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Mikhail Kashchenko

Publications and source records attributed to Mikhail Kashchenko.

8 recordsLinked to original sources

Observation of single antiferromagnetic magnon modes through tunnelling spectroscopy of spin-1/2 Kitaev system a-RuCl3

The small-gap room-temperature semiconductor a-RuCl3, which is known to undergo a Mott-Hubbard transition at low temperatures, is one of the most promising candidates for realisation of an exotic matter form, the quantum spin liquid state, which may have applications in quantum computing. Although extensively investigated by neutron scattering techniques, electronic study of this system in the form of van der Waals heterostructures has been limited mainly to graphene proximity. Here we report a systematic study of planar and tunnelling electronic properties of a-RuCl3 films, where we observe an n-type field effect on a-RuCl3 films at room temperature, with a Mott insulator nature onset below 120 K. For films of three-layer thickness and below we find inelastic scattering features, below the N\'eel temperature of 7-14.5 K, which we attribute to single magnon modes. Our study confirms preserved low-temperature signatures of the zigzag antiferromagnetic order in the atomically thin limit and its single magnon modes within the continuum through tunnelling spectroscopy.

cond-mat.mes-hall

All-in-plane image sensors free from readout integrated circuits

High resolution image sensors require electrical access to each individual pixel for signal readout. Such access is especially challenging for ultra-miniaturized pixels, for heterogeneously integrated sensing and readout layers in long-wavelength detectors, and for novel light-sensing materials with unestablished integration to silicon chips. Here, we introduce and experimentally validate a novel imaging approach that does not require electrical connections to individual pixels. The sensor matrix involves photoresistive pixels connected neighbor-to-neighbor and packed into a rectangular lattice. The signal readout is based on electrical impedance tomography applied to the photoresistance: the photovoltage is measured at the matrix boundary at various positions of injected bias current, and the image is reconstructed algorithmically. We present experimental validations for moderate-size infrared imagers based on multilayer graphene (24 pixels) and amorphous vanadium oxide (264 pixels). The reconstruction procedure is mathematically stable, sustainable to variations of pixel resistivity and photosensitivity, and its complexity is that of linear system solution. The proposed method enables unprecedented architecture simplification of imaging devices.

cond-mat.mes-hall

Universal reconstructive polarimetry with graphene-metal infrared photodetectors

Recent advent of smart photodetectors, where in-situ tuning of responsivity enables the reconstruction of light intensity, polarization and spectrum by a single device, has revolutionized the field of optoelectronics. So far, most such reconstructive detectors were realized with non-scalable technology of van der Waals stacking. Here, we demonstrate the infrared reconstructive polarimetry with photodetectors based on conventional gated graphene-metal junctions. The reconstruction exploits the gate tuning of polarization contrast, which enables the determination of both infrared power and polarization angle from photovoltage measurements at two different gate voltages. The physics enabling the polarimetry lies in polarization-dependent shift of the electron hot spot near the contact, and the gate tuning of photosensitive barrier width. We further show the universality of polarization reconstruction, i.e. its feasibility with different geometries of the junction, and with graphene of different quality, from boron-nitride encapsulated flakes to the scalable chemical vapor deposited films.

cond-mat.mes-hall

Optical probing of Wigner crystallization in monolayer WSe$_2$ via diffraction of longitudinal excitons

Monolayer transition metal dichalcogenides (TMDs) are characterized by relatively large carrier effective masses and suppressed screening of the Coulomb interaction, which substantially enhances the correlation effects in these structures. The direct band gap allows to effectively optically probe these correlations. Here, we present an experimental observation of Wigner crystallization in monolayer $\mathrm{WSe}_2$ probed by the measurement of the exciton diffraction on the Wigner crystal (WC) periodic potential. We observe the formation of the WC phase in the absence of external magnetic fields at temperature range $T<26~\mathrm{K}$ and carrier concentrations $n$ $<2\times10^{11}~\mathrm{cm}^{-2}$. The direct observation of the exciton diffraction is enabled by the strong exciton longitudinal-transverse splitting induced by the long-range intervalley exchange interaction, leading to the large detuning between main exciton peak and first diffraction peak. Our findings highlight that the valley degree of freedom of charge carriers in TMDs facilitates optical probing of correlated electron phases in these structures.

cond-mat.mes-hall

Giant exciton binding energy in bulk CrCl3

Van der Waals (vdW) materials, with their unique combination of electronic, optical, and magnetic properties, are emerging as promising platforms for exploring excitonic phenomena. Thus far, the choice of materials with exceptional excitonic response has been limited to two-dimensional (2D) configurations of vdW materials. At the same time, large interlayer distance and the possibility to create a variety of heterostructures offers an opportunity to control the dielectric screening in van der Waals heterostructures and van der Waals 3D materials, thus engineering the excitonic properties. Here, we reveal that bulk vdW crystal CrCl3 answers this quest with a record exciton binding energy of 1.64 eV owing to a delicate interplay of quasi-2D electronic confinement and local magnetic correlations. We also suggest that the non-local magnetic correlations play an important role in the temperature dependence of photoluminescence intensity. Furthermore, we observe colossal binding energies in vdW crystals NbOCl2 (0.66 eV) and MoCl3 (0.35 eV) and formulate a universal exciton binding energy dependence on bandgap for 2D and 3D vdW materials. Hence, our findings establish a fundamental link between the layered structure of vdW materials and their excitonic properties.

cond-mat.mtrl-sci

Multifunctional 2d infrared photodetectors enabled by asymmetric singular metasurfaces

Two-dimensional materials offering ultrafast photoresponse suffer from low intrinsic absorbance, especially in the mid-infrared wavelength range. Challenges in 2d material doping further complicate the creation of light-sensitive $p-n$ junctions. Here, we experimentally demonstrate a graphene-based infrared detector with simultaneously enhanced absorption and strong structural asymmetry enabling zero-bias photocurrent. A key element for those properties is an asymmetric singular metasurface (ASMS) atop graphene with keen metal wedges providing singular enhancement of local absorbance. The ASMS geometry predefines extra device functionalities. The structures with connected metallic wedges demonstrate polarization ratios up to 200 in a broad range of carrier densities at a wavelength of 8.6 $\mu$m. The structures with isolated wedges display gate-controlled switching between polarization-discerning and polarization-stable photoresponse, a highly desirable yet scarce property for polarized imaging.

cond-mat.mes-hall

Ultralow-noise terahertz detection by p-n junctions in gapped bilayer graphene

Graphene shows a strong promise for detection of terahertz (THz) radiation due to its high carrier mobility, compatibility with on-chip waveguides and transistors, and small heat capacitance. At the same time, weak reaction of graphene's physical properties on the detected radiation can be traced down to the absence of band gap. Here, we study the effect of electrically-induced band gap on THz detection in graphene bilayer with split-gate p-n junction. We show that gap induction leads to simultaneous increase in current and voltage responsivities. At operating temperatures of ~25 K, the responsivity at 20 meV band gap is from 3 to 20 times larger than that in the gapless state. The maximum voltage responsivity of our devices at 0.13 THz illumination exceeds 50 kV/W, while the noise equivalent power falls down to 36 fW/Hz^0.5. These values set new records for semiconductor-based cryogenic terahertz detectors, and pave the way for efficient and fast terahertz detection.

cond-mat.mes-hall

Tight-binding terahertz plasmons in chemical vapor deposited graphene

Transistor structures comprising graphene and sub-wavelength metal gratings hold a great promise for plasmon-enhanced terahertz detection. Despite considerable theoretical effort, little experimental evidence for terahertz plasmons in such structures was found so far. Here, we report an experimental study of plasmons in graphene-insulator-grating structures using Fourier transform spectroscopy in 5-10 THz range. The plasmon resonance is clearly visible above the Drude absorption background even in chemical vapor deposited (CVD) graphene with low carrier mobility $\sim 10^3$ cm$^2$/(V s). We argue that plasmon lifetime is weakly sensistive to scattering by grain boundaries and macoscopic defects which limits the mobility of CVD samples. Upon placing the grating in close proximity to graphene, the plasmon field becomes tightly bound below the metal stripes, while the resonant frequency is determined by the stripe width but not by grating period. Our results open the prospects of large-area commercially available graphene for resonant terahertz detectors.

physics.app-ph