arXiv subjects

Murray J. Holland

Publications and source records attributed to Murray J. Holland.

At least 37 records · Page 2Linked to original sources

arXiv2021

Collective emission of an atomic beam into an off-resonant cavity mode

We study the collective emission of a beam of atomic dipoles into an optical cavity. Our focus lies on the effect of a finite detuning between the atomic transition frequency and the cavity resonance frequency. By developing a theoretical description of the coupled atom-cavity dynamics we analyze the stationary atomic configurations including a superradiant phase where the atoms undergo continuous monochromatic collective emission. In addition, we derive an analytical formula for the cavity pulling coefficient which characterizes the displacement of the emission frequency towards the cavity frequency. We find that the pulling is small if the cavity linewidth is much larger than the collective linewidth of the atomic beam. This regime is desired for building stable lasers because the emission frequency is robust against cavity length fluctuations. Furthermore, we investigate the stability of the atomic phases and compare our theoretical predictions with numerical results. Remarkably, we also find polychromatic emission regimes, where the spectrum has several frequency components while the light output is still superradiant.

quant-ph↗

arXiv2021

Superradiant emission of a thermal atomic beam into an optical cavity

We theoretically analyze the collective dynamics of a thermal beam of atomic dipoles that couple to a single mode when traversing an optical cavity. For this setup we derive a semiclassical model and determine the onset of superradiant emission and its stability. We derive analytical expressions for the linewidth of the emitted light and compare them with numerical simulations. In addition, we find and predict two different superradiant phases; a steady-state superradiant phase and a multi-component superradiant phase. In the latter case we observe sidebands in the frequency spectrum that can be calculated using a stability analysis of the amplitude mode of the collective dipole. We show that both superradiant phases are robust against free-space spontaneous emission and $T_2$ dephasing processes.

quant-ph↗

arXiv2021

Entropy transfer from a quantum particle to a classical coherent light field

In the field of light-matter interactions, it is often assumed that a classical light field that interacts with a quantum particle remains almost unchanged and thus contains nearly no information about the manipulated particles. To investigate the validity of this assumption, we develop and theoretically analyze a simple Gedankenexperiment which involves the interaction of a coherent state with a quantum particle in an optical cavity. We quantify the resulting alteration of the light field by measuring the fidelity of its initial and equilibrium states. Using Bayesian inference, we demonstrate the information transfer through photon measurements. In addition, we employ the concepts of quantum entropy and mutual information to quantify the entropy transfer from the particle to the light field. In the weak coupling limit, we validate the usually assumed negligible alteration of the light field and entropy transfer. In the strong coupling limit, however, we observe that the information of the initial particle state can be fully encoded in the light field, even for large photon numbers. Nevertheless, we show that spontaneous emission is a sufficient mechanism for removing the entropy initially stored in the particle. Our analysis provides a deeper understanding of the entropy exchange between quantum matter and classical light.

quant-ph↗

arXiv2021

Subradiant-to-Subradiant Phase Transition in the Bad Cavity Laser

We show that the onset of steady-state superradiance in a bad cavity laser is preceded by a dissipative phase transition between two distinct phases of steady-state subradiance. The transition is marked by a non-analytic behavior of the cavity output power and the mean atomic inversion, as well as a discontinuity in the variance of the collective atomic inversion. In particular, for repump rates below a critical value, the cavity output power is strongly suppressed and does not increase with the atom number, while it scales linearly with atom number above this value. Remarkably, we find that the atoms are in a macroscopic entangled steady state near the critical region with a vanishing fraction of unentangled atoms in the large atom number limit.

quant-ph↗

arXiv2020

Rugged mHz-Linewidth Superradiant Laser Driven by a Hot Atomic Beam

We propose a new type of superradiant laser based on a hot atomic beam traversing an optical cavity. We show that the theoretical minimum linewidth and maximum power are competitive with the best ultracoherent clock lasers. Also, our system operates naturally in continuous wave mode, which has been elusive for superradiant lasers so far. Unlike existing ultracoherent lasers, our design is simple and rugged. This makes it a candidate for the first widely accessible ultracoherent laser, as well as the first to realize sought-after applications of ultracoherent lasers in challenging environments.

quant-ph↗

arXiv2020

Regular and bistable steady-state superradiant phases of an atomic beam traversing an optical cavity

We investigate the different photon emission regimes created by a preexcited and collimated atomic beam passing through a single mode of an optical cavity. In the regime where the cavity degrees of freedom can be adiabatically eliminated, we find that the atoms undergo superradiant emission when the collective linewidth exceeds the transit-time broadening. We analyze the case where the atomic beam direction is slanted with respect to the cavity axis. For this situation, we find that a phase of continuous light emission similar to steady-state superradiance is established providing the tilt of the atomic beam is sufficiently small. However, if the atoms travel more than half a wavelength along the cavity axis during one transit time we predict a dynamical phase transition to a new bistable superradiant regime. In this phase the atoms undergo collective spontaneous emission with a frequency that can be either blue or red detuned from the free-space atomic resonance. We analyze the different superradiant regimes and the quantum critical crossover boundaries. In particular we find the spectrum of the emitted light and show that the linewidth exhibits features of a critical scaling close to the phase boundaries.

quant-ph↗

arXiv2020

Broadening of the drumhead mode spectrum due to in-plane thermal fluctuations of two-dimensional trapped ion crystals in a Penning trap

Two-dimensional crystals of ions stored in Penning traps are a leading platform for quantum simulation and sensing experiments. For small amplitudes, the out-of-plane motion of such crystals can be described by a discrete set of normal modes called the drumhead modes, which can be used to implement a range of quantum information protocols. However, experimental observations of crystals with Doppler-cooled and even near-ground-state-cooled drumhead modes reveal an unresolved drumhead mode spectrum. In this work, we establish in-plane thermal fluctuations in ion positions as a major contributor to the broadening of the drumhead mode spectrum. In the process, we demonstrate how the confining magnetic field leads to unconventional in-plane normal modes, whose average potential and kinetic energies are not equal. This property, in turn, has implications for the sampling procedure required to choose the in-plane initial conditions for molecular dynamics simulations. For current operating conditions of the NIST Penning trap, our study suggests that the two dimensional crystals produced in this trap undergo in-plane potential energy fluctuations of the order of $10$ mK. Our study therefore motivates the need for designing improved techniques to cool the in-plane degrees of freedom.

quant-ph↗

arXiv2020

Speeding Up Particle Slowing using Shortcuts to Adiabaticity

We propose a method for slowing particles by laser fields that potentially has the ability to generate large forces without the associated momentum diffusion that results from the random directions of spontaneously scattered photons. In this method, time-resolved laser pulses with periodically modified detunings address an ultranarrow electronic transition to reduce the particle momentum through repeated absorption and stimulated emission cycles. We implement a shortcut to adiabaticity approach that is based on Lewis-Riesenfeld invariant theory. This affords our scheme the advantages of adiabatic transfer, where there can be an intrinsic insensitivity to the precise strength and detuning characteristics of the applied field, with the advantages of rapid transfer that is necessary for obtaining a short slowing distance. For typical parameters of a thermal oven source that generates a particle beam with a central velocity on the order of meters per second, this could result in slowing the particles to near stationary in less than a millimeter. We compare the slowing scheme to widely-implemented slowing techniques that rely on radiation pressure forces and show the advantages that potentially arise when the excited state decay rate is small. Thus, this scheme is a particularly promising candidate to slow narrow-linewidth systems that lack closed cycling transitions, such as occurs in certain molecules.

physics.atom-ph↗

arXiv2020

Sawtooth Wave Adiabatic Passage in a Magneto-Optical Trap

We investigate theoretically the application of Sawtooth Wave Adiabatic Passage (SWAP) in a 1D magneto-optical trap (MOT). As opposed to related methods that have been previously discussed, our approach utilizes repeated cycles of stimulated absorption and emission processes to achieve both trapping and cooling, thereby reducing the adverse effects that arise from photon scattering. Specifically, we demonstrate this method's ability to cool, slow, and trap particles with fewer spontaneously emitted photons, higher forces and in less time when compared to a traditional MOT scheme that utilizes the same narrow linewidth transition. We calculate the phase space compression that is achievable and characterize the resulting system equilibrium cloud size and temperature.

physics.atom-ph↗

arXiv2019

Superradiant optomechanical phases of cold atomic gases in optical resonators

We theoretically analyze superradiant emission of light from a cold atomic gas, when mechanical effects of photon-atom interactions are considered. The atoms are confined within a standing-wave resonator and an atomic metastable dipolar transition couples to a cavity mode. The atomic dipole is incoherently pumped in the parameter regime that would correspond to stationary superradiance in absence of inhomogeneous broadening. Starting from the master equation for cavity field and atomic degrees of freedom we derive a mean-field model that allows us to determine a threshold temperature, above which thermal fluctuations suppress superradiant emission. We then analyze the dynamics of superradiant emission when the motion is described by a mean-field model. In the semiclassical regime and below the threshold temperature we observe that the emitted light can be either coherent or chaotic, depending on the incoherent pump rate. We then analyze superradiant emission from an ideal Bose gas at zero temperature when the superradiant decay rate $Λ$ is of the order of the recoil frequency $ω_R$. We show that the quantized exchange of mechanical energy between the atoms and the field gives rise to a threshold, $Λ_c$, below which superradiant emission is damped down to zero. When $Λ>Λ_c$ superradiant emission is accompanied by the formation of matter-wave gratings diffracting the emitted photons. The stability of these gratings depends on the incoherent pump rate $w$ with respect to a second threshold value $w_c$. For $w>w_c$ the gratings are stable and the system achieves stationary superradiance. Below this second threshold the coupled dynamics becomes chaotic. We characterize the dynamics across these two thresholds and show that the three phases we predict (incoherent, coherent, chaotic) can be revealed via the coherence properties of the light at the cavity output.

cond-mat.quant-gas↗

arXiv2019

Dynamical phase transitions to optomechanical superradiance

We theoretically analyze superradiant emission of light from an ultracold gas of bosonic atoms confined in a bad cavity. A metastable dipolar transition of the atoms couples to the cavity field and is incoherently pumped, the mechanical effects of cavity-atom interactions tend to order the atoms in the periodic cavity potential. By means of a mean-field model we determine the conditions on the cavity parameters and pump rate that lead to the buildup of a stable macroscopic dipole emitting coherent light. We show that this occurs when the superradiant decay rate and the pump rate exceed threshold values of the order of the photon recoil energy. Above these thresholds superradiant emission is accompanied by the formation of stable matter-wave gratings that diffract the emitted photons. Outside of this regime, instead, the optomechanical coupling can give rise to dephasing or chaos, for which the emitted light is respectively incoherent or chaotic. These behaviors exhibit the features of a dynamical phase transitions and emerge from the interplay between global optomechanical interactions, quantum fluctuations, and noise.

quant-ph↗

arXiv2018

Modeling near ground-state cooling of two-dimensional ion crystals in a Penning trap using electromagnetically induced transparency

Penning traps, with their ability to control planar crystals of tens to hundreds of ions, are versatile quantum simulators. Thermal occupations of the motional drumhead modes, transverse to the plane of the ion crystal, degrade the quality of quantum simulations. Laser cooling using electromagnetically induced transparency (EIT cooling) is attractive as an efficient way to quickly initialize the drumhead modes to near ground-state occupations. We numerically investigate the efficiency of EIT cooling of planar ion crystals in a Penning trap, accounting for complications arising from the nature of the trap and from the simultaneous cooling of multiple ions. We show that, in spite of challenges, the large bandwidth of drumhead modes (hundreds of kilohertz) can be rapidly cooled to near ground-state occupations within a few hundred microseconds. Our predictions for the center-of-mass mode include a cooling time constant of tens of microseconds and an enhancement of the cooling rate with increasing number of ions. Successful experimental demonstrations of EIT cooling in the NIST Penning trap [E. Jordan, K. A. Gilmore, A. Shankar, A. Safavi-Naini, M. J. Holland, and J. J. Bollinger, "Near ground-state cooling of two-dimensional trapped-ion crystals with more than 100 ions", (2018), submitted.] validate our predictions.

quant-ph↗

arXiv2018

Near ground-state cooling of two-dimensional trapped-ion crystals with more than 100 ions

We study, both experimentally and theoretically, electromagnetically induced transparency cooling of the drumhead modes of planar 2-dimensional arrays with up to $N\approx 190$ Be${}^+$ ions stored in a Penning trap. Substantial sub-Doppler cooling is observed for all $N$ drumhead modes. Quantitative measurements for the center-of-mass mode show near ground state cooling with motional quantum numbers of $\bar{n} = 0.3\pm0.2$ obtained within $200~μs$. The measured cooling rate is faster than that predicted by single particle theory, consistent with a quantum many-body calculation. For the lower frequency drumhead modes, quantitative temperature measurements are limited by apparent damping and frequency instabilities, but near ground state cooling of the full bandwidth is strongly suggested. This advancement will greatly improve the performance of large trapped ion crystals in quantum information and quantum metrology applications.

physics.atom-ph↗

arXiv2018

Laser Cooling by Sawtooth Wave Adiabatic Passage

We provide a theoretical analysis for a recently demonstrated cooling method. Two-level particles undergo successive adiabatic transfers upon interaction with counter-propagating laser beams that are repeatedly swept over the transition frequency. We show that particles with narrow linewidth transitions can be cooled to near the recoil limit. This cooling mechanism has a reduced reliance on spontaneous emission compared to Doppler cooling, and hence shows promise for application to systems lacking closed cycling transitions, such as molecules.

quant-ph↗

arXiv2017

Narrow-line Laser Cooling by Adiabatic Transfer

We propose and demonstrate a novel laser cooling mechanism applicable to particles with narrow-linewidth optical transitions. By sweeping the frequency of counter-propagating laser beams in a sawtooth manner, we cause adiabatic transfer back and forth between the ground state and a long-lived optically excited state. The time-ordering of these adiabatic transfers is determined by Doppler shifts, which ensures that the associated photon recoils are in the opposite direction to the particle's motion. This ultimately leads to a robust cooling mechanism capable of exerting large forces via a weak transition and with reduced reliance on spontaneous emission. We present a simple intuitive model for the resulting frictional force, and directly demonstrate its efficacy for increasing the total phase-space density of an atomic ensemble. We rely on both simulation and experimental studies using the 7.5~kHz linewidth $^1$S$_0$ to $^3$P$_1$ transition in $^{88}$Sr. The reduced reliance on spontaneous emission may allow this adiabatic sweep method to be a useful tool for cooling particles that lack closed cycling transitions, such as molecules.

physics.atom-ph↗

arXiv2017

Semiclassical theory of synchronization-assisted cooling

We analyse the dynamics leading to radiative cooling of an atomic ensemble confined inside an optical cavity when the atomic dipolar transitions are incoherently pumped and can synchronize. Our study is performed in the semiclassical regime and assumes that cavity decay is the largest rate in the system dynamics. We identify three regimes characterising the cooling. At first hot atoms are individually cooled by the cavity friction forces. After this stage, the atoms' center-of-mass motion is further cooled by the coupling to the internal degrees of freedom while the dipoles synchronize. In the latest stage dipole-dipole correlations are stationary and the center-of-mass motion is determined by the interplay between friction and dispersive forces due to the coupling with the collective dipole. We analyse this asymptotic regime by means of a mean-field model and show that the width of the momentum distribution can be of the order of the photon recoil. Furthermore, the internal excitations oscillate spatially with the cavity standing wave forming an antiferromagnetic-like order.

quant-ph↗

arXiv2015

Synchronization of Interacting Quantum Dipoles

Macroscopic ensembles of radiating dipoles are ubiquitous in the physical and natural sciences. In the classical limit the dipoles can be described as damped-driven oscillators, which are able to spontaneously synchronize and collectively lock their phases. Here we investigate the correspond- ing phenomenon in the quantum regime with arrays of quantized two-level systems coupled via long-range and anisotropic dipolar interactions. Our calculations demonstrate that the dipoles may overcome the decoherence induced by quantum fluctuations and inhomogeneous couplings and evolve to a synchronized steady-state. This steady-state bears much similarity to that observed in classical systems, and yet also exhibits genuine quantum properties such as quantum correlations and quan- tum phase diffusion (reminiscent of lasing). Our predictions could be relevant for the development of better atomic clocks and a variety of noise tolerant quantum devices.

quant-ph↗

arXiv2013

Evaporative cooling of reactive polar molecules confined in a two-dimensional geometry

Recent experimental developments in the loading of ultracold KRb molecules into quasi-two-dimensional traps, combined with the ability to tune the ratio between elastic and loss (inelastic/reactive) collisions through application of an external electric field, are opening the door to achieving efficient evaporative cooling of reactive polar molecules. In this paper, we use Monte Carlo simulations and semianalytic models to study theoretically the experimental parameter regimes in which evaporative cooling is feasible under current trapping conditions. We investigate the effect of the anisotropic character of dipole-dipole collisions and reduced dimensionality on evaporative cooling. We also present an analysis of the experimentally relevant anti-evaporation effects that are induced by chemical reactions that take place when more than one axial vibrational state is populated.

quant-ph↗