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Motohiko Yoshimura

Publications and source records attributed to Motohiko Yoshimura.

24 records · Page 2Linked to original sources

Vibrational two-photon emission from coherently excited solid parahydrogen

We report observation of two-photon emission from coherently excited vibrational state of solid parahydrogen, known as one of quantum solids. The coherent state between the ground and the excited states is prepared by stimulated Raman scattering using two visible laser pulses. The two-photon emission is triggered by another mid-infrared laser pulse. The observed two-photon emission persists even when the trigger pulse is injected long after the excitation. The observed phenomenon is due to a long decoherence time of the vibrational states of solid parahydrogen, which is attributed to special nature as quantum solid. Dependence of the decoherence on target temperature and residual orthohydrogen concentration are studied along with its time evolution. It is found that the emission intensity increases even after the excitation pulses pass through the target completely. The coherence development is highly suppressed at high target temperature and high residual orthohydrogen concentration. Effects of target annealing and laser-induced damage on the target are also observed.

physics.chem-ph↗

Externally triggered coherent two-photon emission from hydrogen molecules

We report coherent enhancement of two-photon emission from the excited vibrational state of molecular hydrogen triggered by irradiating mid-infrared pulses externally. We previously observed the two-photon emission triggered by the internally generated fourth Stokes photons. By injecting independent mid-infrared pulses externally, it is possible to control experimental parameters and investigate the mechanism in more detail. In this article, we describe the two-photon emission using the external trigger pulses. Its spectrum and dependence on the energy and timing of the trigger pulse are presented along with numerical simulations based on the Maxwell-Bloch equations. The measured number of emitted photons is 6 10^11 photons/pulse and the resulting enhancement factor from the spontaneous emission is more than 10^18. This value is three orders of magnitude higher than that of the previous experiment. External control of emission process is expected to be essential for observation of weaker process of radiative emission of neutrino pair.

physics.atom-ph↗

Observation of coherent two-photon emission from the first vibrationally-excited state of hydrogen molecules

In this paper, we describe an experiment which was conducted to explore the macro-coherent amplification mechanism using a two-photon emission process from the first vibrationally-excited state of para-hydrogen molecule. Large coherence in the initial state was prepared by the adiabatic Raman population transfer method, and the lowest Stokes sideband was used as a trigger field. We observed the coherent two-photon emission consistent with the expectation of the paired super-radiance master equation.

physics.atom-ph↗

I$_{2}$ molecule for neutrino mass spectroscopy: ab initio calculation of spectral rate

It has recently been argued that atoms and molecules may become good targets of determining neutrino parameters still undetermined, if atomic/molecular process is enhanced by a new kind of coherence. We compute photon energy spectrum rate arising from coherent radiative neutrino pair emission processes of metastable excited states of I$_2$ and its iso-valent molecules, $|Av \rangle \rightarrow |Xv' \rangle + γ+ ν_iν_j$ and $|A'v \rangle \rightarrow |Xv' \rangle + γ+ ν_iν_j$ with $γ$ an IR photon and $ν_{i(j)}$ $i(j)-$th neutrino mass eigenstates, and show how fundamental neutrino parameters may be determined. Energies of electronically excited states of I$_2$, including the effect of spin-orbit couplings were calculated by the multiconfigurational second order perturbation (CASPT2) method. Summation over many vibrational levels of intermediate states is fully incorporated. Unlike atomic candidate of a much larger energy difference such as Xe, I$_2$ transitions from a vibrational level $A(v=0)$ to $X(v' = 24)$ give an opportunity of determination of the mass type (Majorana vs Dirac distinction) and determination of Majorana CPV (charge-conjugation parity violating) phases, although the rate is much smaller.

hep-ph↗

Neutrino Spectroscopy with Atoms and Molecules

We give a comprehensive account of our proposed experimental method of using atoms or molecules in order to measure parameters of neutrinos still undetermined; the absolute mass scale, the mass hierarchy pattern (normal or inverted), the neutrino mass type (Majorana or Dirac), and the CP violating phases including Majorana phases. There are advantages of atomic targets, due to the closeness of available atomic energies to anticipated neutrino masses, over nuclear target experiments. Disadvantage of using atomic targets, the smallness of rates, is overcome by the macro-coherent amplification mechanism. The atomic or molecular process we use is a cooperative deexcitation of a collective body of atoms in a metastable level |e> emitting a neutrino pair and a photon; |e> -> |g> + gamma + nu_i nu_j where nu_i's are neutrino mass eigenstates. The macro-coherence is developed by trigger laser irradiation. We discuss aspects of the macro-coherence development by setting up the master equation for the target quantum state and propagating electric field. With a choice of heavy target atom or molecule such as Xe or I_2 that has a large M1 x E1 matrix element between |e> and |g>, we show that one can determine three neutrino masses along with the mass hierarchy pattern by measuring the photon spectral shape. If one uses a target of available energy of a fraction of 1 eV, Majorana CP phases may be determined. Our master equation, when applied to E1 x E1 transition such as pH_2 vibrational transition Xv=1 -> 0, can describe explosive PSR events in which most of the energy stored in |e> is released within a few nanoseconds. The present paper is intended to be self-contained explaining some details related theoretical works in the past, and further reports new simulations and our ongoing experimental efforts of the project to realize the neutrino mass spectroscopy using atoms/molecules.

hep-ph↗

Curvaton Scenario in the Presence of Two Dilatons Coupled to the Scalar Curvature

The possibility of the realization of a curvaton scenario is studied in a theory in which two dilatons are introduced along with coupling to the scalar curvature. It is shown that when the two dilatons have an approximate O(2) symmetric coupling, a scalar field playing the role of the curvaton may exist in the framework of this theory without introducing any other scalar field for the curvaton. Thus the curvaton scenario can be realized, and in the simple version of the curvaton scenario, in which the curvaton potential is quadratic, the curvature perturbation with a sufficient amplitude and a nearly scale-invariant spectrum suggested by observations obtained from WMAP can be generated.

hep-ph↗