arXiv subjects

Ming-Guang Hu

Publications and source records attributed to Ming-Guang Hu.

At least 19 recordsLinked to original sources

arXiv2024

Experimental Demonstration of Logical Magic State Distillation

Realizing universal fault-tolerant quantum computation is a key goal in quantum information science. By encoding quantum information into logical qubits utilizing quantum error correcting codes, physical errors can be detected and corrected, enabling substantial reduction in logical error rates. However, the set of logical operations that can be easily implemented on such encoded qubits is often constrained, necessitating the use of special resource states known as 'magic states' to implement universal, classically hard circuits. A key method to prepare high-fidelity magic states is to perform 'distillation', creating them from multiple lower fidelity inputs. Here we present the experimental realization of magic state distillation with logical qubits on a neutral-atom quantum computer. Our approach makes use of a dynamically reconfigurable architecture to encode and perform quantum operations on many logical qubits in parallel. We demonstrate the distillation of magic states encoded in d=3 and d=5 color codes, observing improvements of the logical fidelity of the output magic states compared to the input logical magic states. These experiments demonstrate a key building block of universal fault-tolerant quantum computation, and represent an important step towards large-scale logical quantum processors.

quant-ph↗

arXiv2024

Large-scale quantum reservoir learning with an analog quantum computer

Quantum machine learning has gained considerable attention as quantum technology advances, presenting a promising approach for efficiently learning complex data patterns. Despite this promise, most contemporary quantum methods require significant resources for variational parameter optimization and face issues with vanishing gradients, leading to experiments that are either limited in scale or lack potential for quantum advantage. To address this, we develop a general-purpose, gradient-free, and scalable quantum reservoir learning algorithm that harnesses the quantum dynamics of neutral-atom analog quantum computers to process data. We experimentally implement the algorithm, achieving competitive performance across various categories of machine learning tasks, including binary and multi-class classification, as well as timeseries prediction. Effective and improving learning is observed with increasing system sizes of up to 108 qubits, demonstrating the largest quantum machine learning experiment to date. We further observe comparative quantum kernel advantage in learning tasks by constructing synthetic datasets based on the geometric differences between generated quantum and classical data kernels. Our findings demonstrate the potential of utilizing classically intractable quantum correlations for effective machine learning. We expect these results to stimulate further extensions to different quantum hardware and machine learning paradigms, including early fault-tolerant hardware and generative machine learning tasks.

quant-ph↗

arXiv2023

Quantum interference and entanglement in ultracold atom-exchange reactions

Coherent superpositions and entanglement are hallmarks of quantum mechanics, but they are fragile and can easily be perturbed by their environment. Selected isolated physical systems can maintain coherence and generate entanglement using well-controlled interactions. Chemical reactions, where bonds break and form, are highly dynamic quantum processes. A fundamental question is whether coherence can be preserved in chemical reactions and then harnessed to generate entangled products. Here we investigate this question by studying the 2KRb $\rightarrow$ K$_2$ + Rb$_2$ reaction at 500 nK, focusing on the the nuclear spin degrees of freedom. We prepare the initial nuclear spins in KRb in an entangled state and characterize the preserved coherence in nuclear spin wavefunction after the reaction. The data are consistent with full coherence at the end of the reaction. This suggests that entanglement can be prepared within the reactants, followed by a chemical reaction that produces separate, entangled molecules. We additionally demonstrate control of the reaction product state distribution by deliberately decohering the reactants.

physics.atom-ph↗

arXiv2021

A model for nuclear spin product-state distributions of ultracold chemical reactions in magnetic fields

Based on a theoretical model where the nuclear spins remain unchanged during a collision, we provide an analytical and general expression for the nuclear spin state-to-state distribution of an ultracold chemical reaction in a magnetic field, for given rotational transitions of the molecules. It simply requires knowledge of the field-dependent eigenfunctions of the molecular reactants and products of the chemical reaction. The final state-to-state distribution drastically changes with the magnetic field. When the distribution is summed over all the final products, a simplified expression is found where only the knowledge of the eigenfunctions of the molecular reactants is required. The present theoretical formalism has been successfully used to explain the magnetic field behavior of the product-state distribution in chemical reactions of ultracold KRb molecules [Hu et al., Nat. Chem. 13, 435 (2021)].

physics.atom-ph↗

arXiv2021

Detection of Long-Lived Complexes in Ultracold Atom-Molecule Collisions

We investigate collisional loss in an ultracold mixture of $^{40}$K$^{87}$Rb molecules and $^{87}$Rb atoms, where chemical reactions between the two species are energetically forbidden. Through direct detection of the KRb$_{2}^{*}$ intermediate complexes formed from atom-molecule collisions, we show that a $1064$ nm laser source used for optical trapping of the sample can efficiently deplete the complex population via photo-excitation, an effect which can explain the universal two-body loss observed in the mixture. By monitoring the time-evolution of the KRb$_{2}^{*}$ population after a sudden reduction in the $1064$ nm laser intensity, we measure the lifetime of the complex ($0.39(6)$ ms), as well as the photo-excitation rate for $1064$ nm light ($0.50(3)$ $μ$s$^{-1}($kW/cm$^{2})^{-1}$). The observed lifetime is ${\sim}10^{5}$ times longer than recent estimates based on the Rice-Ramsperger-Kassel-Marcus statistical theory, which calls for new insight to explain such a dramatic discrepancy.

physics.atom-ph↗

arXiv2020

Precision test of statistical dynamics with state-to-state ultracold chemistry

Chemical reactions represent a class of quantum problems that challenge both the current theoretical understanding and computational capabilities. Reactions that occur at ultralow temperatures provide an ideal testing ground for quantum chemistry and scattering theories, as they can be experimentally studied with unprecedented control, yet display dynamics that are highly complex. Here, we report the full product state distribution for the reaction 2KRb $\rightarrow$ K$_2$ + Rb$_2$. Ultracold preparation of the reactants grants complete control over their initial quantum degrees of freedom, while state-resolved, coincident detection of both products enables the measurement of scattering probabilities into all 57 allowed rotational state-pairs. Our results show an overall agreement with a state-counting model based on statistical theory, but also reveal several deviating state-pairs. In particular, we observe a strong suppression of population in the state-pair closest to the exoergicity limit, which we precisely determine to be $9.7711^{+0.0007}_{-0.0005}$ cm$^{-1}$, as a result of the long-range potential inhibiting the escape of products. The completeness of our measurements provides a valuable benchmark for quantum dynamics calculations beyond the current state-of-the-art.

physics.chem-ph↗

arXiv2020

State-to-state control of ultracold molecular reactions

Quantum control of reactive systems has enabled microscopic probes of underlying interaction potentials, the opening of novel reaction pathways, and the alteration of reaction rates using quantum statistics. However, extending such control to the quantum states of reaction outcomes remains challenging. In this work, we realize this goal through the nuclear spin degree of freedom, a result which relies on the conservation of nuclear spins throughout the reaction. Using resonance-enhanced multiphoton ionization spectroscopy to investigate the products formed in bimolecular reactions between ultracold KRb molecules, we find that the system retains a near-perfect memory of the reactants' nuclear spins, manifested as a strong parity preference for the rotational states of the products. We leverage this effect to alter the occupation of these product states by changing the coherent superposition of initial nuclear spin states with an external magnetic field. In this way, we are able to control both the inputs and outputs of a bimolecular reaction with quantum state resolution. The techniques demonstrated here open up the possibilities to study quantum interference between reaction pathways, quantum entanglement between reaction products, and ultracold reaction dynamics at the state-to-state level.

physics.atom-ph↗

arXiv2020

Steering ultracold reactions through long-lived transient intermediates

Controlling the pathways and outcomes of reactions is a broadly pursued goal in chemistry. In gas phase reactions, this is typically achieved by manipulating the properties of the reactants, including their translational energy, orientation, and internal quantum state. In contrast, here we influence the pathway of a reaction via its intermediate complex, which is generally too short-lived to be affected by external processes. In particular, the ultracold preparation of potassium-rubidium (KRb) reactants leads to a long-lived intermediate complex (K$_2$Rb$_2^*$), which allows us to steer the reaction away from its nominal ground-state pathway onto a newly identified excited-state pathway using a laser source at 1064 nm, a wavelength commonly used to confine ultracold molecules. Furthermore, by monitoring the change in the complex population after the sudden removal of the excitation light, we directly measure the lifetime of the complex to be $360 \pm 30$ ns, in agreement with our calculations based on the Rice-Ramsperger-Kassel-Marcus (RRKM) statistical theory. Our results shed light on the origin of the two-body loss widely observed in ultracold molecule experiments. Additionally, the long complex lifetime, coupled with the observed photo-excitation pathway, opens up the possibility to spectroscopically probe the structure of the complex with high resolution, thus elucidating the reaction dynamics.

physics.atom-ph↗

arXiv2019

Probing ultracold chemistry using ion spectrometry

Rapid progress in atomic, molecular, and optical (AMO) physics techniques enabled the creation of ultracold samples of molecular species and opened opportunities to explore chemistry in the ultralow temperature regime. In particular, both the external and internal quantum degrees of freedom of the reactant atoms and molecules are controlled, allowing studies that explored the role of the long range potential in ultracold reactions. The kinetics of these reactions have typically been determined using the loss of reactants as proxies. To extend such studies into the short-range, we developed an experimental apparatus that combines the production of quantum-state-selected ultracold KRb molecules with ion mass and kinetic energy spectrometry, and directly observed KRb + KRb reaction intermediates and products [Science, 2019, 366, 1111]. Here, we present the apparatus in detail. For future studies that aim for detecting the quantum states of the reaction products, we demonstrate a photodissociation based scheme to calibrate the ion kinetic energy spectrometer at low energies.

physics.chem-ph↗

arXiv2019

Direct observation of bimolecular reactions of ultracold KRb molecules

Femtochemistry techniques have been instrumental in accessing the short time scales necessary to probe transient intermediates in chemical reactions. Here we take the contrasting approach of prolonging the lifetime of an intermediate by preparing reactant molecules in their lowest ro-vibronic quantum state at ultralow temperatures, thereby drastically reducing the number of exit channels accessible upon their mutual collision. Using ionization spectroscopy and velocity-map imaging of a trapped gas of potassium-rubidium molecules at a temperature of 500~nK, we directly observe reactants, intermediates, and products of the reaction $^{40}$K$^{87}$Rb + $^{40}$K$^{87}$Rb $\rightarrow$ K$_2$Rb$^*_2$ $\rightarrow$ K$_2$ + Rb$_2$. Beyond observation of a long-lived energy-rich intermediate complex, this technique opens the door to further studies of quantum-state resolved reaction dynamics in the ultracold regime.

physics.atom-ph↗

arXiv2016

Bose polarons in the strongly interacting regime

When an impurity is immersed in a Bose-Einstein condensate, impurity-boson interactions are expected to dress the impurity into a quasiparticle, the Bose polaron. We superimpose an ultracold atomic gas of $^{87}$Rb with a much lower density gas of fermionic $^{40}$K impurities. Through the use of a Feshbach resonance and RF spectroscopy, we characterize the energy, spectral width and lifetime of the resultant polaron on both the attractive and the repulsive branches in the strongly interacting regime. The width of the polaron in the attractive branch is narrow compared to its binding energy, even as the two-body scattering length formally diverges.

cond-mat.quant-gas↗

arXiv2014

Looking for "avalanche-mechanism" loss at an atom-molecule Efimov resonance

The "avalanche mechanism" has been used to relate Efimov trimer states to certain enhanced atom loss features observed in ultracold atom gas experiments. These atom loss features are argued to be a signature of resonant atom-molecule scattering that occurs when an Efimov trimer is degenerate with the atom-molecule scattering threshold. However, observation of these atom loss features has yet to be combined with the direct observation of atom-molecule resonant scattering for any particular atomic species. In addition, recent Monte-Carlo simulations were unable to reproduce a narrow loss feature. We experimentally search for enhanced atom loss features near an established scattering resonance between 40K87Rb Feshbach molecules and 87Rb atoms. Our measurements of both the three-body recombination rate in a gas of 40K and 87Rb atoms and the ratio of the number loss for the two species do not show any broad loss feature and are therefore inconsistent with theoretical predictions that use the avalanche mechanism.

cond-mat.quant-gas↗

arXiv2013

Feshbach molecule formation in a Bose-Fermi mixture

We investigate magnetoassociation of ultracold fermionic Feshbach molecules in a mixture of $^{40}$K and $^{87}$Rb atoms, where we can create as many as $7\times 10^4$ $^{40}$K$^{87}$Rb molecules with a conversion efficiency as high as 45%. In the perturbative regime, we find that the conversion efficiency depends linearly on the density overlap of the two gases, with a slope that matches a parameter-free model that uses only the atom masses and the known Feshbach resonance parameters. In the saturated regime, we find that the maximum number of Feshbach molecules depends on the atoms' phase-space density. At higher temperatures, our measurements agree with a phenomenological model that successfully describes the formation of bosonic molecules from either Bose or Fermi gases. However, for quantum degenerate atom gas mixtures, we measure significantly fewer molecules than this model predicts.

cond-mat.quant-gas↗

arXiv2013

Tests of universal three-body physics in an ultracold Bose-Fermi mixture

Recent measurements of Efimov resonances in a number of ultracold atom species have revealed an unexpected universality, in which three-body scattering properties are determined by the van der Waals length of the two-body interaction potential. To investigate whether this universality extends to heteronuclear mixtures, we measure loss rate coefficients in an ultracold trapped gas of $^{40}$K and $^{87}$Rb atoms. We find an Efimov-like resonance in the rate of inelastic collisions between $^{40}$K$^{87}$Rb Feshbach molecules and $^{87}$Rb atoms. However, we do not observe any Efimov-related resonances in the rates of inelastic collisions between three atoms. These observations are compared to previous measurements by the LENS group of Efimov resonances in a $^{41}$K and $^{87}$Rb mixture as well as to recent predictions.

cond-mat.quant-gas↗

arXiv2009

Geometric phase of a two-level system in a dissipative environment

The geometric (Berry) phase of a two-level system in a dissipative environment is analyzed by using the second-quantized formulation, which provides a unified and gauge-invariant treatment of adiabatic and nonadiabatic phases and is thus applicable to a quantitative analysis of transitional regions away from ideal adiabaticity. In view of the recent experimental observation of the Berry phase in a superconducting qubit, we illustrate our formulation for a concrete adiabatic case in the Ohmic dissipation. The correction to the total phase together with the geometry-dependent dephasing time is given in a transparent way. The behavior of the geometric phase away from ideal adiabaticity is also analyzed in some detail.

quant-ph↗

arXiv2009

Proposed all-versus-nothing violation of local realism in the Kitaev spin-lattice model

We investigate the nonlocal property of the fractional statistics in Kitaev's toric code model. To this end, we construct the Greenberger-Horne-Zeilinger paradox which builds a direct conflict between the statistics and local realism. It turns out that the fractional statistics in the model is purely a quantum effect and independent of any classical theory.We also discuss a feasible experimental scheme using anyonic interferometry to test this contradiction.

quant-ph↗

arXiv2008

Exact Solution of a Yang-Baxter Spin-1/2 Chain Model and Quantum Entanglement

Entanglement is believed to be crucial in macroscopic physical systems for understanding the collective quantum phenomena such as quantum phase transitions. We start from and solve exactly a novel Yang-Baxter spin-1/2 chain model with inhomogeneous and anisotropic short-range interactions. For the ground state, we show the behavior of neighboring entanglement in the parameter space and find that the inhomogeneous coupling strengths affect entanglement in a distinctive way from the homogeneous case, but this would not affect the coincidence between entanglement and quantum criticality.

quant-ph↗

arXiv2008

Maximal Quantum Violation of the CGLMP Inequality on Its Both Sides

We investigate the maximal violations for both sides of the $d$-dimensional CGLMP inequality by using the Bell operator method. It turns out that the maximal violations have a decelerating increase as the dimension increases and tend to a finite value at infinity. The numerical values are given out up to $d=10^6$ for positively maximal violations and $d=2\times 10^5$ for negatively maximal violations. Counterintuitively, the negatively maximal violations tend to be a little stronger than the positively maximal violations. Further we show the states corresponding to these maximal violations and compare them with the maximally entangled states by utilizing entangled degree defined by von Neumann entropy. It shows that their entangled degree tends to some nonmaximal value as the dimension increases.

quant-ph↗