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Mikael Käll

Publications and source records attributed to Mikael Käll.

17 recordsLinked to original sources

Deep learning enables large-scale inverse design of free-form metasurfaces

Metasurfaces are ultrathin optical elements that control light through carefully engineered structures smaller than the wavelength of light, enabling compact devices with functionalities that are difficult to achieve with conventional optics. However, exploiting their full design freedom over large areas has been prohibited by the large computational cost of repeated electromagnetic simulations required for inverse design. Here we introduce a physics-tailored deep-learning surrogate model that exploits the locality and symmetries of electromagnetic interactions to generalize from small-scale simulations to metasurfaces orders of magnitude larger. The model captures nonlocal interactions while predicting optical fields more than four orders of magnitude faster than the conventional electromagnetic solver it is trained on, enabling gradient-based topology optimization under arbitrary illumination. We validate the approach through the inverse design and experimental realization of free-form metagratings with diffraction angles up to 75 degrees, as well as a millimeter-scale free-form holographic metasurface more than 1,000 wavelengths across and comprising 1.6 billion degrees of freedom. By decoupling the scale of electromagnetic simulation from the scale of inverse design, our approach enables system-scale free-form photonic devices that retain nanoscale design freedom.

physics.optics↗

Transverse optical gradient force in untethered rotating metaspinners

Nanostructured dielectric metasurfaces offer unprecedented opportunities to control light-matter momentum exchange, and thereby the forces and torques that light can exert on matter. Here we introduce optical metasurfaces as components of ultracompact untethered microscopic metaspinners capable of efficient light-induced rotation in a liquid environment. Illuminated by weakly focused light, a metaspinner generates torque via photon recoil through the metasurfaces ability to bend light towards high angles despite their sub-wavelength thickness, thereby creating orbital angular momentum. We find that a metaspinner is subject to an anomalous transverse lateral optical gradient force that acts in concert with the classical gradient force. Consequently, when two or more metaspinners are trapped together in a laser beam, they collectively orbit the optical axis in the opposite direction to their spinning motion, in stark contrast to rotors coupled through hydrodynamic or mechanical interactions. The metaspinners delineated herein not only serve to illustrate the vast possibilities of utilizing optical metasurfaces for fundamental exploration of optical torques, but they also represent potential building-blocks of artificial active matter systems, light-driven micromachinery, and general-purpose optomechanical devices.

physics.optics↗

Microscopic Geared Mechanisms

The miniaturization of mechanical machines is critical for advancing nanotechnology and reducing device footprints. Traditional efforts to downsize gears and micromotors have faced limitations at around 0.1 mm for over thirty years due to the complexities of constructing drives and coupling systems at such scales. Here, we present an alternative approach utilizing optical metasurfaces to locally drive microscopic machines, which can then be fabricated using standard lithography techniques and seamlessly integrated on the chip, achieving sizes down to tens of micrometers with movements precise to the sub-micrometer scale. As a proof of principle, we demonstrate the construction of microscopic gear trains powered by a single driving gear with a metasurface activated by a plane light wave. Additionally, we develop a versatile pinion and rack micromachine capable of transducing rotational motion, performing periodic motion, and controlling microscopic mirrors for light deflection. Our on-chip fabrication process allows for straightforward parallelization and integration. Using light as a widely available and easily controllable energy source, these miniaturized metamachines offer precise control and movement, unlocking new possibilities for micro- and nanoscale systems.

physics.optics↗

Nanoalignment by Critical Casimir Torques

The manipulation of microscopic objects requires precise and controllable forces and torques. Recent advances have led to the use of critical Casimir forces as a powerful tool, which can be finely tuned through the temperature of the environment and the chemical properties of the involved objects. For example, these forces have been used to self-organize ensembles of particles and to counteract stiction caused by Casimir-Liftshitz forces. However, until now, the potential of critical Casimir torques has been largely unexplored. Here, we demonstrate that critical Casimir torques can efficiently control the alignment of microscopic objects on nanopatterned substrates. We show experimentally and corroborate with theoretical calculations and Monte Carlo simulations that circular patterns on a substrate can stabilize the position and orientation of microscopic disks. By making the patterns elliptical, such microdisks can be subject to a torque which flips them upright while simultaneously allowing for more accurate control of the microdisk position. More complex patterns can selectively trap 2D-chiral particles and generate particle motion similar to non-equilibrium Brownian ratchets. These findings provide new opportunities for nanotechnological applications requiring precise positioning and orientation of microscopic objects.

cond-mat.soft↗

Roadmap for Optical Tweezers

Optical tweezers are tools made of light that enable contactless pushing, trapping, and manipulation of objects ranging from atoms to space light sails. Since the pioneering work by Arthur Ashkin in the 1970s, optical tweezers have evolved into sophisticated instruments and have been employed in a broad range of applications in life sciences, physics, and engineering. These include accurate force and torque measurement at the femtonewton level, microrheology of complex fluids, single micro- and nanoparticle spectroscopy, single-cell analysis, and statistical-physics experiments. This roadmap provides insights into current investigations involving optical forces and optical tweezers from their theoretical foundations to designs and setups. It also offers perspectives for applications to a wide range of research fields, from biophysics to space exploration.

physics.optics↗

Tunable critical Casimir forces counteract Casimir-Lifshitz attraction

Casimir forces in quantum electrodynamics emerge between microscopic metallic objects because of the confinement of the vacuum electromagnetic fluctuations occurring even at zero temperature. Their generalization at finite temperature and in material media are referred to as Casimir--Lifshitz forces. These forces are typically attractive, leading to the widespread problem of stiction between the metallic parts of micro- and nanodevices. Recently, repulsive Casimir forces have been experimentally realized but their reliance on specialized materials prevents their dynamic control and thus limits their further applicability. Here, we experimentally demonstrate that repulsive critical Casimir forces, which emerge in a critical binary liquid mixture upon approaching the critical temperature, can be used to actively control microscopic and nanoscopic objects with nanometer precision. We demonstrate this by using critical Casimir forces to prevent the stiction caused by the Casimir--Lifshitz forces. We study a microscopic gold flake above a flat gold-coated substrate immersed in a critical mixture. Far from the critical temperature, stiction occurs because of dominant Casimir--Lifshitz forces. Upon approaching the critical temperature, however, we observe the emergence of repulsive critical Casimir forces that are sufficiently strong to counteract stiction. This experimental demonstration can accelerate the development of micro- and nanodevices by preventing stiction as well as providing active control and precise tunability of the forces acting between their constituent parts.

cond-mat.soft↗

Microscopic Metavehicles Powered and Steered by Embedded Optical Metasurfaces

Nanostructured dielectric metasurfaces offer unprecedented opportunities to manipulate light by imprinting an arbitrary phase-gradient on an impinging wavefront. This has resulted in the realization of a range of flat analogs to classical optical components like lenses, waveplates and axicons. However, the change in linear and angular optical momentum associated with phase manipulation also results in previously unexploited forces acting on the metasurface itself. Here, we show that these optomechanical effects can be utilized to construct optical metavehicles - microscopic particles that can travel long distances under low-power plane-wave illumination while being steered through the polarization of the incident light. We demonstrate movement in complex patterns, self-correcting motion, and an application as transport vehicles for microscopic cargo, including unicellular organisms. The abundance of possible optical metasurfaces attests to the prospect of developing a wide variety of metavehicles with specialized functional behavior.

physics.optics↗

Strong transient flows generated by thermoplasmonic bubble nucleation

The challenge of inducing and controlling localized fluid flows for generic force actuation and for achieving efficient mass transport in microfluidics is key to the development of next generation miniaturized systems for chemistry and life sciences. Here we demonstrate a methodology for the robust generation and precise quantification of extremely strong flow transients driven by vapor bubble nucleation on spatially isolated plasmonic nanoantennas excited by light. The system is capable of producing peak flow speeds of the order mm/s at modulation rates up to 100 Hz in water, thus allowing for a variety of high-throughput applications. Analysis of flow dynamics and fluid viscosity dependence indicate that the transient originates in the rapid bubble expansion that follows nucleation rather than being strictly thermocapillary in nature.

physics.app-ph↗

Non-equilibrium Properties of an Active Nanoparticle in a Harmonic Potential

Active particles break out of thermodynamic equilibrium thanks to their directed motion, which leads to complex and interesting behaviors in the presence of confining potentials. When dealing with active nanoparticles, however, the overwhelming presence of rotational diffusion hinders directed motion, leading to an increase of their effective temperature, but otherwise masking the effects of self-propulsion. Here, we demonstrate an experimental system where an active nanoparticle immersed in a critical solution and held in an optical harmonic potential features far-from-equilibrium behavior beyond an increase of its effective temperature. When increasing the laser power, we observe a cross-over from a Boltzmann distribution to a non-equilibrium state, where the particle performs fast orbital rotations about the beam axis. These findings are rationalized by solving the Fokker-Planck equation for the particle's position and orientation in terms of a moment expansion. The proposed self-propulsion mechanism results from the particle's non-sphericity and the lower critical point of the solute.

cond-mat.soft↗

Metasurface optical characterization using quadriwave lateral shearing interferometry

An optical metasurface consists of a dense and usually non-uniform layer of scattering nanostructures behaving as a continuous and extremely thin optical component, with predefined phase and intensity transmission/reflection profiles. To date, various sorts of metasurfaces (metallic, dielectric, Huygens-like, Pancharatman-Berry, etc.) have been introduced to design ultrathin lenses, beam deflectors, holograms, or polarizing interfaces. Their actual efficiencies depend on the ability to predict their optical properties and to fabricate non-uniform assemblies of billions of nanoscale structures on macroscopic surfaces. To further help improve the design of metasurfaces, precise and versatile post-characterization techniques need to be developed. Today, most of the techniques used to characterize metasurfaces rely on light intensity measurements. Here, we demonstrate how quadriwave lateral shearing interferometry (QLSI), a quantitative phase microscopy technique, can easily achieve full optical characterization of metasurfaces of any kind, as it can probe the local phase imparted by a metasurface with high sensitivity and spatial resolution. As a means to illustrate the versatility of this technique, we present measurements on two types of metasurfaces, namely Pancharatnam-Berry and effective-refractive-index metasurfaces, and present results on uniform metasurfaces, metalenses and deflectors.

physics.optics↗

Circular dichroism mode splitting and bounds to its enhancement with cavity-plasmon-polaritons

The ability to differentiate chiral molecules of different handedness is of great importance for chemical and life sciences. Since most of the relevant chiral molecules have their chiral transitions in the UV region, detecting their circular dichroism (CD) signal is associated with practical experimental challenges of performing optical measurements in that spectral range. To address this problem, here, we study the possibility of shifting CD signal of a model chiral medium by reaching the strong coupling regime with an optical microcavity. Specifically, we show that by strongly coupling chiral plasmonic nanoparticles to a non-chiral Fabry-Pérot microcavity one can imprint the hybrid mode splitting, the hallmark of strongly coupled systems, on the CD spectrum of the coupled system and thereby effectively shift the chiral resonance of the model system to lower energies. We first predict the effect using analytical transfer-matrix method as well as numerical finite-difference time-domain (FDTD) simulations. Furthermore, we confirm the validity of theoretical predictions in a proof-of-principle experiment involving chiral plasmonic nanoparticles coupled to a Fabry-Pérot microcavity.

physics.optics↗

Transition metal dichalcogenide nanodisks as high-index dielectric Mie nanoresonators

Monolayer transition metal dichalcogenides (TMDCs) have recently been proposed as a unique excitonic platform for advanced optical and electronic functionalities. However, in spite of intense research efforts, it has been largely overlooked that, in addition to displaying rich exciton physics, TMDCs also possess a very high refractive index. This opens a possibility to utilize these materials for constructing resonant nanoantennas based on subwavelength geometrical modes. Here we show that nanodisks fabricated from exfoliated multilayer WS$_2$ support distinct Mie resonances and so-called anapole states that can be easily tuned in wavelength over the visible and near-infrared spectral range by varying the nanodisks' size and aspect ratio. We argue that the TMDC material anisotropy and the presence of excitons substantially enrich nanophotonics by complementing traditional approaches based on plasmonics and well-known high-index materials such as silicon. As a proof-of-concept, we demonstrate a novel regime of light-matter interaction, anapole-exciton polaritons, which we realize within a single WS$_2$ nanodisk. Our results thus suggest that nanopatterned TMDCs are promising materials for high-index nanophotonics applications with enriched functionalities and superior prospects.

physics.optics↗

Optically Controlled Stochastic Jumps of Individual Gold Nanorod Rotary Motors

Brownian microparticles diffusing in optical potential energy landscapes constitute a generic testbed for nonequilibrium statistical thermodynamics and has been used to emulate a wide variety of physical systems, ranging from Josephson junctions to Stirling engines. Here we demonstrate that it is possible to scale down this approach to nanometric length-scales by constructing a tilted washboard potential for the rotation of plasmonic gold nanorods. The potential depth and tilt can be precisely adjusted by modulating the light polarization. This allows for a gradual transition from continuous rotation to discrete stochastic jumps, which are found to follow Kramers dynamics in excellent agreement with stochastic simulations. The results widen the possibilities for fundamental experiments in statistical physics and provide new insights in how to construct light-driven nanomachines and multifunctional sensing elements.

physics.optics↗

Comparative study of plasmonic antennas for strong coupling and quantum nonlinearities with single emitters

Realizing strong coupling between a single quantum emitter (QE) and an optical cavity is of crucial importance in the context of various quantum optical applications. While Rabi splitting of single quantum emitters coupled to high-Q diffraction limited cavities have been reported in numerous configurations, attaining single emitter Rabi splitting with a plasmonic nanostructure is still elusive. Here, we establish the analytical condition for strong coupling between a single QE and a plasmonic nanocavity and apply it to study various plasmonic arrangements that were shown to enable Rabi splitting. We investigate numerically the optical response and the resulting Rabi splitting in metallic nanostructures such as bow-tie nanoantennas, nanosphere dimers and nanospheres on a surface and find the optimal geometries for emergence of the strong coupling regime with single QEs. We also provide a master equation approach to show the saturation of a single QE in the gap of a silver bow-tie nanoantenna. Our results will be useful for implementation of realistic quantum plasmonic nanosystems involving single QEs.

physics.optics↗

Schottky barrier formation and band bending revealed by first principles calculations

An atomistic insight into potential barrier formation and band bending at the interface between a metal and an n-type semiconductor is achieved by ab initio simulations and model analysis of a prototype Schottky diode, i.e., niobium doped rutile titania in contact with gold (Au/Nb:TiO$_2$). The local Schottky barrier height is found to vary between 0 and 1.26 eV depending on the position of the dopant. The band bending is caused by a dopant induced dipole field between the interface and the dopant site, whereas the pristine Au/TiO$_2$ interface does not show any band bending. These findings open the possibility for atomic scale optimization of the Schottky barrier and light harvesting in metal-semiconductor nanostructures.

cond-mat.mes-hall↗

Realizing strong light-matter interactions between single nanoparticle plasmons and molecular excitons at ambient conditions

Realizing strong light-matter interactions between individual 2-level systems and resonating cavities in atomic and solid state systems opens up possibilities to study optical nonlinearities on a single photon level, which can be useful for future quantum information processing networks. However, these efforts have been hampered by the unfavorable experimental conditions, such as cryogenic temperatures and ultrahigh vacuum, required to study such systems and phenomena. Although several attempts to realize strong light-matter interactions at room-temperature using so-called plasmon resonances have been made, successful realizations on the single nanoparticle level are still lacking. Here, we demonstrate strong coupling between plasmons confined within a single silver nanoprism and excitons in molecular J-aggregates at ambient conditions. Our findings show that the deep subwavelength mode volumes, $V$, together with high quality factors, $Q$, associated with plasmons in the nanoprisms result in strong coupling figure-of-merit -- $Q/\sqrt{V}$ as high as $\sim6\times10^{3}$~$μ$m$^{-3/2}$ -- a value comparable to state-of-art photonic crystal and microring resonator cavities, thereby suggesting that plasmonic nanocavities and specifically silver nanoprisms can be used for room-temperature quantum optics.

cond-mat.mes-hall↗

Surface-enhanced Raman scattering and fluorescence near metal nanoparticles

We present a general model study of surface-enhanced resonant Raman scattering and fluorescence, focusing on the interplay between electromagnetic (EM) effects and the molecular dynamics as treated by a density matrix calculation. The model molecule has two electronic levels, is affected by radiative and non-radiative damping mechanisms, and a Franck-Condon mechanism yields electron-vibration coupling. The coupling between the molecule and the electromagnetic field is enhanced by placing it between two Ag nanoparticles. The results show that the Raman scattering cross section can, for realistic parameter values, increase by some 10 orders of magnitude (to $\sim10^{-14}$ cm$^2$) compared with the free-space case. Also the fluorescence cross section grows with increasing EM enhancement, however, at a slower rate, and this increase eventually stalls when non-radiative decay processes become important. Finally, we find that anti-Stokes Raman scattering is possible with strong incident laser intensities, $\sim 1$ mW/$μ$m.

cond-mat.other↗