arXiv subjects

Mohit K. Sharma

Publications and source records attributed to Mohit K. Sharma.

26 records · Page 2Linked to original sources

arXiv2018

Evidence of large magnetic cooling power and double glass transition in Tb5Pd2

We report a detailed dc magnetization, ac susceptibility and magnetocaloric properties of a binary intermetallic compound Tb5Pd2. Our dc magnetization and heat capacity results reveal absence of long range ordering in this compound. Two distinct frequency dependent peaks (Tf1~60 K and Tf2~21 K) had been observed in the ac-susceptibility. Analysis of these frequency dependent peaks by Mydosh parameter, power and Vogel-Fulcher law reveals that around Tf1 the compound is at the boundary of spin glass (SG) like-cluster glass (CG) like state and it undergoes a cluster glass-like freezing below Tf2. Zero field cooled memory effect and non-linear dc susceptibility also confirmed the presence of two glassy transitions in this compound. The transformation from SG/CG boundary to CG phase was also confirmed by the magnetic relaxation measurement and Arrott plots study. Remarkably, a significant magnetic entropy change was also observed in the temperature range of 60-120 K. Additionally a large relative cooling power also observed in this compound. The observed value is comparable to those of promising refrigerant material in this temperature range and is quite notable as in this compound magnetic hysteresis was absent in this temperature range. It was noted that in this compound short-range interactions persist up to a higher temperature above Tf1 and this is responsible for the observation of significant MCE over a wide temperature range. Our studies suggest that this compound is an example of a glassy magnetic compound which shows large magnetocaloric effect.

cond-mat.mtrl-sci↗

arXiv2017

Magnetic and universal magnetocaloric behavior of rare-earth substituted DyFe0.5Cr0.5O3

We report the effect of partial substitution of Dy-site by rare-earths (R=Gd, Er and La)on the magnetic and magnetocaloric behavior of a mixed metal oxide DyFe0.5Cr0.5O3.Structural studies reveal that substitution of Dy by R has a minimal influence on the crystal structure. Magnetic and heat capacity studies show that the magnetic transition around 121 K observed for DyFe0.5Cr0.5O3 remains unchanged with rare-earth substitution, whereas the lower magnetic transition temperature is suppressed/enhanced by magnetic/non-magnetic substitution. In all these compounds, the second order nature of magnetic transition is confirmed by Arrott plots. As compared to DyFe0.5Cr0.5O3, the values of magnetic entropy change and relative cooling power are increased with magnetic rare-earth substitution while it decreases with non-magnetic rare-earth substitution. In all these compounds, magnetic entropy change follows the power law dependence of magnetic field and the value of the exponent n indicate the presence of ferromagnetic correlation in an antiferromagnetic state. A phenomenological universal master curve is also constructed for all the compounds by normalizing the entropy change with rescaled temperature using a single reference temperature. This master curve also reiterates the second order nature of the magnetic phase transition in such mixed metal oxides.

cond-mat.mtrl-sci↗

arXiv2017

Complex magnetic behaviour and evidence of superspin glass state in a binary intermetallic compound Er5Pd2

A binary intermetallic compound Er5Pd2 has been investigated using dc and ac magnetic susceptibilities, magnetic memory effect, isothermal magnetization, non-linear dc susceptibility, heat capacity and magnetocaloric effect studies. Interestingly, even though the compound does not show geometrical frustration it undergoes glassy magnetic phase transition below 17.2 K. Investigation of dc magnetisation and heat capacity data divulged absence of long-ranged magnetic ordering. Through magnetic memory effect, time dependent magnetization and ac susceptibility studies it was revealed that the compound undergoes glass-like freezing below 17.2 K. Analysis of frequency dependence of this transition temperature through scaling and Arrhenius law; along with Mydosh parameter indicate, that the dynamics in Er5Pd2 is due to the presence of strongly interacting superspins rather than individual spins. This phase transition was further investigated by non-linear dc susceptibility and was characterized by static critical exponents γ and δ. Our results indicate that this compound show signature of superspin glass at low temperature. Additionally, both conventional and inverse magnetocaloric effect was observed with large value of magnetic entropy change and relative cooling power. Our results suggest that Er5Pd2 can be classified as a superspin glass system with large magnetocaloric effect.

cond-mat.mtrl-sci↗

arXiv2017

On Distributed Power Control for Uncoordinated Dual Energy Harvesting Links: Performance Bounds and Near-Optimal Policies

In this paper, we consider a point-to-point link between an energy harvesting transmitter and receiver, where neither node has the information about the battery state or energy availability at the other node. We consider a model where data is successfully delivered only in slots where both nodes are active. Energy loss occurs whenever one node turns on while the other node is in sleep mode. In each slot, based on their own energy availability, the transmitter and receiver need to independently decide whether or not to turn on, with the aim of maximizing the long-term time-average throughput. We present an upper bound on the throughput achievable by analyzing a genie-aided system that has noncausal knowledge of the energy arrivals at both the nodes. Next, we propose an online policy requiring an occasional one-bit feedback whose throughput is within one bit of the upper bound, asymptotically in the battery size. In order to further reduce the feedback required, we propose a time-dilated version of the online policy. As the time dilation gets large, this policy does not require any feedback and achieves the upper bound asymptotically in the battery size. Inspired by this, we also propose a near-optimal fully uncoordinated policy. We use Monte Carlo simulations to validate our theoretical results and illustrate the performance of the proposed policies.

cs.IT↗

arXiv2016

Effect of rare-earth (Er and Gd) substitution on the magnetic and multiferroic properties of DyFe0.5Cr0.5O3

We report the results of our investigations on the influence of partial substitution of Er and Gd for Dy on the magnetic and magnetoelectric properties of DyFe0.5Cr0.5O3, which is known to be a multiferroic system. Magnetic susceptibility and heat capacity data, apart from confirming the occurrence of magnetic transitions at ~ 121 and 13 K in DyFe0.5Cr0.5O3, bring out that the lower transition temperature only is suppressed by rare-earth substitution. Multiferroic behavior is found to persist in Dy0.4Ln0.6Fe0.5Cr0.5O3 (Ln= Er and Gd). There is an evidence for magnetoelectric coupling in all these materials with qualitative differences in its behavior as the temperature is changed across these two transitions. Remnant electric polarization is observed for all the compounds. The most notable observation is that electric polarization is seen to get enhanced as a result of rare-earth substitution with respect to that in DyFe0.5Cr0.5O3. Interestingly, similar trend is seen in magnetocaloric effect, consistent with the existence of magnetoelectric coupling. The results thus provide evidence for the tuning of magnetoelectric coupling by rare-earth substitution in this family of oxides.

cond-mat.str-el↗

arXiv2015

On the basis-set extrapolation

A possible solution for the problem of memory-size and computer-time, is the extrapolation of basis-set$^1$. This extrapolation has two exponents $α$ and $β$, corresponding to the HF (reference energy) and the energy of correlations (EC), respectively. For a given system, the exponents are taken as constant$^2$, and potential energy surfaces (PES) are generated. We have found that the values of $α$ and $β$ are not constant, but vary from position to position in the system. How to deal with such situation and get very accurate PES, is discussed.

physics.chem-ph↗

arXiv2015

Detection of TiH$_2$ molecule in the interstellar medium is less probable

Identification of TiH$^1$ and TiO$^2$ has been historical, as the Titanium was first time discovered in the interstellar medium (ISM). After finding TiO$_2$$^3$, there is an obvious question about the search of titanium dihydride (TiH$_2$). The existence of TiH$_2$ in the ISM is quite probable, as the atomic abundance of hydrogen is about 1900 times larger than that of oxygen. We have discussed that the detection of TiH$_2$ in the ISM is less probable, though it has a large electric dipole moment.

astro-ph.GA↗

arXiv2015

Earth Similarity Index with two free parameters

We have derived Earth Similarity Index (ESI) with two free parameters m and T. These free parameters are optimized with the consideration that the planet Mars is almost similar to the Earth. For the optimized values of free parameters, the interior-ESI, surface-ESI and ESI for some planets are calculated. The results for m = 0.8 and T = 0.8 are compared with the values obtained by Schulze-Makuch {\it et al.} (2011). We have found that the exoplanet 55 Cnc f is within 10% away from the threshold value T. The exoplanets HD 69830 c, 55 Cnc c, 55 Cnc f, 61 Vir d and HIP 57050 b are found to have ESI within 10% from the threshold value.

astro-ph.EP↗