SearcharxivSearch

arXiv subjects

Moritz Meinecke

Publications and source records attributed to Moritz Meinecke.

2 recordsLinked to original sources

Photonic Cluster State Generation from a Quantum Dot Emitting in the Telecom C-band

Photonic cluster states are a key resource for photonic quantum information processing. So far, deterministic generation of these states has been limited to the near-infrared wavelength range. To achieve quantum advantage in communication while maintaining compatibility with silicon photonics, operation in the telecom wavelength range is required. In this work, we demonstrate deterministic cluster state generation directly in the telecom C-band. This is achieved through repetitive excitation of a hole spin confined in an indium-arsenide quantum dot subjected to an external magnetic field. We characterize the quantum process that generates the cluster state by measuring its process map, obtaining a fidelity of $\mathrm{F} = 0.71 \pm 0.01$ to the ideal case. As part of this characterization, we observe spin--photon polarization entanglement with a negativity of $\mathrm{N} = 0.27 \pm 0.02$. The emitted photons exhibit indistinguishability of at least 83%, demonstrating the potential for future fusion gates necessary for photonic cluster state generation beyond linear connectivity.

quant-ph

Kinetic Modeling of Transient Electroluminescence reveals TTA as Efficiency-Limiting Process in Exciplex-Based TADF OLEDs

Organic light emitting diodes (OLEDs) based on thermally activated delayed fluorescence (TADF) show increased efficiencies due to efficient upconversion of non-emissive triplet states to emissive singlets states via reverse intersystem crossing (RISC). To assess the influence of the characteristic efficiency-enhancing RISC process as well as possible efficiency-limiting effects in operational OLEDs, we performed temperature-dependent measurements of transient electroluminescence (trEL). With kinetic modeling, we quantify and separate the impact of different temperature-dependent depopulation processes and contributions to EL in the established donor:acceptor model system m-MTDATA:3TPYMB. The underlying rate equations adapted for EL measurements on TADF systems include radiative and non-radiative first- and second-order effects. In this way, we are able to evaluate the non-radiative recombination and annihilation processes with respect to their efficiency-limiting effects on these OLEDs. On the one hand, we evaluate the depopulation of intermolecular exciplex triplet states via non-radiative direct triplet decay, RISC and triplet-triplet annihilation (TTA). On the other hand, we determine the contribution to EL from the formation of singlet exciplex states via polarons, RISC and TTA. Our results show that TTA accounts for a significant part to triplet depopulation and contributes to EL while limiting the overall device quantum efficiency.

physics.app-ph