arXiv subjects

Min Gu

Publications and source records attributed to Min Gu.

27 records · Page 2Linked to original sources

arXiv2020

Giant Polarization and Abnormal Flexural Deformation in Bent Freestanding Perovskite Oxides

Recent realizations of ultrathin freestanding perovskite oxides offer a unique platform to probe novel properties in two-dimensional oxides. Here, we observed a giant flexoelectric response in freestanding BiFeO3 and SrTiO3 in their bent state arising from strain gradients up to 4x10e7/m, suggesting a promising approach for realizing extremely large polarizations. Additionally, a substantial reversible change in thickness was discovered in bent freestanding BiFeO3, which implies an unusual bending-expansion/shrinkage and thickness-dependence Poisson's ratios in this ferroelectric membrane that has never been seen before in crystalline materials. Our theoretical modeling reveals that this unprecedented flexural deformation within the membrane is attributable to a flexoelectricity-piezoelectricity interplay. The finding unveils intriguing nanoscale electromechanical properties and provides guidance for their practical applications in flexible nanoelectromechanical systems.

cond-mat.mtrl-sci↗

arXiv2019

Three-dimensional femtosecond laser nanolithography of crystals

Nanostructuring hard optical crystals has so far been exclusively feasible at their surface, as stress induced crack formation and propagation has rendered high precision volume processes ineffective. We show that the inner chemical etching reactivity of a crystal can be enhanced at the nanoscale by more than five orders of magnitude by means of direct laser writing. The process allows to produce cm-scale arbitrary three-dimensional nanostructures with 100 nm feature sizes inside large crystals in absence of brittle fracture. To showcase the unique potential of the technique, we fabricate photonic structures such as sub-wavelength diffraction gratings and nanostructured optical waveguides capable of sustaining sub-wavelength propagating modes inside yttrium aluminum garnet crystals. This technique could enable the transfer of concepts from nanophotonics to the fields of solid state lasers and crystal optics.

physics.optics↗

arXiv2018

Topological insulator materials for advanced optoelectronic devices

Topological insulators are quantum materials that have an insulating bulk state and a topologically protected metallic surface state with spin and momentum helical locking and a Dirac-like band structure. Unique and fascinating electronic properties, such as the quantum spin Hall effect, quantum anomalous Hall effect, and topological magnetoelectric effect, as well as magnetic monopole images and Majorana fermions, have been observed in the topological insulator materials. With these unique properties, topological insulator materials have great potential applications in spintronics and quantum information processing, as well as magnetoelectric devices with higher efficiency and lower energy consumption. On the other hand, topological insulator materials also exhibit a number of excellent optical properties, including Kerr and Faraday rotation, ultrahigh bulk refractive index, near-infrared frequency transparency, unusual electromagnetic scattering, and ultra-broadband surface plasmon resonances. Specifically, Dirac plasmon excitations have been observed in Bi2Se3 micro-ribbon arrays at THz frequencies. Ultraviolet and visible frequency plasmonics have been observed in nanoslit and nanocone arrays of Bi1.5Sb0.5Te1.8Se1.2 crystals. High transparency has been observed in Bi2Se3 nanoplates. An ultrahigh refractive index has been observed in bulk Bi1.5Sb0.5Te1.8Se1.2 crystals as well as in Sb2Te3 thin films. These excellent optical properties mean that topological insulator materials are suitable for various optoelectronic devices, including plasmonic solar cells, ultrathin holograms, plasmonic and Fresnel lens, broadband photodetectors, and nanoscale waveguides. In this chapter, we focus on the excellent electronic and optical properties of topological insulator materials and their wide applications in advanced optoelectronic devices.

physics.optics↗

arXiv2018

Direct demonstration of the emergent magnetism resulting from the multivalence Mn in a LaMnO3 epitaxial thin film system

Atomically engineered oxide heterostructures provide a fertile ground for creating novel states. For example, a two-dimensional electron gas at the interface between two oxide insulators, giant thermoelectric Seebeck coefficient, emergent ferromagnetism from otherwise nonmagnetic components, and colossal ionic conductivity. Extensive research efforts reveal that oxygen deficiency or lattice strain play an important role in determining these unexpected properties. Herein, by studying the abrupt presence of robust ferromagnetism (up to 1.5 uB/Mn) in LaMnO3-based heterostructures, we find the multivalence states of Mn that play a decisive role in the emergence of ferromagnetism in the otherwise antiferromagnetic LaMnO3 thin films. Combining spatially resolved electron energy-loss spectroscopy, X-ray absorption spectroscopy and X-ray magnetic circular dichroism techniques, we determine unambiguously that the ferromagnetism results from a conventional Mn3+-O-Mn4+ double-exchange mechanism rather than an interfacial effect. In contrast, the magnetic dead layer of 5 unit cell in proximity to the interface is found to be accompanied with the accumulation of Mn2+ induced by electronic reconstruction. These findings provide a hitherto-unexplored multivalence state of Mn on the emergent magnetism in undoped manganite epitaxial thin films, such as LaMnO3 and BiMnO3, and shed new light on all-oxide spintronic devices.

cond-mat.mtrl-sci↗

arXiv2017

Photo-induced change of refractive index and transparency in Bi2Te3 films

We report on an 800 nm femtosecond laser beam induced giant refractive index modulation and enhancement of near-infrared transparency in topological insulator material Bi2Te3 thin films. An ultrahigh refractive index of up to 5.9 was observed in the Bi2Te3 thin film in near-infrared frequency. The refractive index dramatically decreases by a factor of ~ 3 by an exposure to the 800 nm femtosecond laser beam. Simultaneously, the transmittance of the Bi2Te3 thin films markedly increases to ~ 96% in the near-infrared frequency. The Raman spectra provides strong evidences that the observed both refractive index modulation and transparency enhancement result from laser beam induced photooxidation effects in the Bi2Te3 thin films. The Bi2Te3 compound transfers into Bi2O3 and TeO2 under the laser beam illumination. These experimental results pave the way towards the design of various optical devices, such as near-infrared flat lenses, waveguide and holograms, based on topological insulator materials.

cond-mat.mtrl-sci↗

arXiv2016

Photocurrent Enhancement of Graphene Photodetectors by Photon Tunneling of Light into Surface Plasmons

We demonstrate that surface plasmon resonances excited by photon tunneling through an adjacent dielectric medium enhance photocurrent detected by a graphene photodetector. The device is created by overlaying a graphene sheet over an etched gap in a gold film deposited on glass. The detected photocurrents are compared for five different excitation wavelengths, ranging from nm to nm. The photocurrent excited with incident p-polarized light (the case for resonant surface plasmon excitation) is significantly amplified in comparison with that for s-polarized light (without surface plasmon resonances). We observe that the photocurrent is greater for shorter wavelengths (for both s and p-polarizations) due to the increased photothermal current resulting from higher damping of surface plasmons at shorter wavelength excitation. Position-dependent Raman spectroscopic analysis of the optically-excited graphene photodetector indicates the presence of charge carriers near the metallic edge. In addition, we show that the polarity of photocurrent switches across the gap as the incident light spot moves across the gap. Graphene-based photodetectors offer a simple architecture which can be fabricated on dielectric waveguides to exploit the plasmonic photocurrent enhancement of the evanescent field for detection. Applications for these devices include photo-detection, optical sensing and direct plasmonic detection.

physics.optics↗

arXiv2013

Group Theory of Circular-Polarization Effects in Chiral Photonic Crystals with Four-Fold Rotation Axes, Applied to the Eight-Fold Intergrowth of Gyroid Nets

We use group or representation theory and scattering matrix calculations to derive analytical results for the band structure topology and the scattering parameters, applicable to any chiral photonic crystal with body-centered cubic symmetry I432 for circularly-polarised incident light. We demonstrate in particular that all bands along the cubic [100] direction can be identified with the irreducible representations E+/-,A and B of the C4 point group. E+ and E- modes represent the only transmission channels for plane waves with wave vector along the ? line, and can be identified as non-interacting transmission channels for right- (E-) and left-circularly polarised light (E+), respectively. Scattering matrix calculations provide explicit relationships for the transmission and reflectance amplitudes through a finite slab which guarantee equal transmission rates for both polarisations and vanishing ellipticity below a critical frequency, yet allowing for finite rotation of the polarisation plane. All results are verified numerically for the so-called 8-srs geometry, consisting of eight interwoven equal-handed dielectric Gyroid networks embedded in air. The combination of vanishing losses, vanishing ellipticity, near-perfect transmission and optical activity comparable to that of metallic meta-materials makes this geometry an attractive design for nanofabricated photonic materials.

physics.optics↗

arXiv2013

Group Theory of Chiral Photonic Crystals with 4-fold Symmetry: Band Structure and S-Parameters of Eight-Fold Intergrown Gyroid Nets

The Single Gyroid, or srs, nanostructure has attracted interest as a circular-polarisation sensitive photonic material. We develop a group theoretical and scattering matrix method, applicable to any photonic crystal with symmetry I432, to demonstrate the remarkable chiral-optical properties of a generalised structure called 8-srs, obtained by intergrowth of eight equal-handed srs nets. Exploiting the presence of four-fold rotations, Bloch modes corresponding to the irreducible representations E- and E+ are identified as the sole and non-interacting transmission channels for right- and left-circularly polarised light, respectively. For plane waves incident on a finite slab of the 8-srs, the reflection rates for both circular polarisations are identical for all frequencies and transmission rates are identical up to a critical frequency below which scattering in the far field is restricted to zero grating order. Simulations show the optical activity of the lossless dielectric 8-srs to be large, comparable to metallic metamaterials, demonstrating its potential as a nanofabricated photonic material.

physics.optics↗

arXiv2005

Bandgap properties of two-dimensional low-index photonic crystals

We study the bandgap properties of two-dimensional photonic crystals created by a lattice of rods or holes conformed in a symmetric or asymmetric triangular structure. Using the plane-wave analysis, we calculate a minimum value of the refractive index contrast for opening both partial and full two-dimensional spectral gaps for both TM and TE polarized waves. We also analyze the effect of ellipticity of rods and holes and their orientation on the threshold value and the relative size of the bandgap.

physics.optics↗