arXiv subjects

Misaki Sasaki

Publications and source records attributed to Misaki Sasaki.

4 recordsLinked to original sources

arXiv2026

Single-crystal structural phase diagram of stoichiometric bilayer nickelate La3Ni2O7 under hydrostatic pressure

The bilayer nickelate La3Ni2O7 has attracted intense interest following the discovery of high-temperature superconductivity under pressure, representing the first nickelate superconductor realized in bulk form. However, the crystal structure of the superconducting phase remains under active discussion, complicating efforts to establish its microscopic origin. Here we resolve these structural controversies by establishing a definitive pressure-temperature phase diagram, including the superconducting region of stoichiometric La3Ni2O7 single crystals under hydrostatic conditions using helium as the pressure-transmitting medium. At ambient pressure, La3Ni2O7 adopts a polar orthorhombic Am2m structure characterized by charge order between inequivalent Ni sites and NiO6 octahedral tilting. Upon compression, the system undergoes a direct transition from the charge-ordered Am2m phase to the tetragonal I4/mmm phase near 10 GPa, coinciding with the onset of bulk superconductivity. These results establish the intrinsic structural evolution of La3Ni2O7 and provide a structural framework for microscopic theories of nickelate superconductivity.

cond-mat.supr-con↗

arXiv2026

High-pressure magnetic transition in iron observed via diamond quantum sensing

Diamond quantum sensors offer high precision and spatial resolution as magnetic probes, making them promising for a wide range of applications. While diamond anvil cells (DACs) can generate extremely high pressures, techniques for magnetometry under such conditions remain limited. By fabricating an ensemble of NV centers directly on the anvil diamond surface, we enable precise magnetic measurements under high pressure. In this work, we employ this NV ensemble to image the stray magnetic field of iron up to 30 GPa, enabling the observation of the magnetic transition ($α$-$\varepsilon$ transition) in iron.

physics.app-ph↗

arXiv2025

GPa Pressure Imaging Using Nanodiamond Quantum Sensors

We demonstrate wide-field optical microscopy of the pressure distribution at approximately 20 GPa in a diamond anvil cell (DAC), using nitrogen-vacancy (NV) centers in nanodiamonds (NDs) as quantum sensors. Pressure and non-hydrostaticity maps are obtained by fitting optically detected magnetic resonance (ODMR) spectra with models incorporating hydrostatic and uniaxial stress conditions. Two methods for introducing NDs with a pressure-transmitting medium are compared, revealing that the embedding approach affects the degree of non-hydrostaticity. This ND-based technique offers a powerful imaging platform for probing pressure-induced phenomena and is extendable to other physical quantities such as magnetic fields.

cond-mat.mtrl-sci↗

arXiv2025

Enhancement of superconductivity on thin film of Sn under high pressure

We investigated the pressure effects of a superconductivity on thin films of Sn. Elemental superconductor Sn with a body-centered tetragonal structure, $β$-Sn, exhibits superconductivity below the superconducting transition temperature ($T_{\rm c}=3.72$ K) at ambient pressure. $T_{\rm c}$ of Sn increases with lowering dimension such as in thin film and nanowire growth, or by high-pressure application. For thin films, $T_{\rm c}$ exhibits a slight increase up to approximately 4 K compared to the bulk value, attributable to the crystalline size and lattice disorder. By applying pressure on a bulk Sn, $T_{\rm c}$ initially decreases from 3.72 K as the pressure increases. Further increasing pressure up to 10 GPa, $T_{\rm c}$ increases to 5.3 K with the structural transformation. However, the combination of these effects on thin films of Sn, namely, thin-film growth and pressure effects, remains underexplored. In this study, we combined film-growth and pressure-application techniques to further increase $T_{\rm c}$ using a diamond anvil cell with boron-doped diamond electrodes. The drop of the electrical resistance suggesting the onset of $T_{\rm c}$ on the thin film reached above 6 K in $γ$-Sn phase. Further, the upper critical magnetic field was drastically enhanced. Atomic force microscopy suggests that the refinement of the grain size of the thin film under the non-hydrostatic pressure conditions contributes to stabilizing the higher $T_{\rm c}$ of $γ$-Sn.

cond-mat.supr-con↗