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Moumita Naskar

Publications and source records attributed to Moumita Naskar.

9 recordsLinked to original sources

Spin-liquid-like ground states in the double hydroxyperovskites CuSn(OD)6 and MnSn(OD)6 evidenced by {\mu}SR spectroscopy

Double hydroxide perovskites with magnetic transition-metal ions were recently identified as a unique class of materials that combine magnetic frustration with correlated proton disorder-a prerequisite for quantum-disordered fluctuating magnetic ground states resembling spin liquids. Here we present the results of muon spin relaxation ({\mu}SR) measurements carried out on fully deuterated samples of the double hydroxyperovskites CuSn(OH)6 (S = 1/2) and MnSn(OH)6 (S = 5/2) over the temperature range 0.053-50 K. The absence of any long-range magnetic order is confirmed down to 0.053 K. We observe no oscillations of the muon asymmetry down to the lowest temperature. The muon relaxation rates show a continuous increase with decreasing temperature, indicating persistent spin fluctuations in both compounds. Spin correlations are consistent with homogeneous spin dynamics. These observations reinforce the assertion that both compounds have a quantum-dynamic magnetic ground state that is consistent with a spin-liquid-like phase stabilized by proton disorder.

cond-mat.str-el

Disorder effects on the metastability of classical Heisenberg ferromagnets

In the present work, we investigate the effects of disorder on the reversal time ($\tau$) of classical anisotropic Heisenberg ferromagnets in three dimensions by means of Monte Carlo simulations. Starting from the pure system, our analysis suggests that $\tau$ increases with increasing anisotropy strength. On the other hand, for the case of randomly distributed anisotropy, generated from various statistical distributions, a set of results is obtained: (i) For both bimodal and uniform distributions the variation of $\tau$ with the strength of anisotropy strongly depends on temperature. (ii) At lower temperatures, the decrement in $\tau$ with increasing width of the distribution is more prominent. (iii) For the case of normally distributed anisotropy, the variation of $\tau$ with the width of the distribution is non-monotonic, featuring a minimum value that decays exponentially with the temperature. Finally, we elaborate on the joint effect of longitudinal ($h_z$) and transverse ($h_x$) fields on $\tau$, which appear to obey a scaling behavior of the form $\tau h_z^{n} \sim f(h_x)$.

cond-mat.stat-mech

Theoretical studies on switching of magnetisation in thin film

In the present chapter, we focus on the switching of magnetisation, or the metastable lifetime of a ferromagnetic system. In this regard, particularly the Ising model and the Blume-Capel model, have been simulated in the presence of an externally applied magnetic field by the Monte-Carlo simulation technique based on the Metropolis algorithm. Magnetisation switching is found to be faster in the presence of disorder, modelled here by a quenched random field. The strength of the random field is observed to play a similar role to that played by temperature. Becker-D\"oring theory of classical nucleation (originally proposed for the spin-1/2 Ising system) has been verified in the random field Ising model. However, a stronger random field affects the nucleation regime. In a cubic Ising lattice, surface reversal time is found to be different from the bulk reversal time. That distinct behaviour of the surface in contrast to the bulk has been studied here by introducing a relative interfacial interaction strength ($R$). Depending on $R$, temperature, and applied field, a competitive switching of magnetisation of surface and bulk is noticed. The effect of anisotropy ($D$) on the metastable lifetime has been investigated. We report a linear dependency of the mean macroscopic reversal time on a suitably defined microscopic reversal time. The saturated magnetisation $M_f$, after the reversal, is noticed to be strongly dependent on $D$. $M_f$, $D$, and $h$ (field) are found to follow a proposed scaling relation. Finally, Becker-D\"oring theory as well as Avrami's law are verified in spin-$s$ Ising and Blume-Capel models. The switching time depends on the number of accessible spin states.

cond-mat.stat-mech

Experimental and first-principles studies of superconductivity in topological nodal line semimetal SnTaS$_2$

We report a detailed study of superconductivity in polycrystalline SnTaS$_2$ using electrical transport, magnetization and heat capacity measurements. SnTaS$_2$ crystallizes in centrosymmetric hexagonal structure with space group $P6_3/mmc$. Electrical resistivity, magnetization and specific heat data suggest SnTaS$_2$ to be a weakly coupled, type-II superconductor with $T_c \approx$ 2.8 K. First-principles calculations show signature for nodal line topology in the electronic band structure, protected by the spatial-inversion and time-reversal symmetries, that strongly gapped out by the inclusion of spin-orbit coupling (SOC). Superconductivity in layered SnTaS$_2$ with nodal line topological state makes it a strong candidate to be considered for a 3D topological superconductor.

cond-mat.supr-con

Competitive metastable behaviours of surface and bulk in Ising ferromagnet

The reversal of magnetisation has been studied in a three dimensional Ising ferromagnet by Monte Carlo simulation with Metropolis single spin flip algorithm using random updating scheme. The outer layers are considered as surface. The surface interacts with core with a relative ferromagnetic interaction strength. Depending on the relative interaction strength, the time of reversal of the surface was found to be different from that of the bulk. For weaker relative strength, surface reversal was found to be faster than that of bulk and vice versa for stronger relative interaction strength. A critical value ($R_c$) of relative interaction strength provides same time of reversal of surface and bulk. This critical relative interaction strength was found to be a function of the temperature ($T$) and applied magnetic field ($h$). The scaling relation $R_c \sim h^{-\beta}f(Th^{\alpha})$, where, $\alpha=0.23\pm0.01$ and $\beta = -0.06\pm0.01$, has been proposed, numerically by the method of data collapse. The metastable volume fractions, for both surface and bulk, were found to follow the Avrami's law. The critical relative interaction strength ($R_c$) has been observed to decrease in an exponential ($e^{bL^{-1.5}})$ fashion with the system size ($L$).

cond-mat.stat-mech

Metastable behavior of the spin-s Ising and Blume-Capel ferromagnets: A Monte Carlo study

We present an extensive Monte Carlo investigation of the metastable lifetime through the reversal of the magnetization of spin-$s$ Ising and Blume-Capel models, where $s=\{1/2, 1, 3/2, 2, 5/2, 3, 7/2\}$. The mean metastable lifetime (or reversal time) is studied as a function of the applied magnetic field and for both models is found to obey the Becker-Doring theory, as was initially developed for the case of $s=1/2$ Ising ferromagnet within the classical nucleation theory. Moreover, the decay of metastable volume fraction nicely follows the Avrami's law for all values of $s$ and for both models considered.

cond-mat.stat-mech

Metastability in graded and step like variation of field and anisotropy of the Blume-Capel ferromagnet

The metastable behaviour of two dimensional anisotropic Blume-Capel ferromagnet, under the influence of graded and stepped like variations of magnetic field, has been investigated by extensive Monte Carlo simulation using Metropolis single spin flip algorithm. Starting from the initial perfectly ordered state, reversal of magnetisation has been studied in presence of the field. Metastable lifetime or the reversal time of magnetisation for the system having uniform anisotropy and in the presence of both graded and stepped field has been studied. Also the same has been explored for a {\it graded and stepped anisotropic system} in presence of a uniform field. Finite size effect is analyzed for the variation of reversal time with gradient of field ($G_h$) and a scaling relation $\langle \tau \rangle \sim L^{-\beta} f(G_h L^\alpha)$ is proposed. Spatial variation of density profile for the projection states (i.e., +1, 0 and -1) has also been studied at the moment of reversal of magnetisation. The spatial variation of the number of spin flips per site is studied. Motion of the interface (or domain wall) with the gradient of field and gradient of anisotropy are investigated and are found to follow the hyperbolic tangent like behaviours in both cases. Since, both the anisotropy and the applied field have significant impact on the metastable lifetime, an interesting competitive scenario is observed for a {\it graded anisotropic system in graded field} and a {\it stepped anisotropic system in stepped field}. A line of marginal competition has been found out for both the cases separating the regions of field dominated reversal and anisotropy dominated reversal. The decay of the metastable volume fraction was found to follow the Avrami's law. The mean reversal time was observed to decrease monotonically across the phase boundary of the ferro-para transition.

cond-mat.stat-mech

Anisotropy driven reversal of magnetisation in Blume-Capel ferromagnet: A Monte Carlo study

The two dimensional Spin-1 Blume-Capel ferromagnet is studied by Monte Carlo simulation with Metropolis algorithm. Starting from initial ordered spin configuration the reversal of magnetisation is investigated in presence of a magnetic field ($h$) applied in the opposite direction. The variations of the reversal time with the strength of single site anisotropy are investigated in details. The exponential dependence was observed. The systematic variations of the mean reversal time with positive and negative anisotropy was found. The mean macroscopic reversal time was observed to be linearly dependent on a suitably defined microscopic reversal time. The saturated magnetisation $M_f$ after the reversal was noticed to be dependent of the strength of anisotropy $D$. An interesting scaling relation was obtained, $|M_f| \sim |h|^{\beta}f(D|h|^{-\alpha})$ with the scaling function of the form $f(x)= \frac{1}{1+e^{(x-a)/b}}$. The temporal evolution of density of $S_i^z=0$ (surrounded by all $S_i^z=+1$) is observed to be exponentially decaying. The growth of mean density of $S_i^z=-1$ has been fitted in a function $\rho_{-1}(t) \sim \frac{1}{a+e^{(t_c-t)/c}}$. The characteristic time shows $t_c \sim e^{-rD}$ and a crossover in the rate of exponential falling is observed at $D=1.5$. The metastable volume fraction has been found to obey the Avrami's law.

cond-mat.stat-mech

Effects of random fields on the reversal of magnetisation of Ising ferromagnet

We have studied the reversal time of the magnetisation in two dimensional Ising ferromagnet in the presence of externally applied uniform magnetic field using Monte Carlo simulation based on Metropolis single spin flip algorithm. Then we have investigated the change in reversal time due to the presence of quenched random field in addition to the uniform magnetic field. We report the results of statistical distribution of reversal times in the presence of three different types of the distributions (namely, uniform, bimodal and normal) of random fields and compared the results with those obtained for uniform field only. We have observed that the reversal time decreases due to the presence of any kind (of distribution) of the random fields. The metastable volume fraction is observed to follow the Avrami's law. Dependence of reversal times on temperature and different widths of the distributions of random fields are also reported. We have also checked whether the system obeyed Becker-Doring theory of classical nucleation in presence of additional random field and tried to investigate the range of the width of the distribution of random field. For larger width of the distribution of random field, the system fails to show the reversal via the nucleation of a single droplet (for small values of uniform field only). The possible reason is analysed.

cond-mat.stat-mech