arXiv subjects

N. Dauphas

Publications and source records attributed to N. Dauphas.

12 recordsLinked to original sources

arXiv2023

Science Priorities for the Extraction of the Solid MSR Samples from their Sample Tubes

Preservation of the chemical and structural integrity of samples that will be brought back from Mars is paramount to achieving the scientific objectives of MSR. Given our knowledge of the nature of the samples retrieved at Jezero by Perseverance, at least two options need to be tested for opening the sample tubes: (1) One or two radial cuts at the end of the tube to slide the sample out. (2) Two radial cuts at the ends of the tube and two longitudinal cuts to lift the upper half of the tube and access the sample. Strategy 1 will likely minimize contamination but incurs the risk of affecting the physical integrity of weakly consolidated samples. Strategy 2 will be optimal for preserving the physical integrity of the samples but increases the risk of contamination and mishandling of the sample as more manipulations and additional equipment will be needed. A flexible approach to opening the sample tubes is therefore required, and several options need to be available, depending on the nature of the rock samples returned. Both opening strategies 1 and 2 may need to be available when the samples are returned to handle different sample types (e.g., loosely bound sediments vs. indurated magmatic rocks). This question should be revisited after engineering tests are performed on analogue samples. The MSR sample tubes will have to be opened under stringent BSL4 conditions and this aspect needs to be integrated into the planning.

astro-ph.IM↗

arXiv2021

Terrestrial planet formation by torque-driven convergent migration of planetary embryos

Massive cores of the giant planets are thought to have formed in a gas disk by accretion of pebble-size particles whose accretional cross-section is enhanced by aerodynamic gas drag [1][2]. A commonly held view is that the terrestrial planet system formed later (30-200 Myr after the dispersal of the gas disk) by giant collisions of tens of roughly Mars-size protoplanets [3]. Here we propose, instead, that the terrestrial planets formed earlier by gas-driven convergent migration of protoplanets toward $\sim\!1\,{\rm au}$ (related ref. [4] invoked a different process to concentrate planetesimals). To investigate situations in which convergent migration occurs, we developed a radiation-hydrodynamic model with realistic opacities [5][6] to determine the thermal structure of the gas and pebble disks in the terrestrial planet zone. We find that protoplanets rapidly grow by mutual collisions and pebble accretion, and gain orbital eccentricities by gravitational scattering and the hot-trail effect [7][8]. The orbital structure of the terrestrial planet system is well reproduced in our simulations, including its tight mass concentration at 0.7-1 au and the small sizes of Mercury and Mars. The early-stage protosolar disk temperature exceeds 1500 K inside 0.4 au implying that Mercury grew in a highly reducing environment, next to the evaporation lines of iron and silicates, influencing Mercury's bulk composition [9]. In a late-stage cold gas disk, accretion of icy/hydrated pebbles would contribute to Earth's water budget.

astro-ph.EP↗

arXiv2019

Evidence of presolar SiC in the Allende Curious Marie calcium aluminum rich inclusion

Calcium aluminum rich inclusions (CAIs) are one of the first solids to have condensed in the solar nebula, while presolar grains formed in various evolved stellar environments. It is generally accepted that CAIs formed close to the Sun at temperatures above 1500 K, where presolar grains could not survive, and were then transported to other regions of the nebula where the accretion of planetesimals took place. In this context, a commonly held view is that presolar grains are found solely in the fine-grained rims surrounding chondrules and in the low-temperature fine-grained matrix that binds the various meteoritic components together. Here we demonstrate, based on noble gas isotopic signatures, that presolar SiC have been incorporated into fine-grained CAIs in the Allende carbonaceous chondrite at the time of their formation, and have survived parent body processing. This finding provides new clues on the conditions in the nascent solar system at the condensation of first solids.

astro-ph.EP↗

arXiv2018

Jupiter's influence on the building blocks of Mars and Earth

Radiometric dating indicates that Mars accreted in the first ~4 Myr of solar system formation, which coincides with the formation and possible migration of Jupiter. While nebular gas from the protoplanetary disk was still present, Jupiter may have migrated inwards and tacked at 1.5 AU in a 3:2 resonance with Saturn. This migration excited planetary building blocks in the inner solar system, resulting in extensive mixing and planetesimal removal. Here we evaluate the plausible nature of Mars' building blocks, focusing in particular on how its growth was influenced by the formation and migration of Jupiter. We use a combination of dynamical simulations and an isotopic mixing model that traces the accretion of elements with different affinities for metal. Dynamical simulations show that Jupiter's migration causes the late stages of Earth's and Mars' accretion to be dominated by EC-type (enstatite chondrite) material due to the loss of OC (ordinary chondrite) planetesimals. Our analysis of available isotopic data for SNC meteorites shows that Mars consists of approximately 68%$^{+0}_{-39}$ EC + 32%$^{+35}_{-0}$ OC by mass (2{\sigma}). The large uncertainties indicate that isotopic analyses of martian samples are for the most part too imprecise to definitely test model predictions; in particular it remains uncertain whether or not Mars accreted predominantly EC material in the latter stages of its formation history. Dynamical simulations also provide no definitive constraint on Mars' accretion history due to the great variety of dynamical pathways that the martian embryo exhibits. The present work calls for new measurements of isotopic anomalies in SNC meteorites targeting siderophile elements (most notably Ni, Mo and Ru) to constrain Mars' accretion history and its formation location.

astro-ph.EP↗

arXiv2015

Thulium anomalies and rare earth element patterns in meteorites and Earth: Nebular fractionation and the nugget effect

This study reports the bulk rare earth element (REEs, La-Lu) compositions of 41 chondrites, including 32 falls and 9 finds from carbonaceous (CI, CM, CO and CV), enstatite (EH and EL) and ordinary (H, L and LL) groups, as well as 2 enstatite achondrites (aubrite). The CI-chondrite-normalized REE patterns and Eu anomalies in ordinary and enstatite chondrites show more scatter in more metamorphosed than in unequilibrated chondrites. This is due to parent-body redistribution of the REEs in various carrier phases during metamorphism. The dispersion in REE patterns of equilibrated ordinary chondrites is explained by the nugget effect associated with concentration of REEs in minor phosphate grains. Terrestrial rocks and samples from ordinary and enstatite chondrites display negative Tm anomalies of ~-4.5 % relative to ca chondrites. In contrast, CM, CO and CV (except Allende) show no significant Tm anomalies. Allende CV chondrite shows large excess Tm (~+10 %). These anomalies are similar to those found in group II refractory inclusions in meteorites but of much smaller magnitude. The presence of Tm anomalies in meteorites and terrestrial rocks suggests that either (i) the material in the inner part of the solar system was formed from a gas reservoir that had been depleted in refractory dust and carried positive Tm anomalies or (ii) CI chondrites are enriched in refractory dust and are not representative of solar composition for refractory elements. The observed Tm anomalies in ordinary and enstatite chondrites and terrestrial rocks, relative to carbonaceous chondrites, indicate that material akin to carbonaceous chondrites must have represented a small fraction of the constituents of the Earth.

astro-ph.EP↗

arXiv2014

Radiogenic p-isotopes from SNIa, nuclear physics uncertainties and Galactic chemical evolution compared with values in primitive meteorites

The nucleosynthesis of proton-rich isotopes is calculated for multi-dimensional Chandrasekhar-mass models of Type Ia supernovae with different metallicities. The predicted abundances of the short-lived radioactive isotopes 92Nb, 97Tc, 98Tc and 146Sm are given in this framework. The abundance seeds are obtained by calculating s-process nucleosynthesis in the material accreted onto a carbon-oxygen white dwarf from a binary companion. A fine grid of s-seeds at different metallicities and 13C-pocket efficiencies is considered. A galactic chemical evolution model is used to predict the contribution of SNIa to the solar system p-nuclei composition measured in meteorites. Nuclear physics uncertainties are critical to determine the role of SNeIa in the production of 92Nb and 146Sm. We find that, if standard Chandrasekhar-mass SNeIa are at least 50% of all SNIa, they are strong candidates for reproducing the radiogenic p-process signature observed in meteorites.

astro-ph.SR↗

arXiv2013

Constraining the astrophysical origin of the p-nuclei through nuclear physics and meteoritic data

A small number of naturally occurring, proton-rich nuclides (the p-nuclei) cannot be made in the s- and r-process. Their origin is not well understood. Massive stars can produce p-nuclei through photodisintegration of pre-existing intermediate and heavy nuclei. This so-called gamma-process requires high stellar plasma temperatures and occurs mainly in explosive O/Ne burning during a core-collapse supernova. Although the gamma-process in massive stars has been successful in producing a large range of p-nuclei, significant deficiences remain. An increasing number of processes and sites has been studied in recent years in search of viable alternatives replacing or supplementing the massive star models. A large number of unstable nuclei, however, with only theoretically predicted reaction rates are included in the reaction network and thus the nuclear input may also bear considerable uncertainties. The current status of astrophysical models, nuclear input, and observational constraints is reviewed. After an overview of currently discussed models, the focus is on the possibility to better constrain those models through different means. Meteoritic data not only provide the actual isotopic abundances of the p-nuclei but can also put constraints on the possible contribution of proton-rich nucleosynthesis. The main part of the review focusses on the nuclear uncertainties involved in the determination of the astrophysical reaction rates required for the extended reaction networks used in nucleosynthesis studies. Experimental approaches are discussed together with their necessary connection to theory, which is especially pronounced for reactions with intermediate and heavy nuclei in explosive nuclear burning, even close to stability.

astro-ph.SR↗

arXiv2012

A general moment NRIXS approach to the determination of equilibrium Fe isotopic fractionation factors: application to goethite and jarosite

We measured the reduced partition function ratios for iron isotopes in goethite FeO(OH), potassium-jarosite KFe3(SO4)2(OH)6, and hydronium-jarosite (H3O)Fe3(SO4)2(OH)6, by Nuclear Resonant Inelastic X-Ray Scattering (NRIXS, also known as Nuclear Resonance Vibrational Spectroscopy -NRVS- or Nuclear Inelastic Scattering -NIS) at the Advanced Photon Source. These measurements were made on synthetic minerals enriched in 57Fe. A new method (i.e., the general moment approach) is presented to calculate {\beta}-factors from the moments of the NRIXS spectrum S(E). The first term in the moment expansion controls iron isotopic fractionation at high temperature and corresponds to the mean force constant of the iron bonds, a quantity that is readily measured and often reported in NRIXS studies.

cond-mat.mtrl-sci↗

arXiv2008

Nucleosynthetic osmium isotope anomalies in acid leachates of the Murchison meteorite

We present osmium isotopic results obtained by sequential leaching of the Murchison meteorite, which reveal the existence of very large internal anomalies of nucleosynthetic origin. The Os isotopic anomalies are correlated, and can be explained by the variable contributions of components derived from the s, r and p-processes of nucleosynthesis. Much of the s-process rich osmium is released by relatively mild leaching, suggesting the existence of an easily leachable s-process rich presolar phase, or alternatively, of a chemically resistant r-process rich phase. The s-process composition of Os released by mild leaching diverges slightly from that released by aggressive digestion techniques, perhaps suggesting that the presolar phases attacked by these differing procedures condensed in different stellar environments. The correlation between 190Os and 188Os can be used to constrain the s-process 190Os/188Os ratio to be 1.275 pm 0.043. Such a ratio can be reproduced in a nuclear reaction network for a MACS value for 190Os of ~200 pm 22 mbarn at 30 keV. We also present evidence for extensive internal variation of 184Os abundances in the Murchison meteorite. This suggests that p process rich presolar grains (e.g., supernova condensates) may be present in meteorites in sufficient quantities to influence the Os isotopic compositions of the leachates.

astro-ph↗

arXiv2008

Iron-60 evidence for early injection and efficient mixing of stellar debris in the protosolar nebula

Among extinct radioactivities present in meteorites, 60Fe (t1/2 = 1.49 Myr) plays a key role as a high-resolution chronometer, a heat source in planetesimals, and a fingerprint of the astrophysical setting of solar system formation. A critical issue with 60Fe is that it could have been heterogeneously distributed in the protoplanetary disk, calling into question the efficiency of mixing in the solar nebula or the timing of 60Fe injection relative to planetesimal formation. If this were the case, one would expect meteorites that did not incorporate 60Fe (either because of late injection or incomplete mixing) to show 60Ni deficits (from lack of 60Fe decay) and collateral effects on other neutron-rich isotopes of Fe and Ni (coproduced with 60Fe in core-collapse supernovae and AGB-stars). Here, we show that measured iron meteorites and chondrites have Fe and Ni isotopic compositions identical to Earth. This demonstrates that 60Fe must have been injected into the protosolar nebula and mixed to less than 10 % heterogeneity before formation of planetary bodies.

astro-ph↗

arXiv2001

Molybdenum Evidence for Inherited Planetary Scale Isotope Heterogeneity of the Protosolar Nebula

Isotope anomalies provide important information about early solar system evolution. Here we report molybdenum isotope abundances determined in samples of various meteorite classes. There is no fractionation of molybdenum isotopes in our sample set within 0.1 permil and no contribution from the extinct radionuclide 97Tc at mass 97 (97Tc/92Mo<3E-6). Instead, we observe clear anomalies in bulk iron meteorites, mesosiderites, pallasites, and chondrites characterized by a coupled excess in p- and r- or a mirror deficit in s-process nuclides (Mo-HL). This large scale isotope heterogeneity of the solar system observed for molybdenum must have been inherited from the interstellar environment where the sun was born, illustrating the concept of ``cosmic chemical memory''. The presence of molybdenum anomalies is used to discuss the filiation between planetesimals.

astro-ph↗

arXiv2001

Inference on the Nature and the Mass of Earth's Late Veneer from Noble Metals and Gases

Noble metals and gases are very sensitive to the late accretion to the Earth of asteroids and comets. We present mass balance arguments based on these elements that indicate that 0.7E22-2.7E22 kg of extraterrestrial bodies struck the Earth after core formation and that comets comprised less than 1E-5 by mass of the impacting population. These results imply that the dynamics of asteroids and comets changed drastically with time and that biogenic elements and prebiotic molecules were not delivered to the Earth by comets but rather by carbonaceous asteroids.

astro-ph↗