arXiv subjects

N. Bontemps

Publications and source records attributed to N. Bontemps.

At least 19 recordsLinked to original sources

arXiv2006

Temperature dependence of the spectral weight in p- and n-type cuprates: a study of normal state partial gaps and electronic kinetic energy

The optical conductivity of CuO2 (copper-oxygen) planes in p- and n-type cuprates thin films at various doping levels is deduced from highly accurate reflectivity data. The temperature dependence of the real part sigma1(omega) of this optical conductivity and the corresponding spectral weight allow to track the opening of a partial gap in the normal state of n-type Pr{2-x}Ce(x)CuO4 (PCCO), but not of p-type Bi2Sr2CaCu2O(8+delta} (BSCCO) cuprates. This is a clear difference between these two families of cuprates, which we briefly discuss. In BSCCO, the change of the electronic kinetic energy Ekin - deduced from the spectral weight- at the superconducting transition is found to cross over from a conventional BCS behavior (increase of Ekin below Tc to an unconventional behavior (decrease of Ekin below Tc) as the free carrier density decreases. This behavior appears to be linked to the energy scale over which spectral weight is lost and goes into the superfluid condensate, hence may be related to Mott physics.

cond-mat.supr-con↗

arXiv2005

Comment to the paper "In-plane spectral weight shift of charge-carriers in YBa2Cu3O(6.9)" by A. V. Boris et al., Science 304, p. 708 (2004)

Recently, A. V. Boris and colleagues claimed to deduce a decrease of intraband spectral weight (SW), and a transfer of SW from intraband to inter-band frequencies, when optimally-doped or slightly underdoped cuprates become superconducting [A. V. Boris et al., Science 304, p. 708 (2004)]. We show that, while their data agree with others [H. J. A. Molegraaf et al., Science 295, p. 2239 (2002) ; A.F. Santander-Syro et al., Europhys.Lett 62, p. 568 (2003)], their analysis is flawed. They cannot disprove the results which yield a superconductivity-induced increase of intraband SW, and a transfer of SW from high to low frequencies, in underdoped or nearly optimally doped Bi-2212.

cond-mat.supr-con↗

arXiv2005

Kinetic energy change with doping upon superfluid condensation in high temperature superconductors

In conventional BCS superconductors, the electronic kinetic energy increases upon superfluid condensation (the change DEkin is positive). Here we show that in the high critical temperature superconductor Bi-2212, DEkin crosses over from a fully compatible conventional BCS behavior (DEkin>0) to an unconventional behavior (DEkin<0) as the free carrier density decreases. If a single mechanism is responsible for superconductivity across the whole phase diagram of high critical temperature superconductors, this mechanism should allow for a smooth transition between such two regimes around optimal doping.

cond-mat.supr-con↗

arXiv2004

On the optical conductivity of Electron-Doped Cuprates I: Mott Physics

The doping and temperature dependent conductivity of electron-doped cuprates is analysed. The variation of kinetic energy with doping is shown to imply that the materials are approximately as strongly correlated as the hole-doped materials. The optical spectrum is fit to a quasiparticle scattering model; while the model fits the optical data well, gross inconsistencies with photoemission data are found, implying the presence of a large, strongly doping dependent Landau parameter.

cond-mat.str-el↗

arXiv2004

Infrared Properties of Electron Doped Cuprates: Tracking Normal State Gaps and Quantum Critical Behavior in Pr(2-x)Ce(x)CuO(4)

We report the temperature dependence of the infrared-visible conductivity of Pr(2-x)Ce(x)CuO(4) thin films. When varying the doping from a non-superconducting film (x = 0.11) to a superconducting overdoped film (x = 0.17), we observe, up to optimal doping (x = 0.15), a partial gap opening. A model combining a spin density wave gap and a frequency and temperature dependent self energy reproduces our data reasonably well. The magnitude of this gap extrapolates to zero for x ~ 0.17 indicating the coexistence of magnetism and superconductivity in this material and the existence of a quantum critical point at this Ce concentration.

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arXiv2004

Infrared Signature of the Superconducting State in Pr(2-x)Ce(x)CuO(4)

We measured the far infrared reflectivity of two superconducting Pr(2-x)Ce(x)CuO(4) films above and below Tc. The reflectivity in the superconducting state increases and the optical conductivity drops at low energies, in agreement with the opening of a (possibly) anisotropic superconducting gap. The maximum energy of the gap scales roughly with Tc as 2 Delta_{max} / kB Tc ~ 4.7. We determined absolute values of the penetration depth at 5 K as lambda_{ab} = (3300 +/- 700) A for x = 0.15 and lambda_{ab} = (2000 +/- 300) A for x = 0.17. A spectral weight analysis shows that the Ferrell-Glover-Tinkham sum rule is satisfied at conventional low energy scales \~ 4 Delta_{max}.

cond-mat.supr-con↗

arXiv2004

The in-plane electrodynamics of the superconductivity in Bi2Sr2CaCu2O8+d: energy scales and spectral weight distribution

The in-plane infrared and visible (3 meV-3 eV) reflectivity of Bi2Sr2CaCu2O8+d (Bi-2212) thin films is measured between 300 K and 10 K for different doping levels with unprecedented accuracy. The optical conductivity is derived through an accurate fitting procedure. We study the transfer of spectral weight from finite energy into the superfluid as the system becomes superconducting. In the over-doped regime, the superfluid develops at the expense of states lying below 60 meV, a conventional energy of the order of a few times the superconducting gap. In the underdoped regime, spectral weight is removed from up to 2 eV, far beyond any conventional scale. The intraband spectral weight change between the normal and superconducting state, if analyzed in terms of a change of kinetic energy is ~1 meV. Compared to the condensation energy, this figure addresses the issue of a kinetic energy driven mechanism.

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arXiv2004

Optical properties of (Pr,Ce)2CuO4

We studied the optical conductivity of electron doped Pr{1-x)Ce(x)CuO(4) from the underdoped to the overdoped regime. The observation of low to high frequency spectral weight transfer reveals the presence of a gap, except in the overdoped regime. A Drude peak at all temperatures shows the partial nature of this gap. The close proximity of the doping at which the gap vanishes to the antiferromagnetic phase boundary leads us to assign this partial gap to a spin density wave.

cond-mat.supr-con↗

arXiv2004

Sum rules and energy scales in BiSrCaCuO

From very high accuracy reflectivity spectra, we have derived the optical conductivity and estimated the spectral weight up to various cut-off frequencies in underdoped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ (Bi-2212). We show that, when evaluating the optical spectral weight over the full conduction band (1 eV), the kinetic energy decreases in the superconducting state, unlike in conventional BCS superconductors. As a consequence, the Ferrell-Glover-Tinkham sum rule is not satisfied up to this energy scale. This stands as a very unconventional behavior, contrasted with the overdoped Bi-2212 sample.

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arXiv2001

Pairing in cuprates from high energy electronic states

The in-plane optical conductivity of Bi2Sr2CaCu2O8+d thin films with small carrier density (underdoped) up to large carrier density (overdoped) is analyzed with unprecedented accuracy. Integrating the conductivity up to increasingly higher energies points to the energy scale involved when the superfluid condensate builds up. In the underdoped sample, states extending up to 2 eV contribute to the superfluid. This anomalously large energy scale may be assigned to a change of in-plane kinetic energy at the superconducting transition, and is compatible with an electronic pairing mechanism.

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arXiv2001

Absence of a pseudogap in the in-plane infrared response of Bi2Sr2CaCu2O(8+d)

The ab-plane reflectance of Bi2Sr2CaCu2O(8+d) thin films was measured in the 30-25000 cm^(-1) range for one underdoped (Tc = 70 K), and one overdoped sample (Tc = 63 K) as a function of temperature (10-300 K). We find qualitatively similar behaviors in the temperature dependence of the normal-state infrared response of both samples. Above Tc, the effective spectral weight, obtained from the integrated conductivity, does not decrease when T decreases, so that no opening of an optical pseudogap is seen. We suggest that these are consequences of the pseudogap opening first in the k=(0, pi) direction, according to ARPES, and of the in-plane infrared conductivity being mostly sensitive to the k=(pi, pi) direction.

cond-mat.supr-con↗

arXiv2001

Localization by disorder in the infrared conductivity of (Y,Pr)Ba2Cu3O7 films

The ab-plane reflectivity of (Y{1-x}Prx)Ba2Cu3O7 thin films was measured in the 30-30000 cm-1 range for samples with x = 0 (Tc = 90 K), x = 0.4 (Tc = 35 K) and x = 0.5 (Tc = 19 K) as a function of temperature in the normal state. The effective charge density obtained from the integrated spectral weight decreases with increasing x. The variation is consistent with the higher dc resistivity for x = 0.4, but is one order of magnitude smaller than what would be expected for x = 0.5. In the latter sample, the conductivity is dominated at all temperatures by a large localization peak. Its magnitude increases as the temperature decreases. We relate this peak to the dc resistivity enhancement. A simple localization-by-disorder model accounts for the optical conductivity of the x = 0.5 sample.

cond-mat.supr-con↗

arXiv2000

Triple approach to determination of the c-axis penetration depth in BSCCO crystals

The c-axis penetration depth $λ_c$ in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ (BSCCO) single crystals as a function of temperature has been determined using three high-frequency techniques, namely: (i) measurements of the ac-susceptibility at a frequency of 100 kHz for different sample alignments with respect to the ac magnetic field; (ii) measurements of the surface impedance in both superconducting and normal states of BSCCO crystals at 9.4 GHz; (iii) measurements of the surface barrier field $H_J(T)\propto 1/λ_c(T)$ at which Josephson vortices penetrate into the sample. Careful analysis of these measurements, including both numerical solution of the electrodynamic problem of the magnetic field distribution in an anisotropic plate at an arbitrary temperature and influence of defects in the sample, has allowed us to estimate $λ_c(0)\approx 50 μ$m in BSCCO crystals overdoped with oxygen ($T_c\approx 84$ K) and $λ_c(0)\approx 150 μ$m at the optimal doping level ($T_c\approx 90$ K). The results obtained by different techniques are in reasonable agreement.

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arXiv2000

Penetration of Josephson vortices and measurement of the c-axis penetration depth in $Bi_{2}Sr_{2}CaCu_{2}O_{8+δ}$: Interplay of Josephson coupling, surface barrier and defects

The first penetration field H_{J}(T) of Josephson vortices is measured through the onset of microwave absorption in the locked state, in slightly overdoped $\rm{Bi_{2}Sr_{2}CaCu_{2}O_{8+δ}}$ single crystals (T_{c} ~ 84 K). The magnitude of H_{J}(T) is too large to be accounted for by the first thermodynamic critical field H_{c1}(T). We discuss the possibility of a Bean-Livingston barrier, also supported by irreversible behavior upon flux exit, and the role of defects, which relates H_{J}(T) to the c-axis penetration depth $λ_{c}(T)$. The temperature dependence of the latter, determined by a cavity perturbation technique and a theoretical estimate of the defect-limited penetration field are used to deduce from H_{J}(T) the absolute value of $λ_{c}(0)=(35 \pm 15) μm$.

cond-mat.supr-con↗

arXiv2000

c-axis penetration depth in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ single crystals measured by ac-susceptibility and cavity perturbation technique

The $c$-axis penetration depth $Δλ_c$ in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ (BSCCO) single crystals as a function of temperature has been determined using two techniques, namely, measurements of the ac-susceptibility at a frequency of 100 kHz and the surface impedance at 9.4 GHz. Both techniques yield an almost linear function $Δλ_c(T)\propto T$ in the temperature range T<0.5 T_c. Electrodynamic analysis of the impedance anisotropy has allowed us to estimate $λ_c(0)\approx 50 μ$m in BSCCO crystals overdoped with oxygen ($T_c\approx 84$ K) and $λ_c(0)\approx 150 μ$m at the optimal doping level ($T_c\approx 90$ K).

cond-mat.supr-con↗

arXiv2000

Microwave Induced Instability Observed in BSCCO 2212 in a Static Magnetic Field

We have measured the microwave dissipation at 10 GHz through the imaginary part of the susceptibility, $χ^"$, in a BSCCO 2212 single crystal in an external static magnetic field $H$ parallel to the c-axis at various fixed temperatures. The characteristics of $χ^"(H)$ exhibit a sharp step at a field $H_{step}$ which strongly depends on the amplitude of the microwave excitation $h_{ac}$. The characteristics of $h_{ac}$ vs. $H_{step}$, qualitatively reveal the behavior expected for the magnetic field dependence of Josephson coupling.

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arXiv1998

Onset of decoupling at the melting field of the vortex lattice in Bi2Sr2CaCu2O8 from microwave dissipation

We have measured the microwave dissipation at 10 GHz in a Bi2Sr2CaCu2O8 single crystal, between 75 and 50 K, as a function of the static magnetic field applied parallel to the c axis. We observe a clear-cut onset in the dissipation precisely at the melting field Hm(T), that we identify in the same sample by a step in the static magnetization. We show that this onset can be assigned to the c-axis resistivity becoming finite in our whole temperature range, whereas the in-plane resistivity displays a thermally activated behavior. This suggests that pinning is efficient even at 10 GHz. The normal state dissipation is recovered at field much higher than the melting field, implying that decoupling develops mostly gradually over a large field range.

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arXiv1998

Electronic Raman scattering in HgBa_{2}Ca_{2}Cu_{3}O_{8+δ} single crystals. Analysis of the superconducting state

Electronic Raman scattering measurements have been performed on $HgBa_{2}Ca_{2}Cu_{3}O_{8+δ} $ single crystals in the superconducting state. Pure electronic Raman spectra with no phonon structures hindering the analysis of the electronic continuum have been obtained. As a consequence, the spectra in the pure $B_{1g} $ and $B_{2g} $ symmetries are directly and reliably analyzed and the pure $A_{1g} $ contribution can be easily identified. Below the critical temperature $T_{c}, $ two electronic structures at $2Δ\sim 6.4 k_{B}T_{c} $ and $2Δ\sim 9.4 $ $k_{B}T_{c} $ are clearly seen. Both are observed simultaneously in pure $A_{1g} $ symmetry, the highest energy one being located at the energy of the $B_{1g} $ maximum. These two maxima disappear at $T_{c} $ and do not soften significantly as the temperature is raised up to $T_{c}. $ The low energy frequency dependence of the $B_{1g} $ electronic response is strongly linear, for various excitation lines in the 476.5 to 647.1 nm range. Such experimental data cannot be reconciled with a pure $d_{x^{2}-y^{2}} $ symmetry. Instead, they strongly advocate in favor of an anisotropic superconducting gap with two distinct gap maxima and of nodes existing outside the [110] and [1,$\bar{1}$,0] directions in {\bf k}-space. We discuss in detail the simplest order parameter compatible with our experimental findings.

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