arXiv subjects

Minoru Yamashita

Publications and source records attributed to Minoru Yamashita.

At least 19 recordsLinked to original sources

arXiv2026

Signatures of field-induced multi-color kagome spin liquids in the dipole-octupole pyrochlore $\mathrm{Ce_2Hf_2O_7}$

We report low-temperature magnetization and magnetostriction measurements on the dipole-octupole pyrochlore $\mathrm{Ce_2Hf_2O_7}$, revealing an unconventional field response for $\mathbf B\parallel[111]$. The magnetization shows no kagome-ice plateau; instead it evolves continuously and exhibits two rapid changes in slope near 0.35~T and 1.2~T, accompanied by magnetostriction features at the same field scales. Classical Monte Carlo simulations, exact diagonalization, and ground-state analysis of the Hamiltonian show that a representative QSI-compatible parameter set captures the data. For this parameter set, the lower-field anomaly marks a closely spaced transition sequence from a two-color kagome spin liquid (KSL) through a narrow three-color KSL into a mixed two-/three-color KSL, while the upper-field anomaly marks the transition from the mixed KSL into a nearly polarized state. These results identify $\mathrm{Ce_2Hf_2O_7}$, and dipole-octupole pyrochlore magnets more broadly, as promising platforms for exotic KSLs beyond conventional spin ice.

cond-mat.str-el↗

arXiv2026

Anomalies in the thermal conductivity of honeycomb antiferromagnet MnPS$_{3}$

Intrinsic two-dimensional magnets serve as a good platform to explore collective, charge-neutral and low-energy excitations. Distinguishing the crucial role of them in experimental aspect remains a challenge for decades. Here, we study the thermal transport in honeycomb antiferromagnet MnPS$_{3}$ with $T_N$=78 K down to very low temperatures (<0.01$T_N$). At high temperatures (>0.1$T_N$), the field dependence of the thermal Hall conductivity exhibits a linear phonon Hall effect and a peak associated with the spin-flop transition due to a strong spin-lattice coupling, well reproducing the previous report (Phys. Rev. B 110, 165147 (2024)). Notably, below 2 K, we find that the field dependence of the thermal Hall conductivity exhibits sign reversals within the spin-flop phase, at which the field dependence of the longitudinal thermal conductivity also shows multiple valleys. We suggest that these anomalies are caused by the redistribution of Berry curvature in magnon bands, demonstrating the superior performance of the thermal Hall measurements to detect the Berry curvature distributions in magnetic insulators.

cond-mat.mtrl-sci↗

arXiv2025

Field-Angle Dependence of Phonon Thermal Hall Effect in Na2X2TeO6 (X = Co, Zn)

The mechanism behind thermal Hall effects by phonons, which are observed in various materials, is not clarified despite the dominant contribution as heat carriers. Theoretically, mechanisms based on the intrinsic Berry phase and those on extrinsic impurity-induced scatterings have been proposed, which can be distinguished by comparing the field-angle dependence of the thermal Hall effect and that of the magnetic anisotropy. Here, we investigate the field-angle dependence of the thermal Hall effects in the antiferromagnet Na2Co2TeO6 and its non-magnetic isostructural analogue Na2Zn2TeO6 in the ac plane. We find that the field-angle dependence of the thermal Hall conductivity in both materials well follows that of the out-of-plane magnetization, showing a common mechanism by extrinsic impurity-induced scatterings in both the phonon thermal Hall effect and that enhanced by a coupling with the magnetism.

cond-mat.mtrl-sci↗

arXiv2025

Observation of Anomalous Thermal Hall Effect in a Kagome Superconductor

Broken time-reversal symmetry (TRS) in superconductors can induce not only spontaneous magnetization by the finite angular momentum of Cooper pairs, but also anomalous thermal Hall effects (ATHEs), whose detection has been extremely challenging. Here we report the successful observation of an ATHE developing below the superconducting transition temperature at zero magnetic field in the kagome-lattice superconductor CsV3Sb5. This finding is verified by the absence of a signal in a conventional type-II superconductor using the same setup and by ruling out the trapped-vortex effects through micro-Hall array measurements. Remarkably, both the temperature dependence and the magnitude of the observed anomalous thermal Hall conductivity are quite different from those expected for the quantized thermal edge current of an intrinsic ATHE, but consistent with extrinsic impurity-induced ATHEs in chiral superconductivity. Our study of ATHE offers an alternative approach to probe TRS breaking in the superconducting states.

cond-mat.supr-con↗

arXiv2025

Huge anisotropic magneto-thermal switching in high-purity polycrystalline compensated metals

Magneto-thermal transport is a promising physical property for thermal management applications. Magneto-thermal switching enables active control of heat flows, and a high switching ratio is desirable for improving performance. Here, we report on the observation of a huge magneto-thermal switching (MTS) effect in high-purity (5N) Pb polycrystalline wires, where magnetic fields perpendicular to the heat current direction are applied at low temperatures. At T = 3 K and B = 0.1 T, the measured thermal conductivity (\k{appa}) of the Pb wire is about 2500 W m-1 K-1 but is reduced to ~150 and ~5 W m-1 K-1 at B = 1 and 9 T, respectively. This strong suppression is attributed to magnetoresistance in compensated metals. Although the huge magnetoresistance has been studied in single crystals with field along the selected orbitals, our results demonstrate that a huge MTS can similarly be realized even in flexible polycrystalline wires. This finding highlights the practical potential of magneto-thermal control in low-temperature thermal management, including applications in space environments where temperatures are around 3 K.

cond-mat.mtrl-sci↗

arXiv2025

Rotational Grüneisen ratio: a probe for quantum criticality in anisotropic systems

The Grüneisen ratio $Γ$ and its magnetic analog, the magnetic Grüneisen ratio $Γ_H$, are powerful probes to study the nature of quantum phase transitions. Here, we propose a Grüneisen parameter, the rotational Grüneisen ratio $Γ_ϕ$, by introducing the orientation of the external field as a control parameter. We investigate $Γ_ϕ$ of the highly anisotropic paramagnets CeRhSn and CeIrSn by measuring the rotational magnetocaloric effect in a wide range of temperatures and magnetic fields. We find that the $Γ_ϕ$ data of both compounds are scaled by using the same critical exponents and the field-invariant critical field angle. Remarkably, the scaling function for the $Γ_ϕ$ data reveals the presence of highly anisotropic quantum criticality that develops as a function of the easy-axis component of the magnetic field from the quantum critical line. This paper provides a thermodynamic approach to detect and identify magnetic quantum criticality in highly anisotropic systems.

cond-mat.str-el↗

arXiv2024

Magnetic structure of polar magnet GaV$_4$Se$_8$ with Néel-type skyrmion lattice probed by $^{51}$V NMR

We report the magnetization and the $^{51}$V NMR measurements in the polar magnet GaV$_4$Se$_8$ in which a magnetic skyrmion lattice appears in the structural domain with the polar axis parallel to the magnetic field. Although we successfully separate the $^{51}$V NMR signals in the domain from those in the other structural domains, only the high-frequency region of NMR spectrum is observed due to a significant increase of the spin-echo decay rate in the low-frequency region. In $B_{\rm{ext}}\parallel[111]$, we find the NMR signals from the supermagnetized cycloidal state in the parallel domains as well as from the conical state in domains where the polar axis is tilted from the magnetic field. No NMR signal from the skyrmion lattice state is observed, suggesting a significant increase of the decay rate by additional low-energy excitations caused by dynamics of the skyrmions. In $B_{\rm{ext}}\parallel[001]$, where all the structural domains are magnetically equivalent, multiple NMR peaks converge into one peak at the saturation magnetic field. This field dependence is explained by the closing of magnetic cones as approaching the forced-ferromagnetic state.

cond-mat.str-el↗

arXiv2024

Incommensurate magnetic order in an axion insulator candidate EuIn$_2$As$_2$ investigated by NMR measurement

Magnetic topological insulators exhibit unique electronic states due to the interplay between the electronic topology and the spin structure. The antiferromagnetic metal $\rm{EuIn_2As_2}$ is a prominent candidate material in which exotic topological phases, including an axion insulating state, are theoretically predicted depending on the magnetic structure of the $\rm{Eu}^{2+}$ moments. Here, we report experimental results of the nuclear magnetic resonance (NMR) measurements of all the nuclei in $\rm{EuIn_2As_2}$ to investigate the coupling between the magnetic moments in the Eu ions and the conduction electrons in $\rm{In_2As_2}$ layers and the magnetic structure. The $^{75}\rm{As}$ and $^{115}\rm{In}$ NMR spectra observed at zero external magnetic field reveal the appearance of internal fields of $4.9$ and $3.6\ \rm{T}$ respectively at the lowest temperature, suggesting a strong coupling between the conduction electrons in the $\rm{In_2As_2}$ layer and the ordered magnetic moments in the Eu ions. The $^{75}\rm{As}$ NMR spectra under in-plane external magnetic fields show broad distributions of the internal fields produced by an incommensurate fan-like spin structure which turns into a forced ferromagnetic state above $0.7\ \rm{T}$. We propose a spin reorientation process that an incommensurate helical state at zero external magnetic field quickly changes into a fan state by applying a slight magnetic field.

cond-mat.str-el↗

arXiv2024

Doping-tunable Fermi surface with persistent topological Hall effect in axion candidate EuIn$_2$As$_2$

Rare-earth Zintl compound EuIn$_2$As$_2$ has been theoretically recognized as a candidate for realizing an intrinsic antiferromagnetic (AFM) bulk axion insulator and a higher-order topological state, which provides a fertile platform to explore novel topological transport phenomena. However, the axion state has yet to be realized because EuIn$_2$As$_2$ is highly hole-doped. Here, we synthesized a series of high-quality Ca-doped EuIn2As2 (Ca$_x$Eu$_{1-x}$In$_2$As$_2$, x = 0 ~ 0.25) single crystals to tune the Fermi energy above the hole pocket. Our Hall measurements reveal that the isovalent Ca substitution decreases the hole carrier density by shrinking the lattice spacing, which is also confirmed by our first-principles calculations. We further find that both the temperature dependence of the magnetic susceptibility with a local maximum at the Néel temperature and the topological Hall effect originating from the finite real-space spin chirality persist in the Ca-doped samples as observed in the pristine EuIn$_2$As$_2$, despite that the nonmagnetic Ca substitution decreases the effective moment and the Néel temperature. These results show that the Ca substitution tunes the Fermi energy while keeping the AFM magnetic structure, suggesting that the axion insulating state may be realized by further Ca substitution.

cond-mat.mtrl-sci↗

arXiv2024

$J_{\rm{eff}}$ = 1/2 Hyperoctagon Lattice in Cobalt Oxalate Metal-Organic-Framework

We report the magnetic properties of a cobalt oxalate metal-organic-framework featuring the hyperoctagon lattice. Our thermodynamic measurements reveal the $J_{\rm{eff}}$ = 1/2 state of the high-spin Co$^{2+}$ (3$\textit{d}^{7}$) ion and the two successive magnetic transitions at zero field with two-stage entropy release. $^{13}$C-NMR measurements reveal the absence of an internal magnetic field in the intermediate temperature phase. Multiple field-induced phases are observed before full saturation at around 40 T. We argue the unique cobalt oxalate network gives rise to the Kitaev interaction and/or a bond frustration effect, providing an unconventional platform for frustrated magnetism on the hyperoctagon lattice.

cond-mat.str-el↗

arXiv2023

Modulation vector of the Fulde-Ferrell-Larkin-Ovchinnikov state in CeCoIn5 revealed by high-resolution magnetostriction measurements

The Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state is an exotic superconducting phase formed by Cooper pairs with finite center-of-mass momentum $q$. On theoretical grounds, the superconducting order parameter in the FFLO state is spatially modulated along the $q$ vector, and the emergence of an associated anisotropy is expected at the phase transition from the Abrikosov state to the FFLO state. Here, we report the results of high-resolution magnetostriction measurements for a single crystal of CeCoIn$_5$ around $B \parallel c$. We find two anomalies in the magnetostriction along the $c$ axis, parallel to the magnetic-field orientation. In sharp contrast, this $B_{\rm K}$ anomaly disappears in the magnetostriction along the $a$-axis direction, perpendicular to the magnetic-field orientation. To explain this uniaxial expansion, we suggest a possibility that the FFLO transition occurs slightly below the upper critical field, and the FFLO modulation vector parallel to the applied magnetic field gives rise to the anisotropic response.

cond-mat.supr-con↗

arXiv2023

Emergent SU(3) magnons and thermal Hall effect in the antiferromagnetic skyrmion lattice

Complexity of quantum phases of matter is often understood by the underlying gauge structures, as was recognized by the $\mathbb{Z}_2$ and U(1) gauge theory description of spin liquid in frustrated magnets. Anomalous Hall effect of conducting electrons can intrisically arise from U(1) gauges expressing the spatial modulation of ferromagnetic moments or from SU(2) gauges representing the spin-orbit coupling effect. Similarly, in insulating ferro and antiferromagnets, the magnon excitations can contribute to anomalous transports by feeling the U(1) and SU(2) gauges arising from the features of ordered moments or interactions. In this work, we report the emergent higher rank SU(3) gauge structure in the magnon transport based on the thermal conductivity measurements of MnSc$_2$S$_4$ in an applied field up to 14\,T. The thermal Hall coefficient takes a substantial value when the material enters a three-sublattice antiferromagnetic skyrmion phase, which is confirmed by the large-scale spin wave theory. The excited magnons are dressed with SU(3) gauge field, which is a mixture of three species of U(1) gauge fields originating from the slowly varying magnetic moments on these sublattices.

cond-mat.str-el↗

arXiv2022

Planar Thermal Hall Effects in Kitaev Spin Liquid Candidate Na2Co2TeO6

We investigate both the longitudinal thermal conductivity ($κ_{xx}$) and the planar thermal Hall conductivity ($κ_{xy}$) in the Kitaev spin liquid candidate of Co-based honeycomb antiferromagnet Na$_2$Co$_2$TeO$_6$ in a magnetic field ($B$) applied along the $a$ and $a^*$ axes. A finite $κ_{xy}$ is resolved for both field directions in the antiferromagnetic (AFM) phase below the Néel temperature of 27 K. The temperature dependence of $κ_{xy}/T$ shows the emergence of topological bosonic excitations. In addition, the field dependence of $κ_{xy}$ shows sign reversals at the critical fields in the AFM phase, suggesting the changes in the Chern number distribution of the topological magnons. Remarkably, a finite $κ_{xy}$ is observed in $B \parallel a^*$ between the first-order transition field in the AFM phase and the saturation field, which is prohibited in a disordered state by the two-fold rotation symmetry around the $a^*$ axis of the honeycomb lattice, showing the presence of a magnetically ordered state that breaks the two-fold rotation symmetry. Our results demonstrate the presence of topological magnons in this compound in the whole field range below the saturation field.

cond-mat.str-el↗

arXiv2022

Topological Thermal Hall Effect of Magnons in Magnetic Skyrmion Lattice

Topological transports of fermions are governed by the Chern numbers of the energy bands lying below the Fermi energy. For bosons, e.g. phonons and magnons in a crystal, topological transport is dominated by the Chern number of the lowest energy band when the band gap is comparable to the thermal energy. Here, we demonstrate the presence of topological transport by bosonic magnons in a lattice of magnetic skyrmions - topological defects formed by a vortex-like texture of spins. We find a distinct thermal Hall signal in the magnetic skyrmion phase of an insulating polar magnet GaV4Se8, identified as the topological thermal Hall effect of magnons governed by the Chern number of the lowest energy band of the magnons in a triangular lattice of magnetic skyrmions. Our findings lay a foundation for studying topological phenomena of other bosonic excitations through thermal Hall probe.

cond-mat.str-el↗

arXiv2022

Charge and spin interplay in a molecular-dimer-based organic Mott insulator

Triangular lattice quasi-two-dimensional Mott insulators based on BEDT-TTF molecule and its analogies present a possibility to produce exotic phases by coupling charge and spin degrees of freedom. In this work we discuss magnetic properties of one of such materials, $κ$-(BEDT-TTF)$_2$Hg(SCN)$_2$Cl, which is found at the border of the phase transition between a Mott insulator into a charge ordered state. Our magnetic susceptibility and cantilever magnetisation measurements demonstrate how the charge degree of freedom defines magnetic properties for few different charge phases observed in this material as a function of temperature. Between $T_{CO}=30~K$ and $T_S=24~K$ we observe charge and spin separation due to one-dimensional charge stripes formed in this material below $T_{CO}=30~K$. Below $T_S=24~K$ charge and spin degrees of freedom demonstrate coupling. Spin singlet correlations develop below 24~K, however melting of charge order below 15~K prevents the spin singlet state formation, leaving the system in the inhomogeneous state with charge ordered spin singlet domains and charge and spin fluctuating ones.

cond-mat.str-el↗

arXiv2022

Resistivity and Thermal Conductivity of an Organic Insulator beta'-EtMe3Sb[Pd(dmit)2]2

A finite residual linear term in the thermal conductivity at zero temperature in insulating magnets indicates the presence of gapless excitations of itinerant quasiparticles, which has been observed in some candidate materials of quantum spin liquids (QSLs). In the organic triangular insulator beta'-EtMe3Sb[Pd(dmit)2]2, a QSL candidate material, the low-temperature thermal conductivity depends on the cooling process and the finite residual term is observed only in samples with large thermal conductivity. Moreover, the cooling rate dependence is largely sample dependent. Here we find that, while the low-temperature thermal conductivity significantly depends on the cooling rate, the high-temperature resistivity is almost perfectly independent of the cooling rate. These results indicate that in the samples with the finite residual term, the mean free path of the quasiparticles that carry the heat at low temperatures is governed by disorders, whose characteristic length scale of the distribution is much longer than the electron mean free path that determines the high-temperature resistivity. This explains why recent X-ray diffraction and nuclear magnetic resonance measurements show no cooling rate dependence. Naturally, these measurements are unsuitable for detecting disorders of the length scale relevant for the thermal conductivity, just as they cannot determine the residual resistivity of metals. Present results indicate that very careful experiments are needed when discussing itinerant spin excitations in beta'-EtMe3Sb[Pd(dmit)2]2.

cond-mat.str-el↗

arXiv2021

Ferromagnetism out of charge fluctuation of strongly correlated electrons in $κ$-(BEDT-TTF)$_2$Hg(SCN)$_2$Br

We perform magnetic susceptibility and magnetic torque measurements on the organic $κ$-(BEDT-TTF)$_2$Hg(SCN)$_2$Br, which is recently suggested to host an exotic quantum dipole-liquid in its low-temperature insulating phase. Below the metal-insulator transition temperature, the magnetic susceptibility follows a Curie-Weiss law with a positive Curie-Weiss temperature, and a particular $M\propto \sqrt{H}$ curve is observed. The emergent ferromagnetically interacting spins amount to about 1/6 of the full spin moment of localized charges. Taking account of the possible inhomogeneous quasi-charge-order that forms a dipole-liquid, we construct a model of antiferromagnetically interacting spin chains in two adjacent charge-ordered domains, which are coupled via fluctuating charges on a Mott-dimer at the boundary. We find that the charge fluctuations can draw a weak ferromagnetic moment out of the spin singlet domains.

cond-mat.str-el↗

arXiv2020

Thermal Hall Effects of Spins and Phonons in Kagome Antiferromagnet Cd-Kapellasite

We have investigated the thermal-transport properties of the kagome antiferromagnet Cd-kapellasite (Cd-K). We find that a field suppression effect on the longitudinal thermal conductivity k_xx sets in below ~25 K, suggesting a large spin contribution k_xx^sp in k_xx. We also find clear thermal Hall signals in the spin liquid phase in all Cd-K samples. The magnitude of the thermal Hall conductivity k_xy shows a significant dependence on the sample's scattering time. On the other hand, the temperature dependence of k_xy is similar in all Cd-K samples; k_xy shows a peak at almost the same temperature of the peak of the phonon thermal conductivity k_xy^ph which is estimated by k_xx at 15 T. These results indicate the presence of a dominant phonon thermal Hall k_xy^ph at 15 T. In addition to k_xy^ph, we find that the field dependence of k_xy at low fields turns out to be non-linear at low temperatures, concomitantly with the appearance of the field suppression of k_xx, indicating the presence of a spin thermal Hall k_xy^sp at low fields. Remarkably, by assembling the k_xx dependene of k_xy^sp data of other kagome antiferromagnets, we find that, whereas k_xy^sp stays a constant in the low-k_xx region, k_xy^sp starts to increase as k_xx does in the high-k_xx region. This k_xx dependence of k_xy^sp indicates the presence of both intrinsic and extrinsic mechanisms in the spin thermal Hall effect in kagome antiferromagnets. Furthermore, both k_xy^ph and k_xy^sp disappear in the antiferromagnetic ordered phase at low fields, showing that phonons alone do not exhibit the thermal Hall effect. A high field above ~7 T induces k_xy^ph, concomitantly with a field-induced increase of k_xx and the specific heat, suggesting a coupling of the phonons to the field-induced spin excitations as the origin of k_xy^ph.

cond-mat.str-el↗