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Milena Grifoni

Publications and source records attributed to Milena Grifoni.

At least 19 recordsLinked to original sources

Impact of Nonlinearities on Local Kinetic and Thermokinetic Uncertainty Relations in Bosonic Transport

The precision of transport observables can be bounded by the entropy production and the activity of the transport process via kinetic and thermokinetic uncertainty relations. In linear bosonic systems, such uncertainty relations can provide tight bounds when the activity is replaced by a local activity of the measurement contact of interest---even in the strong-coupling regime. How much nonlinearities (or interactions) impact the validity and predictiveness of these local bounds and how much this impact depends on the concrete definition of activity are open questions that we address for two experimentally relevant model systems, a harmonic oscillator network and the intrinsically nonlinear spin-boson model. We thereby provide experimentally testable predictions on how nonlinearities impact or even break local kinetic and thermokinetic precision bounds.

quant-ph

Transcendental momentum quantization in semiconducting Rashba nanowires and zero energy states in their normal and superconducting phase

We study finite system properties of the canonical low energy model for a semiconducting nanowire with Rashba spin-orbit coupling. The case of an isolated wire as well as of one proximitized by an s-wave superconductor are considered. Already for the normal wire, the presence of spin-orbit coupling leads to eigenstates of the finite system composed of more than two momentum eigenstates. The quantization condition for the wavevectors is not that of a quantum box, but given instead by a transcendental equation linking the involved wavevectors. For the wire with superconducting pairing, the presence of electron and hole channels complicates the composition of the eigenstates. In this case we derive an approximate quantization condition close to the phase boundary, and a condition for the appearance of exact zero energy states. It can be satisfied both in the topological and in the trivial phase. Both the trivial and topological zero energy states contribute to the linear transport through Andreev reflection and direct transmission processes, with their relative importance depending on the degree of the states' localization at the boundary.

cond-mat.mes-hall

A universal route to chiral Ising superconductivity in monolayer TaS$_2$ and NbSe$_2$

We investigate Ising superconductivity in two archetypal intrinsic superconductors, monolayer 1H-TaS$_2$ and 1H-NbSe$_2$, in a bottom-up approach. Using ab initio-based tight-binding parameterizations for the relevant low-energy d-bands, the screened interaction is evaluated microscopically, in a scheme including Bloch overlaps. In direct space, the screened potential displays for both systems long-range Friedel oscillations alternating in sign. Upon scaling, the oscillation pattern becomes universal, with the periodic features locked to the lattice. Solving the momentum-resolved gap equations, a chiral ground state with p-like symmetry is generically found. Due to the larger Ising spin-orbit coupling, the chiral gap is more anisotropic in TaS$_2$ than in NbSe$_2$. This is reflected in tunneling spectra displaying V-shaped features for the former, in quantitative agreement with low-temperature scanning tunneling experiments on TaS$_2$. At the same time, our results reconcile the apparent discordance with hard gap tunneling spectra reported for the sibling NbSe$_2$.

cond-mat.supr-con

Thermal rectification in a qubit-resonator system

A qubit-oscillator junction connecting as a series two bosonic heat baths at different temperatures can display heat valve and diode effects. In particular, the rectification can change in magnitude and even in sign, implying an inversion of the preferential direction for the heat current with respect to the temperature bias. We perform a systematic study of these effects in a circuit QED model of qubit-oscillator system and find that the features of current and rectification crucially depend on the qubit-oscillator coupling. While at small coupling, transport occurs via a resonant mechanism between the sub-systems, in the ultrastrong coupling regime the junction is a unique, highly hybridized system and the current becomes largely insensitive to the detuning. Correspondingly, the rectification undergoes a change of sign. In the nonlinear transport regime, the coupling strength determines whether the current scales sub- or super-linearly with the temperature bias and whether the rectification, which increases in magnitude with the bias, is positive or negative. We also find that steady-state coherence largely suppresses the current and enhances rectification. An insight on these behaviors with respect to changes in the system parameters is provided by analytical approximate formulas.

quant-ph

Friedel oscillations and chiral superconductivity in monolayer NbSe$_2$

In 1965 Kohn and Luttinger proposed a genuine electronic mechanism for superconductivity. Despite the bare electrostatic interaction between two electrons being repulsive, in a metal electron-hole fluctuations can give rise to Friedel oscillations of the screened Coulomb potential. Cooper pairing among the electrons then emerges when taking advantage of the attractive regions. The nature of the leading pairing mechanism in some two-dimensional transition metal dichalcogenides is still debated. Focusing on NbSe$_2$, we show that superconductivity can be induced by the Coulomb interaction when accounting for screening effects on the trigonal lattice with multiple orbitals. Using ab initio-based tight-binding parametrizations for the relevant low-energy d-bands, we evaluate the screened interaction microscopically, in a scheme including Bloch overlaps. In the direct space, we find long-range Friedel oscillations alternating in sign, a key to the Kohn-Luttinger mechanism. The momentum-resolved gap equations predict two degenerate solutions at the critical temperature Tc, signaling the unconventional nature of the pairing. Their complex linear combination, i.e., a chiral gap with p-like symmetry, provides the ground state of the system. Our prediction of a fully gapped chiral phase well below Tc is in excellent agreement with the spectral function extracted from tunneling spectroscopy measurements of single-layer NbSe$_2$.

cond-mat.supr-con

Non-equilibrium cotunneling in interacting Josephson junctions

We investigate non-equilibrium transport through interacting superconducting nanojunctions using a Liouville space approach. The formalism allows us to study finite gap effects, and to account for both quasiparticle and Cooper pair tunneling. With focus on the weak tunneling limit, we study the stationary dc and ac current up to second order (cotunneling) in the hybridization energy. We identify the characteristic virtual processes that yield the Andreev and Josephson current and obtain the dependence on the gate and bias voltage for the dc current, the critical current and the phase-dependent dissipative current. In particular, the critical current is characterized by regions in the stability diagram in which its sign changes from positive to negative, resulting in a multitude of 0-\pi transitions. The latter signal the interplay between strong interactions and tunneling at finite bias.

cond-mat.mes-hall

A particle conserving approach to AC-DC driven interacting quantum dots with superconducting leads

The combined action of a DC bias and a microwave drive on the transport characteristic of a superconductor-quantum dot-superconductor junction is investigated. To cope with time dependent non-equilibrium effects and interactions in the quantum dot, we develop a general formalism for the dynamics of the density operator based on a particle conserving approach to superconductivity. Without invoking a broken U (1) symmetry, we identify a dynamical phase connected to the coherent transfer of Cooper pairs across the junction. In the weak coupling limit, we show that besides quasiparticle transport, proximity induced superconducting correlations manifest in anomalous pair tunneling involving the transfer of a Cooper pair. The resulting generalized master equation in presence of the microwave drive showcases the characteristic bichromatic response due to the combination of the AC Josephson effect and an AC voltage. Analytical expressions for all harmonics in the driving frequency of both the current and the reduced dot operator are given for arbitrary driving strength. For the net DC current the resulting photon assisted processes give rise to rich current-voltage characteristics. In addition to photon assisted subgap transport we find regions of total current inversion in the stability diagram. There, the junction acts as a pump with the net DC current flowing against the applied DC bias. The first harmonic of the current, being closely related to the nonlinear dynamic susceptibility of the junction, is discussed at finite applied DC bias.

cond-mat.mes-hall

Topological transitions in two-dimensional Floquet superconductors

We demonstrate the occurrence of a topological phase transition induced by an effective magnetic field in a two-dimensional electron gas with spin-orbit coupling and in proximity to an $s$-wave superconductor. The effective, perpendicular magnetic field is generated by an in plane, off-resonant ac-magnetic field or by circularly polarized light. The conditions for entering the topological phase do not rely on fine parameter tuning: For fixed frequency, one requires a minimal amplitude of the effective field which can be evaluated analytically. In this phase, chiral edge states generally emerge for a system in stripe geometry unless the Rashba and Dresselhaus coupling have the same magnitude. In this special case, for magnetic field driving the edge states become Majorana flat bands, due to the presence of a chiral symmetry; the light irradiated system is a trivial superconductor.

cond-mat.mes-hall

Two bands Ising superconductivity from Coulomb interactions in monolayer NbSe$_2$

The nature of superconductivity in monolayer transition metal dichalcogenides is still an object of debate. It has already been argued that repulsive Coulomb interactions, combined with the disjoint Fermi surfaces around the $K$, $K'$ valleys and at the $Γ$ point, can lead to superconducting instabilities in monolayer NbSe$_2$. Here, we demonstrate the two bands nature of superconductivity in NbSe$_2$. It arises from the competition of repulsive long range intravalley and short range intervalley interactions together with Ising spin-orbit coupling. The two distinct superconducting gaps, one for each spin-orbit split band, consist of a mixture of s-wave and f-wave components. Their different amplitudes are due to different normal densities of states of the two bands at the Fermi level. Using a microscopic multiband BCS approach, we derive and self-consistently solve the gap equation, demonstrating the stability of nontrivial solutions in a realistic parameter range. We find a universal behavior of the temperature dependence of the gaps and of the critical in-plane field which is consistent with various sets of existing experimental data.

cond-mat.supr-con

$4π$-periodic supercurrent tuned by an axial magnetic flux in topological insulator nanowires

Topological insulator (TI) nanowires in proximity with conventional superconductors have been proposed as a tunable platform to realize topological superconductivity and Majorana zero modes (MZM). The tuning is done using an axial magnetic flux $Φ$ which allows transforming the system from trivial at $Φ=0$ to topologically nontrivial when half a magnetic flux quantum $Φ_0/2$ threads the wire's cross-section. Here we explore the expected topological transition in TI-wire-based Josephson junctions as a function of magnetic flux by probing the $4π$-periodic fraction of the supercurrent, which is considered as an indicator of topological superconductivity. Our data suggest that this $4π$-periodic supercurrent is at lower magnetic field largely of trivial origin, but that at magnetic fields above $\simΦ_{0}/4$ topological $4π$-periodic supercurrents take over.

cond-mat.mes-hall

Supercurrent and phase slips in a ballistic carbon nanotube embedded into a van der Waals heterostructure

We demonstrate long-range superconducting correlations in a several micrometer-long carbon nanotube encapsulated in a van der Waals stack between hBN and NbSe$_2$. We show that a substantial supercurrent flows through the nanotube section beneath the NbSe$_2$ crystal as well as through the 2 $μ$m-long section not in contact with it. As expected for superconductors of nanoscopic cross section, the current-induced breakdown of superconductivity is characterized by resistance steps due to the nucleation of phase slip centers. All elements of our hybrid device are active building blocks of several recently proposed setups for realization of Majorana fermions in carbon nanotubes.

cond-mat.supr-con

Linear and non-linear transport across a finite Kitaev chain: an exact analytical study

We present exact analytical results for the differential conductance of a finite Kitaev chain in an N-S-N configuration, where the topological superconductor is contacted on both sides with normal leads. Our results are obtained with the Keldysh non-equilibrium Green's functions technique, using the full spectrum of the Kitaev chain without resorting to minimal models. A closed formula for the linear conductance is given, and the analytical procedure to obtain the differential conductance for the transport mediated by higher excitations is described. The linear conductance attains the maximum value of $e^2/h$ only for the exact zero energy states. Also the differential conductance exhibits a complex pattern created by numerous crossings and anticrossings in the excitation spectrum. We reveal the crossings to be protected by the inversion symmetry, while the anticrossings result from a pairing-induced hybridization of particle-like and hole-like solutions with the same inversion character. Our comprehensive treatment of the Kitaev chain allows us also to identify the contributions of both local and non-local transmission processes to transport at arbitrary bias voltage. Local Andreev reflection processes dominate the transport within the bulk gap and diminish for higher excited states, but reemerge when the bias voltage probes the avoided crossings. The non-local direct transmission is enhanced above the bulk gap, but contributes also to the transport mediated by the topological states.

cond-mat.mes-hall

Interference and shot noise in a degenerate Anderson-Holstein model

We study the transport properties of an Anderson-Holstein model with orbital degeneracies and a tunneling phase that allows for the formation of dark states. The resulting destructive interference yields a characteristic pattern of positive and negative differential conductance features with enhanced shot noise, without further asymmetry requirements in the coupling to the leads. The transport characteristics are strongly influenced by the Lamb-shift renormalization of the system Hamiltonian. Thus, the electron-vibron coupling cannot be extracted by a simple fit of the current steps to a Poisson distribution. For strong vibronic relaxation, a simpler effective model with analytical solution allows for a better understanding and moreover demonstrates the robustness of the described effects.

cond-mat.mes-hall

Exact eigenvectors and eigenvalues of the finite Kitaev chain and its topological properties

We present a comprehensive, analytical treatment of the finite Kitaev chain for arbitrary chemical potential. We derive the momentum quantization conditions and present exact analytical formulae for the resulting energy spectrum and eigenstate wave functions, encompassing boundary and bulk states. In accordance with an analysis based on the winding number topological invariant, and as expected from the bulk-edge correspondence, the boundary states are topological in nature. They can have zero, exponentially small or even finite energy. A numerical analysis confirms their robustness against disorder.

cond-mat.mes-hall

Unhiding a concealed resonance by multiple Kondo transitions in a quantum dot

Kondo correlations are responsible for the emergence of a zero-bias peak in the low temperature differential conductance of Coulomb blockaded quantum dots. In the presence of a global SU(2)$\otimes$SU(2) symmetry, which can be realized in carbon nanotubes, they also inhibit inelastic transitions which preserve the Kramers pseudospins associated to the symmetry. We report on magnetotransport experiments on a Kondo correlated carbon nanotube where resonant features at the bias corresponding to the pseudospin-preserving transitions are observed. We attribute this effect to a simultaneous enhancement of pseudospin-non-preserving transitions occurring at that bias. This process is boosted by asymmetric tunneling couplings of the two Kramers doublets to the leads and by asymmetries in the potential drops at the leads. Hence, the present work discloses a fundamental microscopic mechanisms ruling transport in Kondo systems far from equilibrium.

cond-mat.str-el

Transmission spectra of an ultrastrongly coupled qubit-dissipative resonator system

We calculate the transmission spectra of a flux qubit coupled to a dissipative resonator in the ultrastrong coupling regime. Such a qubit-oscillator system constitutes the building block of superconducting circuit QED platforms. The calculated transmission of a weak probe field quantifies the response of the qubit, in frequency domain, under the sole influence of the oscillator and of its dissipative environment, an Ohmic heat bath. We find the distinctive features of the qubit-resonator system, namely two-dip structures in the calculated transmission, modified by the presence of the dissipative environment. The relative magnitude, positions, and broadening of the dips are determined by the interplay among qubit-oscillator detuning, the strength of their coupling, and the interaction with the heat bath.

quant-ph

Transverse profile and 3D spin canting of a Majorana state in carbon nanotubes

The full spatial 3D profile of Majorana bound states (MBS) in a nanowire-like setup featuring a semiconducting carbon nanotube (CNT) as the central element is discussed. By accurate tight-binding calculations we show that the chiral nature of the CNT lattice is imprinted in the MBS wave function which has a helical structure, anisotropic in the transverse direction. The local spin canting angle displays a similar spiral pattern, varying around the CNT circumference. We reconstruct the intricate 3D profile of the MBS wave function analytically, using an effective low energy Hamiltonian accounting both for the electronic spin and valley degrees of freedom of the CNT. We find that the four components of the Majorana spinor are related by the three symmetries of our Bogoliubov-de Gennes (BdG) Hamiltonian, reducing the number of independent components to one. A Fourier transform analysis uncovers the presence of three contributions to the MBS, one from the $Γ$-point and one from each of the Fermi points, with further complexity added by the presence of two valley states in each contribution.

cond-mat.mes-hall

Dark states in a carbon nanotube quantum dot

Illumination of atoms by resonant lasers can pump electrons into a coherent superposition of hyperfine levels which can no longer absorb the light. Such superposition is known as dark state, because fluorescent light emission is then suppressed. Here we report an all-electric analogue of this destructive interference effect in a carbon nanotube quantum dot. The dark states are a coherent superposition of valley (angular momentum) states which are decoupled from either the drain or the source leads. Their emergence is visible in asymmetric current-voltage characteristics, with missing current steps and current suppression which depend on the polarity of the applied source-drain bias. Our results demonstrate for the first time coherent-population trapping by all-electric means in an artificial atom.

cond-mat.mes-hall