arXiv subjects

N. A. M. Araujo

Publications and source records attributed to N. A. M. Araujo.

At least 19 recordsLinked to original sources

arXiv2026

Imbibition dynamics under dissolution-driven fluid thickening

The imbibition of milk into a biscuit provides an example of a broader class of processes in which a liquid invades a porous material, dissolving components of the solid and thereby modifying its own rheology. This coupling between imbibition, dissolution, and evolving fluid rheology also occurs in food processing, filtration, and reactive porous media. While the resulting changes in fluid viscosity are known to affect imbibition, a quantitative description of how this evolving rheology determines the imbibition dynamics is still lacking. Here, we establish such a description for dissolution-driven fluid thickening. For a capillary tube in the well-mixed limit, we derive a generalized Washburn law showing that the evolving viscosity can be incorporated through a rescaled time given by the accumulated inverse viscosity. This predicts a collapse of the imbibition dynamics for different dissolution rates, which we confirm numerically using coupled free-surface and solute-transport simulations. When diffusion is slower, concentration and viscosity become spatially heterogeneous, resulting in a weaker retardation of the advancing liquid than predicted by the well-mixed theory. We then consider disordered porous media and quantify how dissolution-driven thickening and variations in pore geometry affect the dynamics. Our results extend the classical Washburn description to imbibition with evolving fluid properties and provide a quantitative basis for understanding fluid uptake when interactions with the solid progressively modify the rheology of the invading liquid.

cond-mat.soft↗

arXiv2024

Healing Regimes for Microscopic Wounds in the Vertex Model of Cell Tissues

Wounds in epithelial tissues compromise their vital role in homeostasis. A rapid and efficient wound healing encompasses different mechanisms, which includes the formation of a contractile actin-myosin cable around its edge, known as the purse-string mechanism. We combine mean-field calculations and numerical simulations of the Vertex model to study the interplay between tissue properties and the purse-string mechanism and its impact on the healing process. We find different regimes, where the wound opens, closes partially or completely. We also derive an analytic expression for the closure time which is validated by numerical simulations. This study establishes under which conditions the purse-string mechanism suffices for closure, providing an analytical mean-field expression for the respective thresholds.

cond-mat.soft↗

arXiv2023

Structural criterion for the onset of rigidity in a colloidal gel

Identifying the necessary conditions for the onset of rigidity in a gel remains a challenge. It has been suggested that local particle coordination could be used to establish such conditions, but rigid gels occur for various coordination numbers. Combining simulations, oscillatory rheology, and a percolation analysis, for particles where the valence can be controlled, we find that the onset of rigidity coincides with the percolation of particles with three or more bonds, which arises after the connectivity percolation. We show that the rigidity results from an interplay of bonding and non-bonding interactions, providing insight into low-valence colloidal gel rigidity.

cond-mat.soft↗

arXiv2021

Dynamical demixing of a binary mixture under sedimentation

We investigate the sedimentation dynamics of a binary mixture, the species of which differ by their Stokes coefficients but are identical otherwise. We analyze the sedimentation dynamics and the morphology of the final deposits using Brownian dynamics simulations for mixtures with a range of sedimentation velocities of both species. In addition, we use the lattice Boltzmann method to study hydrodynamic effects. We found a threshold in the difference of the sedimentation velocities above which the species in the final deposit are segregated. The degree of segregation increases with the difference in the Stokes coefficients or the sedimentation velocities above the threshold. We propose a simple analytical model that captures the main features of the simulated deposits.

cond-mat.soft↗

arXiv2021

Hierarchical structure of the energy landscape in the Voronoi model of dense tissue

The Voronoi model is a popular tool for studying confluent living tissues. It exhibits an anomalous glassy behavior even at very low temperatures or weak active self-propulsion, and at zero temperature the model exhibits a disordered solid structure with no evidence of a rigidity transition. Here we investigate the properties of the energy landscape in this limit. We find two disordered solid phases that have similar structural features but that differ in the ultrametricity of their energy landscapes; the crossover between these two states shares phenomenological properties with a Gardner transition. We further highlight how the metric used to calculate distances between configurations influences the ability to detect hierarchical arrangements of basins in the energy landscape.

cond-mat.soft↗

arXiv2020

Cracking urban mobility

Assessing the resilience of a road network is instrumental to improve existing infrastructures and design new ones. Here we apply the optimal path crack model (OPC) to investigate the mobility of road networks and propose a new proxy for resilience of urban mobility. In contrast to static approaches, the OPC accounts for the dynamics of rerouting as a response to traffic jams. Precisely, one simulates a sequence of failures (cracks) at the most vulnerable segments of the optimal origin-destination paths that are capable to collapse the system. Our results with synthetic and real road networks reveal that their levels of disorder, fractions of unidirectional segments and spatial correlations can drastically affect the vulnerability to traffic congestion. By applying the OPC to downtown Boston and Manhattan, we found that Boston is significantly more vulnerable than Manhattan. This is compatible with the fact that Boston heads the list of American metropolitan areas with the highest average time waste in traffic. Moreover, our analysis discloses that the origin of this difference comes from the intrinsic spatial correlations of each road network. Finally, we argue that, due to their global influence, the most important cracks identified with OPC can be used to pinpoint potential small rerouting and structural changes in road networks that are capable to substantially improve urban mobility.

physics.soc-ph↗

arXiv2020

Heterogeneous impact of a lockdown on inter-municipality mobility

Without a vaccine, the fight against the spreading of the coronavirus has focused on maintaining physical distance. To study the impact of such measures on inter-municipality traffic, we analyze a mobile dataset with the daily flow of people in Portugal in March and April 2020. We find that the reduction in inter-municipality traffic depends strongly on its initial outflow. In municipalities where the mobility is low, the outflow reduced by $10-20\%$ and this decrease was independent of the population size. Whereas, for municipalities of high mobility, the reduction was a monotonic increasing function of the population size and it even exceeded $60\%$ for the largest municipalities. As a consequence of such heterogeneities, there were significant structural changes on the most probable paths for the spreading of the virus, which must be considered when modeling the impact of control measures.

physics.soc-ph↗

arXiv2020

How to design cell-mediated self-assembled colloidal scaffolds

A critical step in tissue engineering is the design and synthesis of 3D biocompatible matrices (scaffolds) to support and guide the proliferation of cells and tissue growth. Most existing techniques rely on the processing of scaffolds under controlled conditions and then implanting them \textit{in vivo}, with questions related to biocompatibility and the implantation process that are still challenging. As an alternative, it was proposed to assemble the scaffolds \textit{in loco} through the self-organization of colloidal particles mediated by cells. In this study, we combine experiments, particle-based simulations, and mean-field calculations to show that, in general, the size of the self-assembled scaffold scales with the cell-to-particle ratio. However, we found an optimal value of this ratio, for which the size of the scaffold is maximal when cell-cell adhesion is suppressed. These results suggest that the size and structure of the self-assembled scaffolds may be designed by tuning the adhesion between cells in the colloidal suspension.

cond-mat.soft↗

arXiv2020

Optimal Number of Faces for Fast Self-Folding Kirigami

We study the spontaneous folding of a 2D template of microscopic panels into a 3D pyramid, driven by thermal fluctuations. Combining numerical simulations and analytical calculations, we find that the total folding time is a non-monotonic function of the number of faces, with a minimum for five faces. The motion of each face is consistent with a Brownian process and folding occurs through a sequence of irreversible binding events that close edges between pairs of faces. The first edge closing is well-described by a first-passage process in 2D, with a characteristic time that decays with the number of faces. By contrast, the subsequent edge closings are all first-passage processes in 1D and so the time of the last one grows logarithmically with the number of faces. It is the interplay between these two different sets of events that explains the non-monotonic behavior. Implications in the self-folding of more complex structures are discussed.

cond-mat.soft↗

arXiv2018

Mechanical equilibrium of aggregates of dielectric spheres

Industrial as well as natural aggregation of fine particles is believed to be associated with electrostatics. Yet like charges repel, so it is unclear how similarly treated particles aggregate. To resolve this apparent contradiction, we analyze conditions necessary to hold aggregates together with electrostatic forces. We find that aggregates of particles charged with the same sign can be held together due to dielectric polarization, we evaluate the effect of aggregate size, and we briefly summarize consequences for practical aggregation.

cond-mat.soft↗

arXiv2018

Multiple timescale contact charging

Contact charging between insulators is one of the most basic, yet least well understood, of physical processes. For example we have no clear theory for how insulators recruit enough charge carriers to deposit charge but not enough to discharge. In this letter we note that charging and discharging kinetics may be distinct, and from this observation we develop a mathematical model. The model surprisingly predicts that charging can decrease as contact frequency increases: we confirm this prediction experimentally and propose future steps.

cond-mat.soft↗

arXiv2018

Fundraising and vote distribution: a non-equilibrium statistical approach

The number of votes correlates strongly with the money spent in a campaign, but the relation between the two is not straightforward. Among other factors, the output of a ballot depends on the number of candidates, voters, and available resources. Here, we develop a conceptual framework based on Shannon entropy maximization and Superstatistics to establish a relation between the distributions of money spent by candidates and their votes. By establishing such a relation, we provide a tool to predict the outcome of a ballot and to alert for possible misconduct either in the report of fundraising and spending of campaigns or on vote counting. As an example, we consider real data from a proportional election with $6323$ candidates, where a detailed data verification is virtually impossible, and show that the number of potential misconducting candidates to audit can be reduced to only nine.

physics.soc-ph↗

arXiv2018

Dynamics of a network fluid within the liquid-gas coexistence region

Low-density networks of molecules or colloids are formed at low temperatures when the interparticle interactions are valence limited. Prototypical examples are networks of patchy particles, where the limited valence results from highly directional pairwise interactions. We combine extensive Langevin simulations and Wertheim's theory of association to study these networks. We find a scale-free (relaxation) dynamics within the liquid-gas coexistence region, which differs from that usually observed for isotropic particles. While for isotropic particles the relaxation dynamics is driven by surface tension (coarsening), when the valence is limited, the slow relaxation proceeds through the formation of an intermediate non-equilibrium gel via a geometrical percolation transition in the Random Percolation universality class.

cond-mat.soft↗

arXiv2017

Thermal gas rectification using a sawtooth channel

We study the rectification of a two-dimensional thermal gas in a channel of asymmetric dissipative walls. For an ensemble of smooth Lennard-Jones particles, our numerical simulations reveal a non-monotonic dependence of the flux on the thermostat temperature, channel asymmetry, and particle density, with three distinct regimes. Theoretical arguments are developed to shed light on the functional dependence of the flux on the model parameters.

cond-mat.soft↗

arXiv2017

Dynamical design of spatial patterns of colloidal suspensions

We study the collective dynamics of colloidal suspensions in the presence of a time-dependent potential, by means of dynamical density functional theory. We consider a non-linear diffusion equation for the density and show that spatial patterns emerge from a sinusoidal external potential with a time-dependent wavelength. These patterns are characterized by a sinusoidal density with the average wavelength and a Bessel-function envelope with an induced wavelength that depends only on the amplitude of the temporal oscillations. As a generalization of this result, we propose a design strategy to obtain a family of spatial patterns using time-dependent potentials of practically arbitrary shape.

cond-mat.soft↗

arXiv2016

Percolation study for the capillary ascent of a liquid through a granular soil

Capillary rise plays a crucial role in the construction of road embankments in flood zones, where hydrophobic compounds are added to the soil to suppress the rising of water and avoid possible damage of the pavement. Water rises through liquid bridges, menisci and trimers, whose width and connectivity depends on the maximal half-length λ of the capillary bridges among grains. Low λ generate a disconnect structure, with small clusters everywhere. On the contrary, for high λ, create a percolating cluster of trimers and enclosed volumes that form a natural path for capillary rise. Hereby, we study the percolation transition of this geometric structure as a function of λ on a granular media of monodisperse spheres in a random close packing. We determine both the percolating threshold λ_{c} = (0.049 \pm 0.004)R (with R the radius of the granular spheres), and the critical exponent of the correlation length ν = (0.830 \pm 0.051), suggesting that the percolation transition falls into the universality class of ordinary percolation.

physics.comp-ph↗

arXiv2015

Relaxation dynamics of functionalized colloids on attractive substrates

Particle-based simulations are performed to study the post-relaxation dynamics of functionalized (patchy) colloids adsorbed on an attractive substrate. Kinetically arrested structures that depend on the number of adsorbed particles and the strength of the particle-particle and particle-substrate interactions are identified. The radial distribution function is characterized by a sequence of peaks, with relative intensities that depend on the number of adsorbed particles. The first-layer coverage is a non-monotonic function of the number of particles, with an optimal value around one layer of adsorbed particles. The initial relaxation towards these structures is characterized by a fast (exponential) and a slow (power-law) dynamics. The fast relaxation timescale is a linearly increasing function of the number of adsorbed particles in the submonolayer regime, but it saturates for more than one adsorbed layer. The slow dynamics exhibits two characteristic exponents, depending on the surface coverage.

cond-mat.soft↗

arXiv2015

Schramm-Loewner Evolution and isoheight lines of correlated landscapes

Real landscapes are usually characterized by long-range height-height correlations, which are quantified by the Hurst exponent $H$. We analyze the statistical properties of the isoheight lines for correlated landscapes of $H\in [-1,1]$. We show numerically that, for $H\leq 0$ the statistics of these lines is compatible with $SLE$ and that established analytic results are recovered for $H=-1$ and $H=0$. This result suggests that for negative $H$, in spite of the long-range nature of correlations, the statistics of isolines is fully encoded in a Brownian motion with a single parameter in the continuum limit. By contrast, for positive $H$ we find that the one-dimensional time series encoding the isoheight lines is not Markovian and therefore not consistent with $SLE$.

cond-mat.stat-mech↗