Miho Odagiri | Searcharxiv

arXiv2024

Maximizing bipolar sensitivity for anomalous Nernst thermopiles in heat flux sensing in amorphous GdCo alloys

A Heat Flux Sensor (HFS) facilitates the visualization of heat flow, unlike a temperature sensor, and is anticipated to be a key technology in managing waste heat. Recently, an HFS utilizing the Anomalous Nernst Effect (ANE) has been proposed garnering significant interest in enhancing the transverse Seebeck coefficient. However, ideal materials for HFS not only require a large transverse Seebeck coefficient but also meet several criteria including low thermal conductivity and a bipolar nature of the transverse Seebeck coefficient, especially a negative coefficient. In this study, we have investigated ANE in amorphous ferrimagnetic GdCo alloys, revealing their numerous advantages as HFS materials. These include a large transverse Seebeck coefficient, extremely low thermal conductivity, large negative sensitivity, unparalleled bipolar sensitivity, versatility for deposition on various substrates, and a small longitudinal Seebeck coefficient. These qualities position GdCo films as promising candidates for the advancement of HFS technology.

cond-mat.mtrl-sci↗

arXiv2024

Coexistence of large anomalous Nernst effect and large coercive force in amorphous ferrimagnetic TbCo alloy films

The Anomalous Nernst Effect (ANE) has garnered significant interest for practical applications, particularly in energy harvesting and heat flux sensing. For these applications, it is crucial for the module to operate without an external magnetic field, necessitating a combination of a large ANE and a substantial coercive force. However, most materials exhibiting a large ANE typically have a relatively small coercive force. In our research, we have explored the ANE in amorphous ferrimagnetic TbCo alloy films, noting that the coercive force peaks at the magnetization compensation point (MCP). We observed that transverse Seebeck coefficients are amplified with Tb doping, reaching more than 1.0 uV/K over a wide composition range near the MCP, which is three times greater than that of pure Co. Our findings indicate that this enhancement is primarily due to direct conversion, a product of the transverse thermoelectric component and electrical resistivity. TbCo films present several significant advantages for practical use: a large ANE, the capability to exhibit both positive and negative ANE, the flexibility to be deposited on any substrate due to their amorphous nature, a low thermal conductivity, and a large coercive force. These attributes make TbCo films a promising material for advancing ANE-based technologies.

cond-mat.mes-hall↗