arXiv subjects

N. Ahmed

Publications and source records attributed to N. Ahmed.

9 recordsLinked to original sources

arXiv2021

Low-dimensional magnetism of BaCuTe$_{2}$O$_{6}$

X-ray diffraction, thermodynamic measurements, and density-functional band-structure calculations are used to study the magnetic behavior of BaCuTe$_{2}$O$_{6}$, a member of the $A$CuTe$_2$O$_6$ structural family that hosts complex three-dimensional frustrated spin networks with possible spin-liquid physics. Temperature-dependent magnetic susceptibility and heat capacity of the Ba compound are well described by the one-dimensional spin-$\frac12$ Heisenberg chain model reminiscent of the Sr analog SrCuTe$_2$O$_6$. While the intrachain coupling $J/k_{\rm B}\simeq 37$ K is reduced compared to 49 K in the Sr compound, the Néel temperature increases from 5.5 K (Sr) to 6.1 K (Ba). Unlike the Sr compound, BaCuTe$_2$O$_6$ undergoes only one magnetic transition as a function of temperature and shows signatures of weak spin canting. We elucidate the microscopic difference between the Sr and Ba compounds and suggest that one of the interchain couplings changes sign as a result of negative pressure caused by the Sr/Ba substitution. The Néel temperature of BaCuTe$_2$O$_6$ is remarkably insensitive to the magnetic dilution with Zn$^{2+}$ up to the highest reachable level of about 20%.

cond-mat.mtrl-sci↗

arXiv2021

Quasi-one-dimensional magnetism in the spin-$\frac12$ antiferromagnet BaNa$_{2}$Cu(VO$_{4}$)$_{2}$

We report synthesis and magnetic properties of quasi-one-dimensional spin-$\frac{1}{2}$ Heisenberg antiferromagnetic chain compound BaNa$_2$Cu(VO$_4$)$_2$. This orthovanadate has a centrosymmetric crystal structure, $C2/c$, where the magnetic Cu$^{2+}$ ions form spin chains. These chains are arranged in layers, with the chain direction changing by 62$^0$ between the two successive layers. Alternatively, the spin lattice can be viewed as anisotropic triangular layers upon taking the inter-chain interactions into consideration. Despite this potential structural complexity, temperature-dependent magnetic susceptibility, heat capacity, ESR intensity, and NMR shift agree well with the uniform spin-$1/2$ Heisenberg chain model with an intrachain coupling of $J/k_{\rm B} \simeq 5.6$ K. The saturation field obtained from the magnetic isotherm measurement consistently reproduces the value of $J/k_{\rm B}$. Further, the $^{51}$V NMR spin-lattice relaxation rate mimics the 1D character in the intermediate temperature range, whereas magnetic long-range order sets in below $T_{\rm N} \simeq 0.25$ K. The effective interchain coupling is estimated to be $J_{\perp}/k_{\rm B} \simeq 0.1$ K. The theoretical estimation of exchange couplings using band-structure calculations reciprocate our experimental findings and unambiguously establish the 1D character of the compound. Finally, the spin lattice of BaNa$_2$Cu(VO$_4$)$_2$ is compared with the chemically similar but not isostructural compound BaAg$_2$Cu(VO$_4)_2$.

cond-mat.mtrl-sci↗

arXiv2018

Electrostatic rogue waves in double pair plasmas

A nonlinear Schrödinger equation is derived to investigate the modulational instability (MI) of ion-acoustic (IA) waves (IAWs) in a double pair plasma system containing adiabatic positive and negative ion fluids along with super-thermal electrons and positrons. The analytical analysis predicts two types of modes, viz. fast ($ω_f$) and slow ($ω_s$) IA modes. The possible stable and unstable parametric regions for the IAWs in presence of external perturbation can be observed for both $ω_f$ and $ω_s$. The number density of the negative ions and positrons play a vital role in generating the IA rogue waves (IARWs) in the modulationally unstable region. The applications of our present work in astrophysical environments [viz. D-region ($\rm H^+, O_2^-$) and F-region ($\rm H^+, H^-$) of the Earth's ionosphere] as well as in laboratory plasmas [viz. pair-ion Fullerene ($\rm C^+, C^-$)] are pinpointed.

physics.plasm-ph↗

arXiv2018

Hyperbolic Metamaterial Resonator-Antenna Scheme for Large, Broadband Emission Enhancement and Single Photon Collection

We model the broadband enhancement of single-photon emission from color centres in silicon carbide nanocrystals coupled to a planar hyperbolic metamaterial, HMM resonator. The design is based on positioning the single photon emitters within the HMM resonator, made of a dielectric index-matched with silicon-carbide material. The broadband response results from the successive resonance peaks of the lossy Fabry Perot structure modes arising within the high-index HMM cavity. To capture this broadband enhancement in the single photon emitters spontaneous emission, we placed a simple gold based cylindrical antenna on top of the HMM resonator. We analyzed the performance of this HMM coupled antenna structure in terms of the Purcell enhancement, quantum efficiency, collection efficiency and overall collected photon rate. For perpendicular dipole orientation relative to the interface, the HMM coupled antenna resonator leads to a significantly large spontaneous emission enhancement with Purcell factor of the order of 250 along with a very high average total collected photon rate, CPR of about 30 over a broad emission spectrum, 700 nm to 1000 nm. The peak CPR increases to about 80 at 900 nm, corresponding to the emission of silicon-carbide quantum emitters. This is a state of the art improvement considering the previous computational designs have reported a maximum average CPR of 25 across the nitrogen-vacancy centre emission spectrum, 600 nm to 800 nm with the highest value being about 40 at 650 nm.

quant-ph↗

arXiv2018

Self-gravitating envelope solitons in a degenerate quantum plasma system

The existence and the basic features of ion-acoustic (IA) envelope solitons in a self-gravitating degenerate quantum plasma system (SG-DQPS), containing inertial non-relativistically degenerate light and heavy ion species as well as inertialess non-relativistically degenerate positron and electron species, have been theoretically investigated by deriving the nonlinear Schrödinger (NLS) equation. The NLS equation, which governs the dynamics of the IA waves, has disclosed the modulationally stable and unstable regions for the IA waves. The unstable region allows to generate bright envelope solitons which are modulationaly stable. It is found that the stability and the growth rate dependent on the plasma parameters (like, mass and number density of the plasma species). The implications of our results in astronomical compact object (viz. white dwarfs, neutron stars, and black holes, etc.) are briefly discussed.

physics.plasm-ph↗

arXiv2015

Alternating-spin-chain compound AgVOAsO$_4$ probed by $^{75}$As NMR

$^{75}$As NMR measurements were performed on a polycrystalline sample of spin-1/2 alternating-spin-chain Heisenberg antiferromagnet AgVOAsO$_4$. Temperature-dependent NMR shift $K(T)$, which is a direct measure of the intrinsic spin susceptibility, agrees very well with the spin-1/2 alternating-chain model, justifying the assignment of the spin lattice. From the analysis of $K(T)$, magnetic exchange parameters were estimated as follows: the leading exchange $J/k_{\rm B} \simeq 38.4$ K, alternation ratio $α= J'/J \simeq 0.68$, and spin gap $Δ/k_{\rm B} \simeq 15$ K. The transferred hyperfine coupling between the $^{75}$As nucleus and V$^{4+}$ spins obtained by comparing the NMR shift with bulk susceptibility amounts to $A_{\rm hf} \simeq 3.3$ T/$μ_{\rm B}$. Our temperature-dependent spin-lattice relaxation rate $1/T_1(T)$ also shows an activated behaviour at low temperatures, thus confirming the presence of a spin gap in AgVOAsO$_4$.

cond-mat.mtrl-sci↗

arXiv2015

Multiple magnetic transitions in the spin-$\frac12$ chain antiferromagnet SrCuTe2O6

Using thermodynamic measurements and density-functional band-structure calculations, we explore magnetic behavior of SrCuTe2O6. Despite being a structural sibling of a three-dimensional frustrated system PbCuTe2O6, this spin-1/2 quantum magnet shows remarkably different low-temperature behavior. Above 7 K, magnetic susceptibility of SrCuTe2O6 follows the spin-chain model with the antiferromagnetic intrachain coupling of J = 49.3 K. We ascribe this quasi-one-dimensional behavior to the leading third-neighbor coupling that involves a weakly bent Cu--O......O--Cu superexchange pathway with a short O.....O contact of 2.79 Å. Below 5 K, SrCuTe2O6 undergoes two consecutive magnetic transitions that may be triggered by the frustrated nature of interchain couplings. Field dependence of the magnetic transitions (phase diagram) is reported.

cond-mat.mtrl-sci↗

arXiv2015

Antiferromagnetism of Zn$_2$VO(PO$_4)_2$ and the dilution with Ti$^{4+}$

We report static and dynamic properties of the antiferromagnetic compound Zn$_{2}$(VO)(PO$_{4}$)$_{2}$, and the consequences of non-magnetic Ti$^{4+}$ doping at the V$^{4+}$ site. $^{31}$P nuclear magnetic resonance (NMR) spectra and spin-lattice relaxation rate ($1/T_1$) consistently show the formation of the long-range antiferromagnetic order below $T_N= 3.8-3.9$\,K. The critical exponent $β=0.33 \pm 0.02$ estimated from the temperature dependence of the sublattice magnetization measured by $^{31}$P NMR at 9.4\,MHz is consistent with universality classes of three-dimensional spin models. The isotropic and axial hyperfine couplings between the $^{31}$P nuclei and V$^{4+}$ spins are $A_{\rm hf}^{\rm iso} = (9221 \pm 100)$ Oe/$μ_{\rm B}$ and $A_{\rm hf}^{\rm ax} = (1010 \pm 50)$ Oe/$μ_{\rm B}$, respectively. Magnetic susceptibility data above 6.5\,K and heat capacity data above 4.5\,K are well described by quantum Monte-Carlo simulations for the Heisenberg model on the square lattice with $J\simeq 7.7$\,K. This value of $J$ is consistent with the values obtained from the NMR shift, $1/T_1$ and electron spin resonance (ESR) intensity analysis. Doping Zn$_2$VO(PO$_4)_2$ with non-magnetic Ti$^{4+}$ leads to a marginal increase in the $J$ value and the overall dilution of the spin lattice. In contrast to the recent \textit{ab initio} results, we find neither evidence for the monoclinic structural distortion nor signatures of the magnetic one-dimensionality for doped samples with up to 15\% of Ti$^{4+}$. The Néel temperature $T_{\rm N}$ decreases linearly with increasing the amount of the non-magnetic dopant.

cond-mat.mtrl-sci↗

arXiv2003

Experimental study of weak antilocalization effect in a high mobility InGaAs/InP quantum well

The magnetoresistance associated with quantum interference corrections in a high mobility, gated InGaAs/InP quantum well structure is studied as a function of temperature, gate voltage, and angle of the tilted magnetic field. Particular attention is paid to the experimental extraction of phase-breaking and spin-orbit scattering times when weak anti- localization effects are prominent. Compared with metals and low mobility semiconductors the characteristic magnetic field $B_{tr} = \hbar/4eD τ$ in high mobility samples is very small and the experimental dependencies of the interference effects extend to fields several hundreds of times larger. Fitting experimental results under these conditions therefore requires theories valid for arbitrary magnetic field. It was found, however, that such a theory was unable to fit the experimental data without introducing an extra, empirical, scale factor of about 2. Measurements in tilted magnetic fields and as a function of temperature established that both the weak localization and the weak anti-localization effects have the same, orbital origin. Fits to the data confirmed that the width of the low field feature, whether a weak localization or a weak anti-localization peak, is determined by the phase-breaking time and also established that the universal (negative) magnetoresistance observed in the high field limit is associated with a temperature independent spin-orbit scattering time.

cond-mat.mes-hall↗