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Min Xiao

Publications and source records attributed to Min Xiao.

At least 91 records · Page 5Linked to original sources

$\mathcal{PT}$ symmetry in a fractional Schrödinger equation

We investigate the fractional Schrödinger equation with a periodic $\mathcal{PT}$-symmetric potential. In the inverse space, the problem transfers into a first-order nonlocal frequency-delay partial differential equation. We show that at a critical point, the band structure becomes linear and symmetric in the one-dimensional case, which results in a nondiffracting propagation and conical diffraction of input beams. If only one channel in the periodic potential is excited, adjacent channels become uniformly excited along the propagation direction, which can be used to generate laser beams of high power and narrow width. In the two-dimensional case, there appears conical diffraction that depends on the competition between the fractional Laplacian operator and the $\mathcal{PT}$-symmetric potential. This investigation may find applications in novel on-chip optical devices.

physics.optics↗

Diffraction-free beams in fractional Schrödinger equation

We investigate the propagation of one-dimensional and two-dimensional (1D, 2D) Gaussian beams in the fractional Schrödinger equation (FSE) without a potential, analytically and numerically. Without chirp, a 1D Gaussian beam splits into two nondiffracting Gaussian beams during propagation, while a 2D Gaussian beam undergoes conical diffraction. When a Gaussian beam carries linear chirp, the 1D beam deflects along the trajectories $z=\pm2(x-x_0)$, which are independent of the chirp. In the case of 2D Gaussian beam, the propagation is also deflected, but the trajectories align along the diffraction cone $z=2\sqrt{x^2+y^2}$ and the direction is determined by the chirp. Both 1D and 2D Gaussian beams are diffractionless and display uniform propagation. The nondiffracting property discovered in this model applies to other beams as well. Based on the nondiffracting and splitting properties, we introduce the Talbot effect of diffractionless beams in FSE.

physics.optics↗

Efficient Thermal Conductance in Organometallic Perovskite CH3NH3PbI3 Films

Perovskite-based optoelectronic devices have shown great promise for solar conversion and other optoelectronic applications, but their long-term performance instability is regarded as a major obstacle to their widespread deployment. Previous works have shown that the ultralow thermal conductivity and inefficient heat spreading might put an intrinsic limit on the lifetime of perovskite devices. Here, we report the observation of a remarkably efficient thermal conductance, with conductivity of 11.2 +/- 0.8 W m^-1 K^-1 at room temperature, in densely-packed perovskite CH3NH3PbI3 films, via noncontact time-domain thermal reflectance measurements. The temperature-dependent experiments suggest the important roles of organic cations and structural phase transitions, which are further confirmed by temperature-dependent Raman spectra. The thermal conductivity at room temperature observed here is over one order of magnitude larger than that in the early report, suggesting that perovskite device performance will not be limited by thermal stability.

cond-mat.mtrl-sci↗

Coupled orbital angular momentum conversions in a quasi-periodically poled LiTaO3 crystal

We experimentally demonstrate the orbital angular momentum (OAM) conversion by the coupled nonlinear optical processes in a quasi-periodically poled LiTaO3 crystal. In such crystal, third-harmonic generation (THG) is realized by the coupled second-harmonic generation (SHG) and sum-frequency generation (SFG) processes, i.e., SHG is dependent on SFG and vice versa. The OAMs of the interacting waves are proved to be conserved in such coupled nonlinear optical processes. As increasing the input OAM in the experiment, the conversion efficiency decreases because of the reduced fundamental power intensity. Our results provide better understanding for the OAM conversions, which can be used to efficiently produce an optical OAM state at a short wavelength.

physics.optics↗

Probing Carrier Transport and Structure-property Relationship of Highly Ordered Organic Semiconductors at Two-dimensional Limit

One of the basic assumptions in organic field-effect transistors, the most fundamental device unit in organic electronics, is that charge transport occurs two-dimensionally in the first few molecular layers near the dielectric interface. Although the mobility of bulk organic semiconductors has increased dramatically, direct probing of intrinsic charge transport in the two-dimensional limit has not been possible due to excessive disorders and traps in ultrathin organic thin films. Here, highly ordered mono- to tetra-layer pentacene crystals are realized by van der Waals (vdW) epitaxy on hexagonal BN. We find that the charge transport is dominated by hopping in the first conductive layer, but transforms to band-like in subsequent layers. Such abrupt phase transition is attributed to strong modulation of the molecular packing by interfacial vdW interactions, as corroborated by quantitative structural characterization and density functional theory calculations. The structural modulation becomes negligible beyond the second conductive layer, leading to a mobility saturation thickness of only ~3nm. Highly ordered organic ultrathin films provide a platform for new physics and device structures (such as heterostructures and quantum wells) that are not possible in conventional bulk crystals.

cond-mat.mes-hall↗

Photonic Floquet Topological Insulator in an Atomic Ensemble

We demonstrate the photonic Floquet topological insulator (PFTI) in an atomic vapor with nonlinear susceptibilities. The interference of three coupling fields splits the energy levels periodically to form a periodic refractive index structure with honeycomb symmetry that can be adjusted by the choice of frequency detunings and intensities of the coupling fields, which all affect the appearance of Dirac cones in the momentum space. When the honeycomb lattice sites are helically ordered along the propagation direction, we obtain a PFTI in the atomic vapor in which an obliquely incident beam moves along the zigzag edge without scattering energy into the PFTI, due to the confinement of the edge states. The appearance of Dirac cones and the formation of PFTI is strongly affected by the nonlinear susceptibilities; i.e. the PFTI can be shut off by the third-order nonlinear susceptibility and re-opened up by the fifth-order one.

physics.optics↗

Propagation dynamics of a light beam in fractional Schr\"odinger equation

Dynamics of wavepackets in fractional Schrodinger equation is still an open problem. The difficulty stems from the fact that the fractional Laplacian derivative is essentially a nonlocal operator. We investigate analytically and numerically the propagation of optical beams in fractional Schr\"odinger equation with a harmonic potential. We find that the propagation of one- and two-dimensional (1D, 2D) input chirped Gaussian beams is not harmonic. In 1D, the beam propagates along a zigzag trajectory in the real space, which corresponds to a modulated anharmonic oscillation in the momentum space. In 2D, the input Gaussian beam evolves into a breathing ring structure in both real and momentum spaces, which forms a filamented funnel-like aperiodic structure. The beams remain localized in propagation, but with increasing distance display increasingly irregular behavior, unless both the linear chirp and the transverse displacement of the incident beam are zero.

physics.optics↗

Dual accelerating Airy-Talbot recurrence effect

We demonstrate the dual accelerating Airy-Talbot recurrence effect, i.e., the self-imaging of accelerating optical beams, by propagating a superposition of Airy beams with successively changing transverse displacements. The dual Airy-Talbot effect is a spontaneous recurring imaging of the input and of the input with alternating component signs. It results from the constructive interference of Airy wave functions, which is also responsible for other kinds of Airy beams, for example, Airy breathers. An input composed of finite-energy Airy beams also displays the dual Airy-Talbot effect, but it demands a large transverse displacement and diminishes fast along the propagation direction.

physics.optics↗

Single Photon Emission from Single Perovskite Nanocrystals of Cesium Lead Bromide

The power conversion efficiency of photovoltaic devices based on semiconductor perovskites has reached ~20% after just several years of research efforts. With concomitant discoveries of other promising applications in lasers, light-emitting diodes and photodetectors, it is natural to anticipate what further excitements these exotic perovskites could bring about. Here we report on the observation of single photon emission from single CsPbBr3 perovskite nanocrystals (NCs) synthesized from a facile colloidal approach. Compared with traditional metal-chalcogenide NCs, these CsPbBr3 NCs exhibit nearly two orders of magnitude increase in their absorption cross sections at similar emission colors. Moreover, the radiative lifetime of CsPbBr3 NCs is greatly shortened at both room and cryogenic temperatures to favor an extremely fast output of single photons. The above findings have not only added a novel member to the perovskite family for the integration into current optoelectronic architectures, but also paved the way towards quantum-light applications of single perovskite NCs in various quantum information processing schemes.

cond-mat.mtrl-sci↗

Storage and retrieval of photons under their mutual interaction in Rydberg medium

Stopping and regenerating a pair of single-photon pulses at adjacent locations in coherently prepared Rydberg atomic ensembles are significantly affected by their effective interaction mediated by Rydberg excitations, and the similar processes can differ notably from the one exhibiting the common Rydberg blockade as with the stationary propagation of multi-photon light beams in the same medium. Based on the complete dynamics, we reveal the detailed features in such processes by finding how the profiles of the involved quantum fields evolve in various situations. The findings help to determine the proper regimes for implementing photonic gates and transistors. In addition, we discuss the non-adiabatic corrections associated with quickly changing control fields, and illustrate a method that restores the photon pulses' original amplitude during their retrieval unless they are heavily damped before storage.

quant-ph↗

Quantum noise effects with Kerr nonlinearity enhancement in coupled gain-loss waveguides

It is generally difficult to study the dynamical properties of a quantum system with both inherent quantum noises and non-perturbative nonlinearity. Due to the possibly drastic intensity increase of an input coherent light in the gain-loss waveguide couplers with parity-time (PT) symmetry, the Kerr effect from a nonlinearity added into the systems can be greatly enhanced, and is expected to create the macroscopic entangled states of the output light fields with huge photon numbers. Meanwhile, the quantum noises also coexist with the amplification and dissipation of the light fields. Under the interplay between the quantum noises and nonlinearity, the quantum dynamical behaviors of the systems become rather complicated. However, the important quantum noise effects have been mostly neglected in the previous studies about nonlinear PT-symmetric systems. Here we present a solution to this non-perturbative quantum nonlinear problem, showing the real-time evolution of the system observables. The enhanced Kerr nonlinearity is found to give rise to a previously unknown decoherence effect that is irrelevant to the quantum noises, and imposes a limit on the emergence of macroscopic nonclassicality. In contrast to what happen in the linear systems, the quantum noises exert significant impact on the system dynamics, and can create the nonclassical light field states in conjunction with the enhanced Kerr nonlinearity. This first study on the noise involved quantum nonlinear dynamics of the coupled gain-loss waveguides can help to better understand the quantum noise effects in the broad nonlinear systems.

quant-ph↗

Electromagnetically Induced Entanglement

We present a novel quantum phenomenon named electromagnetically induced entanglement in the conventional Lambda-type three-level atomic system driven by a strong pump field and a relatively weak probe field. Nearly perfect entanglement between the pump and probe fields can be achieved with a low coherence decay rate between the two lower levels, high pump-field intensity, and large optical depth of the atomic ensemble. The physical origin is quantum coherence between the lower doublet produced by the pump and probe fields, similar to the well-known electromagnetically induced transparency. This method would greatly facilitate the generation of nondegenerate narrow-band continuous-variable entanglement between bright light beams by using only coherent laser fields, and may find potential and broad applications in realistic quantum information processing.

quant-ph↗

Cyclic permutation-time symmetric structure with coupled gain-loss microcavities

We study the coupled even number of microcavities with the balanced gain and loss between any pair of their neighboring components. The effective non-Hermitian Hamiltonian for such structure has the cyclic permutation-time symmetry with respect to the cavity modes, and this symmetry determines the patterns of the dynamical evolutions of the cavity modes. The systems also have multiple exceptional points for the degeneracy of the existing supermodes, exhibiting the "phase transition" of system dynamics across these exceptional points. We illustrate the quantum dynamical properties of the systems with the evolutions of cavity photon numbers and correlation functions. Moreover, we demonstrate the effects of the quantum noises accompanying the amplification and dissipation of the cavity modes. The reciprocal light transportation predicted with the effective non-Hermitian models for the similar couplers is violated by the unavoidable quantum noises.

quant-ph↗

Magnetic dipolar interaction between correlated triplets created by singlet fission in tetracene crystals

Singlet fission (SF) can potentially break the Shockley-Queisser efficiency limit in single-junction solar cells by splitting one photo-excited singlet exciton (S1) into two triplets (2T1) in organic semiconductors. A dark multi-exciton (ME) state has been proposed as the intermediate connecting S1 to 2T1. However, the exact nature of this ME state, especially how the doubly-excited triplets interact, remains elusive. Here, we report a quantitative study on the magnetic dipolar interaction between SF-induced correlated triplets in tetracene crystals by monitoring quantum beats relevant to the ME sublevels at room temperature. The resonances of ME sublevels approached by tuning an external magnetic field are observed to be avoided, which agrees well with the theoretical predictions considering a magnetic dipolar interaction of ~ 0.008 GHz. Our work paves a way to quantify the magnetic dipolar interaction in organic materials and marks an important step towards understanding the underlying physics of the ME state.

physics.chem-ph↗

Feedback-optimized Extraordinary Optical Transmission of Continuous-variable Entangled States

We report on the feedback-optimized extraordinary optical transmission of continuous-variable entangled states through a hexagonal metal-hole array. The continuous-variable entanglements from a nondegenerate optical parametric amplifier are first demonstrated to survive after a photon-plasmon-photon conversion process. By controlling the reflected light from the metal-hole array, a significant enhancement of quantum correlations has then been experimentally achieved comparing to the case of without such coherent feedback control. This result presents a useful technique to efficiently recover the substantial reflective losses in the plasmonic circuits for quantum information processing.

quant-ph↗

Polarization-dependent exciton dynamics in tetracene single crystals

We conduct polarization-dependent ultrafast spectroscopy to study the dynamics of singlet fission in tetracene single crystals. The spectrotemporal species for singlet and triplet excitons in transient absorption spectra are found to be strongly dependent on probe polarization. By carefully analyzing the polarization dependence, the signals contributed by different transitions related to singlet excitons have been disentangled, which is further applied to construct the correlation between dynamics of singlet and triplet excitons. The anisotropy of exciton dynamics provides an alternative approach to tackle the long-standing challenge in understanding the mechanism of singlet fission in organic semiconductors.

cond-mat.mtrl-sci↗

Strong coupling of an optomechanical system to an anomalously dispersive atomic medium

We investigate a hybrid optomechanical system in which a membrane oscillator is coupled to a collective spin of ground states of an intracavity $Λ$-type three-level atomic medium. The cavity field response is greatly modified by atomic coherence and the anomalous dispersion generated by two Raman pumping beams near two-photon resonance. The optomechanical interaction, therefore radiation pressure force, is substantially enhanced due to superluminal propagation of photons in the cavity. Such improvement facilitates ground-state cooling of the mechanical oscillator with room temperature thermal environment. Moreover, it can greatly improve the sensitivity and bandwidth of displacement measurement. In such system, optically-controlled strong-coupling interaction between the mechanical oscillator and cavity field could be implemented on small intracavity photon number, even at the single quanta level, which is important for weak-light nonlinear photonics and the generation of nonclassical quantum states in the mechanical field.

physics.optics↗

Ultrafast spectroscopy of quasiparticle dynamics in cuprate superconductors

Ultrafast pump-probe spectroscopy is a powerful tool to study the nonequilibrium dynamics in high-Tc cuprate superconductors. The photo-induced quasiparticle (QP) dynamics revealed by pump-probe spectroscopy are sensitive to the near-Fermi level electronic structures. Here we review several selected examples to illustrate the enduring challenges including pairing glue, phase separation, and phase transitions in cuprate superconductors. We also present the data obtained on thin films of YBa2Cu3O7-δ in connection to these issues.

cond-mat.supr-con↗