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N. D. Scielzo

Publications and source records attributed to N. D. Scielzo.

At least 19 recordsLinked to original sources

Exploration for Astromers near $^{132}$Sn with the Canadian Penning Trap

Nuclear isomers can have significant impacts on astrophysical nucleosynthesis processes, with recent efforts demonstrating that the population of isomeric states with different half-lives may require separate treatment in reaction networks to accurately capture the differences in heating or in identifiable electromagnetic signals. Several potential so-called ``astromers'' in tin and antimony isotopes near doubly-magic $^{132}$Sn were identified and direct mass measurements of their ground and isomeric states were performed with the Canadian Penning Trap at Argonne National Laboratory's CARIBU facility, and their impact on astrophysical reaction rates and in reaction networks calculated. It was found that $^{129g,m}$Sn, with measured mass excesses of $-80 593.2(25)$ keV and $-80 557.4(25)$ keV, respectively, and an excitation energy of $35.8(35)$ keV, behaves as an astromer during neutron capture in the $i$-process and in the $r$-process.

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Beta-decay Half Lives beyond $^{54}$Ca: A Systematic Survey of Decay Properties approaching the Neutron Dripline

In an experiment performed at the Facility for Rare Isotope Beams (FRIB) using the FRIB Decay Station initiator (FDSi), 15 new half lives of isotopes near $^{54}$Ca were measured. A new method of extracting lifetimes from experimental data, taking into account the unknown $β$-delayed neutron emission branches of very neutron-rich nuclei, was developed to enable systematic uncertainty analysis. The experiment observed a dramatic change in the half-life systematics for the isotopes with neutron number N =34. Beyond N =34, the decline of nuclear lifetime is much slower, leading to longer than anticipated lifetimes for near-dripline nuclei. State-of-the-art shell-model calculations can explain the experimental results for Z$>$19 nuclei, revealing the imprint of shell effects and the need for modification of single-particle neutron states. The results from a newly developed QRPA model with potential for making global predictions were also tested against the experimental results and good agreement was found.

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Universal Effective Charges in the $sd$ and $fp$ Shells

The 247-keV state in $^{54}$Sc, populated in the $β$ decay of $^{54}$Ca, is reported here as a nanosecond isomer with a half-life of 26.0(22) ns. The state is interpreted as the $1^+$ member of the $πf_{7/2}\otimesνf_{5/2}$ spin-coupled multiplet, which decays to the $3^+,πf_{7/2} \otimes νp_{1/2}$ ground state. The new half-life corresponds to a pure $E2$ transition with a strength of 1.93(16) W.u., providing the most precise, unambiguous $B(E2)$ value in the neutron-rich $fp$ region to date for a nucleus with valence protons above $Z=20$. Notably, it is roughly four times larger than the $B(E2; 1/2^{-} \rightarrow 5/2^{-})$ value in $^{55}$Ca. The results, as compared to semi-empirical and ab initio shell-model calculations, indicate (1) a weak $N=34$ sub-shell gap relative to $N = 32$, (2) a large $E2$ enhancement in Sc as compared to Ca due to $1p-1h$ proton excitations across $Z=28$, and (3) empirical effective proton and neutron charges, $e_π$ = 1.30(8)$e$ and $e_ν$ = 0.452(7)$e$, respectively, that are in contrast to reports of $e_π\approx 1.1-1.15e$ and $e_ν\approx 0.6-0.8e$ for $fp$-shell nuclei near $N = Z$. We demonstrate that these reports are erroneous and that, in fact, a universal set of effective charges can be used across the $sd$ and $fp$ shells.

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Mass measurements of neutron-rich nuclides using the Canadian Penning Trap to inform predictions in the $r$-process rare-earth peak region

Studies aiming to determine the astrophysical origins of nuclei produced by the rapid neutron capture process ($r$ process) rely on nuclear properties as inputs for simulations. The solar abundances can be used as a benchmark for such calculations, with the $r$-process rare-earth peak (REP) around mass number ($A$) 164 being of special interest due to its presently unknown origin. With the advancement of rare isotope beam production over the last decade and improvement in experimental sensitivities, many of these REP nuclides have become accessible for measurement. Masses are one of the most critical inputs as they impact multiple nuclear properties, namely the neutron-separation energies, neutron capture rates, $β$-decay rates, and $β$-delayed neutron emission probabilities. In this work, we report masses of 20 neutron-rich nuclides (along the Ba, La, Ce, Pr, Nd, Pm, Gd, Dy and Ho isotopic chains) produced at the CAlifornium Rare Isotope Breeder Upgrade (CARIBU) facility at Argonne National Laboratory. The masses were measured with the Canadian Penning trap (CPT) mass spectrometer using the Phase-Imaging Ion-Cyclotron-Resonance (PI-ICR) technique. We then use these new masses along with previously published CPT masses to inform predictions for a Markov Chain Monte Carlo (MCMC) procedure aiming to identify the astrophysical conditions consistent with both solar data and mass measurements. We show that the MCMC responds to this updated mass information, producing refined results for both mass predictions and REP abundances.

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On the half life of $^{71}$Ge and the Gallium Anomaly

Recent discussions about the origin of the Gallium Anomaly have motivated a remeasurement of the half life of $^{71}$Ge. We have conducted three separate measurements using dedicated planar Ge detectors: one with $^{55}$Fe as a standard, one with $^{57}$Co as a standard, and one stand alone 71Ge measurement. Our results yield a half life of 11.468 +- 0.008 days, which is consistent with but significantly more precise than the currently accepted value. With this experiment, the potential explanation of the Gallium Anomaly being due to an unexpectedly long $^{71}$Ge half life has been ruled out, leaving the origin of the anomaly as an open question.

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The Beta-decay Paul Trap Mk IV: Design and commissioning

The Beta-decay Paul Trap is an open-geometry, linear trap used to measure the decays of $^8$Li and $^8$B to search for a tensor contribution to the weak interaction. In the latest $^8$Li measurement of Burkey et al. (2022), $β$ scattering was the dominant experimental systematic uncertainty. The Beta-decay Paul Trap Mk IV reduces the prevalence of $β$ scattering by a factor of 4 through a redesigned electrode geometry and the use of glassy carbon and graphite as electrode materials. The trap has been constructed and successfully commissioned with $^8$Li in a new data campaign that collected 2.6 million triple coincidence events, an increase in statistics by 30% with 4 times less $β$ scattering compared to the previous $^8$Li data set.

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Nuclear $β$ decay as a probe for physics beyond the Standard Model

This white paper was submitted to the 2022 Fundamental Symmetries, Neutrons, and Neutrinos (FSNN) Town Hall Meeting in preparation for the next NSAC Long Range Plan. We advocate to support current and future theoretical and experimental searches for physics beyond the Standard Model using nuclear $β$ decay.

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Impact of clustering on the $^8$Li $β$ decay and recoil form factors

We place unprecedented constraints on recoil corrections in the $β$ decay of $^8$Li, by identifying a strong correlation between them and the $^8$Li ground state quadrupole moment in large-scale ab initio calculations. The results are essential for improving the sensitivity of high-precision experiments that probe the weak interaction theory and test physics beyond the Standard Model (BSM). In addition, our calculations predict a $2^+$ state of the $α+α$ system that is energetically accessible to $β$ decay but has not been observed in the experimental $^8$Be energy spectrum, and has an important effect on the recoil corrections and $β$ decay for the $A=8$ systems. This state and an associated $0^+$ state are notoriously difficult to model due to their cluster structure and collective correlations, but become feasible for calculations in the ab initio symmetry-adapted no-core shell-model framework.

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Improved Limit on Tensor Currents in the Weak Interaction from $^8$Li $β$ Decay

The electroweak interaction in the Standard Model (SM) is described by a pure vector-axial-vector structure, though any Lorentz-invariant component could contribute. In this work, we present the most precise measurement of tensor currents in the low-energy regime by examining the $β$-$\barν$ correlation of trapped $^{8}$Li ions with the Beta-decay Paul Trap. We find $a_{βν} = -0.3325 \pm 0.0013_{stat} \pm 0.0019_{syst}$ at $1σ$ for the case of coupling to right-handed neutrinos $(C_T=-C_T')$, which is consistent with the SM prediction.

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Search for Majorana neutrinos exploiting millikelvin cryogenics with CUORE

The possibility that neutrinos may be their own antiparticles, unique among the known fundamental particles, arises from the symmetric theory of fermions proposed by Ettore Majorana in 1937. Given the profound consequences of such Majorana neutrinos, among which is a potential explanation for the matter-antimatter asymmetry of the universe via leptogenesis, the Majorana nature of neutrinos commands intense experimental scrutiny globally; one of the primary experimental probes is neutrinoless double beta ($0 νββ$) decay. Here we show results from the search for $0 νββ$ decay of $^{130}$Te, using the latest advanced cryogenic calorimeters with the CUORE experiment. CUORE, operating just 10 millikelvin above absolute zero, has pushed the state of the art on three frontiers: the sheer mass held at such ultra-low temperatures, operational longevity, and the low levels of ionising radiation emanating from the cryogenic infrastructure. We find no evidence for $0 νββ$ decay and set a lower bound of $T_{1/2}^{0 ν} > 2.2 \times 10^{25}$ years at a 90% credibility interval. We discuss potential applications of the advances made with CUORE to other fields such as direct dark matter, neutrino and nuclear physics searches and large-scale quantum computing, which can benefit from sustained operation of large payloads in a low-radioactivity, ultra-low temperature cryogenic environment.

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Search for Double-Beta Decay of $\mathrm{^{130}Te}$ to the $0^+$ States of $\mathrm{^{130}Xe}$ with CUORE

The CUORE experiment is a large bolometric array searching for the lepton number violating neutrino-less double beta decay ($0νββ$) in the isotope $\mathrm{^{130}Te}$. In this work we present the latest results on two searches for the double beta decay (DBD) of $\mathrm{^{130}Te}$ to the first $0^{+}_2$ excited state of $\mathrm{^{130}Xe}$: the $0νββ$ decay and the Standard Model-allowed two-neutrinos double beta decay ($2νββ$). Both searches are based on a 372.5 kg$\times$yr TeO$_2$ exposure. The de-excitation gamma rays emitted by the excited Xe nucleus in the final state yield a unique signature, which can be searched for with low background by studying coincident events in two or more bolometers. The closely packed arrangement of the CUORE crystals constitutes a significant advantage in this regard. The median limit setting sensitivities at 90\% Credible Interval (C.I.) of the given searches were estimated as $\mathrm{S^{0ν}_{1/2} = 5.6 \times 10^{24} \: \mathrm{yr}}$ for the ${0νββ}$ decay and $\mathrm{S^{2ν}_{1/2} = 2.1 \times 10^{24} \: \mathrm{yr}}$ for the ${2νββ}$ decay. No significant evidence for either of the decay modes was observed and a Bayesian lower bound at $90\%$ C.I. on the decay half lives is obtained as: $\mathrm{(T_{1/2})^{0ν}_{0^+_2} > 5.9 \times 10^{24} \: \mathrm{yr}}$ for the $0νββ$ mode and $\mathrm{(T_{1/2})^{2ν}_{0^+_2} > 1.3 \times 10^{24} \: \mathrm{yr}}$ for the $2νββ$ mode. These represent the most stringent limits on the DBD of $^{130}$Te to excited states and improve by a factor $\sim5$ the previous results on this process.

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Measurement of the 2$νββ$ Decay Half-life of $^{130}$Te with CUORE

We measured two-neutrino double beta decay of $^{130}$Te using an exposure of 300.7 kg$\cdot$yr accumulated with the CUORE detector. Using a Bayesian analysis to fit simulated spectra to experimental data, it was possible to disentangle all the major background sources and precisely measure the two-neutrino contribution. The half-life is in agreement with past measurements with a strongly reduced uncertainty: $T^{2ν}_{1/2} = 7.71^{+0.08}_{-0.06}\mathrm{(stat.)}^{+0.12}_{-0.15}\mathrm{(syst.)}\times10^{20}$ yr. This measurement is the most precise determination of the $^{130}$Te 2$νββ$ decay half-life to date.

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Development of a Reference Database for Beta-Delayed Neutron Emission

Beta-delayed neutron emission is important for nuclear structure and astrophysics as well as for reactor applications. Significant advances in nuclear experimental techniques in the past two decades have led to a wealth of new measurements that remain to be incorporated in the databases. We report on a coordinated effort to compile and evaluate all the available beta-delayed neutron emission data. The different measurement techniques have been assessed and the data have been compared with semi-microscopic and microscopic-macroscopic models. The new microscopic database has been tested against aggregate total delayed neutron yields, time-dependent group parameters in 6-and 8-group re-presentation, and aggregate delayed neutron spectra. New recommendations of macroscopic delayed-neutron data for fissile materials of interest to applications are also presented. The new Reference Database for Beta-Delayed Neutron Emission Data is available online at: http://www-nds.iaea.org/beta-delayed-neutron/database.html.

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New results from the CUORE experiment

The Cryogenic Underground Observatory for Rare Events (CUORE) is the first cryogenic experiment searching for neutrinoless double-beta ($0νββ$) decay that has been able to reach the one-ton scale. The detector, located at the Laboratori Nazionali del Gran Sasso in Italy, consists of an array of 988 TeO$_2$ crystals arranged in a compact cylindrical structure of 19 towers. Following the completion of the detector construction in August 2016, CUORE began its first physics data run in 2017 at a base temperature of about 10 mK. Following multiple optimization campaigns in 2018, CUORE is currently in stable operating mode. In 2019, CUORE released its 2\textsuperscript{nd} result of the search for $0νββ$ with a TeO$_2$ exposure of 372.5 kg$\cdot$yr and a median exclusion sensitivity to a $^{130}$Te $0νββ$ decay half-life of $1.7\cdot 10^{25}$ yr. We find no evidence for $0νββ$ decay and set a 90\% C.I. (credibility interval) Bayesian lower limit of $3.2\cdot 10^{25}$ yr on the $^{130}$Te $0νββ$ decay half-life. In this work, we present the current status of CUORE's search for $0νββ$, as well as review the detector performance. Finally, we give an update of the CUORE background model and the measurement of the $^{130}$Te two neutrino double-beta ($2νββ$) decay half-life.

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Improved Limit on Neutrinoless Double-Beta Decay in $^{130}$Te with CUORE

We report new results from the search for neutrinoless double-beta decay in $^{130}$Te with the CUORE detector. This search benefits from a four-fold increase in exposure, lower trigger thresholds and analysis improvements relative to our previous results. We observe a background of $(1.38\pm0.07)\cdot10^{-2}$ counts$/($keV$\cdot$kg$\cdot$yr$)$ in the $0νββ$ decay region of interest and, with a total exposure of 372.5 kg$\cdot$yr, we attain a median exclusion sensitivity of $1.7\cdot10^{25}$ yr. We find no evidence for $0νββ$ decay and set a $90\%$ CI Bayesian lower limit of $3.2\cdot10^{25}$ yr on the $^{130}$Te half-life for this process. In the hypothesis that $0νββ$ decay is mediated by light Majorana neutrinos, this results in an upper limit on the effective Majorana mass of 75-350 meV, depending on the nuclear matrix elements used.

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Results of CUORE

The Cryogenic Underground Observatory for Rare Events (CUORE) at the Laboratori Nazionali del Gran Sasso, Italy, is the world's largest bolometric experiment. The detector consists of an array of 988 TeO2 crystals, for a total mass of 742 kg. CUORE is presently in data taking, searching for the neutrinoless double beta decay of 130 Te. CUORE is operational since the spring of 2017. The initial science run already allowed to provide the most stringent limit on the neutrinoless double beta decay half-life of 130Te, and to perform the most precise measurement of the two-neutrino double beta decay half-life. Up to date, we have more than doubled the collected exposure. In this talk, we presenteded the most recent results and discuss the present status of the CUORE experiment.

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Beta-delayed-neutron studies of $^{135,136}$Sb and $^{140}$I performed with trapped ions

Beta-delayed-neutron ($β$n) spectroscopy was performed using the Beta-decay Paul Trap and an array of radiation detectors. The $β$n branching ratios and energy spectra for $^{135,136}$Sb and $^{140}$I were obtained by measuring the time of flight of recoil ions emerging from the trapped ion cloud. These nuclei are located at the edge of an isotopic region identified as having $β$n branching ratios that impact the r-process abundance pattern around the A~130 peak. For $^{135,136}$Sb and $^{140}$I, $β$n branching ratios of 14.6(11)%, 17.6(28)%, and 7.6(28)% were determined, respectively. The $β$n energy spectra obtained for $^{135}$Sb and $^{140}$I are compared with results from direct neutron measurements, and the $β$n energy spectrum for $^{136}$Sb has been measured for the first time.

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Towards Neutron Capture on Exotic Nuclei: Demonstrating $(d,pγ)$ as a Surrogate Reaction for $(n,γ)$

The neutron-capture reaction plays a critical role in the synthesis of the elements in stars and is important for societal applications including nuclear power generation and stockpile-stewardship science. However, it is difficult - if not impossible - to directly measure neutron capture cross sections for the exotic, short-lived nuclei that participate in these processes. In this Letter we demonstrate a new technique which can be used to indirectly determine neutron-capture cross sections for exotic systems. This technique makes use of the $(d,p)$ transfer reaction, which has long been used as a tool to study the structure of nuclei. Recent advances in reaction theory, together with data collected using this reaction, enable the determination of neutron-capture cross sections for short-lived nuclei. A benchmark study of the $^{95}$Mo$(d,p)$ reaction is presented, which illustrates the approach and provides guidance for future applications of the method with short-lived isotopes produced at rare isotope accelerators.

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