arXiv subjects

Mohamed Sennary

Publications and source records attributed to Mohamed Sennary.

7 recordsLinked to original sources

arXiv2026

Attosecond quantum optics

Modern quantum optics primarily operates in the quasistationary regime, isolated from the intrinsic timescales of ultrafast optical fields. Pushing these boundaries into the femtosecond and attosecond domains is a critical frontier. Here, we generate, shape, and interrogate the quantum state of an ultrafast squeezed light field. Our optical metrology reveals a highly dynamic, time dependent squeezing distribution across individual half cycles of the electric field. Incorporating this intracycle squeezing into strong field simulations demonstrates that the temporal redistribution of quantum uncertainty fundamentally reshapes the quantum strong field physics of high harmonic emission. Furthermore, we achieve attosecond scale control of the squeezed state, visualized through inferred effective Wigner representations. Finally, we show that ultrafast squeezed light encodes its quantum properties into a photoinduced tunneling current within a petahertz phototransistor with subfemtosecond resolution, demonstrating a direct optical electronic quantum coupling. This work lays the foundation for the emerging field of ultrafast quantum optics and unlocks new avenues for high speed quantum communication and photonics.

physics.optics↗

arXiv2025

Imaging and controlling electron motion and chemical structural dynamics of biological system in real time and space

Ultrafast electron microscopy (UEM) has found widespread applications in physics, chemistry, and materials science, enabling real-space imaging of dynamics on ultrafast timescales. Recent advances have pushed the temporal resolution of UEM into the attosecond regime, enabling the attomicroscopy technique to directly visualize electron motion. In this work, we extend the capabilities of this powerful imaging tool to investigate ultrafast electron dynamics in a biological system by imaging and controlling light induced electronic and chemical changes in the conductive network of multicellular cable bacteria. Using electron energy loss spectroscopy (EELS), we first observed a laser induced increase in π-electron density, accompanied by spectral peak broadening and a blueshift features indicative of enhanced conductivity and structural modification. We also traced the effect of ultrafast laser pumping on bulk plasmon electron oscillations by monitoring changes in the plasmon like resonance peak. Additionally, we visualized laser induced chemical structural changes in cable bacteria in real space. The imaging results revealed carbon enrichment alongside a depletion of nitrogen and oxygen, highlighting the controllability of chemical dynamics. Moreover, time resolved EELS measurements further revealed a picosecond scale decay and recovery of both π-electron and plasmonic features, attributed to electron phonon coupling. In addition to shedding light on the mechanism of electron motion in cable bacteria, these findings demonstrate ultrafast modulation and switching of conductivity, underscoring their potential as bio-optoelectronic components operating on ultrafast timescales.

physics.chem-ph↗

arXiv2025

Ultrafast quantum light uncertainty dynamics in real time

Advancements in quantum optics and squeezed light generation have transformed various domains of quantum science and technology. However, real-time quantum dynamics remain an underexplored frontier. Here, we extend quantum optics into the ultrafast regime, providing direct experimental evidence that quantum uncertainty is not a static constraint but evolves dynamically with the system state and interactions. Using ultrafast squeezed light generated via a four-wave mixing nonlinear process, we observe the temporal dynamics of amplitude uncertainty, demonstrating that quantum uncertainty is a controllable and tunable physical quantity. This offers new insights into fundamental quantum mechanics in real-time. Additionally, we demonstrate control over the quantum state of light by switching between amplitude and phase squeezing. Our ability to generate and manipulate ultrafast squeezed light waveforms with attosecond resolution unlocks exciting possibilities for quantum technologies, including petahertz scale secure quantum communication, quantum computing, and ultrafast spectroscopy. We also introduce an ultrafast quantum encryption protocol leveraging squeezed light for secure digital communication at unprecedented speeds. This work paves the way for exploring quantum uncertainty dynamics and establishes the foundation for the emerging field of ultrafast quantum science.

physics.optics↗

arXiv2025

Comment on "Comment on Attosecond electron microscopy and diffraction"

Over the past few decades, following the first demonstration of ultrafast electron microscopy, numerous research groups have focused on achieving attosecond temporal resolution in electron microscopy with the goal of imaging electron and atomic motion. Recently, several studies have claimed to achieve attosecond temporal resolution in imaging(1-3). These claims are based on the generation of attosecond electron pulse trains. However, in typical time-resolved measurements used to capture dynamic processes in real-time, the temporal resolution is determined by the envelope of the pulse train. The reliance of using attosecond electron pulse trains fails to account for the distinct temporal resolution advantages enabled by our attosecond optical gating, which are absent in the case of using a continuous-wave or long laser pulse. These oversights highlight the limitations of this methodology (1-3) in studying ultrafast phenomena of matter. It is crucial to clarify this distinction to avoid confusion, misinterpretation, and potential miscitations within the community regarding attosecond temporal resolution in electron microscopy and the attosecond imaging of matter dynamics. In contrast, Hui et al. (4) present the first realistic demonstration of attosecond imaging resolution in electron microscopy, enabling the diffraction imaging of electron motion dynamics in graphene. In a commentary by Peter Baum and Claus Ropers, the authors conjecture that the graphene dynamics observed in our time-resolved diffraction experiment (Fig. 5, Hui et al. 2024) (4) is an optical interference artifact or light modulation of electrons effects, similar to what was reported previously (1-3), in addition to raising other technical concerns. In this reply, we are pleased to address these allegations and provide clarifications to resolve the raised technical questions.

physics.optics↗

arXiv2024

Attomicroscopy imaging and control of electron motion in graphene

Attosecond science has leveraged the highly nonlinear interactions between intense few-cycle laser pulses and matter, allowing for unprecedented observation and control of electron motion with remarkable temporal resolution. However, most existing experiments focusing on laser-controlled attosecond dynamics have dealt with quasi-bound electrons released in the ionization continua of atoms, molecules, or conduction bands in solid-state systems. Here, we employed the recently developed attomicroscopy imaging tool to investigate, visualize, and manipulate the motion of bound electrons in graphene. By adjusting the carrier-envelope phase and the field strength of the driving electric field, we were able to control both the amplitude and direction of the field-induced electron current between carbon atoms in graphene. This research opens new avenues for understanding and controlling dynamic, on-demand electron motion processes, including chemical reactions, molecular bonding, and the electronic properties of materials.

cond-mat.mes-hall↗

arXiv2024

Light-induced quantum tunnelling current in graphene

In the last decade, advancements in attosecond spectroscopy have allowed us to study electron motion dynamics in condensed matter. The access to these electron dynamics and, consequently, its control by an ultrafast light field paves the way for establishing ultrafast optoelectronics. Here, we report the generation of light-induced quantum tunnelling current in graphene phototransistors by ultrafast laser pulses in an ambient environment. This tunnelling effect provides access to the instantaneous field-driven current to demonstrate the current switching (ON and OFF) on a 630 attosecond (1.6 petahertz speed). Moreover, we controlled the tunnelling current and enhanced the graphene phototransistor conductivity by controlling the density of the photoexcited charge carriers at different pump laser powers. Furthermore, we exploited this capability to demonstrate various logic gates. The demonstrated light-induced tunnelling current and ultrafast switching were attained under standard room temperature and pressure conditions. Therefore, the presented scientific advancement in this work is at the technology readiness level suitable for its immediate integration into the development of ultrafast, nearly six orders of magnitude faster, optical transistors, lightwave electronics, and optical quantum computers.

cond-mat.mes-hall↗

arXiv2023

Attosecond Electron Microscopy

The electron motion in atoms and molecules is at the heart of all phenomena in nature that occur outside the nucleus. Recently, ultrafast electron and X-ray imaging tools have been developed to image the ultrafast dynamics of matter in real time and space. The cutting-edge temporal resolution of these imaging tools is on the order of a few tens to a hundred femtoseconds, limiting imaging to atomic dynamics. Hence electron motion imaging remains beyond the reach. Here, we achieved attosecond electron imaging temporal resolution in a transmission electron microscope, orders of magnitude faster than the highest reported imaging resolution, to demonstrate, which we coin it as (attomicroscopy) to image the field-induced electron dynamics in neutral multilayer graphene. Our results show that the electron motion between the carbon atoms in graphene is due to the field-driven electron dynamics in the conduction band and depends on the field waveform, strength, and polarization direction. This attomicroscopy imaging provides more insights into the electron motion of neutral matter in real time and space and would have long-anticipated real-life attosecond science applications in quantum physics, chemistry, and biology.

physics.optics↗