arXiv subjects

Michelle O. Araújo

Publications and source records attributed to Michelle O. Araújo.

11 recordsLinked to original sources

arXiv2026

Temporal dynamics of Levy flights of photons in a three-dimensional geometry for hot vapor

Multiple scattering of light by resonant vapor is characterized by Lévy-type superdiffusion with a step size distribution $P(x) \propto 1/x^{1+α}$, with $0 < α< 2$. The Lévy parameter $α$ was measured from $P(x)$, steady fluorescence, frequency-dependent fluorescence and time-resolved transmission, where the latter was observed for quenched disordered media, not yet for annealed disordered media. Here we report first measurements of this quantity from time-resolved fluorescence for photons that are forward diffused from light pulses exciting a hot rubidium vapor, a medium characterized by annealed disorder, where correlations between the photon steps are absent. Also, the vapor is contained in a three-dimensional geometry, a turned cylinder with respect of the incident photon direction. We show experimentally that $α$ can be extracted from this setup, and the results are consistent with those given by the steady frequency-dependent forward fluorescence. Theoretical simulations are consistent with these results. Also, our simulations show the validity of the one-dimensional theories for our actual geometry and other three-dimensional ones, as thin and thick disks, and a measurement of the number of steps that the photon performed before leaving the medium.

physics.optics↗

arXiv2025

Quantum and classical correlations in four-wave mixing from cold ensembles of two-level atoms

Quantum correlations in four-wave-mixing from ensembles of cold two-level atoms may prevail without filtering over background light with well-known classical interpretations, such as Rayleigh scattering, as recently experimentally demonstrated in Phys. Rev. Lett. {\bf 128}, 083601 (2022). Here we provide an extended investigation of this effect, in which we detail the experimental procedure and the variation of the quantum correlation with various parameters of the system. Particularly, we show that the decay rate of the quantum correlations changes with the number of atoms in the sample, providing another indication of its superradiance-like nature. The nonclassical aspects of the signal occur for short timescales, but the long timescales carry as well a lot of information on the classical correlations of the system. This slow classical regime presents also two clearly distinct timescales, which we explain by two different pathways for the creation of biphotons. From the global analysis of the data in all its timescales, we are able to derive an empirical expression to fit the data, resulting in information on, among other parameters, the sample's temperature and superradiant-like acceleration. In general, the reported quantum correlations present a dependence on critical parameters of the system, such as optical depth and excitation power, that is quite different from other systems used for biphoton generation, and are more robust to changes in these parameters. This opens the possibility of exploring this process for efficient generation of narrow-band biphotons or of other quantum-correlated photonic states of higher order.

quant-ph↗

arXiv2024

Frequency redistribution and step-size distribution of light scattered by atomic vapor: applications to Lévy flight random walk

The propagation of light that undergoes multiple-scattering by resonant atomic vapor can be described as a Lévy flight. Lévy flight is a random walk with heavy tailed step-size (r) distribution, decaying asymptotically as $P(r)\sim r^{-1-α}$, with $α<2$. The large steps, typical of Lévy flights, have its origins in frequency redistribution of the light scattered by the vapor. We calculate the frequency redistribution function and the step-size distribution for light diffusion in atomic vapor. From the step-size distribution we extract a Lévy parameter $α$ that depends on the step's size. We investigate how the frequency redistribution function and step-size distribution are influenced by the finite size of the vapor and the many-level structure typical for alkali vapors. Finite size of the vapor introduces cutoff on the light scattered spectrum and thus in the size of steps. Multi-level structure introduces oscillations in $P(r)$ slope. Both effects might have an impact on measurables related to the Lévy flight random walk.

physics.optics↗

arXiv2024

Enhancing non-classical correlations for light scattered by an ensemble of cold two-level atoms

We report the enhancement of quantum correlations for biphotons generated via spontaneous four-wave mixing in an ensemble of cold two-level atoms. This enhancement is based on the filtering of the Rayleigh linear component of the spectrum of the two emitted photons, favoring the quantum-correlated sidebands reaching the detectors. We provide direct measurements of the unfiltered spectrum presenting its usual triplet structure, with Rayleigh central components accompanied by two peaks symmetrically located at the detuning of the excitation laser with respect to the atomic resonance. The filtering of the central component results in a violation of the Cauchy-Schwarz inequality to $4.8 \pm 1.0 \leq 1$ for a detuning of 60 times the atomic linewidth, representing an enhancement by a factor of four compared with the unfiltered quantum correlations observed at the same conditions.

quant-ph↗

arXiv2022

Observation of nonclassical correlations in biphotons generated from an ensemble of pure two-level atoms

We report the experimental verification of nonclassical correlations for a four-wave-mixing process in an ensemble of cold two-level atoms, confirming theoretical predictions by Du et al. in 2007 for the violation of a Cauchy-Schwarz inequality in the system, and obtaining $R = (1.98\pm0.03) \nleq 1$. Quantum correlations are observed in a nano-seconds timescale, in the interference between the central exciting frequency and sidebands dislocated by the detuning to the atomic resonance. They prevail without filters over the noise background coming from linear scattering from the same optical transition. These correlations are fragile with respect to processes that disturb the phase of the atomic excitation, but are robust to variations in number of atoms and to increasing light intensities.

quant-ph↗

arXiv2021

Lévy flights of photons with infinite mean free path

Multiple scattering of light by resonant vapor is characterized by Lévy-type superdiffusion with a single-step size distribution $p(x)\propto 1/x^{1+α}$. We investigate Lévy flight of light in a hot rubidium vapor collisional-broadened by 50 torr of He gas. The frequent collisions produce Lorentzian absorptive and emissive profiles with $α<1$ and a corresponding divergent mean step size. We extract the Lévy parameter $α\approx0.5$ in a multiple scattering regime from radial profile of the transmission and from violation of the Ohm's law. The measured radial transmission profile and the total diffusive transmission curves are well reproduced by numerical simulations for Lorentzian line shapes.

physics.optics↗

arXiv2018

Subradiance and radiation trapping in cold atoms

We experimentally and numerically study the temporal dynamics of light scattered by large clouds of cold atoms after the exciting laser is switched off in the low intensity (linear optics) regime. Radiation trapping due to multiple scattering as well as subradiance lead to decay much slower than the single atom fluorescence decay. These two effects have already been observed separately, but the interplay between them remained to be understood. Here, we show that with well chosen parameters of the driving field, the two effects can occur at the same time, but follow different scaling behaviors. The subradiant decay is observed at late time and its rate is independent of the detuning, while the radiation trapping decay is observed at intermediate time and depends on the detuning through the optical depth of the sample. Numerical simulations based on random walk process and coupled-dipole equations support our interpretations. Our study clarifies the different interpretations and physical mechanisms at the origin of slow temporal dynamics of light in cold atoms.

physics.atom-ph↗

arXiv2017

Stabilization of a laser on a large-detuned atomic-reference frequency by resonant interferometry

We report a simple technique for stabilization of a laser frequency at the wings of an atomic resonance. The reference signal used for stabilization issues from interference effects obtained in a low-quality cavity filled with a resonant atomic vapour. For a frequency detuned at 2.6 GHz from the $^{133}$Cs D$_2$ 6S$_{1/2}$ F=4 to 6P$_{3/2}$ F'= 5 transition, the fractional frequency Allan deviation is $10^{-8}$ for averaging times of 300 s, corresponding to a frequency deviation of 4 MHz. Adequate choice of the atomic density and of the cell thickness allows locking the laser at detunings larger than 10 GHz. Such a simple technique does not require magnetic fields or signal modulation.

physics.atom-ph↗

arXiv2016

Superradiance in a Large and Dilute Cloud of Cold Atoms in the Linear-Optics Regime

Superradiance has been extensively studied in the 1970s and 1980s in the regime of superfluores-cence, where a large number of atoms are initially excited. Cooperative scattering in the linear-optics regime, or "single-photon superradiance" , has been investigated much more recently, and superra-diant decay has also been predicted, even for a spherical sample of large extent and low density, where the distance between atoms is much larger than the wavelength. Here, we demonstrate this effect experimentally by directly measuring the decay rate of the off-axis fluorescence of a large and dilute cloud of cold rubidium atoms after the sudden switch-off of a low-intensity laser driving the atomic transition. We show that, at large detuning, the decay rate increases with the on-resonance optical depth. In contrast to forward scattering, the superradiant decay of off-axis fluorescence is suppressed near resonance due to attenuation and multiple-scattering effects.

physics.atom-ph↗

arXiv2016

Subradiance in a Large Cloud of Cold Atoms

Since Dicke's seminal paper on coherence in spontaneous radiation by atomic ensembles, superradiance has been extensively studied. Subradiance, on the contrary, has remained elusive, mainly because subradiant states are weakly coupled to the environment and are very sensitive to nonradiative decoherence processes.Here we report the experimental observation of subradiance in an extended and dilute cold-atom sample containing a large number of particles. We use a far detuned laser to avoid multiple scattering and observe the temporal decay after a sudden switch-off of the laser beam. After the fast decay of most of the fluorescence, we detect a very slow decay, with time constants as long as 100 times the natural lifetime of the excited state of individual atoms. This subradiant time constant scales linearly with the cooperativity parameter, corresponding to the on-resonance optical depth of the sample, and is independent of the laser detuning, as expected from a coupled-dipole model.

physics.atom-ph↗

arXiv2014

Measurement of the Kerr nonlinear refractive index of Cs vapor

Atomic vapors are systems well suited for nonlinear optics studies but very few direct measurements of their nonlinear refractive index have been reported. Here we use the z-scan technique to measure the Kerr coefficient, $n_2$, for a Cs vapor. Our results are analyzed through a four-level model, and we show that coherence between excited levels as well as cross-population effects contribute to the Kerr-nonlinearity.

physics.atom-ph↗