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Motoi Kimata

Publications and source records attributed to Motoi Kimata.

33 records · Page 2Linked to original sources

Anisotropy of the Upper Critical Field in the Heavy-Fermion Superconductor UTe2 under Pressure

We studied the anisotropy of the superconducting upper critical field $H_{\rm c2}$ in the heavy-fermion superconductor UTe$_2$ under hydrostatic pressure by magnetoresistivity measurements. In agreement with previous experiments we confirm that superconductivity disappears near a critical pressure $p_{\rm c} \approx 1.5$~GPa, and a magnetically ordered state appears. The unusual $H_{\rm c2}(T)$ at low temperatures for $H \parallel a$ suggests that the multiple superconducting phases which appear under pressure have quite different $H_{\rm c2}$. For a field applied along the hard magnetization $b$ axis $H_{\rm c2} (0)$ is glued to the metamagnetic transition $H_{\rm m}$ which is suppressed near $p_{\rm c}$. The suppression of $H_{\rm m}$ with pressure follows the decrease of temperature $T_χ^{\rm max}$, at the maximum in the susceptibility along $b$. The strong reinforcement of $H_{\rm c2}$ at ambient pressure for $H \parallel b$ above 16~T is rapidly suppressed under pressure due to the increase of $T_{\rm sc}$ and the decrease of $H_{\rm m}$. The change in the hierarchy of the anisotropy of $H_{\rm c2}(0)$ on approaching $p_{\rm c}$ points out that the $c$ axis becomes the hard magnetization axis.

cond-mat.str-el↗

Two-Fold-Symmetric Magnetoresistance in Single Crystals of Tetragonal BiCh2-Based Superconductor LaO0.5F0.5BiSSe

We have investigated the in-plane anisotropy of the c-axis magnetoresistance for single crystals of a BiCh2-based superconductor LaO0.5F0.5BiSSe under in-plane magnetic fields. We observed two-fold symmetry in the c-axis magnetoresistance in the ab-plane of LaO0.5F0.5BiSSe while the crystal possessed a tetragonal square plane with four-fold symmetry. The observed symmetry lowering in magnetoresistance from the structural symmetry may be related to the nematic states, which have been observed in the superconducting states of several unconventional superconductors.

cond-mat.supr-con↗

Thermal Hall effect in a phonon-glass Ba$_3$CuSb$_2$O$_9$

A distinct thermal Hall signal is observed in a quantum spin liquid candidate Ba$_3$CuSb$_2$O$_9$. The transverse thermal conduction shows a power-law temperature dependence below 40 K where a spin gap opens. We suggest that, through the very low longitudinal thermal conductivity and the thermal Hall signals, a phonon Hall effect is induced by strong phonon scatterings by orphan Cu$^{2+}$ spins formed in random domains of Cu$^{2+}$-Sb$^{5+}$ dumbbells.

cond-mat.str-el↗

Spin Relaxation Mechanism in a Highly Doped Organic Polymer Film

We report the systematic studies of spin current transport and relaxation mechanism in highly doped organic polymer film. In this study, we have determined spin diffusion length (SDL), spin lifetime, and spin diffusion constant by using different experimental techniques. The spin lifetime estimated from the electron paramagnetic resonance experiment is much shorter than the previous expectation beyond the experimental ambiguity. This suggests that significantly large spin diffusion constant, which is reasonably explained by the hopping transport mechanism in degenerate semiconductors, exists in highly doped organic semiconductors. The calculated SDL using the spin lifetime and spin diffusion constant estimated from our experiment is comparable to the experimentally obtained SDL of the order of one hundred nanometers. Moreover, the present study revealed that the spin angular momentum is almost preserved in the hopping events. In other words, the spin relaxation mainly occurs due to the spin-orbit coupling at the nanoscale crystalline grains.

cond-mat.mtrl-sci↗

Pressure-induced superconductivity in EuFe2As2 without a quantum critical point: magnetotransport and upper critical field measurements under high pressure

Resistivity and Hall effect measurements of EuFe$_2$As$_2$ up to 3.2\,GPa indicate no divergence of quasiparticle effective mass at the pressure $P_\mathrm{c}$ where the magnetic and structural transition disappears. This is corroborated by analysis of the temperature ($T$) dependence of the upper critical field. $T$-linear resistivity is observed at pressures slightly above $P_\mathrm{c}$. The scattering rates for both electrons and holes are shown to be approximately $T$-linear. When a field is applied, a $T^2$ dependence is recovered, indicating that the origin of the $T$-linear dependence is spin fluctuations.

cond-mat.supr-con↗

Fermi surface in KFe2As2 determined via de Haas-van Alphen oscillation measurements

We have completely determined the Fermi surface in KFe$_2$As$_2$ via de Haas-van Alphen (dHvA) measurements. Fundamental frequencies $ε$, $α$, $ζ$, and $β$ are observed in KFe$_2$As$_2$. The first one is attributed to a hole cylinder near the X point of the Brillouin zone, while the others to hole cylinders at the $Γ$ point. We also observe magnetic breakdown frequencies between $α$ and $ζ$ and suggest a plausible explanation for them. The experimental frequencies show deviations from frequencies predicted by band structure calculations. Large effective masses up to 19 $m_e$ for $B \parallel c$ have been found, $m_e$ being the free electron mass. The carrier number and Sommerfeld coefficient of the specific heat are estimated to be 1.01 -- 1.03 holes per formula unit and 82 -- 94 mJmol$^{-1}$K$^{-2}$, respectively, which are consistent with the chemical stoichiometry and a direct measure of 93 mJmol$^{-1}$K$^{-2}$ [H. Fukazawa \textit{et al}., J. Phys. Soc. Jpn. \textbf{80SA}, SA118 (2011)]. The Sommerfeld coefficient is about 9 times enhanced over a band value, suggesting the importance of low-energy spin and/or orbital fluctuations, and places KFe$_2$As$_2$ among strongly correlated metals. We have also performed dHvA measurements on Ba$_{0.07}$K$_{0.93}$Fe$_2$As$_2$ and have observed the $α$ and $β$ frequencies.

cond-mat.supr-con↗

Cyclotron resonance and mass enhancement by electron correlation in KFe$_2$As$_2$

Cyclotron resonance (CR) measurements for the Fe-based superconductor KFe$_2$As$_2$ are performed. One signal for CR is observed, and is attributed to the two-dimensional $α$ Fermi surface at the $Γ$ point. We found a large discrepancy in the effective masses of CR [(3.4$\pm$0.05)$m_e$ ($m_e$ is the free electron mass)] and de-Haas van Alphen (dHvA) results, a direct evidence of mass enhancement due to electronic correlation. A comparison of the CR and dHvA results shows that both intra- and interband electronic correlations contribute to the mass enhancement in KFe$_2$As$_2$.

cond-mat.mtrl-sci↗

Phase Diagram of Pressure-Induced Superconductivity in EuFe2As2 Probed by High-Pressure Resistivity up to 3.2 GPa

We have constructed a pressure$-$temperature ($P-T$) phase diagram of $P$-induced superconductivity in EuFe$_2$As$_2$ single crystals, via resistivity ($ρ$) measurements up to 3.2 GPa. As hydrostatic pressure is applied, an antiferromagnetic (AF) transition attributed to the FeAs layers at $T_\mathrm{0}$ shifts to lower temperatures, and the corresponding resistive anomaly becomes undetectable for $P$ $\ge$ 2.5 GPa. This suggests that the critical pressure $P_\mathrm{c}$ where $T_\mathrm{0}$ becomes zero is about 2.5 GPa. We have found that the AF order of the Eu$^{2+}$ moments survives up to 3.2 GPa without significant changes in the AF ordering temperature $T_\mathrm{N}$. The superconducting (SC) ground state with a sharp transition to zero resistivity at $T_\mathrm{c}$ $\sim$ 30 K, indicative of bulk superconductivity, emerges in a pressure range from $P_\mathrm{c}$ $\sim$ 2.5 GPa to $\sim$ 3.0 GPa. At pressures close to but outside the SC phase, the $ρ(T)$ curve shows a partial SC transition (i.e., zero resistivity is not attained) followed by a reentrant-like hump at approximately $T_\mathrm{N}$ with decreasing temperature. When nonhydrostatic pressure with a uniaxial-like strain component is applied using a solid pressure medium, the partial superconductivity is continuously observed in a wide pressure range from 1.1 GPa to 3.2 GPa.

cond-mat.supr-con↗

Upper Critical Field of Pressure-Induced Superconductor EuFe$_2$As$_2$

We have carried out high-field resistivity measurements up to 27\,T in EuFe$_2$As$_2$ at $P$\,=\,2.5\,GPa, a virtually optimal pressure for the $P$-induced superconductivity, where $T_\mathrm{c}$\,=\,30\,K. The $B_\mathrm{c2}-T_\mathrm{c}$ phase diagram has been constructed in a wide temperature range with a minimum temperature of 1.6 K ($\approx 0.05 \times T_\mathrm{c}$), for both $B \parallel ab$ ($B_\mathrm{c2}^\mathrm{ab}$) and $B \parallel c$ ($B_\mathrm{c2}^\mathrm{c}$). The upper critical fields $B_\mathrm{c2}^\mathrm{ab}$(0) and $B_\mathrm{c2}^\mathrm{c}$(0), determined by the onset of resistive transitions, are 25 T and 22 T, respectively, which are significantly smaller than those of other Fe-based superconductors with similar values of $T_\mathrm{c}$. The small $B_\mathrm{c2}(0)$ values and the $B_\mathrm{c2}(T)$ curves with positive curvature around 20 K can be explained by a multiple pair-breaking model that includes the exchange field due to the magnetic Eu$^{2+}$ moments. The anisotropy parameter, $Γ=B_\mathrm{c2}^{ab}/B_\mathrm{c2}^{c}$, in EuFe$_2$As$_2$ at low temperatures is comparable to that of other "122" Fe-based systems.

cond-mat.supr-con↗

Comment on "Quantum Criticality and Nodal Superconductivity in the FeAs-Based Superconductor KFe$_2$As$_2$"

In a recent Letter [J. K. Dong et al., Phys. Rev. Lett. 104, 087005 (2010)], Dong \textit{et al}. have observed a $T^{1.5}$ dependence of resistivity $ρ$ in KFe$_2$As$_2$ at the upper critical field $B_{c2}$ = 5 T parallel to the c axis and have suggested the existence of a field-induced quantum critical point (QCP) at $B_{c2}$. In this comment, we argue that observation of a $T^{1.5}$ dependence of $ρ$ in a sample showing broad resistive transitions does not constitute evidence for a QCP and that recent dHvA results do not support the proposed QCP.

cond-mat.supr-con↗

Fermi surface and mass enhancement in KFe$_2$As$_2$ from de Haas-van Alphen effect measurements

We report on a band structure calculation and de Haas-van Alphen measurements of KFe$_2$As$_2$. Three cylindrical Fermi surfaces are found. Effective masses of electrons range from 6 to 18$m_e$, $m_e$ being the free electron mass. Remarkable discrepancies between the calculated and observed Fermi surface areas and the large mass enhancement ($\gtrsim 3$) highlight the importance of electronic correlations in determining the electronic structures of iron pnicitide superconductors.

cond-mat.supr-con↗

Pressure-Induced Antiferromagnetic Bulk Superconductor EuFe$_2$As$_2$

We present the magnetic and superconducting phase diagram of EuFe$_2$As$_2$ for $B \parallel c$ and $B \parallel ab$. The antiferromagnetic phase of the Eu$^{2+}$ moments is completely enclosed in the superconducting phase. The upper critical field vs. temperature curves exhibit strong concave curvatures, which can be explained by the Jaccarino-Peter compensation effect due to the antiferromagnetic exchange interaction between the Eu$^{2+}$ moments and conduction electrons.

cond-mat.supr-con↗

EuFe$_2$As$_2$ under high pressure: an antiferromagnetic bulk superconductor

We report the ac magnetic susceptibility $χ_{ac}$ and resistivity $ρ$ measurements of EuFe$_2$As$_2$ under high pressure $P$. By observing nearly 100% superconducting shielding and zero resistivity at $P$ = 28 kbar, we establish that $P$-induced superconductivity occurs at $T_c \sim$~30 K in EuFe$_2$As$_2$. $ρ$ shows an anomalous nearly linear temperature dependence from room temperature down to $T_c$ at the same $P$. $χ_{ac}$ indicates that an antiferromagnetic order of Eu$^{2+}$ moments with $T_N \sim$~20 K persists in the superconducting phase. The temperature dependence of the upper critical field is also determined.

cond-mat.supr-con↗

Resistivity and upper critical field in KFe$_2$As$_2$ single crystals

We report resistivity measurements performed on KFe$_2$As$_2$ single crystals down to $T$ = 0.3 K and in magnetic fields up to 17.5 T. The in-plane resistivity vs. $T$ curve has a convex shape down to $\sim$50 K and shows a $T^2$ dependence below $\sim$45 K. The ratio of the c-axis to in-plane resistivities is $\sim$10 at room temperature and $\sim$40 at 4.2 K. The superconducting upper critical field $B_{c2}(T)$ has been determined from the resistivity data: $B_{c2}^{ab}$(0) = 4.47 T and $B_{c2}^{c}$(0) = 1.25 T. The anisotropy parameter $Γ$ = $B_{c2}^{ab}$ / $B_{c2}^{c}$ increases with $T$ and is 6.8 at $T$ = $T_c$. The strong curvature of the $B_{c2}^{ab}(T)$ curve indicates the existence of strong spin paramagnetic effects.

cond-mat.supr-con↗

Fermi surface in BaNi$_2$P$_2$

We report measurements of the de Haas-van Alphen (dHvA) oscillation and a band structure calculation for the pnictide superconductor BaNi$_2$P$_2$, which is isostructural to BaFe$_2$As$_2$, the mother compound of the iron-pnictide high-$T_c$ superconductor (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$. Six dHvA-frequency branches with frequencies up to $\sim$8 kT were observed, and they are in excellent agreement with results of the band-structure calculation. The determined Fermi surface is large, enclosing about one electron and hole per formula unit, and three-dimensional. This is in contrast to the small two-dimensional Fermi surface expected for the iron-pnictide high-$T_c$ superconductors. The mass enhancement is about two.

cond-mat.supr-con↗