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N. B. Ivanov

Publications and source records attributed to N. B. Ivanov.

At least 19 recordsLinked to original sources

Heisenberg spin chains with additional isotropic three-site exchange interactions

The $J_1-J_3$ Heisenberg spin models with nearest-neighbor ($J_1$) and additional isotropic three-site ($J_3$) spin interactions remain relatively less explored, although such types of competing exchange terms can naturally emerge from different sources, including the strong-coupling expansion of the multiorbital Hubbard model. Below we present a short survey of the recently published research in this field, the emphasis being on the characteristics of the variety of quantum phases supported by a few generic uniform- and alternating-spin $J_1-J_3$ Heisenberg chains. For the reason that the positive ($J_3>0$) three-site couplings tend towards the formation of local quantum dimers, the $J_1-J_3$ spin models typically experience some spontaneous dimerization upon increasing $J_3$. Actually, it occurred that the established dimer phases in spin-$S$ $J_1-J_3$ Heisenberg chains ($S>{1}/{2}$) serve as complete analogues of the famous gapped Majumdar-Ghosh dimer phase in the spin-${1}/{2}$ Heisenberg chain with next-nearest-neighbor couplings. The same dimerizations have been observed in the alternating-spin ($S,σ$) $J_1-J_3$ chains ($S>σ$), provided that the cell spin $S+σ=\rm{integer}$, whereas for half-integer cell spin, the local dimer formation produces gapless spin-liquid ground states. The alternating-spin $J_1-J_3$ chains also provide some typical examples of spin models supporting the so-called non-Lieb-Mattis magnetic phases.

cond-mat.str-el

Alternating-spin S=3/2 and sigma=1/2 Heisenberg chain with three-body exchange interactions

The promotion of collinear classical spin configurations as well as the enhanced tendency towards nearest-neighbor clustering of the quantum spins are typical features of the frustrating isotropic three-body exchange interactions in Heisenberg spin systems. Based on numerical density-matrix renormalization group calculations, we demonstrate that these extra interactions in the Heisenberg chain constructed from alternating S=3/2 and sigma=1/2 site spins can generate numerous specific quantum spin states, including some partially-polarized ferrimagnetic states as well as a doubly-degenerate non-magnetic gapped phase. In the non-magnetic region of the phase diagram, the model describes a crossover between the spin-1 and spin-2 Haldane-type states.

cond-mat.str-el

Phase diagram of the alternating-spin Heisenberg chain with extra isotropic three-body exchange interactions

For the time being isotropic three-body exchange interactions are scarcely explored and mostly used as a tool for constructing various exactly solvable one-dimensional models, although, generally speaking, such competing terms in generic Heisenberg spin systems can be expected to support specific quantum effects and phases. The Heisenberg chain constructed from alternating S=1 and sigma=1/2 site spins defines a realistic prototype model admitting extra three-body exchange terms. Based on numerical density-matrix renormalization group (DMRG) and exact diagonalization (ED) calculations, we demonstrate that the additional isotropic three-body terms stabilize a variety of partially-polarized states as well as two specific non-magnetic states including a critical spin-liquid phase controlled by two Gaussinal conformal theories as well as a critical nematic-like phase characterized by dominant quadrupolar S-spin fluctuations. Most of the established effects are related to some specific features of the three-body interaction such as the promotion of local collinear spin configurations and the enhanced tendency towards nearest-neighbor clustering of the spins. It may be expected that most of the predicted effects of the isotropic three-body interaction persist in higher space dimensions.

cond-mat.str-el

Discrete antiferromagnetic spin-wave excitations in the giant ferric wheel Fe18

The low-temperature elementary spin excitations in the AFM molecular wheel Fe18 were studied experimentally by inelastic neutron scattering and theoretically by modern numerical methods, such as dynamical density matrix renormalization group or quantum Monte Carlo techniques, and analytical spin-wave theory calculations. Fe18 involves eighteen spin-5/2 Fe(III) ions with a Hilbert space dimension of 10^14, constituting a physical system that is situated in a region between microscopic and macroscopic. The combined experimental and theoretical approach allowed us to characterize and discuss the magnetic properties of Fe18 in great detail. It is demonstrated that physical concepts such as the rotational-band or L&E-band concepts developed for smaller rings are still applicable. In particular, the higher-lying low-temperature elementary spin excitations in Fe18 or AFM wheels in general are of discrete antiferromagnetic spin-wave character.

cond-mat.str-el

Heat capacity uncovers physics of a frustrated spin tube

We report on refined experimental results concerning the low-temperature specific heat of the frustrated spin tube material [(CuCl2tachH)3Cl]Cl2. This substance turns out to be an unusually perfect spin tube system which allows to study the physics of quasi-one dimensional antiferromagnetic structures in rather general terms. An analysis of the specific heat data demonstrates that at low enough temperatures the system exhibits a Tomonaga-Luttinger liquid behavior corresponding to an effective spin-3/2 antiferromagnetic Heisenberg chain with short-range exchange interactions. On the other hand, at somewhat elevated temperatures the composite spin structure of the chain is revealed through a Schottky-type peak in the specific heat located around 2 K. We argue that the dominating contribution to the peak originates from gapped magnon-type excitations related to the internal degrees of freedom of the rung spins.

cond-mat.str-el

Frustrated spin ladder with alternating spin-1 and spin-1/2 rungs

We study the impact of the diagonal frustrating couplings on the quantum phase diagram of a two-leg ladder composed of alternating spin-1 and spin-1/2 rungs. As the coupling strength is increased the system successively exhibits two gapped paramagnetic phases (a rung-singlet and a Haldane-like non-degenerate states) and two ferrimagnetic phases with different ferromagnetic moments per rung. The first two states are similar to the phases studied in the frustrated spin-1/2 ladder, whereas the magnetic phases appear as a result of the mixed-spin structure of the model. A detailed characterization of these phases is presented using density-matrix renormalization-group calculations, exact diagonalizations of periodic clusters, and an effective Hamiltonian approach inspired by the analysis of numerical data. The present theoretical study was motivated by the recent synthesis of the quasi-one-dimensional ferrimagnetic material Fe$^{II}$Fe$^{III}$ (trans-1,4-cyclohexanedicarboxylate) exhibiting a similar ladder structure.

cond-mat.str-el

Spin models of quasi-1D quantum ferrimagnets with competing interactions

We present a brief survey of the recent theoretical work related to generic Heisenberg spin models describing quasi-one-dimensional quantum ferrimagnets. The emphasis is on quantum chains and ladders with strong competing interactions, such as the frustrated $J_1-J_2$ chain with alternating (1,1/2) spins, the spin-1/2 diamond chain with four-spin cyclic couplings, and some generic types of mixed-spin ladders with geometric frustration. As a rule, discussed models exhibit rich quantum phase diagrams and provide some interesting examples of one-dimensional magnetic-paramagnetic quantum phase transitions. A number of open problems in the reviewed research area are discussed.

cond-mat.str-el

Diamond chains with multiple-spin exchange interactions

We study the phase diagram of a symmetric spin-1/2 Heisenberg diamond chain with additional cyclic four-spin exchange interactions. The presented analysis supplemented by numerical exact-diagonalization results for finite periodic clusters implies a rich phase diagram containing, apart from standard magnetic and spin-liquid phases, two different tetramer-dimer phases as well as an exotic four-fold degenerate dimerized phase. The characteristics of the established spin phases as well as the nature of quantum phase transitions are discussed, as well.

cond-mat.str-el

Magnetic phase diagram of a frustrated ferrimagnetic ladder: Relation to the one-dimensional boson Hubbard model

We study the magnetic phase diagram of two coupled mixed-spin $(1,{1/2})$ Heisenberg chains as a function of the frustration parameter related to diagonal exchange couplings. The analysis is performed by using spin-wave series and exact numerical diagonalization techniques. The obtained phase diagram--containing the Luttinger liquid phase, the plateau phase with a magnetization per rung $M=1/2$, and the fully polarized phase--is closely related to the generic $(J/U,μ/U)$ phase diagram of the one-dimensional boson Hubbard model.

cond-mat.str-el

Spin wave analysis of Heisenberg magnets in restricted geometries

In the last decade it has been proven that the standard spin wave theory was able to provide accurate zero-temperature results for a number of low-dimensional Heisenberg spin systems. In this chapter we introduce the main ingredients of the spin-wave technique using as a working model the two-leg mixed-spin ferrimagnetic ladder and the Dyson--Maleev boson formalism up to second order in the spin-wave interaction. In the remainder, we survey typical applications in low-space dimensionality as well as some recent modifications of the theory admitting a quantitative analysis in magnetically disordered phases. The presented spin-wave results are compared with available numerical estimates.

cond-mat.str-el

Phase diagram of a frustrated mixed-spin ladder with diagonal exchange bonds

Using exact numerical diagonalization and the conformal field theory approach, we study the effect of magnetic frustrations due to diagonal exchange bonds in a system of two coupled mixed-spin $(1,{1/2})$ Heisenberg chains. It is established that relatively moderate frustrations are able to destroy the ferrimagnetic state and to stabilize the critical spin-liquid phase typical for half-integer-spin antiferromagnetic Heisenberg chains. Both phases are separated by a narrow but finite region occupied by a critical partially-polarized ferromagnetic phase.

cond-mat.str-el

Study of an Antiferromagnetic Sawtooth Chain with Spin-1/2 and Spin-1 sites

We study the low-energy properties of a sawtooth chain with spin-1's at the bases of the triangles and spin-1/2's at the vertices of the triangles. The spins have Heisenberg antiferromagnetic interactions between nearest neighbors, with a coupling J_2 between a spin-1 and a spin-1/2, and a coupling J_1 = 1 between two spin-1's. Analysis of the exact diagonalization data for periodic chains containing up to N=12 unit cells shows that the ground state is a singlet for exchange couplings up to approximately J_2 = 3.8, whereas for larger J_2, the system exhibits a ferrimagnetic ground state characterized by a net ferromagnetic moment per unit cell of 1/2. In the region of small interactions J_2, the mixed spin sawtooth chain maps on to an effective isotropic spin model representing two weakly interacting and frustrated spin-1/2 Heisenberg chains composed of spin-1/2 sites at odd and even vertices respectively. Finally, we study the phenomenon of a macroscopic magnetization jump which occurs if a magnetic field is applied with a value close to the saturation field for J_2 = 2.

cond-mat.str-el

Magnetic phases of the mixed-spin $J_1-J_2$ Heisenberg model on a square lattice

We study the zero-temperature phase diagram and the low-energy excitations of a mixed-spin ($S_1>S_2$) $J_1-J_2$ Heisenberg model defined on a square lattice by using a spin-wave analysis, the coupled cluster method, and the Lanczos exact-diagonalization technique. As a function of the frustration parameter $J_2/J_1$ ($ >0$), the phase diagram exhibits a quantized ferrimagnetic phase, a canted spin phase, and a mixed-spin collinear phase. The presented results point towards a strong disordering effect of the frustration and quantum spin fluctuations in the vicinity of the classical spin-flop transition. In the extreme quantum system $(S_1,S_2)=(1,{1/2})$, we find indications of a new quantum spin state in the region $0.46< J_2/J_1<0.5$

cond-mat.str-el

Finite size and temperature effects in the $J_1-J_2$ model on a strip

Within Takahashi's spin-wave theory we study finite size and temperature effects near the quantum critical point in the $J_{1}-J_{2}$ Heisenberg antiferromagnet defined on a strip ($L\times\infty$). In the continuum limit, the theory predicts universal finite size and temperature corrections and describes the dimensional crossover in magnetic properties from 2+1 to 1+1 space-time dimensions.

cond-mat.stat-mech

Collective excitations in ferrimagnetic Heisenberg ladders

We study ground-state properties and the low-lying excitations of Heisenberg spin ladders composed of two ferrimagnetic chains with alternating site spins $(S_1>S_2)$ by using the bosonic Dyson-Maleev formalism and Lanczos numerical techniques. The emphasis is on properties of the ferrimagnetic phase which is stable for antiferromagnetic interchain couplings $J_{\perp}\geq 0$. There are two basic implications of the underlying lattice structure: (i) the spin-wave excitations form folded acoustic and optical branches in the extended Brillouin zone and (ii) the ground state parameters (such as the on-site magnetizations and spin-stiffness constant) show a crossover behavior in the weak-coupling region $0<J_{\perp}<1$. The above peculiarities of the ladder ferrimagnetic state are studied up to second order in the quasiparticle interaction and by a numerical diagonalization of ladders containing up to N=12 rungs. The presented results for the ground-state parameters and the excitation spectrum can be used in studies on the low-temperature thermodynamics of ferrimagnetic ladders.

cond-mat.str-el

Magnon dispersions in quantum Heisenberg ferrimagnetic chains at zero temperature

Within the Dyson-Maleev boson formalism, we study the zero-temperature magnon dispersions in a family of one-dimensional quantum Heisenberg ferrimagnets composed of two different spins $(S_1,S_2)$ in the elementary cell. It is shown that the spin-wave theory can produce precise quantitative results for the low-energy excitations. The spin-stiffness constant $ρ_s$ and the optical magnon gap $Δ$ of different $(S_1,S_2)$ ferrimagnetic systems are calculated, respectively, to second and third order in the quasiparticle interaction. The spin-wave results are compared with available numerical estimates.

cond-mat.str-el

Fluctuations in confined nematic liquid crystals in a regime of critical wetting

Within the macroscopic Landau-de Gennes approach, we examine the Gaussian normal mode fluctuations of semi-infinite nematic liquid crystals in a regime of critical wetting. It is argued that surface free-energy potentials that strongly suppress the long-range nematic order favor the appearance of bound biaxial nematic-director fluctuation modes, located in the domain occupied by the thermodynamic phase wetting the wall. Instead, substrates enhancing the orientational order promote the existence of uniaxial nematic-director local excitations. Close to the phase coexistence temperature both types of local exciations are strongly softened as compared to their bulk counterparts and acquire characteristic cusplike low-energy spectra. These spectrum peculiarities are directly connected to the critical behavior of the mean-field interface position and can provide a valuable insight on the nature of surface interactions and critical wetting phenomena in nematic liquid crystals. Possible changes in the local director mode properties resulting from the critical interface position fluctuations and order electricity effects are also discussed.

cond-mat.soft

Frustrated quantum Heisenberg ferrimagnetic chains

We study the ground-state properties of weakly frustrated Heisenberg ferrimagnetic chains with nearest and next-nearest neighbor antiferromagnetic exchange interactions and two types of alternating sublattice spins S_1 > S_2, using 1/S spin-wave expansions, density-matrix renormalization group, and exact- diagonalization techniques. It is argued that the zero-point spin fluctuations completely destroy the classical commensurate- incommensurate continuous transition. Instead, the long-range ferrimagnetic state disappears through a discontinuous transition to a singlet state at a larger value of the frustration parameter. In the ferrimagnetic phase we find a disorder point marking the onset of incommensurate real-space short-range spin-spin correlations.

cond-mat.str-el