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N. B. Bolotina

Publications and source records attributed to N. B. Bolotina.

5 recordsLinked to original sources

3D- (H-theta-phi) magnetic phase diagram of antiferromagnetic metal GdB6 with electron and lattice instability

The origin of charge transport and magnetization anisotropy was studied in GdB6, an antiferromagnetic (AF) metal (Néel temperature TN ~ 15.5 K) with cubic lattice and Gd S-type magnetic ions. Both small static Jahn-Teller distortions and nanoscale electronic instabilities (dynamic charge stripes) were found in precise low temperature X-ray diffraction measurements. The detailed magnetic field (H) vs temperature (T) phase diagrams were constructed with two main magnetic phases AF(I) and AF(II). Using the angular phi-dependences of magnetoresistance and magnetization, impeller-type patterns of the H-phi magnetic phase diagrams in the (110) and (111) planes were found at helium temperatures, which included the AF phases I and II separated from each other by radial and circular boundaries. The results argue in favor of the important role of the spin density wave 5d- component in the magnetic structure of AF(II) state. Charge fluctuations in stripes are proposed to be responsible for the suppression of the Ruderman-Kittel-Kasuya-Yoshida (RKKY) indirect exchange between the first and second neighboring Gd3+ ions located along the <100> and <110> directions. These dynamic charge stripes and vibrationally coupled Gd-Gd pairs produce unusual anisotropy of charge scattering and the impeller-type diagrams in GdB6 with S-type magnetic ion.

cond-mat.str-el↗

Two-gap superconductor ZrB$_{12}$ with dynamic stripes and charge density waves: Crystal structure, physical properties and pairing mechanism

A review of long-term studies of ZrB$_{12}$ and LuB$_{12}$ superconductors with very similar conduction bands and phonon spectra, but with radically different (by a factor of 15-20) critical temperatures and magnetic fields is presented. A detailed analysis of well-known studies in combination with new results of structural, thermodynamic and charge transport measurements obtained here for these metallic dodecaborides with Jahn-Teller instability of the rigid boron network and with dynamic charge stripes allows us to conclude in favor of the primary role of nanoscale effects of electron phase separation, leading to the formation of one-dimensional dynamic chains with different configurations of fluctuating charges, which in the case of ZrB$_{12}$ are predominantly $2p$-states, and for LuB$_{12}$-$5d$-$2p$ states. We propose a new plasmon-phonon pairing mechanism in ZrB$_{12}$, which may be common to different classes of high-$T_c$ superconductors.

cond-mat.supr-con↗

Evidence for spin droplets (ferrons) formation in the heavy fermion metal CeB$_6$ with dynamic charge stripes

The presented studies of resistivity (R), thermal conductivity (k) and specific heat (C) at low temperature 1.8-7 K in magnetic field up to 90 kOe made it possible to detect for the first time the exponential field dependences R(H), 1/k(H), $C(H) \sim \exp(-μ_{\rm eff}H/kBT)$ of the charge transport and thermal characteristics in the so-called antiferroquadrupole (AFQ) phase of the archetypal heavy-fermion CeB$_6$ hexaboride. From magnetoresistance measurements it is shown that in the AFQ state the effective magnetic moment varies in the range $μ_{\rm eff}(T) = 1.4$-1.9$μ$B, and its value is very close to $μ_{\rm eff}(τ)(T) = 2μ$B, derived from the field dependence of the relaxation time $|tau(H)$ observed in the heat capacity and thermal conductivity experiments. The phenomenological model proposed here allowed us to attribute the magnetic moments to spin droplets (ferrons), that appear in the bulk AFQ phase of CeB$_6$ crystals. The relevant electron phase separation at the nanoscale, manifested by dynamic charge stripes, that leads to the formation of ferrons, was revealed from the analysis of low-temperature X-ray diffraction experiments using the maximum entropy method. We argue that the Jahn-Teller collective mode of B$_6$ clusters is responsible for the charge stripe formation, which subsequently induces transverse quasi-local vibrations of Ce ions in the form of pairs and triples. These lead to 4f-5d spin fluctuations providing spin-polarons (ferrons) in the CeB$_6$ matrix.

cond-mat.str-el↗

Checkerboard-type patterns of charge stripes in two-gap superconductor ZrB12

Inhomogeneous superconductivity in the high quality single crystals of ZrB12 (Tc = 6 K) has been studied using the heat capacity and x-ray diffraction (XRD) data. Evidence of two-band superconductivity with two branches of upper critical field Hc2(Tc) is obtained in a magnetic field applied along the [110] axis of the crystal. On the contrary, at H //[100], the only dependence Hc2(Tc) is observed. This finding is supplemented with the checkerboard-type patterns of the charge stripes in ZrB12 deduced from the detailed analysis of XRD data. These patterns are compared to the structure of the charge stripes in the weakly bound superconductor LuB12, whose Tc is 15 times lower than that of ZrB12. Probable nature of the two-gap superconductivity in ZrB12 with strongly enhanced characteristics is discussed.

cond-mat.supr-con↗

Observation of dynamic charge stripes in Tm0.19Yb0.81B12 at the metal-insulator transition

Higher accuracy low temperature charge transport measurements in combination with precise X-ray diffraction experiment have allowed detecting the symmetry lowering in the single domain Tm0.19Yb0.81B12 crystals of the family of dodecaborides with metal-insulator transition. Basing on the fine structure analysis we discover formation of dynamic charge stripes within the semiconducting matrix of Tm0.19Yb0.81B12. The charge dynamics in these metallic nano-size conducting channels is characterized by broad-band optical spectroscopy that allowed estimating the frequency (~2.4 10^11 Hz) of quantum motion of the charge carriers. It is suggested that caused by cooperative Jahn-Teller effect in the boron sub-lattice, the large amplitude rattling modes of the Tm and Yb ions are responsible for modulation of the conduction band along [110] direction through the variation of 5d-2p hybridization of electron states.

cond-mat.str-el↗