arXiv subjects

N. D. Lanzillotti-Kimura

Publications and source records attributed to N. D. Lanzillotti-Kimura.

At least 19 recordsLinked to original sources

arXiv2026

GaAs/AlAs Acoustic Nanocavities for Coherent GHz-THz Phonon Engineering

The controlled confinement of high-frequency acoustic phonons in semiconductor nanostructures has emerged as a key ingredient for functional nanophononic and hybrid quantum technologies. In this Review, we summarize recent advances that have established GaAs/AlAs acoustic nanocavities as a versatile and scalable platform for GHz-THz phonon engineering. Compared with alternative nanophononic platforms, GaAs/AlAs offers a particularly favorable combination of mature epitaxial growth, strong photoelastic coupling, and simultaneous optical-acoustic mode colocalization across the GHz-THz regime. We focus on distributed Bragg reflector (DBR)-based architectures, with particular emphasis on micropillar resonators enabling three-dimensional phonon confinement and strong colocalization of acoustic and optical fields. Recent developments in ultrafast optical techniques, including picosecond ultrasonics and Brillouin scattering, have provided unprecedented access to phonon dynamics, coherence, and dissipation at the nanoscale. These advances, combined with strong optophononic coupling, have enabled efficient coherent generation, detection, and manipulation of confined acoustic modes. We discuss key performance metrics, integration strategies, and remaining challenges, notably in acousto-optic transduction efficiency and scalable electrical control. Finally, we outline near-term perspectives for nonlinear phononics, hybrid quantum systems, and integrated phononic circuits, positioning GaAs/AlAs heterostructures as a robust and scalable platform for next-generation nanophononic functionalities.

cond-mat.mes-hall↗

arXiv2026

Open Nanoacoustic Resonators Based on SrTiO$_3$/YBa$_2$Cu$_3$O$_{7-x}$ Superlattices

We report the design and experimental demonstration of an open nanophononic cavity based on a hybrid oxide superlattice composed of SrTiO$_3$ (STO) and YBa$_2$Cu$_3$O$_{7-x}$ (YBCO), combined with a metallic Ni transducer for coherent phonon generation. The STO/YBCO periodic stack acts as an acoustic distributed Bragg reflector supporting confined longitudinal acoustic phonons in the sub-THz regime, while the Ni layer enables efficient ultrafast optical excitation and detection by time-domain Brillouin scattering. Transient reflectivity measurements reveal confined acoustic dynamics and a well-defined cavity resonance, in agreement with transfer-matrix calculations of acoustic reflectivity and mode profiles. These results demonstrate phonon confinement in multifunctional oxide heterostructures and establish complex oxide superlattices as a platform for hybrid nano-acoustic resonators and ultrafast phonon control of correlated electronic phases.

cond-mat.mes-hall↗

arXiv2026

Coupled Topological Interface States and Phonon Molecules in GaAs/AlAs Superlattices

Topological interface states in one-dimensional superlattices provide spatially localized phonon modes protected by the topology of the underlying band structure. In GaAs/AlAs distributed Bragg reflectors (DBRs), such states can be engineered through band inversion between superlattices with opposite Zak phases within the Su-Schrieffer-Heeger (SSH) framework. Here, we demonstrate topological phonon molecules and extended chains formed by coupled nanophononic interface states. By concatenating three superlattices with alternating topology, we realize two coupled interface states that hybridize into symmetric and antisymmetric modes, whose splitting can be tuned over tens of gigahertz by varying the reflectivity of the central DBR. Extending this concept, we engineer chains of up to N=6 coupled interface states that form narrow topological minibands while remaining strongly localized at the interfaces. We experimentally observe these coupled states in molecular-beam-epitaxy-grown GaAs/AlAs heterostructures using time-domain pump-probe transient reflectivity measurements, and reproduce their behavior using transfer-matrix calculations and a simple analytical model for the mode splitting. These results establish topological interface states as a robust platform for engineering coupled phononic systems and tunable nanophononic architectures in the GHz regime.

cond-mat.mes-hall↗

arXiv2025

Structural, magnetic, and nanoacoustic characterization of Co/Pt superlattices

Superlattices presenting a spatial modulation of the elastic properties appear as a main tool to reach the THz regime in nanoacoustic devices. The exploration of alternative materials with multifunctional properties remains a fertile domain of research. In this work, we study the structural, magnetic, and acoustic characteristics of nanometric superlattices made of Pt/Co. The samples present a well defined periodicity, as determined by X-ray reflectometry, whereas scanning transmission electron microscopy with local compositional analysis reveals that the superlattices present a modulation in composition instead of sharp interfaces. The policrystalline nature of the superlattices is evidenced both by X ray diffraction and transmission electron microscopy. Magnetization measurements show a perpendicular magnetic anisotropy for the higher Co concentrations. Picosecond acoustic experiments evidence that the studied samples support short-lived acoustic modes up to 900 GHz, and up to 7 acoustic echoes at lower frequencies.These are promising results for the development of magnetoacoustic devices working at ultrahigh frequencies.

cond-mat.mtrl-sci↗

arXiv2024

Coupled acoustoplasmonic resonators: the role of geometrical symmetries

Acoustoplasmonic resonators, such as nanobars and crosses, are efficient acousto-optical transducers. The excitation of mechanical modes in these structures strongly depends on the spatial profile of the eigenmodes of the resonator. Using a system of two identical gold elongated bars placed on a silicon dioxide substrate, we examine how breaking mirror symmetries affects the optical and acoustic properties to provide insights in the design of acoustoplasmonic metasurfaces for nonsymmetric acousto-optical transducers. Our findings show that, the absence of mirror symmetries affects differently the optical and nanomechanical response. Broken mirror symmetries not only couple nanomechanical modes existing in single bars, but introduces new torsional resonant modes.

physics.optics↗

arXiv2024

Interference of ultrahigh frequency acoustic phonons from distant quasi-continuous sources

The generation of propagating acoustic waves is essential for telecommunication applications, quantum technologies, and sensing. Up to now, the electrical generation has been at the core of most implementations, but is technologically limited to a few gigahertz. Overcoming this frequency limit holds the prospect of faster modulators, quantum acoustics at higher working temperatures, nanoacoustic sensing from smaller volumes. Alternatively, the optical excitation of acoustic resonators has unlocked frequencies up to 1 THz, but in most cases, the acoustic energy cannot be efficiently extracted from the resonator into a propagating wave. Here, we demonstrate a quasi-continuous and coherent source of 20 GHz acoustic phonons, based on a ridge waveguide, structured in the vertical direction as a high-Q acousto-optic resonator. The high frequency phonons propagate up to 20 $μ$m away from the source, with a decay rate of $\sim$1.14 dB/$μ$m. We demonstrate the coherence between acoustic phonons generated from two distant sources through spatio-temporal interference. This concept could be scaled up to a larger number of sources, which enable a new generation of optically programmed, reconfigurable nanoacoustic devices and applications.

cond-mat.mes-hall↗

arXiv2023

Towards chiral acoustoplasmonics

The possibility of creating and manipulating nanostructured materials encouraged the exploration of new strategies to control electromagnetic properties. Among the most intriguing nanostructures are those that respond differently to helical polarization, i.e., exhibit chirality. Here, we present a simple structure based on crossed elongated bars where light-handedness defines the dominating cross-section absorption or scattering, with a 200% difference from its counterpart (scattering or absorption). The proposed chiral system opens the way to enhanced coherent phonon excitation and detection. We theoretically propose a simple coherent phonon generation (time-resolved Brillouin scattering) experiment using circularly polarized light. In the reported structures, the generation of acoustic phonons is optimized by maximizing the absorption, while the detection is enhanced at the same wavelength -- and different helicity -- by engineering the scattering properties. The presented results constitute one of the first steps towards harvesting chirality effects in the design and optimization of efficient and versatile acoustoplasmonic transducers.

physics.optics↗

arXiv2022

Probing Gigahertz Coherent Acoustic Phonons in TiO$_{2}$ Mesoporous Thin Films

Ultrahigh-frequency acoustic-phonon resonators usually require atomically flat interfaces to avoid phonon scattering and dephasing, leading to expensive fabrication processes, such as molecular beam epitaxy. In contrast, mesoporous thin films are based on inexpensive wet chemical fabrication techniques. Here, we report mesoporous titanium dioxide-based acoustic resonators with resonances up to 90 GHz, and quality factors from 3 to 7. Numerical simulations show a good agreement with the picosecond ultrasonics experiments. We also numerically study the effect of changes in the speed of sound on the performance of the resonator. This change could be induced by liquid infiltration into the mesopores. Our findings constitute the first step towards the engineering of building blocks based on mesoporous thin films for reconfigurable optoacoustic sensors.

cond-mat.mes-hall↗

arXiv2022

Surface acoustic wave lasing in a silicon optomechanical cavity

Integrated optomechanical cavities stand as a promising means to interface mechanical motion and guided optical modes. State-of-the-art demonstrations rely on optical and mechanical modes tightly confined of in micron-scale areas to achieve strong optomechanical coupling. However, the need for tight optomechanical confinement and the general use of suspended devices hinders interaction with external devices, limiting the potential for the implementation of complex circuits. Here, we propose and demonstrate a new approach for optomechanical cavities coupling free-propagating surface acoustic waves (SAWs) and guided optical modes. The cavity is formed by a periodic array of silicon nanopillars with subwavelength separation, implemented in silicon-on-insulator substrate. Optical pumping yields a strong radiation pressure that drives the harmonic vibration of the pillars, periodically deforming the silica under-cladding and exciting the SAW. The propagation of the SAW deforms the cavity period, modulating the resonance wavelength to close the optomechanical coupling loop. Based on this concept, we experimentally demonstrate a phonon laser at room temperature and ambient conditions with optical pump power as low as 1 mW. We also show the possibility to cascade this process, achieving a frequency comb generation with more than 30 harmonic lines. These results open a new path to achieve strong bidirectional coupling between integrated waveguides and SAW, with a great potential for a wide range of applications in quantum and classical domains.

physics.optics↗

arXiv2021

Three-dimensional electrical control of the excitonic fine structure for a quantum dot in a cavity

The excitonic fine structure plays a key role for the quantum light generated by semiconductor quantum dots, both for entangled photon pairs and single photons. Controlling the excitonic fine structure has been demonstrated using electric, magnetic, or strain fields, but not for quantum dots in optical cavities, a key requirement to obtain high source efficiency and near-unity photon indistinguishability. Here, we demonstrate the control of the fine structure splitting for quantum dots embedded in micropillar cavities. We propose a scheme based on remote electrical contacts connected to the pillar cavity through narrow ridges. Numerical simulations show that such a geometry allows for a three-dimensional control of the electrical field. We experimentally demonstrate tuning and reproducible canceling of the fine structure, a crucial step for the reproducibility of quantum light source technology.

quant-ph↗

arXiv2020

Fiber-based angular filtering for high-resolution Brillouin spectroscopy in the 20-300 GHz frequency range

Brillouin spectroscopy emerges as a promising non-invasive tool for nanoscale imaging and sensing. One-dimensional semiconductor superlattice structures are eminently used for selectively enhancing the generation or detection of phonons at few GHz. While commercially available Brillouin spectrometers provide high-resolution spectra, they consist of complex experimental techniques and are not suitable for semiconductor cavities operating at a wide range of optical wavelengths. We develop a pragmatic experimental approach for conventional Brillouin spectroscopy integrating a widely tunable excitation-source. Our setup combines a fibered-based angular filtering and a spectral filtering based on a single etalon and a double grating spectrometer. This configuration allows probing confined acoustic phonon modes in the 20-300 GHz frequency range with excellent laser rejection and high spectral resolution. Remarkably, our scheme based on the excitation and collection of the enhanced Brillouin scattering signals through the optical cavity, allows for better angular filtering for low phonon frequency. It can be implemented for the study of cavity optomechanics and stimulated Brillouin scattering over broadband optical and acoustic frequency ranges.

physics.optics↗

arXiv2020

Fiber-integrated microcavities for efficient generation of coherent acoustic phonons

Coherent phonon generation by optical pump-probe experiments has enabled the study of acoustic properties at the nanoscale in planar heterostructures, plasmonic resonators, micropillars and nanowires. Focalizing both pump and probe on the same spot of the sample is a critical part of pump-probe experiments. This is particularly relevant in the case of small objects. The main practical challenges for the actual implementation of this technique are: stability of the spatio-temporal overlap, reproducibility of the focalization and optical mode matching conditions. In this work, we solve these three challenges for the case of planar and micropillar optophononic cavities. We integrate the studied samples to single mode fibers lifting the need for focusing optics to excite and detect coherent acoustic phonons. The resulting excellent reflectivity contrast of at least 66% achieved in our samples allows us to observe stable coherent phonon signals over at least a full day and signals at extremely low excitation powers of 1uW. The monolithic sample structure is transportable and could provide a means to perform reproducible plug-and-play experiments.

physics.optics↗

arXiv2020

Topological optical and phononic interface mode by simultaneous band inversion

Interface modes have been widely explored in the field of electronics, optics, acoustics and nanophononics. One strategy to generate them is band inversion in one-dimensional superlattices. Most realizations of this type of topological states have so far been explored for a single kind of excitation. Despite its potential in the manipulation and engineering of interactions, platforms for the simultaneous topological confinement of multiple excitations remain an open challenge. GaAs/AlAs heterostructures exhibit enhanced optomechanical interactions due to the intrinsic colocalization of light and sound. In this work, we designed, fabricated, and experimentally studied a multilayered structure based on GaAs/AlAs. Due to the simultaneously inverted band structures for light and phonons, colocalized interface modes for both 1.34 eV photons and 18 GHz phonons appear. We experimentally validated the concept by optical reflectivity and coherent phonon generation and detection. Furthermore, we theoretically analyzed the performance of different topological designs presenting colocalized states in time-domain Brillouin scattering and deduce engineering rules. Potential future applications include the engineering of robust optomechanical resonators, compatible with the incorporation of active media such as quantum wells and quantum dots.

cond-mat.mes-hall↗

arXiv2020

Mesoporous Thin-Films for Acoustic Devices in the Gigahertz Range

The coherent manipulation of acoustic waves on the nanoscale usually requires multilayers with thicknesses and interface roughness defined down to the atomic monolayer. This results in expensive devices with predetermined functionality. Nanoscale mesoporous materials present high surface-to-volume ratio and tailorable mesopores, which allow the incorporation of chemical functionalization to nanoacoustics. However, the presence of pores with sizes comparable to the acoustic wavelength is intuitively perceived as a major roadblock in nanoacoustics. Here we present multilayered nanoacoustic resonators based on mesoporous SiO$_2$ thin-films showing acoustic resonances in the 5-100 GHz range. We characterize the acoustic response of the system using coherent phonon generation experiments. Despite resonance wavelengths comparable to the pore size, we observe for the first time unexpectedly well-defined acoustic resonances with Q-factors around 10. Our results open the path to a promising platform for nanoacoustic sensing and reconfigurable acoustic nanodevices based on soft, inexpensive fabrication methods.

physics.app-ph↗

arXiv2019

Phonon engineering with superlattices: generalized nanomechanical potentials

Earlier implementations to simulate coherent wave propagation in one-dimensional potentials using acoustic phonons with gigahertz-terahertz frequencies were based on coupled nanoacoustic resonators. Here, we generalize the concept of adiabatic tuning of periodic superlattices for the implementation of effective one-dimensional potentials giving access to cases that cannot be realized by previously reported phonon engineering approaches, in particular the acoustic simulation of electrons and holes in a quantum well or a double well potential. In addition, the resulting structures are much more compact and hence experimentally feasible. We demonstrate that potential landscapes can be tailored with great versatility in these multilayered devices, apply this general method to the cases of parabolic, Morse and double-well potentials and study the resulting stationary phonon modes. The phonon cavities and potentials presented in this work could be probed by all-optical techniques like pump-probe coherent phonon generation and Brillouin scattering.

cond-mat.mes-hall↗

arXiv2018

Brillouin Scattering in Hybrid Optophononic Bragg Micropillar Resonators at 300 GHz

We introduce a monolithic Brillouin generator based on a semiconductor micropillar cavity embedding a high frequency nanoacoustic resonator operating in the hundreds of GHz range. The concept of two nested resonators allows an independent design of the ultrahigh frequency Brillouin spectrum and of the optical device. We develop an optical free-space technique to characterize spontaneous Brillouin scattering in this monolithic device and propose a measurement protocol that maximizes the Brillouin generation efficiency in the presence of optically induced thermal effects. The compact and versatile Brillouin generator studied here could be readily integrated into fibered and on-chip architectures.

physics.optics↗

arXiv2018

Coherent generation and detection of acoustic phonons in topological nanocavities

Inspired by concepts developed for fermionic systems in the framework of condensed matter physics, topology and topological states are recently being explored also in bosonic systems. The possibility of engineering systems with unidirectional wave propagation and protected against disorder is at the heart of this growing interest. Topogical acoustic effects have been observed in a variety of systems, most of them based on kHz-MHz sound waves, with typical wavelength of the order of the centimeter. Recently, some of these concepts have been successfully transferred to acoustic phonons in nanoscaled multilayered systems. The reported demonstration of confined topological phononic modes was based on Raman scattering spectroscopy, yet the resolution did not suffice to determine lifetimes and to identify other acoustic modes in the system. Here, we use time-resolved pump-probe measurements using an asynchronous optical sampling (ASOPS) technique to overcome these resolution limitations. By means of one-dimensional GaAs/AlAs distributed Bragg reflectors (DBRs) as building blocks, we engineer high frequency ($\sim$ 200 GHz) topological acoustic interface states. We are able to clearly distinguish confined topological states from stationary band edge modes. The detection scheme reflects the symmetry of the modes directly through the selection rules, evidencing the topological nature of the measured confined state. These experiments enable a new tool in the study of the more complex topology-driven phonon dynamics such as phonon nonlinearities and optomechanical systems with simultaneous confinement of light and sound.

cond-mat.mes-hall↗

arXiv2018

Polarization-Controlled Coherent Phonon Generation in Acousto-Plasmonic Metasurfaces

Acoustic vibrations at the nanoscale (GHz-THz frequencies) and their interactions with electrons, photons and other excitations are the heart of an emerging field in physics: nanophononics. The design of ultrahigh frequency acoustic-phonon transducers, with tunable frequency, and easy to integrate in complex systems is still an open and challenging problem for the development of acoustic nanoscopies and phonon lasers. Here we show how an optimized plasmonic metasurface can act as a high-frequency phonon transducer. We report pump-probe experiments in metasurfaces composed of an array of gold nanostructures, revealing that such arrays can act as efficient and tunable photon-phonon transducers, with a strong spectral dependence on the excitation rate and laser polarization. We anticipate our work to be the starting point for the engineering of phononic metasurfaces based on plasmonic nanostructures.

cond-mat.mes-hall↗