arXiv subjects

Misha Yu. Ivanov

Publications and source records attributed to Misha Yu. Ivanov.

11 recordsLinked to original sources

arXiv2025

Table-top all-attosecond transient absorption spectroscopy

Attosecond transient absorption spectroscopy (ATAS) has emerged as a powerful technique within the field of attosecond science, combining extremely high temporal and excellent spectral resolution. So far, ATAS has been implemented in pump-probe experiments where an attosecond extreme-ultraviolet (XUV) pump or probe pulse was combined with a near-infrared (NIR) pulse in the femtosecond range, with the attosecond time resolution deriving from sub-cycle NIR-driven dynamics. Investigations of ultrafast electron dynamics in atoms, molecules and solids, with potential impact across physics, chemistry, and biology, would benefit significantly from the ability to perform all-attosecond transient absorption spectroscopy (AATAS). Here we demonstrate time-resolved AATAS using a table-top high-harmonic generation (HHG) source. The method is applied to investigate previously unresolved electronic coherences in Xe, revealing oscillatory valence hole motion with a 3-femtosecond period. In addition, systematic investigations of electron dynamics in Kr, Ar, and Ne are presented. Our work shows that, thanks to its broad bandwidth, high stability and easy accessibility, HHG is an ideal source for AATAS, offering the potential for replication in numerous laboratories.

physics.atom-ph↗

arXiv2025

Quantum Optics and Quantum Electrodynamics of Strong Field Processes

In its beginnings, the physics of intense laser-matter interactions was the physics of multiphoton processes. The theory was reduced then to high-order perturbation theory, while treating matter and light in a quantum manner. With the advent of chirped pulse amplification developed by D. Strickland and G. Mourou, which enabled generation of ultra-intense, ultra-short, coherent laser pulses, the need for a quantum electrodynamics description of electromagnetic (EM) fields practically ceased to exist and lost relevance. Contemporary attoscience (AS), and more generally ultrafast laser physics, awarded the Nobel Prize in 2023 to P. Agostini, F. Krausz, and A. L'Huillier, commonly uses the classical description of EM fields while keeping a fully quantum description of matter. The progress and successes of AS in the last 40 years have been spectacular, with an enormous amount of fascinating investigations in basic research and technology. Yet a central question remains: can ultrafast laser physics continue to advance without reintroducing quantum electrodynamics and quantum optics into its description of light-matter interactions? This article discusses future perspectives at the intersection of strong-field physics and quantum optics.

quant-ph↗

arXiv2016

Strong-field ionization of clusters using two-cycle pulses at 1.8~$μ$m

The interaction of intense laser pulses with nano-scale particles leads to the production of high-energy electrons, ions, neutral atoms, neutrons and photons. Up to now, investigations have focused on near-infrared to X-ray laser pulses consisting of many optical cycles. Here we study strong-field ionization of rare-gas clusters ($10^3$ to $10^5$ atoms) using two-cycle 1.8~$μ$m laser pulses to access a new interaction regime in the limit where the electron dynamics are dominated by the laser field and the cluster atoms do not have time to move significantly. The emission of fast electrons with kinetic energies exceeding 3keV is observed using laser pulses with a wavelength of 1.8~$μ$m and an intensity of $1\times 10^{15}$~W/cm$^2$, whereas only electrons below 500eV are observed at 800nm using a similar intensity and pulse duration. Fast electrons are preferentially emitted along the laser polarization direction, showing that they are driven out from the cluster by the laser field. In addition to direct electron emission, an electron rescattering plateau is observed. Scaling to even longer wavelengths is expected to result in a highly directional current of energetic electrons on a few-femtosecond timescale.

physics.atm-clus↗

arXiv2015

A practical scheme for generating isolated elliptically polarized attosecond pulses using bi-chromatic counter rotating circularly polarized laser fields

Spectra of circularly polarized harmonics is calculated by numerically solving the Time-Dependent Schrödinger Equation for a 2D model of Ne atom using circularly polarized fundamental with counter-rotating second harmonic laser fields. We demonstrate strong asymmetry between left- and right- circularly polarized harmonics when a ground state with p-type symmetry is used. It arises due to the circular polarization of individual attosecond pulses in the generated pulse train. Reducing the length of the counter-rotating drivers and introducing a small time-shift between them allows to generate a single elliptically polarized attosecond pulse.

physics.atom-ph↗

arXiv2015

Real-time quantum trajectories for classically allowed dynamics in strong laser fields

Both the physical picture of the dynamics of atoms and molecules in intense infrared fields and its theoretical description use the concept of electron trajectories. Here we address a key question which arises in this context: Are distinctly quantum features of these trajectories, such as the complex-valued coordinates, physically relevant in the classically allowed region of phase space, and what is their origin? First, we argue that solutions of classical equations of motion can account for quantum effects. To this end, we construct an exact solution to the classical Hamilton-Jacobi equation which accounts for dynamics of the wave packet, and show that this solution is physically correct in the limit $\hbar \to 0$. Second, we show that imaginary components of classical trajectories are directly linked to the finite size of the initial wavepacket in momentum space. This way, if the electronic wavepacket produced by optical tunneling in strong infrared fiels is localised both in coordinate and momentum, its motion after tunneling {\em ipso facto\/} cannot be described with purely classical trajectories -- in contrast to popular models in the literature.

physics.atom-ph↗

arXiv2014

The Effect of Multiple Conduction Bands on High Harmonic Emission from Dielectrics

We find that, for sufficiently strong mid-IR fields, transitions between different conduction bands play an important role in the generation of high-order harmonics in a dielectric. The transitions make a significant contribution to the harmonic signal, and they can create a single effective band for the motion of an electron wave packet. We show how high harmonic spectra produced during the interaction of ultrashort laser pulses with periodic solids provide a spectroscopic tool for understanding the effective band structure that controls electron dynamics in these media.

cond-mat.other↗

arXiv2013

Three-body bound states in atomic mixtures with resonant p-wave interaction

We employ the Born-Oppenheimer approximation to find the effective potential in a three-body system consisting of a light particle and two heavy ones when the heavy-light short-range interaction potential has a resonance corresponding to a non-zero orbital angular momentum. In the case of an exact resonance in the p-wave scattering amplitude, the effective potential is attractive and long-range, namely it decreases as the third power of the inter-atomic distance. Moreover, we show that the range and power of the potential, as well as the number of bound states are determined by the mass ratio of the particles and the parameters of the heavy-light short-range potential.

physics.atom-ph↗

arXiv2013

Operational Dynamic Modeling Transcending Quantum and Classical Mechanics

We introduce a general and systematic theoretical framework for Operational Dynamic Modeling (ODM) by combining a kinematic description of a model with the evolution of the dynamical average values. The kinematics includes the algebra of the observables and their defined averages. The evolution of the average values is drawn in the form of Ehrenfest-like theorems. We show that ODM is capable of encompassing wide ranging dynamics from classical non-relativistic mechanics to quantum field theory. The generality of ODM should provide a basis for formulating novel theories.

quant-ph↗

arXiv2010

Enhancement and suppression of tunneling by controlling symmetries of a potential barrier

We present a class of 2D systems which shows a counterintuitive property that contradicts a semi classical intuition: A 2D quantum particle "prefers" tunneling through a barrier rather than traveling above it. Viewing the one particle 2D system as the system of two 1D particles, it is demonstrated that this effect occurs due to a specific symmetry of the barrier that forces excitations of the interparticle degree of freedom that, in turn, leads to the appearance of an effective potential barrier even though there is no "real" barrier. This phenomenon cannot exist in 1D.

quant-ph↗

arXiv2009

An electron in the presence of multiple zero range potentials and an external laser field -- exact solutions for photoionization and stimulated bremsstrahlung

The method of zero range potential (ZRP) for one-electron problems is reviewed. In the absence of an external electromagnetic field, the notion of a ZRP is introduced from different points of view and for an arbitrary dimension of space. Then, three-dimensional problems of motion of an electron in the field of several ZRPs and laser radiation are studied. Exact wave functions for the processes of photoionization and stimulated bremsstrahlung in the presence of the laser field of an arbitrary pulse shape are obtained in the form of one-dimensional integral representations.

physics.atom-ph↗

arXiv2009

Two-electron ionization in strong laser fields below intensity threshold: signatures of attosecond timing in correlated spectra

We develop an analytical model of correlated two-electron ionization in strong infrared laser fields. The model includes all relevant interactions between the electrons, the laser field, and the ionic core nonperturbatively. We focus on the deeply quantum regime, where the energy of the active electron driven by the laser field is insufficient to collisionally ionize the parent ion, and the assistance of the laser field is required to create a doubly charged ion. In this regime, the electron-electron and the electron-ion interactions leave distinct footprints in the correlated two-electron spectra, recording the mutual dynamics of the escaping electrons.

physics.atom-ph↗