arXiv subjects

Michel Brune

Publications and source records attributed to Michel Brune.

At least 19 recordsLinked to original sources

arXiv2026

Measuring the Sr$^+$ 5s$_{1/2}$ Land\'e $g$-factor Using Singlet-Triplet Oscillations in a Circular Rydberg State of Strontium

Circular states of strontium are promising platforms for quantum technologies. They exhibit much longer lifetimes than laser-accessible Rydberg states and possess an optically active ionic core that can be manipulated with laser light. Here we trap circular states in optical tweezers by exploiting the dynamical polarizability of the ionic core. We measure the decay of the orbital component of a n=51 circular state and observe singlet-triplet spin oscillations arising from the interplay of vector light shifts induced by the optical tweezers, spin-orbit coupling associated with the Rydberg electron, and the difference in Land\'e $g$-factor between the ionic core and the Rydberg electrons. By observing the two electron spin dynamics, we measure the spin-orbit interaction and the correction $\delta g \sim$ 10^(-5) of the Land\'e $g$-factor of the Sr$^+$ 5s$_{1/2}$ ionic core electron with respect to that of a free electron. This provides a first high-precision measurement of $g_{\textrm{Sr}^+, 5s_{1/2}}$ = 2.002290(1).

physics.atom-ph↗

arXiv2026

Fast Pulses for High-Fidelity Circularization of Interacting Rydberg atoms

Circular states in Rydberg atoms offer a promising platform for quantum computation, quantum simulation and quantum sensing. However, the final step of their preparation - termed as circularization, a process that involves the transfer of a large amount of angular momentum quanta to the valence electron by means of radio-frequency (RF) pulses - remains as a major bottleneck for all technological applications based on interacting circular Rydberg atoms. Even though successfully implemented to circularize an atom cloud in the dilute regime, previous efforts to speed up the circularization process have focused on the single-atom case, thereby neglecting the interactions which constitute one of the main resources for quantum simulation and computation. In this theoretical work we show how interactions between two atoms disturb the efficiency of pulses designed for single atoms and identify shifts induced by the interactions on relevant transition energies as the dominant disturbance. We demonstrate that the initial efficiency of single-atom pulses can be restored by adapting them to these shifts. Our approach is based on a simple functional form depending only on two linear parameters, which we derive analytically. The adapted pulses prepare two $^{87}$Rb atoms after $65 \,$ns in a $n=52$ circular state with a fidelity of at least $95\,\%$ for interatomic distances down to $6.5\,\mu$m and for all angular configurations, while also complying experimental amplitude and frequency constraints. Finally, we show that when combining our adapted pulses with Krotov's pulse-shaping algorithm we obtain high-fidelity pulses for any pair arrangement with interatomic distances larger than $5.9\,\mu$m. This work demonstrates that fast RF pulses can circularize interacting Rydberg atoms, paving the way toward their technological application.

physics.atom-ph↗

arXiv2025

Full-field-of-view aberration correction for large arrays of focused beams

We propose and implement an aberration correction method for the creation of extended arrays of spots well beyond the isoplanatic region of any optical system. The method relies on an extensive calibration of aberrations in terms of Zernike polynomials over the full accessible field of an optical system. We introduce a modified Gerchberg-Saxton algorithm for generating holographic phase masks creating fully corrected arbitrary arrays of spots. By applying the method to an aspherical lens, and using a liquid-crystal spatial light modulator (SLM), we increase the aberration-free field of view from 50 to 500 $\mu$m, only limited by the largest diffraction angles accessible to the SLM. This opens new perspectives for the generation of large arrays of optical tweezers, especially for neutral atom based quantum processors and simulators.

physics.optics↗

arXiv2025

Non-destructive optical read-out and manipulation of circular Rydberg atoms

Among the thriving quantum computation and quantum simulation platforms based on arrays of Rydberg atoms, those using circular Rydberg atoms are particularly promising. These atoms uniquely combine the strong dipole-dipole interactions typical of Rydberg states with long lifetimes. However, low-angular-momentum ($\ell$) laser-accessible Rydberg levels have been so far mostly used, because circular Rydberg atoms have no optical transitions, hindering their individual detection and manipulation. We remove this limitation with a hybrid platform, combining an array of logical laser-trapped circular Rydberg atoms of rubidium with an auxiliary array of Rb ancilla atoms transiently excited to a low-$\ell$ Rydberg level. We perform a quantum non-demolition detection of the logical qubit with the ancilla, through the blockade of the ancilla optical excitation induced by a F\"orster resonance. Conversely, we locally manipulate the logical qubit through the excitation of the ancilla. This dual-Rydberg platform is highly promising for quantum computation and simulation. It adds to the circular-atom toolbox the mid-circuit measurements, essential for error correction. More strikingly, it gives access to time correlations in long-term quantum simulations, uniquely accessible to circular Rydberg atoms.

physics.atom-ph↗

arXiv2024

Interacting Circular Rydberg Atoms Trapped in Optical Tweezers

Circular Rydberg atoms (CRAs), i.e., Rydberg atoms with maximal orbital momentum, ideally combine long coherence times and strong interactions, a key property of quantum systems, in particular for the development of quantum technologies. However, the dipole-dipole interaction between CRAs has not been observed so far. We report the measurement and characterization of the resonant dipole-dipole interaction between two CRAs, individually trapped in optical tweezers, and find excellent agreement with theoretical predictions. We demonstrate a dynamic control over the strength of the interaction by tuning the orientation of an electric field. We use the interaction between the CRAs as a meter for the interatomic distance, and record the relative motion between two atoms in their traps. This motion, that we induce through the interaction between Rydberg levels with permanent electric dipoles, transiently populated during the preparation of the circular states, is a signature of spin-motion coupling.

physics.atom-ph↗

arXiv2023

Array of Individual Circular Rydberg Atoms Trapped in Optical Tweezers

Circular Rydberg atoms (CRAs), i.e., Rydberg atoms with maximal orbital momentum, are highly promising for quantum computation, simulation and sensing. They combine long natural lifetimes with strong inter-atomic interactions and coupling to electromagnetic fields. Trapping individual CRAs is essential to harness these unique features. We report the first demonstration of CRAs laser-trapping in a programmable array of optical bottle beams. We observe the decay of a trapped Rubidium circular level over 5ms using a novel optical detection method. This first optical detection of alkali CRAs is both spatially- and level selective. We finally observe the mechanical oscillations of the CRAs in the traps. This work opens the route to the use of circular levels in quantum devices. It is also promising for quantum simulation and information processing using the full extent of Rydberg manifolds.

quant-ph↗

arXiv2023

Spin-motion coupling in a circular Rydberg state quantum simulator: case of two atoms

Rydberg atoms are remarkable tools for the quantum simulation of spin arrays. Circular Rydberg atoms open the way to simulations over very long time scales, using a combination of laser trapping of the atoms and spontaneous-emission inhibition, as shown in the proposal of a XXZ spin-array simulator based on chains of trapped circular atoms [T.L. Nguyen $\textit{et al.}$, Phys. Rev. X 8, 011032 (2018)]. Such simulators could reach regimes (thermalization, glassy dynamics) that are out of the reach of those based on ordinary, low-angular-momentum short-lived Rydberg atoms. Over the promised long time scales, the unavoidable coupling of the spin dynamics with the atomic motion in the traps may play an important role. We study here the interplay between the spin exchange and motional dynamics in the simple case of two interacting circular Rydberg atoms confined in harmonic traps. The time evolution is solved exactly when the position dependence of the dipole-dipole interaction terms can be linearized over the extension of the atomic motion. We present numerical simulations in more complex cases, using the realistic parameters of the simulator proposal. We discuss three applications. First, we show that realistic experimental parameters lead to a regime in which atomic and spin dynamics become fully entangled, generating interesting non-classical motional states. We also show that, in other parameter regions, the spin dynamics notably depends on the initial temperature of the atoms in the trap, providing a sensitive motional thermometry method. Last, and most importantly, we discuss the range of parameters in which the motion has negligible influence over the spin dynamics.

physics.atom-ph↗

arXiv2022

Millisecond-lived circular Rydberg atoms in a room-temperature experiment

Circular Rydberg states are ideal tools for quantum technologies, with huge mutual interactions and extremely long lifetimes in the tens of milliseconds range, two orders of magnitude larger than those of laser-accessible Rydberg states. However, such lifetimes are observed only at zero temperature. At room temperature, blackbody-radiation-induced transfers annihilate this essential asset of circular states, which have thus been used mostly so far in specific, complex cryogenic experiments. We demonstrate here, on a laser-cooled atomic sample, a circular state lifetime of more than one millisecond at room temperature for a principal quantum number 60. The inhibition structure is a simple plane-parallel capacitor that efficiently inhibits the blackbody-radiation-induced transfers. One of the capacitor electrodes is fully transparent and provides complete optical access to the atoms, an essential feature for applications. This experiment paves the way to a wide use of circular Rydberg atoms for quantum metrology and quantum simulation.

physics.atom-ph↗

arXiv2021

Optical coherent manipulation of alkaline-earth circular Rydberg states

Rydberg atoms are ideal tools for quantum technologies. Due to their large size, their dipole-dipole interaction at micrometer-scale distances and their coupling to external fields are huge. Recent experiments vividly exhibit their interest for quantum simulation, in spite of limitations due to the relatively short lifetime of optically-accessible Rydberg levels. These limitations motivate a renewed interest for the long-lived circular Rydberg states . However, detecting them is so far either destructive or complex. Moreover, alkali circular states can be manipulated only by microwave fields, unable to address individual atoms. Alkaline earth circular states, with their optically active second valence electron, can circumvent these problems. Here we show how to use the electrostatic coupling between the two valence electrons of strontium to coherently manipulate a circular Rydberg state with optical pulses. We also use this coupling to map the state of the Rydberg electron onto that of the ionic core. This experiment opens the way to a state-selective spatially-resolved non-destructive detection of the circular states and, beyond, to the realization of a hybrid optical-microwave platform for quantum technology.

quant-ph↗

arXiv2020

Autonomous Maxwell's demon in a cavity QED system

We present an autonomous Maxwell's demon scheme. It is first analysed theoretically in term of information exchange in a closed system and then implemented experimentally with a single Rydberg atom and a high-quality microwave resonator. The atom simulates both a qubit interacting with the cavity, and a demon carrying information on the qubit state. While the cold qubit crosses the hot cavity, the demon prevents energy absorption from the cavity mode, apparently violating the second law of thermodynamics. Taking into account the change of the mutual information between the demon and the qubit-cavity system gives rise to a generalized expression of the second law that we establish and measure. Finally, considering the closed qubit-cavity-demon system, we establish and measure that the generalized second law can be recast into an entropy conservation law, as expected for a unitary evolution.

quant-ph↗

arXiv2020

Long-lived circular Rydberg states of laser-cooled Rubidium atoms in a cryostat

The exquisite properties of Rydberg levels make them particularly appealing for emerging quantum technologies. The lifetime of low-angular-momentum laser-accessible levels is however limited to a few $100\,μ\mathrm{s}$ by optical transitions and microwave blackbody radiation (BBR) induced transfers at room temperature. A considerable improvement would be obtained with the few $10\,\mathrm{ms}$ lifetime of circular Rydberg levels in a cryogenic environment reducing the BBR temperature. We demonstrate the preparation of long-lived circular Rydberg levels of laser-cooled Rubidium atoms in a cryostat. We observe a $3.7\,\mathrm{ms}$ lifetime for the circular level of principal quantum number $n=52$. By monitoring the transfers between adjacent circular levels, we estimate in situ the microwave BBR temperature to be $(11\pm 2)\,\mathrm{K}$. The measured atomic coherence time ($270\,μ\mathrm{s}$) is limited here only by technical magnetic field fluctuations. This work opens interesting perspectives for quantum simulation and sensing with cold circular Rydberg atoms.

physics.atom-ph↗

arXiv2019

Evaporative cooling to a Rydberg crystal close to its ground state

We theoretically show how to obtain a long one-dimensional crystal near its quantum ground state. We rely on an evaporative cooling scheme applicable to many-body systems with nonzero-ranged interactions. Despite the absence of periodic potentials, the final state is a crystal which exhibits long-range spatial order. We describe the scheme thermodynamically, applying the truncated Boltzmann distribution to the collective excitations of the chain, and show that it leads to a novel quasi-equilibrium many-body state. For longer chains, comprising about 1000 atoms, we emphasize the quasi-universality of the evaporation curve. Such exceptionally long 1D crystals are only accessible deep in the quantum regime. We perform our analysis on the example of an initially thermal chain of circular Rydberg atoms confined to a one-dimensional (1D) geometry. Our scheme may be applied to other quantum systems with long-ranged interactions such as polar molecules.

cond-mat.quant-gas↗

arXiv2019

Benchmarking maximum-likelihood state estimation with an entangled two-cavity state

The efficient quantum state reconstruction algorithm described in [P. Six et al., Phys. Rev. A 93, 012109 (2016)] is experimentally implemented on the non-local state of two microwave cavities entangled by a circular Rydberg atom. We use information provided by long sequences of measurements performed by resonant and dispersive probe atoms over time scales involving the system decoherence. Moreover, we benefit from the consolidation, in the same reconstruction, of different measurement protocols providing complementary information. Finally, we obtain realistic error bars for the matrix elements of the reconstructed density operator. These results demonstrate the pertinence and precision of the method, directly applicable to any complex quantum system.

quant-ph↗

arXiv2018

Fast and accurate circularization of a Rydberg atom

Preparation of a so-called circular state in a Rydberg atom where the projection of the electron angular momentum takes its maximum value is challenging due to the required amount of angular momentum transfer. Currently available protocols for circular state preparation are either accurate but slow or fast but error-prone. Here, we show how to use quantum optimal control theory to derive pulse shapes that realize fast and accurate circularization of a Rydberg atom. In particular, we present a theoretical proposal for optimized radio-frequency pulses that achieve high fidelity in the shortest possible time, given current experimental limitations on peak amplitudes and spectral bandwidth. We also discuss the fundamental quantum speed limit for circularization of a Rydberg atom, when lifting these constraints.

quant-ph↗

arXiv2018

Towards quantum simulation with circular Rydberg atoms

The main objective of quantum simulation is an in-depth understanding of many-body physics. It is important for fundamental issues (quantum phase transitions, transport, . . . ) and for the development of innovative materials. Analytic approaches to many-body systems are limited and the huge size of their Hilbert space makes numerical simulations on classical computers intractable. A quantum simulator avoids these limitations by transcribing the system of interest into another, with the same dynamics but with interaction parameters under control and with experimental access to all relevant observables. Quantum simulation of spin systems is being explored with trapped ions, neutral atoms and superconducting devices. We propose here a new paradigm for quantum simulation of spin-1/2 arrays providing unprecedented flexibility and allowing one to explore domains beyond the reach of other platforms. It is based on laser-trapped circular Rydberg atoms. Their long intrinsic lifetimes combined with the inhibition of their microwave spontaneous emission and their low sensitivity to collisions and photoionization make trapping lifetimes in the minute range realistic with state-of-the-art techniques. Ultra-cold defect-free circular atom chains can be prepared by a variant of the evaporative cooling method. This method also leads to the individual detection of arbitrary spin observables. The proposed simulator realizes an XXZ spin-1/2 Hamiltonian with nearest-neighbor couplings ranging from a few to tens of kHz. All the model parameters can be tuned at will, making a large range of simulations accessible. The system evolution can be followed over times in the range of seconds, long enough to be relevant for ground-state adiabatic preparation and for the study of thermalization, disorder or Floquet time crystals. This platform presents unrivaled features for quantum simulation.

quant-ph↗

arXiv2017

Coherent transfer between low-angular momentum and circular Rydberg states

We realize a coherent transfer between a laser-accessible low-angular-momentum Rydberg state and the circular Rydberg level with maximal angular momentum. This transfer is induced by a radiofrequency field with a high-purity $σ^+$ polarization tuned at resonance on Stark transitions inside the hydrogenic Rydberg manifold. We observe over a few microseconds more than twenty coherent Rabi oscillations between the initial Rydberg state and the circular Rydberg level. We characterize in details these complex oscillations involving many Rydberg levels and find them to be in perfect agreement with a simple theoretical model. This coherent transfer procedure opens the way to hybrid quantum gates bridging the gap between optical communication and quantum information manipulations based on microwave Cavity and Circuit Quantum Electrodynamics.

quant-ph↗

arXiv2016

A quantum-enabled Rydberg atom electrometer

There is no fundamental limit to the precision of a classical measurement. The position of a meter's needle can be determined with an arbitrarily small uncertainty. In the quantum realm, however, fundamental quantum fluctuations due to the Heisenberg principle limit the measurement precision. The simplest measurement procedures, involving semi-classical states of the meter, lead to a fluctuation-limited imprecision at the standard quantum limit. By engineering the quantum state of the meter system, the measurement imprecision can be reduced down to the fundamental Heisenberg Limit (HL). Quantum-enabled metrology techniques are thus in high demand and the focus of an intense activity. We report here a quantum-enabled measurement of an electric field based on this approach. We cast Rydberg atoms in Schrödinger cat states, superpositions of atomic levels with radically different polarizabilites. We use a quantum interference process to perform a measurement close to the HL, reaching a single-shot sensitivity of 1.2 mV/cm for a 100 ns interaction time, corresponding to 30 $μ$V/cm/Hz^(1/2) at our 3 kHz repetition rate. This highly sensitive, non-invasive space- and time-resolved field measurement extends the realm of electrometric techniques and could have important practical applications. Detection of individual electrons in mesoscopic devices at a ~100 $μ$m distance, with a MegaHertz bandwith is within reach.

quant-ph↗

arXiv2014

Past quantum state analysis of the photon number evolution in a cavity

A quantum system can be monitored through repeated interactions with meters, followed by their detection. The state of the system at time t is thus conditioned on the information obtained until that time. More insight in the state dynamics is provided, however, by the past quantum state (PQS) [S. Gammelmark et al. Phys. Rev. Lett. 111, 160401 (2013)]. It relies on all aspects of the system evolution which are recorded in the past and in the future of t. Using PQS analysis for the quantum non-demolition photon number counting in a cavity, we can reveal information hidden in the standard approach and resolve a wider range of number states. This experiment demonstrates the strong potential of PQS analysis.

quant-ph↗