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Miina Leiviskä

Publications and source records attributed to Miina Leiviskä.

10 recordsLinked to original sources

Demonstration of ultrafast coherent sub-picosecond magnon pulses

Ultrafast magnonics explores routes towards energy-efficient information processing by replacing electrons with pulses of terahertz magnons. The critical, but so far elusive, requirement on the magnon pulses is the combination of high-speed and a long-range propagation while maintaining a well-defined narrow waveform of the pulses. Here, we demonstrate the launching of 0.4-picosecond magnon pulses in the altermagnetic insulator $α$-Fe$_2$O$_3$ (hematite) using broadband terahertz spin-orbit torques by an adjacent platinum layer. Phase-resolved terahertz transmission reveals that these sub-picosecond pulses travel ballistically, coherently and non-dispersively at a constant velocity of 23 nm/ps, transport angular momentum and retain their temporal waveform shape over 160 nm, with an inferred relaxation length in hundreds of nanometers or more. Beyond establishing $α$-Fe$_2$O$_3$ as an optimal platform for ultrafast magnonics, our technique introduces a high-resolution, tabletop method to directly extract dispersion relations up to high wavevectors, and explore ultrafast magnon dynamics in altermagnets and other magnetic materials with teraherz-range dynamics.

cond-mat.mtrl-sci↗

Spin Hall magnetoresistance at the altermagnetic insulator/Pt interface

The resistance of a heavy metal can be modulated by an adjacent magnetic material through the combined effects of the spin Hall effect, inverse spin Hall effect, and dissipation of the spin accumulation at the interface. This phenomenon is known as the spin Hall magnetoresistance. The dissipation of the spin accumulation can occur via various mechanisms, with spin-transfer torque being the most extensively studied. In this work, we report the observation of spin Hall magnetoresistance at the interface between platinum and an insulating altermagnetic candidate, Ba$_2$CoGe$_2$O$_7$. Our findings reveal that this heterostructure exhibits a relatively large spin Hall magnetoresistance signal, which is anisotropic with respect to the crystal orientation of the current channel. We explore and rule out several potential explanations for this anisotropy and propose that our results may be understood in the context of the anisotropies of the spin current channels across the Pt/altermagnetic Ba$_2$CoGe$_2$O$_7$ interface.

cond-mat.mes-hall↗

Even-in-magnetic field part of transverse resistivity as a probe of magnetic transitions

The component of the resistivity tensor $ρ_{ij}$ corresponding to voltage transverse to both an applied current and a magnetic field can be separated into odd and even parts with respect to the applied magnetic field. The former contains information, for example, about the ordinary or anomalous Hall effect. The latter is often ascribed to experimental artefacts and ignored. Here, we show that upon suppressing these artefacts in carefully controlled experiments, useful information remains. We first investigate the well-explored ferromagnet CoFeB, where the even part of $ρ_{yx}$ contains a contribution from the anisotropic magnetoresistance, which we confirm by Stoner--Wohlfarth modelling. We then apply our approach to magnetotransport measurements of $\rm Mn_5Si_3$ thin films, which undergo a transition from non-collinear to an altermagnetic collinear state. In this material, the even part of the transverse signal is sizable only in the low-spin-symmetry phase below $\approx 80$~K. Transverse resistivity measurements thus offer a simple and readily available probe of magnetic order transitions.

cond-mat.mes-hall↗

Imprinting of skyrmions and bimerons in an antiferromagnet

Topologically protected magnetic states in condensed matter physics, particularly antiferromagnetic (AFM) skyrmions (Sks) and bimerons (Bms), offer promising prospects for terahertz dynamics and sustained current-induced motion, thanks to their compensating multiple sub-lattice structure. However, nucleating AFM Sks and Bms is challenging due to the lack of net magnetization. Previous attempts to imprint pre-defined Sks and Bms in a ferromagnet (FM) and transfer them to an AFM using interfacial exchange bias in FM/AFM heterostructures have been hindered by complex multilayers with discontinuities, polycrystallinity, or multipartite chiral AFMs. Employing atomistic spin simulations, we demonstrate the viability of texture imprinting for nucleating Sks and Bms in AFMs, using a prototypical bipartite AFM layer in a multilayer structure free from discontinuities. Such imprinting is a crucial step towards understanding the static and dynamic properties of natural antiferromagnetic textures and their unique properties.

cond-mat.mtrl-sci↗

Anisotropy of the anomalous Hall effect in the altermagnet candidate Mn$_5$Si$_3$ films

Altermagnets are compensated magnets belonging to spin symmetry groups that allow alternating spin polarizations both in the coordinate space of the crystal and in the momentum space of the electronic structure. In these materials the anisotropic local crystal environment of the different sublattices lowers the symmetry of the system so that the opposite-spin sublattices are connected only by rotations, which results in an unconventional spin-polarized band structure in the momentum space. This low symmetry of the crystal structure is expected to be reflected in the anisotropy of the anomalous Hall effect. In this work, we study the anisotropy of the anomalous Hall effect in epitaxial thin films of Mn$_5$Si$_3$, an altermagnetic candidate material. We first demonstrate a change in the relative Néel vector orientation when rotating the external field orientation through systematic changes in both the anomalous Hall effect and the anisotropic longitudinal magnetoresistance. We then show that the anomalous Hall effect in this material is anisotropic with the Néel vector orientation relative to the crystal structure and that this anisotropy requires high crystal quality and unlikely correlates with the magnetocrystalline anisotropy. Our results provide further systematic support to the case for considering epitaxial thin films of Mn$_5$Si$_3$ as an altermagnetic candidate material.

cond-mat.mes-hall↗

Altermagnetic variants in thin films of Mn5Si3

The altermagnet candidate Mn5Si3 has attracted wide attention in the context of non-relativistic spin physics, due to its composition of light elements. However, the presumed structure of the altermagnetic phase had yet to be demonstrated. In this study, we demonstrate a hallmark of altermagnetism in Mn5Si3 thin films, namely the three options, or variants, for the checkerboard distribution of the magnetic Mn atoms. The magnetic symmetries were altered by field-rotation of the Néel vector along relevant crystal directions, resulting in anomalous Hall effect anisotropy. The experimental results in nanoscale devices were corroborated by a theoretical model involving atomic site dependent anisotropy and bulk Dzyaloshinskii-Moriya interaction for a single variant.

cond-mat.mes-hall↗

Detecting slow magnetization relaxation via magnetotransport measurements based on the current-reversal method

Slow magnetization relaxation processes are an important time-dependent property of many magnetic materials. We show that magnetotransport measurements based on a well-established current-reversal method can be utilized to implement a simple and robust screening scheme for such relaxation processes. We demonstrate our approach considering the anomalous Hall effect in a Pt/Co/AlOx trilayer model system, and then explore relaxation in τ -MnAl films. Compared to magnetotransport experiments based on ac lock-in techniques, we find that the dc current-reversal method is particulary sensitive to relaxation processes with relaxation time scales on the order of seconds, comparable to the current-reversal measurement time scales.

cond-mat.mtrl-sci↗

Observation of the anomalous Nernst effect in altermagnetic candidate Mn5Si3

The anomalous Nernst effect generates transverse voltage to the applied thermal gradient in magnetically ordered systems. The effect was previously considered excluded in compensated magnetic materials with collinear ordering. However, in the recently identified class of compensated magnetic materials, dubbed altermagnets, time-reversal symmetry breaking in the electronic band structure makes the presence of the anomalous Nernst effect possible despite the collinear spin arrangement. In this work, we investigate epitaxial Mn5Si3 thin films known to be an altermagnetic candidate. We show that the material manifests a sizable anomalous Nernst coefficient despite the small net magnetization of the films. The measured magnitudes of the anomalous Nernst coefficient reach a scale of microVolts per Kelvin. We support our magneto-thermoelectric measurements by density-functional theory calculations of the material's spin-split electronic structure, which allows for the finite Berry curvature in the reciprocal space. Furthermore, we present our calculations of the intrinsic Berry-curvature Nernst conductivity, which agree with our experimental observations.

cond-mat.mtrl-sci↗

Local setting of spin textures in a granular antiferromagnet

Controlling the magnetic order of antiferromagnets is challenging due to their vanishing net magnetization. For this reason, the study of local spin textures in antiferromagnets is restricted by the difficulty in nucleating such states. Here, using atomistic simulations we demonstrate a method for nucleating localized spin textures in the grains of thin film antiferromagnet, $γ$-IrMn$_3$. Utilising the exchange bias coupling between a ferromagnet and an antiferromagnet, we set the spin texture in the latter from a predefined spin texture in the former by means of a thermal cycling procedure. The local textures set in the antiferromagnetic grains are shown to be stable against field perturbations. We also discuss how various material parameters affect the efficiency of the setting and the characteristics of these set textures. The setting of antiferromagnetic spin textures provides a potential route to antiferromagnetic spintronic devices with non-collinear spin states such as skyrmions, bubbles and domain walls.

cond-mat.mes-hall↗

Macroscopic time reversal symmetry breaking by staggered spin-momentum interaction

Time-reversal (T) symmetry breaking is a fundamental physics concept underpinning a broad science and technology area, including topological magnets, axion physics, dissipationless Hall currents, or spintronic memories. A best known conventional model of macroscopic T-symmetry breaking is a ferromagnetic order of itinerant Bloch electrons with an isotropic spin interaction in momentum space. Anisotropic electron interactions, on the other hand, have been a domain of correlated quantum phases, such as the T-invariant nematics or unconventional superconductors. Here we report discovery of a broken-T phase of itinerant Bloch electrons with an unconventional anisotropic spin-momentum interaction, whose staggered nature leads to the formation of two ferromagnetic-like valleys in the momentum space with opposite spin splittings. We describe qualitatively the effect by deriving a non-relativistic single-particle Hamiltonian model. Next, we identify the unconventional staggered spin-momentum interaction by first-principles electronic structure calculations in a four-sublattice antiferromagnet Mn5Si3 with a collinear checkerboard magnetic order. We show that the staggered spin-momentum interaction is set by nonrelativistic spin-symmetries which were previously omitted in relativistic physics classifications of spin interactions and topological quasiparticles. Our measurements of a spontaneous Hall effect in epilayers of antiferromagnetic Mn5Si3 with vanishing magnetization are consistent with our theory predictions. Bloch electrons with the unconventional staggered spin interaction, compatible with abundant low atomic-number materials, strong spin-coherence, and collinear antiferromagnetic order open unparalleled possibilities for realizing T-symmetry broken spin and topological quantum phases.

cond-mat.mes-hall↗