG-driven linewidth enhancement can reach up to 6.7 times. In addition, at low temperatures and frequencies above 18$\,$GHz, the FMR linewidth deviates from the viscous Gilbert-damping model. These results allow the partial elimination of the damping mechanisms attributed to GGG, which is necessary for the advancement of solid-state quantum technologies.

cond-mat.mes-hall↗

Unidirectional propagation of zero-momentum magnons

We report on experimental observation of unidirectional propagation of zero-momentum magnons in synthetic antiferromagnet consisting of strained CoFeB/Ru/CoFeB trilayer. Inherent non-reciprocity of spin waves in synthetic antiferromagnets with uniaxial anisotropy results in smooth and monotonous dispersion relation around Gamma point, where the direction of the phase velocity is reversed, while the group velocity direction is conserved. The experimental observation of this phenomenon by intensity-, phase-, and time-resolved Brillouin light scattering microscopy is corroborated by analytical models and micromagnetic simulations.

cond-mat.mes-hall↗

Magnetic anisotropy and GGG substrate stray field in YIG films down to millikelvin temperatures

Quantum magnonics investigates the quantum-mechanical properties of magnons such as quantum coherence or entanglement for solid-state quantum information technologies at the nanoscale. The most promising material for quantum magnonics is the ferrimagnetic yttrium iron garnet (YIG), which hosts magnons with the longest lifetimes. YIG films of the highest quality are grown on a paramagnetic gadolinium gallium garnet (GGG) substrate. The literature has reported that ferromagnetic resonance (FMR) frequencies of YIG/GGG decrease at temperatures below 50 K despite the increase in YIG magnetization. We investigated a 97 nm-thick YIG film grown on 500 $\mathrmμ$m-thick GGG substrate through a series of experiments conducted at temperatures as low as 30 mK, and using both analytical and numerical methods. Our findings suggest that the primary factor contributing to the FMR frequency shift is the stray magnetic field created by the partially magnetized GGG substrate. This stray field is antiparallel to the applied external field and is highly inhomogeneous, reaching up to 40 mT in the center of the sample. At temperatures below 500 mK, the GGG field exhibits a saturation that cannot be described by the standard Brillouin function for a paramagnet. Including the calculated GGG field in the analysis of the FMR frequency versus temperature dependence allowed the determination of the cubic and uniaxial anisotropies. We find that the total anisotropy increases more than three times with the decrease in temperature down to 2 K. Our findings enable accurate predictions of the YIG/GGG magnetic systems behavior at low and ultra-low millikelvin temperatures, crucial for developing quantum magnonic devices.

cond-mat.mes-hall↗

Zero-field spin wave turns

Spin-wave computing, a potential successor to CMOS-based technologies, relies on the efficient manipulation of spin waves for information processing. While basic logic devices like magnon transistors, gates, and adders have been experimentally demonstrated, the challenge for complex magnonic circuits lies in steering spin waves through sharp turns. In this study we demonstrate with micromagnetic simulations and Brillouin light scattering microscopy experiments, that dipolar spin waves can propagate through 90-degree turns without distortion. The key lies in carefully designed in-plane magnetization landscapes, addressing challenges posed by anisotropic dispersion. The experimental realization of the required magnetization landscape is enabled by spatial manipulation of the uniaxial anisotropy using corrugated magnonic waveguides. The findings presented in this work should be considered in any magnonic circuit design dealing with anisotropic dispersion and spin wave turns.

cond-mat.mes-hall↗