arXiv subjects

Miha Ravnik

Publications and source records attributed to Miha Ravnik.

At least 19 recordsLinked to original sources

arXiv2026

Molecular chirality controls droplet division and helical fiber formation in liquid crystal emulsions

Molecular chirality is a source of broken mirror symmetry, but using it to control mesoscale structures with a tunable length scale remains challenging. Here, we demonstrate that adding a chiral dopant to nematic liquid crystal droplets bounded by a deformable two-surfactant interface controls their morphogenesis: the ratio of droplet diameter to cholesteric pitch determines whether droplets divide asymmetrically or symmetrically upon cooling, and whether they transform into single- or double-strand helical fibers. The fiber periodicity and thickness both scale linearly with the cholesteric pitch, which varies by less than 2% with temperature across the self-shaping window. Numerical simulations reveal that chirality-driven elastic stresses at the interface destabilize the droplets and trigger cusp-mediated shape transformations. These results establish cholesteric pitch as a design variable to precisely control droplet division and decouple the dimensions of spontaneously formed mesoscale structures from temperature dependence.

cond-mat.soft↗

arXiv2025

Scallop Theorem for Swimming in Anisotropic Fluids

In isotropic fluids like water, micrometer-scale swimmers have evolved swim strokes to translate despite their tiny size. As described by Purcell in his Scallop Theorem, reciprocal motions, like those performed by a scallop, cannot drive swimming when inertial effects are absent, as is typical at micrometer length scales. Thus, microswimmers have evolved complex structures that can perform non-reciprocal swim strokes or body displacements to generate motion. Microswimmer dynamics in structured fluids differ fundamentally from those in isotropic fluids because of their inherent asymmetry. The orientation of elongated constituents and the topological defects that spontaneously form near microswimmers provide broken symmetries, even atequilibrium. This is sufficient for the dynamic disturbance of even the simplest isotropic swimmers to generate propulsion. We combine experiments on magnetically rotated colloids in nematic liquid crystals with analytic non-equilibrium solutions to formulate propulsion strategies for microswimmers in nematic fluids and determine how swimming velocity depends on the rotation rate, materials parameters, and forcing regimes. For example, we find that micro-scale spherical colloids swim effectively under continuous rotation and under reciprocal forcing.Thus, swim strokes that are ineffective in isotropic fluids are highly effective in nematic liquid crystals. In light of these observations, the Scallop Theorem is extended for structured fluids.

cond-mat.soft↗

arXiv2024

Nematic liquid crystal flow driven by time-varying active surface anchoring

We demonstrate the generation of diverse material flow regimes in nematic liquid cells as driven by time-variable active surface anchoring, including no-net flow, oscillatory flow, steady flow, and pulsating flow. Specifically, we numerically simulate a passive nematic fluid inside a cell bounded with two flat solid boundaries at which the time-dependent anchoring is applied with the dynamically variable surface anchoring easy axis. We show that different flow regimes emerge as the result of different anchoring driving directions (i.e. co-rotating or counter-rotating) and relative phase of anchoring driving. The flow magnitude is tunable by cell thickness and anchoring driving frequency. More generally, this work aims towards possible applications of responsive time-variable surfaces, including photonics or synthetic active matter.

cond-mat.soft↗

arXiv2024

Chirality, anisotropic viscosity and elastic anisotropy in three-dimensional active nematic turbulence

Various active materials exhibit strong spatio-temporal variability of their orientational order known as active turbulence, characterised by irregular and chaotic motion of topological defects, including colloidal suspensions, biofilaments, and bacterial colonies.In particular in three dimensions, it has not yet been explored how active turbulence responds to changes in material parameters and chirality.Here, we present a numerical study of three-dimensional (3D) active nematic turbulence, examining the influence of main material constants: (i) the flow-alignment viscosity, (ii) the magnitude and anisotropy of elastic deformation modes (elastic constants), and (iii) the chirality. Specifically, this main parameter space covers contractile or extensile, flow-aligning or flow tumbling, chiral or achiral elastically anisotropic active nematic fluids. The results are presented using time- and space-averaged fields of defect density and mean square velocity. The results also discuss defect density and mean square velocity as possible effective order parameters in chiral active nematics, distinguishing two chiral nematic states -- active nematic blue phase and chiral active turbulence. This research contributes to the understanding of active turbulence, providing a numerical main phase space parameter sweep to help guide future experimental design and use of active materials.

cond-mat.soft↗

arXiv2023

Three-Dimensional Spontaneous Flow Transition in a Homeotropic Active Nematic

We study the three-dimensional spontaneous flow transition of an active nematic in an infinite slab geometry using a combination of numerics and analytics. We show that it is determined by the interplay of two eigenmodes -- called S- and D-mode -- that are unstable at the same activity threshold and spontaneously breaks both rotational symmetry and chiral symmetry. The onset of the unstable modes is described by a non-Hermitian integro-differential operator, which we determine their exponential growth rates from using perturbation theory. The S-mode is the fastest growing. After it reaches a finite amplitude, the growth of the D-mode is anisotropic, being promoted perpendicular to the S-mode and suppressed parallel to it, forming a steady state with a full three-dimensional director field and a well-defined chirality. Lastly, we derive a model of the leading-order time evolution of the system close to the activity threshold.

cond-mat.soft↗

arXiv2023

Nematronics: Reciprocal coupling between ionic currents and nematic dynamics

Adopting a spintronics-inspired approach, we study the reciprocal coupling between ionic charge currents and nematic texture dynamics in a uniaxial nematic electrolyte. Assuming quenched fluid dynamics, we develop equations of motion analogously to spin torque and spin pumping. Based on the principle of least dissipation of energy, we derive the adiabatic "nematic torque" exerted by ionic currents on the nematic director field as well as the reciprocal motive force on ions due to the orientational dynamics of the director. We discuss several simple examples that illustrate the potential functionality of this coupling. Furthermore, using our phenomenological framework, we propose a practical means to extract the coupling strength through impedance measurements on a nematic cell. Exploring further applications based on this physics could foster the development of nematronics -- nematic iontronics.

cond-mat.soft↗

arXiv2023

Defect Line Coarsening and Refinement in Active Nematics

Active matter is naturally out of equilibrium which results in the emergence of diverse dynamic steady states, including the omnipresent chaotic state known as the active turbulence. However, much less is known how active systems dynamically depart out of these configurations, such as get excited or damped to a different dynamic steady state. In this Letter, we demonstrate the coarsening and refinement dynamics of topological defect lines in three-dimensional active nematic turbulence. Specifically, using theory and numerical modelling, we are able to predict the evolution of the active defect density away from the steady state due to time-dependent activity or viscoelastic material properties, establishing a single length scale phenomenological description of defect line coarsening/refinement in a three-dimensional active nematic. The approach is first applied to growth dynamics of a single active defect loop, and then to a full three-dimensional active defect network. More generally, this work provides insight into the general coarsening phenomena between dynamical regimes in 3D active matter, with a possible analogy in other physical systems.

cond-mat.soft↗

arXiv2023

Topological liquid crystal superstructures as structured light lasers

Liquid crystals (LCs) form an extremely rich range of self-assembled topological structures with artificially or naturally created topological defects. Some of the main applications of LCs are various optical and photonic devices, where compared to their solid state counterparts soft photonic systems are fundamentally different in terms of unique properties such as self-assembly, self-healing, large tunability, sensitivity to external stimuli and biocompatibility. Here we show that complex tunable microlasers emitting structured light can be generated from self-assembled topological LC superstructures containing topological defects inserted into a thin Fabry-Pérot microcavity. The topology and geometry of the LC superstructure determine the structuring of the emitted light by providing complex three dimensionally varying optical axis and order parameter singularities, also affecting the topology of the light polarization. The microlaser can be switched between modes by an electric field and its wavelength can be tuned with temperature. The proposed soft matter microlaser approach opens new direction in soft matter photonics research, where structured light with specifically tailored intensity and polarization fields could be designed and implemented.

physics.optics↗

arXiv2022

Controllable shifting, steering, and expanding of light beam based on multi-layer liquid-crystal cells

Shaping and steering of light beams is essential in many modern applications, ranging from optical tweezers, camera lenses, vision correction to 3D displays. However, current realisations require increasingly greater tunability and aim for lesser specificity for use in diverse applications. Here, we demonstrate tunable light beam control based on multi-layer liquid-crystal cells and external electric field, capable of extended beam shifting, steering, and expanding, using a combination of theory and full numerical modelling, both for liquid crystal orientations and the transmitted light. Specifically, by exploiting three different function-specific and tunable birefringent nematic layers, we show an effective liquid-crystal beam control device, capable of precise control of outgoing light propagation, with possible application in projectors or automotive headlamps.

cond-mat.soft↗

arXiv2022

Numerical modeling of optical modes in topological soft matter

Vector and vortex laser beams are desired in many applications and are usually created by manipulating the laser output or by inserting optical components in the laser cavity. Distinctly, inserting liquid crystals into the laser cavity allows for extensive control over the emitted light due to their high susceptibility to external fields and birefringent nature. In this work we demonstrate diverse optical modes for lasing as enabled and stablised by topological birefringent soft matter structures using numerical modelling. We show diverse structuring of light -- with different 3D intensity and polarization profiles -- as realised by topological soft matter structures in radial nematic droplet, in 2D nematic cavities of different geometry and including topological defects with different charges and winding numbers, in arbitrary varying birefringence fields with topological defects and in pixelated birefringent profiles. We use custom written FDFD code to calculate emergent electromagnetic eigenmodes. Control over lasing is of a particular interest aiming towards the creation of general intensity, polarization and topologically shaped laser beams.

cond-mat.soft↗

arXiv2022

Nematic colloidal micro-robots as physically intelligent systems

Physically intelligent micro-robotic systems exploit information embedded in micro-robots, their colloidal cargo, and their milieu to interact, assemble and form functional structures. Nonlinear anisotropic fluids like nematic liquid crystals (NLCs) provide untapped opportunities to embed interactions via their topological defects, complex elastic responses, and their ability to dramatically restructure in dynamic settings. Here we design and fabricate a 4-armed ferromagnetic micro-robot to embed and dynamically reconfigure information in the nematic director field, generating a suite of physical interactions for cargo manipulation. The micro-robot shape and surface chemistry are designed to generate a nemato-elastic energy landscape in the domain that defines multiple modes of emergent, bottom-up interactions with passive colloids. Micro-robot rotation expands the ability to sculpt interactions; the energy landscape around a rotating micro-robot is dynamically reconfigured by complex far-from-equilibrium dynamics of the micro-robot's companion topological defect. These defect dynamics allow transient information to be programmed into the domain and exploited for top-down cargo manipulation. We demonstrate robust micro-robotic manipulation strategies that exploit these diverse modes of nemato-elastic interaction to achieve cargo docking, transport, release, and assembly of complex reconfigurable structures at multi-stable sites. Such structures are of great interest to future developments of LC-based advanced optical device and micro-manufacturing in anisotropic environments.

cond-mat.soft↗

arXiv2021

Topological defect-propelled swimming of nematic colloids

Non-equilibrium dynamics of topological defects can be used as a fundamental propulsion mechanism in microscopic active matter. Here, we demonstrate swimming of topological defect-propelled colloidal particles in (passive) nematic fluids through experiments and numerical simulations. Dynamic swim strokes of the topological defects are driven by colloidal rotation in an external magnetic field, causing periodic defect rearrangement which propels the particles. The swimming velocity is determined by the colloid's angular velocity, sense of rotation and defect polarity. By controlling them we can locomote the particles along different trajectories. We demonstrate scattering -- that is, the effective pair interactions -- of two of our defect-propelled swimmers, which we show is highly anisotropic and depends on the microscopic structure of the defect stroke, including the local defect topology and polarity. More generally, this work aims to develop biomimetic active matter based on the underlying relevance of topology.

cond-mat.soft↗

arXiv2021

Ionically charged topological defects in nematic fluids

Charge profiles in liquid electrolytes are of crucial importance for applications, such as supercapacitors, fuel cells, batteries, or the self-assembly of particles in colloidal or biological settings. However, creating localised (screened) charge profiles in the bulk of such electrolytes, generally requires the presence of surfaces -- for example, provided by colloidal particles or outer surfaces of the material -- which poses a fundamental constraint on the material design. Here, we show that topological defects in nematic electrolytes can perform as regions for local charge separation, forming charged defect cores and in some geometries even electric multilayers, as opposed to the electric double layers found in isotropic electrolytes. Using a Landau-de Gennes-Poisson-Boltzmann theoretical framework, we show that ions highly effectively couple with the topological defect cores via ion solvability, and with the local director-field distortions of the defects via flexoelectricity. The defect charging is shown for different defect types -- lines, points, and walls -- using geometries of ionically screened flat isotropic-nematic interfaces, radial hedgehog point defects and half-integer wedge disclinations in the bulk and as stabilised by (charged) colloidal particles. More generally, our findings are relevant for possible applications where topological defects act as diffuse ionic capacitors or as ionic charge carriers.

cond-mat.soft↗

arXiv2021

Charge-, salt- and flexoelectricity-driven anchoring effects in nematics

We investigate the effects of electric double layers and flexoelectricity on the surface anchoring in general nematic fluids. Within a simplified model, we demonstrate for a nematic electrolyte how the surface anchoring strength can be affected by the surface charge, bulk ion concentration and/or flexoelectricity, effectively changing not only the magnitude of the anchoring but also the anchoring type, such as from planar to tilted. In particular, we envisage possible tuning of the anchoring strength by the salt concentration in the regime where sufficiently strong electrostatic anchoring, as controlled by the (screened) surface charge, can compete with the non-electrostatic anchoring. This effect is driven by the competing energetic-torque couplings between nematic director and the emergent electrostatic potential, due to surface charge, ions and flexoelectricity. Our findings propose a way of influencing surface anchoring by using electrostatic effects, which could be used in various aspects, including in the self-assembly of colloidal particles in nematic fluids, optical and display patterns, and sensing.

cond-mat.soft↗

arXiv2021

Anisotropic electrostatic screening of charged colloids in nematic solvents

The physical behaviour of anisotropic charged colloids is determined by their material dielectric anisotropy, affecting colloidal self-assembly, biological function and even out-of-equilibrium behaviour. However, little is known about anisotropic electrostatic screening, which underlies all electrostatic effective interactions in such soft or biological materials. In this work, we demonstrate anisotropic electrostatic screening for charged colloidal particles in a nematic electrolyte. We show that material anisotropy behaves markedly different from particle anisotropy: The electrostatic potential and pair interactions decay with an anisotropic Debye screening length, contrasting the constant screening length for isotropic electrolytes. Charged dumpling-shaped near-spherical colloidal particles in a nematic medium are used as an experimental model system to explore the effects of anisotropic screening, demonstrating competing anisotropic elastic and electrostatic effective pair interactions for colloidal surface charges tunable from neutral to high, yielding particle-separated metastable states. Generally, our work contributes to the understanding of electrostatic screening in nematic anisotropic media.

cond-mat.soft↗

arXiv2020

Discharging dynamics of topological batteries

Topological constraints have long been known to provide efficient mechanisms for localizing and storing energy across a range of length scales, from knots in DNA to turbulent plasmas. Despite recent theoretical and experimental progress on the preparation of topological states, the role of topology in the discharging dynamics is not well understood. Here, we investigate robust topological energy release protocols in two archetypal soft systems through simulations of 238 knotted elastic fibers and 3D liquid crystals across a range of different topologies. By breaking the elastic fiber or switching the liquid crystal surface anchoring, such topological batteries can perform mechanical work or drive fluid flows. Our study reveals topologically resonant states for which energy release becomes superslow or superfast. Owing to their intrinsic stability we expect such tunable topological batteries to have broad applications to storage and directed release of energy in soft matter.

cond-mat.soft↗

arXiv2020

Spectral energy analysis of bulk three-dimensional active nematic turbulence

We perform energy spectrum analysis of the active turbulence in 3D bulk active nematic using continuum numerical modelling. Specifically, we calculate the spectra of two main energy contributions---kinetic energy and nematic elastic energy---and combine this with the geometrical analysis of the nematic order and flow fields, based on direct defect tracking and calculation of autocorrelations. We show that the active nematic elastic energy is concentrated at scales corresponding to the effective defect-to-defect separation, scaling with activity as $\simζ^{0.5}$, whereas the kinetic energy is largest at somewhat larger scales of typically several 100 nematic correlation lengths. Nematic biaxiallity is shown to have no role in active turbulence at most of length scales, but can affect the nematic elastic energy by an order of magnitude at scales of active defect core size. The effect of an external aligning field on the 3D active turbulence is explored, showing a transition from an effective active turbulent to an aligned regime. The work is aimed to provide a contribution towards understanding active turbulence in general three-dimensions, from the perspective of main energy-relevant mechanisms at different length scales of the system.

cond-mat.soft↗

arXiv2020

Topological-defect-induced surface charge heterogeneities in nematic electrolytes

We show that topological defects in an ion-doped nematic liquid crystal can be used to manipulate the surface charge distribution on chemically homogeneous, charge-regulating external surfaces, using a minimal theoretical model. In particular, the location and type of the defect encodes the precise distribution of surface charges and the effect is enhanced when the liquid crystal is flexoelectric. We demonstrate the principle for patterned surfaces and charged colloidal spheres. More generally, our results indicate an interesting approach to control surface charges on external surfaces without changing the surface chemistry.

cond-mat.soft↗