arXiv subjects

Morgan W. Mitchell

Publications and source records attributed to Morgan W. Mitchell.

At least 19 recordsLinked to original sources

arXiv2026

Sensitivity Scaling and Limits of Cavity Enhancement in Miniaturized Optically Pumped Magnetometers

The sensitivity of miniaturized optically pumped magnetometers (OPMs) is limited by weak atom-light coupling, which an optical cavity can enhance. In this work, we model the photon-shot-noise-limited sensitivity of cavity-enhanced OPMs in the regime of strongly collisionally broadened optical transitions, characteristic of buffer-gas-filled miniaturized vapor cells. The cavity enhancement is benchmarked against a single-pass free-induction-decay OPM employing Faraday-rotation readout, with the probe power and detuning jointly optimized using the Cram\'{e}r-Rao lower bound as a figure of merit. For a Fabry-P\'{e}rot cavity, we compare side-of-fringe, homodyne, Pound-Drever-Hall, and Faraday-rotation readout. All four yield an optimal sensitivity enhancement scaling as $\alpha\sqrt{2\mathcal{F}/\pi}$, where $\mathcal{F}$ is the cavity finesse and $0.5\leq \alpha \leq 1$ is a readout-dependent prefactor. The enhancement is maximized at critical coupling, and we quantify its degradation away from this point. We further show that, despite spin-dependent absorption associated with the ensemble's vector polarizability, near-critical coupling can be maintained throughout spin precession at arbitrary finesse by exceeding a derived probe-power threshold and increasing the atomic detuning with finesse. We also establish a limit to the maximum cavity enhancement set by vector light-shift noise.

physics.atom-ph↗

arXiv2026

A single atom emitting resonance fluorescence into a coherent beam, and its use for non-destructive atom thermometry

Using a far-off-resonance optical dipole trap, we place a single neutral $^{87}$Rb atom in a weak, atom-resonant coherent beam, while also strongly illuminating it from an orthogonal direction to produce resonance fluorescence. The atom-modified coherent beam is then collected and its photon statistics analyzed. We observe first-order interference that can increase or decrease the beam flux, depending on the relative phase of the coherent beam and resonance fluorescence. This confirms predictions of Goncalves et al. [Phys. Rev. A 104, 013724]. The interference visibility is also shown to be a sensitive, time-resolved, non-destructive thermometer: by fitting the resulting photon count distributions, we infer the center-of-mass localization of the atom within the trap. With $1200$ atoms and integration time of $80\mathrm{ms}$ per atom, we demonstrate temperature uncertainties of $4 %$ for $\sim 30 \mu\mathrm{K}$ temperatures at $\sim 200\mu\mathrm{s}$ time resolution.

physics.atom-ph↗

arXiv2026

Local, mm-scale $^1$H magnetic resonance imaging using atomic vapors

We demonstrate a practical and sensitive low-field approach to magnetic resonance imaging (MRI) of $\mu$L-scale samples using an optically pumped magnetometer (OPM). Using a simple setup where a commercial OPM is placed directly adjacent to a sample, without intermediary signal-pickup coils, we perform one- and two-dimensional imaging with a >1 cm field of view and sub-mm Fourier-limited resolution at 10 $\mu$T, near Earth's field. This enables (i) high-throughput, low-field MRI of fluidic and tissue samples, and (ii) a quantitative benchmark of the sensitive volume surrounding the OPM.

physics.chem-ph↗

arXiv2026

Fast, powerful, low-noise optical pumping of an atomic vapor with semiconductor optical amplifiers

We use a $^{87}\text{Rb}$ atomic vapor, suitable for an optically-pumped magnetometer (OPM) in Earth-field conditions, to study the noise properties of three strategies for generating pulsed optical pumping. We compare a frequency-modulated (FM) laser, amplitude modulation (AM) via an acousto-optic modulator (AOM), and amplitude modulation via a semiconductor optical amplifier (SOA). Pumping the ensemble to operate as a Bell-Bloom OPM, and with an equal degree of spin polarization, the three methods give nearly identical sensitivity, showing that the SOA, despite being an active device, can introduce negligible additional noise. Pumping the ensemble to operate as a free-induction-decay OPM, we observe longer unpumped coherence times with the SOA-AM method than with the FM method. Finally, using the higher power available from the SOA, we demonstrate an environment-limited sensitivity of $80\text{fT}/\sqrt{\text{Hz}}$ at $600\text{Hz}$ and 200fT$200\text{fT}/\sqrt{\text{Hz}}$ at $4\text{kHz}$, one to two orders of magnitude beyond what was achievable with the other pumping methods.

physics.atom-ph↗

arXiv2026

Quantum noise scaling in continuously operating multiparameter sensors

We experimentally investigate the quantum noise mechanisms that limit continuously operating multiparameter quantum sensors. Using a hybrid rf-dc optically pumped magnetometer, we map the photon shot noise, spin projection noise, and measurement back-action noise over an order of magnitude in probe power and a factor of three in pump power while remaining quantum-noise-limited. We observe linear, quadratic, and cubic scaling of the respective total noise powers with probe photon flux, together with a quadratic dependence of back-action on pump photon flux, in quantitative agreement with a stochastic Bloch-equation model. At higher probe powers, additional probe-induced relaxation modifies the spin-noise spectrum while preserving the integrated noise scaling. Our results reveal fundamental, resource-dependent trade-offs unique to continuously monitored multiparameter sensors and establish experimentally the quantum limits governing their optimal operation.

quant-ph↗

arXiv2026

Distinguishing synthetic unravelings on quantum computers

Distinct monitoring or intervention schemes can produce different conditioned stochastic quantum trajectories while sharing the same unconditional (ensemble-averaged) dynamics. This is the essence of unravelings of a given Gorini-Kossakowski-Sudarshan-Lindblad (GKSL) master equation: any trajectory-ensemble average of a function that is linear in the conditional state is completely determined by the unconditional density matrix, whereas applying a nonlinear function before averaging can yield unraveling-dependent results beyond the average evolution. A paradigmatic example is resonance fluorescence, where direct photodetection (jump/Poisson) and homodyne or heterodyne detection (diffusive/Wiener) define inequivalent unravelings of the same GKSL dynamics. In earlier work, we showed that nonlinear trajectory averages can distinguish such unravelings, but observing the effect in that optical setting requires demanding experimental precision. Here we translate the same idea to a digital setting by introducing synthetic unravelings implemented as quantum circuits acting on one and two qubits. We design two unravelings - a projective measurement unraveling and a random-unitary "kick" unraveling - that share the same ensemble-averaged evolution while yielding different nonlinear conditional-state statistics. We implement the protocols on superconducting-qubit hardware provided by IBM Quantum to access trajectory-level information. We show that the variance across trajectories and the ensemble-averaged von Neumann entropy distinguish the unravelings in both theory and experiment, while the unconditional state and the ensemble-averaged expectation values that are linear in the state remain identical. Our results provide an accessible demonstration that quantum trajectories encode information about measurement backaction beyond what is fixed by the unconditional dynamics.

quant-ph↗

arXiv2026

Quantum Position Verification with Remote Untrusted Devices

Position information underpins many modern technologies, from navigation and timing to authentication and critical infrastructure. However, classical methods of proving that information originates from a particular position are vulnerable to spoofing. This limitation can be overcome with quantum technologies but current protocols rely on trust in quantum hardware that can be undermined, or require quantum computers and bounds on adversarial computation. Nevertheless, there has been significant interest in experimental demonstrations, and aspects of these protocols have been implemented. Here we introduce and experimentally demonstrate the Bell-test quantum position verification protocol for device-independent quantum position verification that guarantees security with only observed correlations from a loophole-free Bell test across a quantum network. We experimentally implement a version of this device-independent protocol against adversaries who, before each trial, are weakly entangled. Our demonstration achieves a one-dimensional localization 2.47(2) times smaller than the best, necessarily non-remote, classical localization protocol. Compared to classical protocols with identical latencies, the localization volume is 4.53(5) times smaller, and represents a certifiable quantum advantage. The general Bell-test protocol is loss tolerant and secure against adversaries with significant quantum resources. This work allows digital security to be anchored to physically trusted locations, enabling new position-based authentication protocols for applications such as financial transactions, legal agreements, and securing critical infrastructure.

quant-ph↗

arXiv2026

Dynamics of hyperpolarized nuclear spins at Zeeman-insensitive points

Avoided crossing (LAC) transitions are central to spin-based precision measurements since they provide strong observability and field-perturbation insensitivity, but while observed commonly in isolated-atom or engineered solid-state platforms, such transitions are unexploited in molecules in liquids. Here we report a solution-state, nuclear-spin LAC transition in hyperpolarized [1-$^{13}$C]-fumarate. The singlet-triplet LAC, occurring near 400 nT produces pronounced magnetization oscillations at approximately 2 Hz with a coherence time of 25 s, three times longer than the longest single-spin $T_2^*$. In the regime of high spin concentration and high polarization the sample's internal dipolar field couples measurably to the transition, providing a direct probe of nonlinear spin dynamics. These results establish nuclear-spin LACs as a platform for quantum sensing in liquids.

physics.chem-ph↗

arXiv2025

Detection of photon-level signals embedded in sunlight with an atomic photodetector

The detection of few-photon signals in a broadband background is an extreme challenge for photon counting, requiring filtering that accepts a narrow range of optical frequencies while strongly rejecting all others. Recent work [Zarraoa et. al, Phys. Rev. Res. 6, 033338 (2024)] demonstrated that trapped single atoms can act as low dark-count narrow-band photodetectors. Here we show that this ``quantum jump photodetector'' (QJPD) approach can also detect photon-level signals embedded in strong sunlight. Using a single rubidium atom as a QJPD, we count arrivals of individual narrow-band laser photons embedded in sunlight powers of order $10^{10}$ photons/s. We derive a rate-equation model for the atom's internal-state dynamics in sunlight, and find quantitative agreement with experiment. Using this model, we calculate the channel capacity over a noisy communication channel when sending weak coherent states and detecting them in the presence of sunlight, achieving a representative rate of 0.5 bits per symbol when sending 150 probe photons per 10 ms time-bin, embedded in 1 nW of sunlight (of order $10^{10}$ photons/s in the visible and near-infrared bands). The demonstration may benefit background-limited applications such as daytime light detection and ranging (LIDAR), remote magnetometry, and free-space classical and quantum optical communications.

quant-ph↗

arXiv2025

Optimal and efficient inference tools for field tracking with precessing spins

Precise, real-time monitoring of magnetic field evolution is important in applications including magnetic navigation and searches for physics beyond the standard model. One main field-monitoring technique, the spin-precession magnetometer (SPM), observes electron, nucleus, colour centre, or muon spins as they precess in response to their local magnetic field. Here, we study Bayesian signal-recovery methods for SPMs in the free-induction decay (FID) mode. In particular, we study tracking of field changes well within the coherence time of the spin system, and thus well beyond the response bandwidth, as in [R. Jim\'enez-Mart\'inez et al., Phys. Rev. Lett. 120, 040503 (2018)]. We derive the Bayesian Cram\'er-Rao bound that dictates the ultimate precision in estimating the Larmor frequency, which we show to be attained by the computationally expensive prediction error method (PEM). Relative to this benchmark, we show that the extended Kalman filter (EKF) and cubature Kalman filter (CKF) offer near-optimal tracking that is also computationally efficient, with the use of the latter giving better results only for a large spin number. Focusing thus on the EKF, we show that it is sufficient to accurately track fluctuating and unknown transient signals. Our methods can be easily adapted to other types of sensors undergoing nonlinear dissipative dynamics and experiencing intrinsic Gaussian-like stochastic noises.

quant-ph↗

arXiv2025

Magnetotactic bacterial populations studied with a Pound-Drever-Hall atomic magnetometer

We demonstrate an optically pumped magnetometer that monitors spin polarization using Pound Drever Hall (PDH) technique. The instrument exhibits a noise floor of 22.2 pT/sqrt(Hz) limited by optical photon shot noise, short-term instability of 30.8 pT/sqrt(Hz)/sqrt({\tau}) for averaging times {\tau} < 0.2 s , instability below 70 pT for 0.2 s < {\tau} < 20 s and a minimum instability of 47 pT at {\tau} = 6 s. We apply the OPM to investigate the ability of magnetotactic bacteria (Magnetospirillum gryphiswaldense, MSR-1) to orient in externally applied magnetic fields. Observing an opaque, concentrated suspension, we detect deviations from exponential relaxation dynamics on second time-scales, which give information about the dispersion of bacterial magnetic moment and rotational damping coefficient. These parameters are observed to evolve as the population further concentrates due to evaporation and settling. To our knowledge, this is the first time such magnetic inhomogeneities and long-term relaxation deviations have been directly observed. This study showcases both the sensitivity and stability of our OPM and its potential for probing biophysical processes.

physics.atom-ph↗

arXiv2025

Sequential analysis in a continuous spin-noise quantum sensor

Many control and detection applications require real-time analysis of signals from sensors, in order to quickly and accurately act upon events revealed by the sensors. Such signal analysis benefits from statistical models of signal and sensor behavior. This creates a need for data analysis methods that are simultaneously model-based, computationally efficient and causal, in the sense that they employ only sensor data available prior to a specific point in time. In this work, we implement sequential data analysis techniques on a spin-noise-based quantum sensor, to perform two key tasks: hypothesis testing and quickest change-point detection. These online protocols allow us to detect weak magnetic fields by adaptively collecting measurement data until a predefined confidence threshold is reached. We demonstrate these methods in a realistic experimental setting and derive performance bounds for the achievable precision and response time. Our approach has potential utility when detecting small perturbations to the magnetic field, in both applied and fundamental contexts including biomagnetism, geophysical surveys, detection of concealed materials, searches for dark matter candidates and exotic spin interactions. Our results demonstrate that sequential techniques enable faster and more sensitive detection, making them a powerful tool for quantum sensing.

quant-ph↗

arXiv2025

Quantum noise in a squeezed-light-enhanced multiparameter quantum sensor

We study quantum enhancement of sensitivity using squeezed light in a multi-parameter quantum sensor, the hybrid dc-rf optically pumped magnetometer (hOPM) [Phys. Rev. Applied 21, 034054, (2024)]. Using a single spin ensemble, the hOPM acquires both the dc field strength (scalar magnetometry), and resonantly detects one quadrature of the ac magnetic field at a chosen frequency (rf magnetometry). In contrast to the Bell-Bloom scalar magnetometer [Phys. Rev. Lett. 127, 193601 (2021)], the back-action evasion in the hOPM is incomplete, leading to a nontrivial interplay of the three quantum noise sources in this system: photon shot noise, spin projection noise, and measurement back-action noise. We observe these interactions using squeezed light as a tool to control the distribution of optical quantum noise between $S_2$ and $S_3$ polarization Stokes components, and the resulting effect on readout quantum noise and measurement back-action. These results demonstrate quantum-enhanced sensitivity in a continuously operating multi-parameter sensor and reveal fundamental trade-offs between sensitivity, back-action, and bandwidth.

quant-ph↗

arXiv2025

Tracking time-varying signals with quantum-enhanced atomic magnetometers

Quantum entanglement, in the form of spin squeezing, is known to improve the sensitivity of atomic instruments to static or slowly-varying quantities. Sensing transient events presents a distinct challenge, requires different analysis methods, and has not been shown to benefit from entanglement in practically-important scenarios such as spin-precession magnetometry (SPM). Here we adapt estimation control techniques introduced in [PRX Quantum 6, 030331 (2025)] to the experimental setting of SPM and analogous techniques. We demonstrate that real-time tracking of fluctuating fields benefits from measurement-induced spin squeezing and that quantum limits dictated by decoherence are within reach of today's experiments. We illustrate this quantum advantage by single-shot tracking, within the coherence time of a spin-precession magnetometer, of a magnetocardiography signal overlain with broadband noise.

quant-ph↗

arXiv2024

Traceable random numbers from a nonlocal quantum advantage

The unpredictability of random numbers is fundamental to both digital security and applications that fairly distribute resources. However, existing random number generators have limitations-the generation processes cannot be fully traced, audited, and certified to be unpredictable. The algorithmic steps used in pseudorandom number generators are auditable, but they cannot guarantee that their outputs were a priori unpredictable given knowledge of the initial seed. Device-independent quantum random number generators can ensure that the source of randomness was unknown beforehand, but the steps used to extract the randomness are vulnerable to tampering. Here, for the first time, we demonstrate a fully traceable random number generation protocol based on device-independent techniques. Our protocol extracts randomness from unpredictable non-local quantum correlations, and uses distributed intertwined hash chains to cryptographically trace and verify the extraction process. This protocol is at the heart of a public traceable and certifiable quantum randomness beacon that we have launched. Over the first 40 days of operation, we completed the protocol 7434 out of 7454 attempts -- a success rate of 99.7%. Each time the protocol succeeded, the beacon emitted a pulse of 512 bits of traceable randomness. The bits are certified to be uniform with error times actual success probability bounded by $2^{-64}$. The generation of certifiable and traceable randomness represents one of the first public services that operates with an entanglement-derived advantage over comparable classical approaches.

quant-ph↗

arXiv2024

Quantum jump photodetector for narrowband photon counting with a single atom

Using a single neutral 87Rb atom held in an optical trap, and "quantum jump" detection of single-photon-initiated state changes, we demonstrate a single-photon quantum jump photodetector (QJPD) with intrinsically narrow bandwidth and strong rejection of out-of-band photons, of interest for detecting weak optical signals in the presence of a strong broadband background. By analyzing fluorescence photon count distributions for the bright and dark states with and without excitation, we measure quantum efficiency of 2.9(2)$\times 10^{-3}$, a record for single-pass quantum jump production, and signal-photon-unprovoked "dark jump" rate - analogous to the dark count rate of other detectors - 3(10)$\times 10^{-3}$ jumps per second during passive accumulation plus 4.0(4)$\times 10^{-3}$ jumps per readout, orders of magnitude below those of traditional single-photon detectors. Available methods can substantially improve QJPD quantum efficiency, dark jump rate, bandwidth and tunability.

quant-ph↗

arXiv2024

Telling different unravelings apart via nonlinear quantum-trajectory averages

The Gorini-Kossakowski-Sudarshan-Lindblad master equation (ME) governs the density matrix of open quantum systems (OQSs). When an OQS is subjected to weak continuous measurement, its state evolves as a stochastic quantum trajectory, whose statistical average solves the ME. The ensemble of such trajectories is termed an unraveling of the ME. We propose a method to operationally distinguish unravelings produced by the same ME in different measurement scenarios, using nonlinear averages of observables over trajectories. We apply the method to the paradigmatic quantum nonlinear system of resonance fluorescence in a two-level atom. We compare the Poisson-type unraveling, induced by direct detection of photons scattered from the two-level emitter, and the Wiener-type unraveling, induced by phase-sensitive detection of the emitted field. We show that a quantum-trajectory-averaged variance is able to distinguish these measurement scenarios. We evaluate the performance of the method, which can be readily extended to more complex OQSs, under a range of realistic experimental conditions.

quant-ph↗

arXiv2024

Precise, super-resolving intensity measurement by quantum jump spectroscopy of a single neutral atom

We present precise, sub-wavelength optical intensity measurement using a single trapped $^{87}$Rb atom as a sensor. The intensity is measured by the scalar ac Stark shift it produces on the $F=1 \rightarrow F'=2$ hyperfine transition of the D$_{2}$ line, chosen for its $F' = F+1$ structure and very small tensor polarizability. To boost signal and reduce measurement-induced perturbations, we use a quantum jump spectroscopy technique in which a single absorbed photon on a transition of interest induces the scattering of hundreds of photons on a bright closed transition. The method greatly reduces systematic effects associated with the atomic state, optical polarization, probe power, and atom heating, and gives the atomic temperature as a second spectroscopic observable. We demonstrate the method by measuring the intensity at the focus of an optical tweezer.

physics.atom-ph↗