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Mikhail D. Lukin

Publications and source records attributed to Mikhail D. Lukin.

At least 181 records · Page 10Linked to original sources

Quantum interference of electromechanically stabilized emitters in nanophotonic devices

Photon-mediated coupling between distant matter qubits may enable secure communication over long distances, the implementation of distributed quantum computing schemes, and the exploration of new regimes of many-body quantum dynamics. Nanophotonic devices coupled to solid-state quantum emitters represent a promising approach towards realization of these goals, as they combine strong light-matter interaction and high photon collection efficiencies. However, the scalability of these approaches is limited by the frequency mismatch between solid-state emitters and the instability of their optical transitions. Here we present a nano-electromechanical platform for stabilization and tuning of optical transitions of silicon-vacancy (SiV) color centers in diamond nanophotonic devices by dynamically controlling their strain environments. This strain-based tuning scheme has sufficient range and bandwidth to alleviate the spectral mismatch between individual SiV centers. Using strain, we ensure overlap between color center optical transitions and observe an entangled superradiant state by measuring correlations of photons collected from the diamond waveguide. This platform for tuning spectrally stable color centers in nanophotonic waveguides and resonators constitutes an important step towards a scalable quantum network.

physics.app-ph↗

Periodic orbits, entanglement and quantum many-body scars in constrained models: matrix product state approach

We analyze quantum dynamics of strongly interacting, kinetically constrained many-body systems. Motivated by recent experiments demonstrating surprising long-lived, periodic revivals after quantum quenches in Rydberg atom arrays, we introduce a manifold of locally entangled spin states, representable by low-bond dimension matrix product states, and derive equations of motions for them using the time-dependent variational principle. We find that they feature isolated, unstable periodic orbits, which capture the recurrences and represent nonergodic dynamical trajectories. Our results provide a theoretical framework for understanding quantum dynamics in a class of constrained spin models, which allow us to examine the recently suggested explanation of 'quantum many-body scarring' [Nature Physics (2018), doi:10.1038], and establish a connection to the corresponding phenomenon in chaotic single-particle systems.

quant-ph↗

Rotons in Optical Excitation Spectra of Monolayer Semiconductors

Optically generated excitons dictate the absorption and emission spectrum of doped semiconductor transition metal dichalcogenide monolayers. We show that upon increasing the electron density, the elementary optical excitations develop a roton-like dispersion, evidenced by a shift of the lowest energy state to a finite momentum on the order of the Fermi momentum. This effect emerges due to Pauli exclusion between excitons and the electron Fermi sea, but the robustness of the roton minimum in these systems is a direct consequence of the long-range nature of the Coulomb interaction and the nonlocal dielectric screening characteristic of monolayers. Finally, we show that the emergence of rotons could be related to hitherto unexplained aspects of photoluminescence spectra in doped transition metal dichalcogenide monolayers.

cond-mat.mes-hall↗

Electrical control of interlayer exciton dynamics in atomically thin heterostructures

Excitons in semiconductors, bound pairs of excited electrons and holes, can form the basis for new classes of quantum optoelectronic devices. A van der Waals heterostructure built from atomically thin semiconducting transition metal dichalcogenides (TMDs) enables the formation of excitons from electrons and holes in distinct layers, producing interlayer excitons with large binding energy and a long lifetime. Employing heterostructures of monolayer TMDs, we realize optical and electrical generation of long-lived neutral and charged interlayer excitons. We demonstrate the transport of neutral interlayer excitons across the whole sample that can be controlled by excitation power and gate electrodes. We also realize the drift motion of charged interlayer excitons using Ohmic-contacted devices. The electrical generation and control of excitons provides a new route for realizing quantum manipulation of bosonic composite particles with complete electrical tunability.

cond-mat.mes-hall↗

Emergent SU(2) dynamics and perfect quantum many-body scars

Motivated by recent experimental observations of coherent many-body revivals in a constrained Rydberg atom chain, we construct a weak quasi-local deformation of the Rydberg blockade Hamiltonian, which makes the revivals virtually perfect. Our analysis suggests the existence of an underlying non-integrable Hamiltonian which supports an emergent SU(2)-spin dynamics within a small subspace of the many-body Hilbert space. We show that such perfect dynamics necessitates the existence of atypical, nonergodic energy eigenstates - quantum many-body scars. Furthermore, using these insights, we construct a toy model that hosts exact quantum many-body scars, providing an intuitive explanation of their origin. Our results offer specific routes to enhancing coherent many-body revivals, and provide a step towards establishing the stability of quantum many-body scars in the thermodynamic limit.

quant-ph↗

Theory of dipole radiation near a Dirac photonic crystal

We develop an analytic formalism to describe dipole radiation near the Dirac cone of a two-dimensional photonic crystal slab. In contrast to earlier work, we account for all polarization effects and derive a closed-form expression for the dyadic Green's function of the geometry. Using this analytic Green's function, we demonstrate that the dipolar interaction mediated by the slab exhibits winding phases, which are key ingredients for engineering topological systems for quantum emitters, as discussed in detail in J. Perczel et al., (2018), arXiv:1810.12299. As an example, we study the coherent atomic interactions mediated by the Dirac cone, which were recently shown to be unusually long-range with no exponential attenuation. These results pave the way for further, rigorous analysis of emitters interacting in photonic crystals via photonic Dirac cones.

cond-mat.mes-hall↗

Origins of diamond surface noise probed by correlating single spin measurements with surface spectroscopy

The nitrogen vacancy (NV) center in diamond exhibits spin-dependent fluorescence and long spin coherence times under ambient conditions, enabling applications in quantum information processing and sensing. NV centers near the surface can have strong interactions with external materials and spins, enabling new forms of nanoscale spectroscopy. However, NV spin coherence degrades within 100 nanometers of the surface, suggesting that diamond surfaces are plagued with ubiquitous defects. Prior work on characterizing near-surface noise has primarily relied on using NV centers themselves as probes; while this has the advantage of exquisite sensitivity, it provides only indirect information about the origin of the noise. Here we demonstrate that surface spectroscopy methods and single spin measurements can be used as complementary diagnostics to understand sources of noise. We find that surface morphology is crucial for realizing reproducible chemical termination, and use these insights to achieve a highly ordered, oxygen-terminated surface with suppressed noise. We observe NV centers within 10 nm of the surface with coherence times extended by an order of magnitude.

cond-mat.mtrl-sci↗

Hyperpolarization-enhanced NMR spectroscopy with femtomole sensitivity using quantum defects in diamond

Nuclear magnetic resonance (NMR) spectroscopy is a widely used tool for chemical analysis and molecular structure identification. Because it typically relies on the weak magnetic fields produced by a small thermal nuclear spin polarization, NMR suffers from poor molecule-number sensitivity compared to other analytical techniques. Recently, a new class of NMR sensors based on optically-probed nitrogen-vacancy (NV) quantum defects in diamond have allowed molecular spectroscopy from sample volumes several orders of magnitude smaller than the most sensitive inductive detectors. To date, however, NV-NMR spectrometers have only been able to observe signals from pure, highly concentrated samples. To overcome this limitation, we introduce a technique that combines picoliter-scale NV-NMR with fully integrated Overhauser dynamic nuclear polarization (DNP) to perform high-resolution spectroscopy on a variety of small molecules in dilute solution, with femtomole sensitivity. Our technique advances mass-limited NMR spectroscopy for drug and natural product discovery, catalysis research, and single cell studies.

physics.app-ph↗

Collective motion of an atom array under laser illumination

We develop a theoretical formalism for the study of light-induced motion of atoms trapped in a two-dimensional (2D) array, considering the effect of multiple scattering of light between the atoms. We find that the atomic motion can be described by a collective diffusion equation, wherein laser-induced dipole-dipole forces couple the motion of different atoms. This coupling leads to the formation of collective mechanical modes of the array atoms, whose spatial structure and stability depend on the parameters of the illuminating laser and the geometry of the 2D array. We demonstrate the application of our formalism for the analysis of light-induced heating of the 2D array. The presented approach should be useful for treating the optomechanical properties of recently proposed quantum optical platforms made of atomic arrays.

quant-ph↗

Quantum optomechanics of a two-dimensional atomic array

We demonstrate that a two-dimensional (2D) atomic array can be used as a novel platform for quantum optomechanics. Such arrays feature both nearly-perfect reflectivity and ultra-light mass, leading to significantly-enhanced optomechanical phenomena. Considering the collective atom-array motion under continuous laser illumination, we study the nonlinear optical response of the array. We find that the spectrum of light scattered by the array develops multiple sidebands, corresponding to collective mechanical resonances, and exhibits nearly perfect quantum-noise squeezing. Possible extensions and applications for quantum nonlinear optomechanics are discussed.

quant-ph↗

Quantum Nonlinear Optics in Atomically Thin Materials

We show that a nonlinear optical response associated with a resonant, atomically thin material can be dramatically enhanced by placing it in front of a partially reflecting mirror, rendering otherwise weakly nonlinear systems suitable for experiments and applications involving quantum nonlinear optics. Our approach exploits the nonlinear response of long-lived polariton resonances that arise at particular distances between the material and the mirror. The scheme is entirely based on free-space optics, eliminating the need for cavities or complex nanophotonic structures. We analyze a specific implementation based on exciton-polariton resonances in two-dimensional semiconductors and discuss the role of imperfections and loss.

cond-mat.mes-hall↗

Computational complexity of the Rydberg blockade in two dimensions

We discuss the computational complexity of finding the ground state of the two-dimensional array of quantum bits that interact via strong van der Waals interactions. Specifically, we focus on systems where the interaction strength between two spins depends only on their relative distance $x$ and decays as $1/x^6$ that have been realized with individually trapped homogeneously excited neutral atoms interacting via the so-called Rydberg blockade mechanism. We show that the solution to NP-complete problems can be encoded in ground state of such a many-body system by a proper geometrical arrangement of the atoms. We present a reduction from the NP-complete maximum independent set problem on planar graphs with maximum degree three. Our results demonstrate that computationally hard optimization problems can be naturally addressed with coherent quantum optimizers accessible in near term experiments.

quant-ph↗

Quantum Simulation and Optimization in Hot Quantum Networks

We propose and analyze a setup based on (solid-state) qubits coupled to a common multi-mode transmission line, which allows for coherent spin-spin interactions over macroscopic on-chip distances, without any ground-state cooling requirements for the data bus. Our approach allows for the realization of fast deterministic quantum gates between distant qubits, the simulation of quantum spin models with engineered (long-range) interactions, and provides a flexible architecture for the implementation of quantum approximate optimization algorithms.

quant-ph↗

Quantum Optimization for Maximum Independent Set Using Rydberg Atom Arrays

We describe and analyze an architecture for quantum optimization to solve maximum independent set (MIS) problems using neutral atom arrays trapped in optical tweezers. Optimizing independent sets is one of the paradigmatic, NP-hard problems in computer science. Our approach is based on coherent manipulation of atom arrays via the excitation into Rydberg atomic states. Specifically, we show that solutions of MIS problems can be efficiently encoded in the ground state of interacting atoms in 2D arrays by utilizing the Rydberg blockade mechanism. By studying the performance of leading classical algorithms, we identify parameter regimes, where computationally hard instances can be tested using near-term experimental systems. Practical implementations of both quantum annealing and variational quantum optimization algorithms beyond the adiabatic principle are discussed.

quant-ph↗

Numerical study of the chiral $\mathbb{Z}_3$ quantum phase transition in one spatial dimension

Recent experiments on a one-dimensional chain of trapped alkali atoms [arXiv:1707.04344] have observed a quantum transition associated with the onset of period-3 ordering of pumped Rydberg states. This spontaneous $\mathbb{Z}_3$ symmetry breaking is described by a constrained model of hard-core bosons proposed by Fendley $et\, \,al.$ [arXiv:cond-mat/0309438]. By symmetry arguments, the transition is expected to be in the universality class of the $\mathbb{Z}_3$ chiral clock model with parameters preserving both time-reversal and spatial-inversion symmetries. We study the nature of the order-disorder transition in these models, and numerically calculate its critical exponents with exact diagonalization and density-matrix renormalization group techniques. We use finite-size scaling to determine the dynamical critical exponent $z$ and the correlation length exponent $ν$. Our analysis presents the only known instance of a strongly-coupled transition between gapped states with $z \ne 1$, implying an underlying nonconformal critical field theory.

cond-mat.str-el↗

Photon-mediated interactions between quantum emitters in a diamond nanocavity

Photon-mediated interactions between quantum systems are essential for realizing quantum networks and scalable quantum information processing. We demonstrate such interactions between pairs of silicon-vacancy (SiV) color centers strongly coupled to a diamond nanophotonic cavity. When the optical transitions of the two color centers are tuned into resonance, the coupling to the common cavity mode results in a coherent interaction between them, leading to spectrally-resolved superradiant and subradiant states. We use the electronic spin degrees of freedom of the SiV centers to control these optically-mediated interactions. Our experiments pave the way for implementation of cavity-mediated quantum gates between spin qubits and for realization of scalable quantum network nodes.

quant-ph↗

Solid-state magnetic traps and lattices

We propose and analyze magnetic traps and lattices for electrons in semiconductors. We provide a general theoretical framework and show that thermally stable traps can be generated by magnetically driving the particle's internal spin transition, akin to optical dipole traps for ultra-cold atoms. Next we discuss in detail periodic arrays of magnetic traps, i.e. magnetic lattices, as a platform for quantum simulation of exotic Hubbard models, with lattice parameters that can be tuned in real time. Our scheme can be readily implemented in state-of-the-art experiments, as we particularize for two specific setups, one based on a superconducting circuit and another one based on surface acoustic waves.

quant-ph↗

Probing quantum thermalization of a disordered dipolar spin ensemble with discrete time-crystalline order

We investigate thermalization dynamics of a driven dipolar many-body quantum system through the stability of discrete time crystalline order. Using periodic driving of electronic spin impurities in diamond, we realize different types of interactions between spins and demonstrate experimentally that the interplay of disorder, driving and interactions leads to several qualitatively distinct regimes of thermalization. For short driving periods, the observed dynamics are well described by an effective Hamiltonian which sensitively depends on interaction details. For long driving periods, the system becomes susceptible to energy exchange with the driving field and eventually enters a universal thermalizing regime, where the dynamics can be described by interaction-induced dephasing of individual spins. Our analysis reveals important differences between thermalization of long-range Ising and other dipolar spin models.

quant-ph↗